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1. 发明申请

US20060204782A1 Polymer and polymer light-emitting device using same 审中-公开
标题翻译：聚合物和聚合物发光装置使用它
公开(公告)号：US20060204782A1
公开(公告)日：2006-09-14
申请号：US10550209
申请日：2004-03-29
申请人： Akihiko Okada , Tomoyuki Suziki , Hideaki Nakajima
发明人： Akihiko Okada , Tomoyuki Suziki , Hideaki Nakajima
IPC分类号： B32B19/00
CPC分类号： H01L51/0036 , C08G61/00 , C09K11/06 , C09K2211/14 , H01L51/0094 , H01L51/5012 , H05B33/14
摘要： A polymer emitting fluorescence in the solid state, having a polystyrene-reduced weight-average molecular weight of 103 to 108 and having a repeating unit selected from the group consisting of arylene group, divalent heterocyclic group and divalent aromatic amine group, wherein the polymer has an unsaturated hydrocarbon group free of aromatic ring which directly bonds to any one of the repeating units, at least, at one terminal end of the main chain thereof.
摘要翻译：发射固态的荧光的聚合物，其聚苯乙烯换算的重均分子量为10 -3至10 8，并具有选自以下的重复单元：亚芳基，二价杂环基和二价芳族胺基，其中所述聚合物具有不饱和烃基，其至少在其主链的一个末端直接键合到任何一个重复单元上的芳环。

2. 发明授权

US5952431A Process for producing acid-modified polyphenylene ether and polystyrenic resin composition 失效
标题翻译：生产酸改性聚苯醚和聚苯乙烯树脂组合物的方法
公开(公告)号：US5952431A
公开(公告)日：1999-09-14
申请号：US765443
申请日：1997-01-16
申请人： Akihiko Okada
发明人： Akihiko Okada
IPC分类号： C08K3/00 , C08G65/48 , C08K7/00 , C08K7/14 , C08K9/00 , C08K9/04 , C08L7/00 , C08L21/00 , C08L25/00 , C08L27/06 , C08L71/00 , C08L71/12 , C08L73/00 , C08L77/00 , H05K1/03 , C08F283/08
CPC分类号： C08L71/126 , C08G65/485 , C08L25/00 , C08L27/06 , C08L71/12 , C08L77/00 , H05K1/0353
摘要： A process for producing an acid-modified polyphenylene ether comprising conducting modification reaction substantially in the absence of solvents at 300 to 350.degree. C. by using (a) 100 parts by weight of a polyphenylene ether, (b) 0.1 to 5.0 parts by weight of fumaric acid or a derivative of fumaric acid, and optionally (c) 0.1 to 5.0 parts by weight of a radical generating agent having a half-life of 1 minute at a temperature of 300.degree. C. or higher; and a polystyrenic resin composition comprising (d) 100 parts by weight of a styrenic polymer having the syndiotactic configuration or 100 parts by weight of a component composed of a styrenic polymer having the syndiotactic configuration and a rubbery elastomer and/or a polyamide, (e) 0.5 to 5.0 parts by weight of an acid-modified polyphenylene ether obtained by the above process, and optionally (f) 1 to 350 parts by weight of inorganic filler.A convenient process for producing an acid-modified polyphenylene ether which does not cause deterioration of the working environment, enables stable production, and suppresses decrease in the molecular weight has been developed. A polystyrenic resin composition which can exhibit high toughness is provided by using the obtained acid-modified polyphenylene ether.
摘要翻译： PCT No.PCT / JP96 / 01277 Sec。 371日期1997年1月16日 102（e）日期1997年1月16日PCT提交1996年5月15日PCT公布。公开号WO96 / 36658 PCT。日期：1996年11月21日1.一种酸改性聚苯醚的制造方法，其特征在于，使用（a）100重量份聚苯醚，（b）0.1（重量）以上，在300〜350℃下，基本上不存在溶剂进行改性反应至5.0重量份的富马酸或富马酸的衍生物，以及（c）0.1至5.0重量份在300℃或更高温度下半衰期为1分钟的自由基发生剂; 和聚苯乙烯树脂组合物，其包含（d）100重量份具有间同立构构型的苯乙烯聚合物或100重量份由具有间同立构构型的苯乙烯类聚合物组成的组分和橡胶弹性体和/或聚酰胺（e ）0.5〜5.0重量份通过上述方法获得的酸改性聚苯醚，和（f）1〜350重量份无机填料。生产酸改性聚苯醚的方便工艺不会导致工作环境恶化，能够稳定地生产，抑制分子量的降低。通过使用得到的酸改性聚苯醚，可提供韧性高的聚苯乙烯树脂组合物。

3. 发明授权

US5418275A Polystyrene composition 失效
标题翻译：聚苯乙烯组合物
公开(公告)号：US5418275A
公开(公告)日：1995-05-23
申请号：US118335
申请日：1993-09-09
申请人： Akihiko Okada , Nobuyuki Sato
发明人： Akihiko Okada , Nobuyuki Sato
IPC分类号： C08K3/00 , C08L21/00 , C08L25/04 , C08L25/06 , C08L51/08 , C08L53/00 , C08L53/02 , C08L71/00 , C08L71/12 , C08L51/04 , C08L73/00
CPC分类号： C08L25/06 , C08L71/12 , C08L21/00 , C08L51/08
摘要： There are disclosed a polystyrene composition which comprises 100 parts by weight of a syndiotactic polystyrene (SPS)(a) and 1 to 100 parts by weight of a high molecular compound comprising 5 to 95% by weight of polyphenylene ether (PPO) and/or modified PPO and 95 to 5% by weight of a rubbery elastomer (b) and optionally, 1 to 350 parts by weight of an inorganic filler (d) and also a polystyrene composition which comprises 100 parts by weight of the component (a), 0.1 to 30 parts by weight of the component (b) and 1 to 100 parts by weight of a rubbery elastomer (c) and optionally, 1 to 350 parts by weight of the component (d). The above compositions are greatly improved in impact resistance, elongation and retention of physical properties during recycling without detriment to heat resistance and modulus of elasticity.
摘要翻译：公开了一种聚苯乙烯组合物，其包含100重量份的间同立构聚苯乙烯（SPS）（a）和1至100重量份的包含5至95重量％的聚苯醚（PPO）和/或改性PPO和95〜5重量％的橡胶弹性体（b）和任选的1〜350重量份的无机填料（d），以及聚苯乙烯组合物，其包含100重量份的组分（a）， 0.1〜30重量份的组分（b）和1至100重量份的橡胶弹性体（c）和任选的1至350重量份组分（d）。上述组合物在回收期间的耐冲击性，伸长率和物理性能的保持性大大提高，而不损害耐热性和弹性模量。

4. 发明授权

US5352727A Syndiotactic polystyrene composition 失效
标题翻译：间规聚苯乙烯组合物
公开(公告)号：US5352727A
公开(公告)日：1994-10-04
申请号：US118334
申请日：1993-09-09
申请人： Akihiko Okada
发明人： Akihiko Okada
IPC分类号： C08K3/00 , C08L21/00 , C08L25/00 , C08L25/04 , C08L25/06 , C08L51/00 , C08L53/00 , C08L53/02 , C08K7/14
CPC分类号： C08L25/06 , C08L51/003 , C08L21/00 , C08L2205/02 , C08L53/025
摘要： There are disclosed a polystyrene composition which comprises 100 parts by weight of a resin component comprising 0 to 99% by weight of syndiotactic polystyrene (SPS) (a) and 100 to 1% by weight of a modified syndiotactic polystrene (SPS) (b) and 1 to 100 parts by weight of a rubbery elastomer which can react with the functional group of the component (b) as the component (c) and optionally, 1 to 350 parts by weight of an inorganic filler (e); and a polystyrene composition which comprises 100 parts by weight of a resin component comprising 0 to 99% by weight of the component (a) and 100 to 1% by weight of the component (b), 1 to 10 parts by weight of the component (c) and 1 to 100 parts by weight of a rubbery elastomer (d) and optionally, 1 to 350 parts by weight of an organic filler (e). The above compositions are greatly improved in impact resistance, elongation and retention of physical properties during recycling without detriment to heat resistance and modulus of elasticity.
摘要翻译：公开了一种聚苯乙烯组合物，其包含100重量份的包含0至99重量％的间同立构聚苯乙烯（SPS）（a）和100至1重量％的改性间规聚苯乙烯（SPS）（b）的树脂组分，和1〜100重量份的可与组分（b）的组分（b）的官能团反应的橡胶状弹性体和任选的1至350重量份的无机填料（e）; 和聚苯乙烯组合物，其包含100重量份的包含0至99重量％的组分（a）和100至1重量％的组分（b）的树脂组分，1至10重量份的组分（c）和1至100重量份的橡胶状弹性体（d）和任选的1至350重量份的有机填料（e）。上述组合物在回收期间的耐冲击性，伸长率和物理性能的保持性大大提高，而不损害耐热性和弹性模量。

5. 发明授权

US06169146A Styrene resin composition and method of manufacturing the same, and method of manufacturing styrene resin molded products 有权
标题翻译：苯乙烯树脂组合物及其制造方法以及苯乙烯树脂成型体的制造方法
公开(公告)号：US06169146A
公开(公告)日：2001-01-02
申请号：US09228968
申请日：1999-01-12
申请人： Akihiko Okada , Takuma Aoyama
发明人： Akihiko Okada , Takuma Aoyama
IPC分类号： C08L2506
CPC分类号： C08L25/06 , C08L53/02 , C08L71/12 , C08L2205/02 , C08L2666/04 , C08L2666/02
摘要： Disclosed is a resin composition containing the following components (A), and (B) or optionally, (C), (D), and (E): (A) an atactic polystyrene or a mixture of an atactic polystyrene and a rubber-like elastic substance: 30 to 95 parts by weight; (B) a syndiotactic polystyrene having a melting point of not higher than 255° C.: 70 to 5 parts by weight; (C) a polyphenylene ether having an intrinsic viscosity of 0.5 deciliter/g or less as measured in chloroform at 25° C.; (D) an inorganic filler; and (E) a polymer having compatibility or affinity with components (A) and (B) and having a polar group. The styrene resin composition exhibits improved solvent resistance and remarkable impact resistance. The composition of the invention is produced by kneading the components within a resin temperature range between the melting point of component (B) and 270° C. Resin molded products are manufactured through use of the styrene resin composition by adjusting the resin temperature during molding to fall within the range from the melting point of component (B) to 270° C.
摘要翻译：公开了含有下列组分（A）和（B）或任选的（C），（D）和（E）：（A）的无规立构聚苯乙烯或无规聚苯乙烯与橡胶 - 弹性体：30〜95重量份;（B）熔点不高于255℃的间同立构聚苯乙烯：70〜5重量份;（C）特性粘度为0.5分升的聚苯醚 / g以下，在25℃的氯仿中测定;（D）无机填料; 和（E）与组分（A）和（B）具有相容性或亲和性且具有极性基团的聚合物。苯乙烯树脂组合物表现出改进的耐溶剂性和显着的耐冲击性。本发明的组合物通过在树脂温度范围内在组分（B）的熔点和270℃之间的树脂温度范围内捏合来制备。树脂模制产品通过使用苯乙烯树脂组合物通过调节模塑过程中的树脂温度而制备成落在组分（B）的熔点到270℃的范围内。

6. 发明授权

US6013709A Polystyrenic resin composition and molded article thereof 失效
标题翻译：聚苯乙烯树脂组合物及其模制品
公开(公告)号：US6013709A
公开(公告)日：2000-01-11
申请号：US776183
申请日：1997-01-24
申请人： Akitoshi Masuyama , Hiroki Fukui , Akihiko Okada
发明人： Akitoshi Masuyama , Hiroki Fukui , Akihiko Okada
IPC分类号： C08K3/16 , C08K5/00 , C08L25/04 , C08L25/06 , C08L53/02 , C08L71/12 , C08L73/00 , C08L77/00 , C08L101/00 , C08K5/21 , C08K3/10 , C08K5/36
CPC分类号： C08L25/06 , C08K5/005 , C08L77/00 , C08L2205/02 , C08L53/02 , C08L71/12
摘要： A polystyrenic resin composition comprising (A) a styrenic polymer composition containing (a) 1 to 99% by weight of a polystyrenic resin having the syndiotactic configuration, (b) 1 to 99% by weight of a polyamide resin, (c) 0.1 to 10% by weight of a compatibilizer which is compatible with component (a) and has a polar group reactive with component (b), and (d) 0 to 50% by weight of a rubbery elastomer and/or a modified rubbery elastomer, (B) specific amounts of a copper compound and an iodine compound, and optionally, specific amounts of (C) a phenolic compound, (D) N,N'-hexamethylenebis(3,5-di-t-butyl-4-hydroxy-hydrocinnamide), (E) an ester of thiodipropionic acid or a derivative thereof, (F) a copper inhibitor, and (G) inorganic filler; and a molded article prepared from the polystyrenic resin composition.The polystyrenic resin composition shows excellent resistance to heat aging so that little change in physical properties or color is caused even after exposure to a high temperature for a long time, has excellent toughness, rigidity, heat resistance, and water resistance, and can advantageously be used as a material for various types of industrial product.
摘要翻译： PCT No.PCT / JP96 / 01329 Sec。 371日期1997年1月24日 102（e）日期1997年1月24日PCT提交1996年5月20日PCT公布。公开号WO96 / 37552 日期：1996年11月28日一种聚苯乙烯树脂组合物，其包含（A）苯乙烯聚合物组合物，其含有（a）1至99重量％的间同立构构型的聚苯乙烯树脂，（b）1至99重量％的聚酰胺树脂，（c）0.1至10重量％的与组分（a）相容并且具有与组分（b）反应的极性基团的增容剂，和（d）0至50重量％的橡胶弹性体和/或改性橡胶弹性体，（B）特定量的铜化合物和碘化合物，以及任选的特定量的（C）酚类化合物，（D）N，N'-六亚甲基双（3,5-二叔丁基（E）硫代二丙酸或其衍生物的酯，（F）铜抑制剂和（G）无机填料; 和由聚苯乙烯树脂组合物制备的模塑制品。聚苯乙烯树脂组合物显示出优异的耐热老化性，即使长时间暴露于高温后也几乎不引起物理性质或颜色的变化，具有优异的韧性，刚性，耐热性和耐水性，并且可以有利地用作各种工业产品的材料。

7. 发明授权

US5760105A Styrenic resin composition 失效
标题翻译：苯乙烯树脂组合物
公开(公告)号：US5760105A
公开(公告)日：1998-06-02
申请号：US603262
申请日：1996-02-20
申请人： Akihiko Okada , Hiroki Fukui
发明人： Akihiko Okada , Hiroki Fukui
IPC分类号： C08L25/04 , C08L25/06 , C08L51/04 , C08L53/00 , C08L55/02 , C08L67/00 , C08L69/00 , C08L71/12 , C08L77/00 , C08F279/00
CPC分类号： C08L77/00 , C08L25/06 , C08L51/04 , C08L53/00 , C08L67/00 , C08L69/00 , C08L71/126 , C08L2205/02 , C08L25/04 , C08L55/02 , C08L71/12 , Y10S525/902
摘要： There are disclosed a styrenic resin composition which comprises 1 to 95% by weight of a (a) styrenic polymer having syndiotactic configuration (SPS) or modified SPS; 1 to 95% by weight of a (b) thermoplastic resin having a polar group; 1 to 50% by weight of a (c) rubbery elastomer having an affinity for the component (a); and 0.1 to 10% by weight of a (d) compatibilizer having a polar group, a styrenic resin composition same as above except that the component (c) has a polar group capable of reacting with the component (b) as well as an affinity for the component (a) and a styrenic resin composition further comprising 1 to 350% parts by weight of an (e) inorganic filler based on 100 parts by weight of the above resin components. According to the present invention, there are obtained styrenic resin compositions that are well suited for various industrial materials and excellent in rigidity, heat resistance, impact resistance and water resistance.
摘要翻译：公开了苯乙烯树脂组合物，其包含1至95重量％的具有间同立构构型（SPS）或改性SPS的（a）苯乙烯聚合物; 1〜95重量％的具有极性基团的（b）热塑性树脂; 1〜50重量％的对组分（a）具有亲和性的（c）橡胶状弹性体; 和0.1〜10重量％的具有极性基团的（d）增容剂，与上述相同的苯乙烯类树脂组合物，只是组分（c）具有能够与组分（b）反应的极性基团以及亲和力对于组分（a）和苯乙烯树脂组合物，其进一步包含基于100重量份上述树脂组分的1至350重量份的（e）无机填料。根据本发明，获得了非常适合于各种工业材料并且刚性，耐热性，耐冲击性和耐水性优异的苯乙烯树脂组合物。

8. 发明授权

US5444126A Process for producing a modified polyphenylene ether 失效
标题翻译：生产改性聚苯醚的方法
公开(公告)号：US5444126A
公开(公告)日：1995-08-22
申请号：US201035
申请日：1994-02-24
申请人： Akihiko Okada , Akitoshi Masuyama
发明人： Akihiko Okada , Akitoshi Masuyama
IPC分类号： C08F283/08 , C08G65/48 , C08L21/00 , C08L25/06 , C08L51/08 , C08L77/00 , H05K1/03
CPC分类号： C08L25/06 , C08F283/08 , C08G65/485 , C08L77/00 , C08L21/00 , C08L51/08 , H05K1/0373 , Y10S525/905
摘要： There are disclosed a thermoplastic resin composition comprising (A) a styrenic polymer having a high degree of syndiotactic configuration, (B) an inorganic filler and (C) a polyphenylene ether that is modified with a compound having an ethylenic double bond and a polar group in the same molecule, especially maleic anhydride, the ether having a modification rate of 1.3% or more by weight; a thermoplastic resin composition further comprising (D) a rubbery elastomer in addition to the above components (A), (B) and (C); a process for producing modified polyphenylene ether (PPO) comprising reacting 100 parts by weight of PPO with 1 to 20 parts by weight of the above compound or a derivative thereof in an aromatic hydrocarbon solvent in the presence of 15 or less parts by weight of a radical generator; and a process for producing the modified PPO comprising reacting 100 parts by weight of PPO with 1 to 5 parts by weight of the above compound or a derivative thereof at 300.degree. to 350.degree. C. in the presence of 0.1 to 3 parts by weight of a radical generator which exhibits a half-life period of 1 minute at 300.degree. C. or higher. The above thermoplastic resin composition is markedly improved in its dynamical properties especially rigidity and heat resistance.
摘要翻译：公开了一种热塑性树脂组合物，其包含（A）具有高间隔构型的苯乙烯类聚合物，（B）无机填料和（C）用具有烯属双键和极性基团的化合物改性的聚苯醚在相同的分子中，特别是马来酸酐，该醚的改性率为1.3重量％以上; 除上述成分（A），（B）和（C）以外还含有（D）橡胶状弹性体的热塑性树脂组合物; 一种生产改性聚苯醚（PPO）的方法，包括使100重量份的PPO与1至20重量份的上述化合物或其衍生物在芳族烃溶剂中，在15重量份或更少重量份的自由基发生器; 和改性PPO的制造方法，其特征在于，在100〜100重量份的PPO与0.1〜3重量份的上述化合物或其衍生物之间，在100〜350重量份一种自由基发生剂，其在300℃或更高温度下具有1分钟的半衰期。上述热塑性树脂组合物的动力特性，特别是刚性和耐热性显着提高。

9. 发明授权

US5326813A Thermoplastic resin composition containing a modified polyphenylene ether 失效
标题翻译：含有改性聚苯醚的热塑性树脂组合物
公开(公告)号：US5326813A
公开(公告)日：1994-07-05
申请号：US988462
申请日：1992-12-10
申请人： Akihiko Okada , Akitoshi Masuyama
发明人： Akihiko Okada , Akitoshi Masuyama
IPC分类号： C08F283/08 , C08G65/48 , C08L21/00 , C08L25/06 , C08L51/08 , C08L77/00 , H05K1/03 , C08L71/02
CPC分类号： C08L25/06 , C08F283/08 , C08G65/485 , C08L77/00 , C08L21/00 , C08L51/08 , H05K1/0373 , Y10S525/905
摘要： There are disclosed a thermoplastic resin composition comprising (A) a styrenic polymer having a high degree of syndiotactic configuration, (B) an inorganic filler and (C) a polyphenylene ether that is modified with a compound having an ethylenic double bond and a polar group in the same molecule, especially maleic anhydride, the ether having a modification rate of 1.3% or more by weight; a thermoplastic resin composition further comprising (D) a rubbery elastomer in addition to the above components (A), (B) and (C); a process for producing modified polyphenylene ether (PPO) comprising reacting 100 parts by weight of PPO with 1 to 20 parts by weight of the above compound or a derivative thereof in an aromatic hydrocarbon solvent in the presence of 15 or less parts by weight of a radical generator; and a process for producing the modified PPO comprising reacting 100 parts by weight of PPO with 1 to 5 parts by weight of the above compound or a derivative thereof at 300.degree. to 350.degree. C. in the presence of 0.1 to 3 parts by weight of a radical generator which exhibits a half-life period of 1 minute at 300.degree. C. or higher. The above thermoplastic resin composition is markedly improved in its dynamical properties especially rigidity and heat resistance.
摘要翻译：公开了一种热塑性树脂组合物，其包含（A）具有高间隔构型的苯乙烯类聚合物，（B）无机填料和（C）用具有烯属双键和极性基团的化合物改性的聚苯醚在相同的分子中，特别是马来酸酐，该醚的改性率为1.3重量％以上; 除上述成分（A），（B）和（C）以外还含有（D）橡胶状弹性体的热塑性树脂组合物; 一种生产改性聚苯醚（PPO）的方法，包括使100重量份的PPO与1至20重量份的上述化合物或其衍生物在芳族烃溶剂中，在15重量份或更少重量份的自由基发生器; 和改性PPO的制造方法，其特征在于，在100〜100重量份的PPO与0.1〜3重量份的上述化合物或其衍生物之间，在100〜350重量份一种自由基发生剂，其在300℃或更高温度下具有1分钟的半衰期。上述热塑性树脂组合物的动力特性，特别是刚性和耐热性显着提高。

10. 发明授权

US06926973B2 Copolymer, polymer composition and polymer light-emitting device 有权
标题翻译：共聚物，聚合物组合物和聚合物发光装置
公开(公告)号：US06926973B2
公开(公告)日：2005-08-09
申请号：US10322046
申请日：2002-12-18
申请人： Tomoyuki Suzuki , Shuji Doi , Takanobu Noguchi , Akihiko Okada
发明人： Tomoyuki Suzuki , Shuji Doi , Takanobu Noguchi , Akihiko Okada
IPC分类号： C08G61/00 , C08G61/02 , H05B33/14 , C09K11/06
CPC分类号： H01L51/0043 , C08G61/02 , C08L65/00 , C09K11/06 , C09K2211/1416 , C09K2211/1433 , H01L51/0035 , H01L51/0037 , H01L51/0039 , H01L51/5012 , H05B33/14 , Y10S428/917
摘要： A copolymer has a polystyrene reduced number average molecular weight of 103-108, and includes repeating units represented by formulas (1), (2), and (3), —Ar1— (3) The copolymer has an excellent solubility in an organic solvent, and a high glass transition temperature in good valance. Further, a polymer LED has high performance, such as low-voltage driving and high luminance.
摘要翻译：共聚物的聚苯乙烯换算数均分子量为10 -3 -10 8，并且包括由式（1），（2）和（3）表示的重复单元， -Ar 1 - （3）共聚物在有机溶剂中的溶解性优异，玻璃化转变温度高。此外，聚合物LED具有高性能，例如低电压驱动和高亮度。

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