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1. 发明授权

US06174839B1 Phenylacetylene derivatives 失效
标题翻译：苯乙炔衍生物
公开(公告)号：US06174839B1
公开(公告)日：2001-01-16
申请号：US09255959
申请日：1999-02-23
申请人： Akihiko Yanagi , Shin-ichi Narabu , Toshio Goto , Seishi Ito , Natsuko Minegishi , Tatsuya Yamaoka , Chieko Ueno
发明人： Akihiko Yanagi , Shin-ichi Narabu , Toshio Goto , Seishi Ito , Natsuko Minegishi , Tatsuya Yamaoka , Chieko Ueno
IPC分类号： A01N43647
CPC分类号： C07D231/38 , A01N43/54 , A01N43/56 , A01N43/713 , A01N43/82 , A01N47/20 , A01N55/00 , C07D239/22 , C07D239/54 , C07D257/04 , C07D271/113 , C07D405/04 , C07F7/0812
摘要： The invention is related to a novel phenylacetylene derivates of formula: wherein X represents hydrogen, halogen, optionally substituted C1-6 alkyl; Y represents hydrogen, halogen, cyano, nitro, optionally substituted C1-6 alkyl, C1-6 alkoxy, C3-8 cycloalkoxy, optionally substituted C1-6 alkylthio, C3-8 cycloalkylthio, C1-6 alkylsulfinyl, optionally substituted C1-6 alkylsulfonyl, C3-8 cycloalkylsulfonyl, C1-6 alkylsulfonyloxy, optionally substituted sulfonamide, optionally substituted carboxamide, etc., or Y may form together with Z which is bonded to the vicinal carbon atom a 5- or 6-membered ring; n is 0 or 1; Z represents hydrogen or halogen; m is 1 or 2; R represents hydrogen, halogen, C1-6 alkyl, tri(C1-6 alkyl)silyl, COORc or CONRdRe; Q represents a heterocyclic group, and their use as herbicid.
摘要翻译：本发明涉及下式的新型苯乙炔衍生物：其中X表示氢，卤素，任选取代的C 1-6烷基; Y代表氢，卤素，氰基，硝基，任选取代的C 1-6烷基，C 1-6烷氧基，C 3-8环烷氧基，任选取代的C 1-6烷硫基，C 3-8环硫基，C 1-6烷基亚磺酰基，任选取代的C 1-6烷基磺酰基，C 3-8环烷基磺酰基，C 1-6烷基磺酰氧基，任选取代的磺酰胺，任选取代的羧酰胺等，或Y可以与连接在邻位碳原子上的5或6元环一起形成; n为0或1; Z表示氢或卤素; m为1或2; R表示氢，卤素，C 1-6烷基，三（C 1-6烷基）甲硅烷基，COOR c或CONR d Re; Q表示杂环基，它们用作除草剂。

2. 发明授权

US5935907A Phenylacetylene derivatives 失效
标题翻译：苯乙炔衍生物
公开(公告)号：US5935907A
公开(公告)日：1999-08-10
申请号：US47260
申请日：1998-03-24
申请人： Akihiko Yanagi , Shin-ichi Narabu , Toshio Goto , Seishi Ito , Natsuko Minegishi , Tatsuya Yamaoka , Chieko Ueno
发明人： Akihiko Yanagi , Shin-ichi Narabu , Toshio Goto , Seishi Ito , Natsuko Minegishi , Tatsuya Yamaoka , Chieko Ueno
IPC分类号： C07D249/12 , A01N43/08 , A01N43/36 , A01N43/38 , A01N43/50 , A01N43/54 , A01N43/56 , A01N43/58 , A01N43/653 , A01N43/707 , A01N43/713 , A01N43/76 , A01N43/78 , A01N43/82 , A01N43/824 , A01N43/88 , A01N43/90 , A01N47/20 , A01N55/00 , C07D207/24 , C07D207/27 , C07D207/277 , C07D207/38 , C07D207/40 , C07D209/48 , C07D231/20 , C07D231/38 , C07D233/76 , C07D237/14 , C07D239/22 , C07D239/54 , C07D253/06 , C07D257/04 , C07D263/18 , C07D263/44 , C07D271/10 , C07D271/113 , C07D273/04 , C07D277/20 , C07D277/42 , C07D277/60 , C07D285/12 , C07D307/66 , C07D307/90 , C07D405/04 , C07D471/04 , C07D487/04 , C07D513/04 , C07F7/08 , C07D413/04 , A01N43/80 , C07D417/04
CPC分类号： C07D231/38 , A01N43/54 , A01N43/56 , A01N43/713 , A01N43/82 , A01N47/20 , A01N55/00 , C07D239/22 , C07D239/54 , C07D257/04 , C07D271/113 , C07D405/04 , C07F7/0812
摘要： The invention is related to a novel phenylacetylene derivates of formula: ##STR1## wherein X represents hydrogen, halogen, optionally substituted C.sub.1-6 alkyl; Y represents hydrogen, halogen, cyano, nitro, optionally substituted C.sub.1-6 alkyl, C.sub.1-6 alkoxy, C.sub.3-8 cycloalkoxy, optionally substituted C.sub.1-6 alkylthio, C.sub.3-8 cycloalkylthio, C.sub.1-6 alkylsulfinyl, optionally substituted C.sub.1-6 alkylsulfonyl, C.sub.3-8 cycloalkylsulfonyl, C.sub.1-6 alkylsulfonyloxy, optionally substituted sulfonamide, optionally substituted carboxamide, etc., or Y may form together with Z which is bonded to the vicinal carbon atom a 5- or 6-membered ring; n is 0 or 1; Z represents hydrogen or halogen; m is 1 or 2; R represents hydrogen, halogen, C.sub.1-6 alkyl, tri(C.sub.1-6 alkyl)silyl, COOR.sup.c or CONR.sup.d R.sup.e ; Q represents a heterocyclic group, and their use as herbicid.
摘要翻译：本发明涉及下式的新型苯乙炔衍生物：其中X表示氢，卤素，任选取代的C 1-6烷基; Y代表氢，卤素，氰基，硝基，任选取代的C 1-6烷基，C 1-6烷氧基，C 3-8环烷氧基，任选取代的C 1-6烷硫基，C 3-8环硫基，C 1-6烷基亚磺酰基，任选取代的C 1-6烷基磺酰基，C 3-8环烷基磺酰基，C 1-6烷基磺酰氧基，任选取代的磺酰胺，任选取代的羧酰胺等，或Y可以与连接在邻位碳原子上的5或6元环一起形成; n为0或1; Z表示氢或卤素; m为1或2; R表示氢，卤素，C 1-6烷基，三（C 1-6烷基）甲硅烷基，COOR c或CONR d Re; Q表示杂环基，它们用作除草剂。

3. 发明授权

US5776858A 1-azinyl-tetrazolinones 失效
标题翻译： 1-吖嗪基 - 四唑啉酮
公开(公告)号：US5776858A
公开(公告)日：1998-07-07
申请号：US736867
申请日：1996-10-25
申请人： Toshio Goto , Seishi Ito , Natsuko Minegishi , Tatsuya Yamaoka , Chieko Ueno , Koichi Moriya , Fritz Maurer , Ryo Watanabe
发明人： Toshio Goto , Seishi Ito , Natsuko Minegishi , Tatsuya Yamaoka , Chieko Ueno , Koichi Moriya , Fritz Maurer , Ryo Watanabe
IPC分类号： C07D401/06 , A01N43/713 , A01N47/38 , C07D257/04 , C07D401/14 , C07D403/04 , C07D403/06 , C07D403/14 , A01N43/58 , A01N43/60 , A01N43/66 , C07D403/02
CPC分类号： C07D403/04 , A01N47/38
摘要： 1-Azinyl-tetraozolinones of the following formulae (I) and (II): ##STR1## wherein R.sup.1 and R.sup.2 are independently represent alkyl, haloalkyl, cycloalkyl, alkenyl, haloalkenyl, alkynyl or optionally substituted phenyl, or R.sup.1 and R.sup.2, together with the nitrogen atom to which they are bonded, may form a 5- or 6-membered heterocyclic ring which may optionally contain a further heteroatom, and said heterocyclic ring may optionally be benzo-condensed and/or be substituted by one or more of C.sub.1-4 alkyl(s), and R.sup.3 is a 6-membered heterocyclic aromatic group consisting of carbon atoms and 2 or 3 nitrogen atoms, which may optionally be substituted by halogen, C.sub.1-4 alkyl, C.sub.1-4 alkoxy, C.sub.1-4 alkylthio, di(C.sub.1-4 alkyl)amino or phenyl. The compounds of the formula (I) exhibit an excellent herbicidal activity and the compounds of the formula (II) are useful as starting materials in the production of the compounds of the formula (I).
摘要翻译：下式（I）和（II）的1-氮杂环丁烷基 - 四唑啉酮：其中R 1和R 2独立地表示烷基，卤代烷基，环烷基，烯基，卤代烯基，炔基或任意取代的苯基或R 1和R 2与它们所键合的氮原子一起可以形成可以任选地含有另外的杂原子的5-或6-元杂环，并且所述杂环可任选地被苯并稠合和/或被一个或多个C 1-4烷基取代，并且R 3是由碳原子和2或3个氮原子组成的6元杂环芳基，其可任选被卤素，C 1-4烷基，C 1 -4-烷氧基，C 1-4烷硫基，二（C 1-4烷基）氨基或苯基。式（I）的化合物显示出优异的除草活性，并且式（II）的化合物可用作制备式（I）化合物的原料。

4. 发明授权

US5641725A Sulphonylaminophenyluracil herbicides for paddy field 失效
标题翻译：用于稻田的磺酰基氨基苯基尿嘧啶除草剂
公开(公告)号：US5641725A
公开(公告)日：1997-06-24
申请号：US562923
申请日：1995-11-27
申请人： Toshio Goto , Seishi Ito , Chieko Ueno , Tatsuya Yamaoka , Kazuhiro Ukawa , Natsuko Minegishi
发明人： Toshio Goto , Seishi Ito , Chieko Ueno , Tatsuya Yamaoka , Kazuhiro Ukawa , Natsuko Minegishi
IPC分类号： A01N43/54
CPC分类号： A01N43/54
摘要： A herbicide for paddy field comprising sulphonylaminophenyluracil derivative as an active ingredient which is represented by the formula (I): ##STR1## wherein R.sup.1 represents hydrogen or methyl,R.sup.2 represents C.sub.1-5 alkyl, fluro-substituted C.sub.1-2 alkyl or C.sup.3-6 cycloalkyl,optionally applied in combination with another herbicide.
摘要翻译：一种稻田除草剂，其包含由式（I）表示的磺酰氨基苯基尿嘧啶衍生物作为活性成分：其中R1表示氢或甲基，R2表示C1-5烷基，氟取代的C1-2烷基或C3- 6环烷基，任选地与另一种除草剂组合施用。

5. 发明授权

US06969697B2 Substituted benzoylcyclohexenones 失效
标题翻译：取代的苯甲酰基环己烯酮
公开(公告)号：US06969697B2
公开(公告)日：2005-11-29
申请号：US10220711
申请日：2001-03-01
申请人： Klaus-Helmut Müller , Hans-Georg Schwarz , Stefan Herrmann , Dorothee Hoischen , Stefan Lehr , Otto Schallner , Mark Wilhelm Drewes , Peter Dahmen , Dieter Feucht , Rolf Pontzen , Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
发明人： Klaus-Helmut Müller , Hans-Georg Schwarz , Stefan Herrmann , Dorothee Hoischen , Stefan Lehr , Otto Schallner , Mark Wilhelm Drewes , Peter Dahmen , Dieter Feucht , Rolf Pontzen , Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
IPC分类号： A01N43/50 , A01N43/54 , A01N43/56 , A01N43/653 , A01N43/713 , C07D233/14 , C07D233/32 , C07D233/36 , C07D239/10 , C07D249/12 , C07D249/14 , C07D257/04 , A01N43/84 , C07D407/04
CPC分类号： C07D239/10 , A01N43/50 , A01N43/54 , A01N43/653 , A01N43/713 , C07D233/32 , C07D233/36 , C07D249/12 , C07D257/04
摘要： The invention relates to novel substituted benzoylcyclohexenones of the formula (I), in which n, A, R1, R2, R3, R4, Y and Z are each as defined in the description, and also to processes for their preparation and to their use as herbicides.
摘要翻译：本发明涉及式（I）的新型取代的苯甲酰基环己烯酮，其中n，A，R 1，R 2，R 3， R 4，Y和Z各自如说明书中所定义，并且还涉及其制备方法及其作为除草剂的用途。

6. 发明授权

US06624121B1 Herbicidal tetrazolinone derivatives 失效
标题翻译：除草四唑啉酮衍生物
公开(公告)号：US06624121B1
公开(公告)日：2003-09-23
申请号：US10049405
申请日：2002-02-05
申请人： Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
发明人： Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
IPC分类号： A01N43713
CPC分类号： C07D257/04 , A01N43/713 , A01N43/80 , C07D403/10 , C07D413/10
摘要： Novel tetrazolinones with herbicidal activity are disclosed. The tetrazolinones of the present invention are represented by the general formula (I) wherein R1, R2, m, n and Q are as defined in the specification. A process for making the tetrazolinones of the present invention is also disclosed.
摘要翻译：公开了具有除草活性的新型四唑啉酮。本发明的四唑啉酮由通式（I）表示，其中R 1，R 2，m，n和Q如说明书中所定义。还公开了制备本发明的四唑啉酮的方法。

7. 发明授权

US06936570B2 Tetrazolinone derivatives 失效
标题翻译：四唑啉酮衍生物
公开(公告)号：US06936570B2
公开(公告)日：2005-08-30
申请号：US10873357
申请日：2004-06-21
申请人： Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
发明人： Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
IPC分类号： A01N43/713 , A01N43/80 , C07D257/04 , C07D403/10 , C07D413/10 , C08D413/10
CPC分类号： C07D257/04 , A01N43/713 , A01N43/80 , C07D403/10 , C07D413/10
摘要： The invention relates to novel tetrazolinone derivatives of general formula (I) wherein R1 represents halogen, C1-4 alkyl, C1-4 haloalkyl, C1-4 alkoxy, C1-4 alkylthio, C1-4 alkylsulfonyl, C1-4 alkylsulfonyloxy, C2-5 alkoxycarbonyl, C2-6 alkoxyalkyl, C2-6 alkylthioalkyl, nitro or cyano, R2 represents a hydrogen atom, C1-6 alkyl, C3-6 cycloalkyl which may be optionally substituted with halogen or C1-3 alkyl, C1-4 haloalkyl, or phenyl which may be optionally substituted with halogen, C1-3 alkyl, C1-3 haloalkyl or nitro, m represents 0, 1 or 2, n represents 0 or 1, Q represents one of the groups which are mentioned in the description. The invention further relates to their use as herbicides and a process together with the intermediates for their preparation.
摘要翻译：本发明涉及通式（I）的新的四唑啉酮衍生物，其中R 1表示卤素，C 1-4烷基，C 1-4烷基，卤代烷基，C 1-4烷氧基，C 1-4烷基硫基，C 1-4烷基磺酰基，C 1-4烷基磺酰基，烷基磺酰氧基，C 2-5烷氧基羰基，C 2-6烷氧基烷基，C 2-6烷硫基烷基，硝基或氰基，R SUP > 2表示氢原子，C 1-6烷基，C 3-6环烷基，其可任选被卤素或C 1 -C 6烷基取代， C 1-4烷基，C 1-4卤代烷基或可任选被卤素取代的苯基，C 1-3烷基，C 1-3烷基卤代烷基或硝基，m表示0,1或2，n表示0或1，Q表示说明书中提到的基团之一。本发明还涉及它们作为除草剂的用途以及与其制备中间体一起的方法。

8. 发明授权

US06790810B2 Tetrazolinone derivatives 失效
标题翻译：四唑啉酮衍生物
公开(公告)号：US06790810B2
公开(公告)日：2004-09-14
申请号：US10610301
申请日：2003-06-30
申请人： Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
发明人： Akihiko Yanagi , Shinichi Narabu , Toshio Goto , Seishi Ito , Chieko Ueno
IPC分类号： A01N43713
CPC分类号： C07D257/04 , A01N43/713 , A01N43/80 , C07D403/10 , C07D413/10
摘要： The invention relates to novel tetrazolinone derivatives of general formula (I) wherein R1 represents halogen, C1-4 alkyl, C1-4 haloalkyl, C1-4 alkoxy, C1-4 alkylthio, C1-4 alkylsulfonyl, C1-4 alkylsulfonyloxy, C2-5 alkoxycarbonyl, C2-6 alkoxyalkyl, C2-6 alkylthioalkyl, nitro or cyano, R2 represents a hydrogen atom, C1-6 alkyl, C3-6 cycloalkyl which may be optionally substituted with halogen, or C1-3 alkyl, C1-4 haloalkyl or phenyl which may be optionally substituted with halogen, or C1-3 aklyl, C1-4 haloalkyl or nitro, m represents 0, 1 or 2, n represents 0 or 1, Q represents one of the groups which are mentioned in the description. The invention further relates to their use as herbicides and a process together with the intermediates for their preparation.
摘要翻译：本发明涉及通式（I）的新的四唑啉酮衍生物，其中R 1表示卤素，C 1-4烷基，C 1-4卤代烷基，C 1-4烷氧基，C 1-4烷硫基，C 1-4烷基磺酰基，C 1-4烷基磺酰氧基，C 2-5烷氧基羰基，C 2-6烷氧基烷基，C 2-6烷硫基烷基，硝基或氰基，R 2表示氢原子，可以任选被卤素取代的C 1-6烷基，C 3-6环烷基或C 1-3 烷基，C 1-4卤代烷基或可被卤素任意取代的苯基，或C 1-3烷基，C 1-4卤代烷基或硝基，m表示0,1或2，n表示0或1，Q表示在说明书中提到。本发明还涉及它们作为除草剂的用途以及与其制备中间体一起的方法。

9. 发明授权

US5654257A 1-cycloalkenyltetrazolinones 失效
标题翻译： 1-环烯基四唑啉酮
公开(公告)号：US5654257A
公开(公告)日：1997-08-05
申请号：US601748
申请日：1996-02-15
申请人： Toshio Goto , Yoshinori Kitagawa , Seishi Ito , Katsuhiko Shibuya , Tatsuya Yamaoka , Chieko Ueno , Yoshiko Kyo
发明人： Toshio Goto , Yoshinori Kitagawa , Seishi Ito , Katsuhiko Shibuya , Tatsuya Yamaoka , Chieko Ueno , Yoshiko Kyo
IPC分类号： C07D401/06 , A01N47/38 , C07D257/04 , C07D403/06 , A01N43/713
CPC分类号： C07D257/04 , A01N47/38
摘要： 1-cycloalkenyltetrazolinone derivatives of the following herbicidal formula ##STR1## R.sup.1 is cycloalkenyl which may optionally be substituted by halogen C.sub.1-4 alkyl, or bicycloalkenyl which may optionally be substituted by halogen or C.sub.1-4 alkyl, andR.sup.2 and R.sup.3 each independently is alkyl, cycloalkyl, phenyl (optionally substituted by a member selected from the group consisting of nitro, cyano, halogen, alkyl, haloalkyl, alkoxy, haloalkoxy and alkylthio), alkenyl and alkynyl,orR.sup.2 and R.sup.3 together with the N-atom to which they are bonded form, a 5- or 6-membered heterocyclic ring which may optionally contain a further hetero atom, said heterocyclic ring optionally being benzo-condensed, or a C-.sub.1-4 alkyl,and intermediates therefore of the formula ##STR2##
摘要翻译：以下除草式R 1的1-环烯基四唑啉酮衍生物是可任选被卤素C 1-4烷基取代的环烯基，或可任意被卤素或C 1-4烷基取代的双环烯基，R 2和R 3各自独立地为烷基，环烷基，苯基（任选被选自硝基，氰基，卤素，烷基，卤代烷基，烷氧基，卤代烷氧基和烷硫基的成员取代），烯基和炔基，或者R 2和R 3与它们的N-原子一起键合形式，可任选地含有另外的杂原子的所述5或6元杂环，所述杂环任选地被苯并稠合，或C 1-4烷基，因此具有下式的中间体：

10. 发明授权

US5605920A Tetrazolinones 失效
标题翻译：四唑啉酮
公开(公告)号：US5605920A
公开(公告)日：1997-02-25
申请号：US618954
申请日：1996-03-20
申请人： Toshio Goto , Yoshinori Kitagawa , Seishi Ito , Katsuhiko Shibuya , Tatsuya Yamaoka , Chieko Ueno , Yoshiko Kyo
发明人： Toshio Goto , Yoshinori Kitagawa , Seishi Ito , Katsuhiko Shibuya , Tatsuya Yamaoka , Chieko Ueno , Yoshiko Kyo
IPC分类号： C07D401/06 , A01N47/38 , C07D257/04 , C07D401/12 , C07D403/06 , C07D403/12 , A01N43/713 , A61K31/41
CPC分类号： C07D257/04 , A01N47/38 , C07D401/12 , C07D403/12
摘要： Disclosed are herbicidal tetrazolinone derivatives, selective in paddy fields of the formula ##STR1## wherein X represents C.sub.1-4 alkyl,n represents 1, 2, 3 or 4,R.sup.1 and R.sup.2 each independently represents C.sub.1-6 alkyl, C.sub.2-4 alkenyl, C.sub.2-6 alkynyl, C.sub.3-8 cycloalkyl, aryl which may optionally be substituted (wherein the substituent is at least one radical selected from the group consisting of halogen, C.sub.1-4 alkyl, C.sub.1-2 haloalkyl, C.sub.1-2 haloalkoxy, C.sub.1-2 haloalkylthio, acyl, nitro and cyano) or aralkyl optionally substituted by halogen orR.sup.1 and R.sup.2 form, together with the N-atom to which they are bonded, a cyclic ring which may be substituted. Also, disclosed are novel intermediates useful in the preparation of the compounds of formula (I).
摘要翻译：公开了除草性四唑啉酮衍生物，其在式（I）的水田中是选择性的，其中X表示C1-4烷基，n表示1,2,3或4，R1和R2各自独立地表示C1-6烷基，C2- 4链烯基，C 2-6炔基，C 3-8环烷基，可任选取代的芳基（其中取代基是至少一个选自卤素，C 1-4烷基，C 1-2卤代烷基，C 1-2卤代烷氧基，C 1-2卤代烷硫基，酰基，硝基和氰基）或任选被卤素或R 1和R 2形式取代的芳烷基与它们所键合的N-原子一起可以被取代的环状基团。还公开了可用于制备式（I）化合物的新型中间体。

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