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1. 发明授权

EP1816112B1 Method of forming a ceramic to ceramic joint 有权
标题翻译：一种用于形成陶瓷 - 陶瓷的接合方法
公开(公告)号：EP1816112B1
公开(公告)日：2014-03-05
申请号：EP07250176.0
申请日：2007-01-17
申请人： Air Products and Chemicals, Inc. , Ceramatec, Inc.
发明人： Cutler, Raymond Ashton , Kleinlein, Brian Paul , Hutchings, Kent Neal , Carolan, Michael Francis
IPC分类号： C04B37/00 , B32B18/00
CPC分类号： C04B35/6261 , B32B2315/02 , C04B35/01 , C04B35/2641 , C04B35/6264 , C04B35/6342 , C04B37/005 , C04B37/008 , C04B2235/3208 , C04B2235/3227 , C04B2235/3275 , C04B2235/5409 , C04B2235/6025 , C04B2235/6562 , C04B2235/6565 , C04B2235/79 , C04B2235/94 , C04B2237/04 , C04B2237/06 , C04B2237/064 , C04B2237/068 , C04B2237/34 , C04B2237/343 , C04B2237/348

2. 发明公开

EP1816112A3 Method of forming a ceramic to ceramic joint 有权
标题翻译：一种用于形成陶瓷 - 陶瓷的接合方法
公开(公告)号：EP1816112A3
公开(公告)日：2010-08-04
申请号：EP07250176.0
申请日：2007-01-17
申请人： Air Products and Chemicals, Inc. , Ceramatec, Inc.
发明人： Cutler, Raymond Ashton , Kleinlein, Brian Paul , Hutchings, Kent Neal , Carolan, Michael Francis
IPC分类号： C04B37/00 , B32B18/00
CPC分类号： C04B35/6261 , B32B2315/02 , C04B35/01 , C04B35/2641 , C04B35/6264 , C04B35/6342 , C04B37/005 , C04B37/008 , C04B2235/3208 , C04B2235/3227 , C04B2235/3275 , C04B2235/5409 , C04B2235/6025 , C04B2235/6562 , C04B2235/6565 , C04B2235/79 , C04B2235/94 , C04B2237/04 , C04B2237/06 , C04B2237/064 , C04B2237/068 , C04B2237/34 , C04B2237/343 , C04B2237/348
摘要： A method of joining at least two sintered bodies to form a composite structure includes: providing a joint material between joining surfaces of first and second sintered bodies; applying pressure from 1 kPa to less than 5 MPa to provide an assembly; heating the assembly to a conforming temperature sufficient to allow the joint material to conform to the joining surfaces; and further heating the assembly to a joining temperature below a minimum sintering temperature of the first and second sintered bodies. The joint material includes organic component(s) and ceramic particles. The ceramic particles constitute 40-75 vol.% of the joint material, and include at least one element of the first and/or second sintered bodies. Composite structures produced by the method are also disclosed.

3. 发明公开

EP1816112A2 Method of forming a ceramic to ceramic joint 有权
标题翻译： Verfahren zur Bildung einer Keramik-Keramik-Verbindung
公开(公告)号：EP1816112A2
公开(公告)日：2007-08-08
申请号：EP07250176.0
申请日：2007-01-17
申请人： Air Products and Chemicals, Inc. , CERAMATEC, INC.
发明人： Cutler, Raymond Ashton , Kleinlein, Brian Paul , Hutchings, Kent Neal , Carolan, Michael Francis
IPC分类号： C04B37/00 , B32B18/00
CPC分类号： C04B35/6261 , B32B2315/02 , C04B35/01 , C04B35/2641 , C04B35/6264 , C04B35/6342 , C04B37/005 , C04B37/008 , C04B2235/3208 , C04B2235/3227 , C04B2235/3275 , C04B2235/5409 , C04B2235/6025 , C04B2235/6562 , C04B2235/6565 , C04B2235/79 , C04B2235/94 , C04B2237/04 , C04B2237/06 , C04B2237/064 , C04B2237/068 , C04B2237/34 , C04B2237/343 , C04B2237/348
摘要： A method of joining at least two sintered bodies to form a composite structure includes: providing a joint material between joining surfaces of first and second sintered bodies; applying pressure from 1 kPa to less than 5 MPa to provide an assembly; heating the assembly to a conforming temperature sufficient to allow the joint material to conform to the joining surfaces; and further heating the assembly to a joining temperature below a minimum sintering temperature of the first and second sintered bodies. The joint material includes organic component(s) and ceramic particles. The ceramic particles constitute 40-75 vol.% of the joint material, and include at least one element of the first and/or second sintered bodies. Composite structures produced by the method are also disclosed.
摘要翻译：连接至少两个烧结体以形成复合结构的方法包括：在第一和第二烧结体的接合表面之间提供接合材料; 施加1kPa至小于5MPa的压力以提供组件; 将组件加热到足以允许接头材料与接合表面一致的适形温度; 并且进一步将组件加热到低于第一和第二烧结体的最小烧结温度的接合温度。接头材料包括有机组分和陶瓷颗粒。陶瓷颗粒构成接合材料的40-75体积％，并且包括第一和/或第二烧结体的至少一种元素。还公开了通过该方法生产的复合结构。

4. 发明公开

EP1466693A2 Method of joining ITM materials using a partially- or fully-transient liquid phase 有权
标题翻译：一种用于使用部分或完全瞬态液相接合材料ITM方法
公开(公告)号：EP1466693A2
公开(公告)日：2004-10-13
申请号：EP04006693.8
申请日：2004-03-19
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Butt, Darryl P. , Rynders, Steven Walton , Cutler, Raymond Ashton , Carolan, Michael Francis
IPC分类号： B23K20/22
CPC分类号： B01D53/228 , B01D2256/12 , B23K35/001 , C04B35/01 , C04B37/005 , C04B2235/3208 , C04B2235/3213 , C04B2235/3215 , C04B2235/3227 , C04B2235/3272 , C04B2235/3281 , C04B2235/6025 , C04B2235/656 , C04B2235/6562 , C04B2235/6565 , C04B2235/6567 , C04B2235/76 , C04B2237/06 , C04B2237/34 , Y10T428/24926 , Y10T428/249953
摘要： A method of forming a composite structure includes: (1) providing first and second sintered bodies containing first and second multicomponent metallic oxides having first and second identical crystal structures that are perovskitic or fluoritic; (2) providing a joint material containing at least one metal oxide: (a) containing (i) at least one metal of an identical IUPAC Group as at least one sintered body metal in one of the multicomponent metallic oxides, (ii) a first row D-Block transition metal not contained in the multicomponent metallic oxides, and/or (iii) a lanthanide not contained in the multicomponent metallic oxides; (b) free of metals contained in the multicomponent metallic oxides; (c) free of cations of boron, silicon, germanium, tin, lead, arsenic, antimony, phosphorus and tellurium; and (d) having a melting point below the sintering temperatures of the sintered bodies; and (3) heating to a joining temperature above the melting point and below the sintering temperatures.
摘要翻译：形成复合结构的方法，包括：（1）提供包含具有第一和第二相同的晶体结构也是perovskitic或fluoritic第一和第二多组分金属氧化物的第一和第二烧结体; （2）提供含有至少一种金属氧化物的接合材料：（a）包含（ⅰ）相同的IUPAC族中的至少一种金属的至少一个烧结体金属的多组分金属氧化物中的一种，（ii）第一行D挡过渡金属不包含在多组分金属氧化物，和/或（iii）不包含在多组分金属氧化物的镧系元素; （B）自由包含在多组分金属氧化物的金属; （C）游离的硼，硅，锗，锡，铅，砷，锑，磷和碲阳离子; 和具有低于烧结体的烧结温度的熔点（D）; 和（3）加热到高于熔化接合点和低于烧结温度的温度。

5. 发明公开

EP1466694A3 Method of forming a joint 有权
标题翻译：一种制造接缝的方法
公开(公告)号：EP1466694A3
公开(公告)日：2009-08-26
申请号：EP04006694.6
申请日：2004-03-19
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Butt, Darryl P. , Rynders, Steven Walton , Cutler, Raymond Ashton , Carolan, Michael Francis
IPC分类号： B23K20/22
CPC分类号： B01D53/228 , B01D2256/12 , B23K35/001 , C04B35/01 , C04B37/005 , C04B2235/3208 , C04B2235/3213 , C04B2235/3215 , C04B2235/3227 , C04B2235/3272 , C04B2235/3281 , C04B2235/6025 , C04B2235/656 , C04B2235/6562 , C04B2235/6565 , C04B2235/6567 , C04B2235/76 , C04B2237/06 , C04B2237/34
摘要： A method of joining at least two sintered bodies to form a composite structure, including providing a first multicomponent metallic oxide having a perovskitic or fluorite crystal structure; providing a second sintered body including a second multicomponent metallic oxide having a crystal structure of the same type as the first; and providing at an interface a joint material containing at least one metal oxide containing at least one metal identically contained in at least one of the first and second multicomponent metallic oxides. The joint material is free of cations of Si, Ge, Sn, Pb, P and Te and has a melting point below the sintering temperatures of both sintered bodies. The joint material is heated to a temperature above the melting point of the metal oxide(s) and below the sintering temperatures of the sintered bodies to form the joint. Structures containing such joints are also disclosed.

6. 发明授权

EP1254862B1 Ceria based solid electrolytes 有权
标题翻译：含有固体电解质的氧化铈
公开(公告)号：EP1254862B1
公开(公告)日：2006-01-04
申请号：EP02009246.6
申请日：2002-04-26
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Cutler, Raymond Ashton , Richards, Robin Edward
IPC分类号： C01G23/00 , H01M8/12 , C01F17/00
CPC分类号： B01D53/326 , C01G23/002 , C01G23/006 , C01P2006/10 , H01M8/126 , Y02E60/525 , Y02P70/56

7. 发明授权

EP1466694B1 Method of forming a joint 有权
标题翻译：一种制造接缝的方法
公开(公告)号：EP1466694B1
公开(公告)日：2012-10-31
申请号：EP04006694.6
申请日：2004-03-19
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Butt, Darryl P. , Rynders, Steven Walton , Cutler, Raymond Ashton , Carolan, Michael Francis
IPC分类号： C04B35/01 , C04B37/00 , B01D53/22 , B01D69/10 , B01D69/12 , B01D71/02
CPC分类号： B01D53/228 , B01D2256/12 , B23K35/001 , C04B35/01 , C04B37/005 , C04B2235/3208 , C04B2235/3213 , C04B2235/3215 , C04B2235/3227 , C04B2235/3272 , C04B2235/3281 , C04B2235/6025 , C04B2235/656 , C04B2235/6562 , C04B2235/6565 , C04B2235/6567 , C04B2235/76 , C04B2237/06 , C04B2237/34

8. 发明公开

EP1254862A3 Ceria based solid electrolytes 有权
标题翻译：含有固体电解质的氧化铈
公开(公告)号：EP1254862A3
公开(公告)日：2003-09-17
申请号：EP02009246.6
申请日：2002-04-26
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Cutler, Raymond Ashton , Richards, Robin Edward
IPC分类号： C01G23/00 , H01M8/12 , C01F17/00
CPC分类号： B01D53/326 , C01G23/002 , C01G23/006 , C01P2006/10 , H01M8/126 , Y02E60/525 , Y02P70/56
摘要： The present invention relates to compositions of matter represented by the general formulaLn x Ln' x' A y Ti z Ce 1-x-x'-y-z O 2-δ wherein Ln is selected from the group consisting of Sm, Gd, Y, and mixtures thereof; Ln' is selected from the group consisting of La, Pr, Nd, Pm, Eu, Tb, Dy, Ho, Er, Tm, Yb, Lu, A is selected from the group consisting of Mg, Ca, Sr and Ba, 0.05 ≤ x ≤ 0.25, 0 ≤ x' ≤ 0.25, 0 ≤ y ≤ 0.03, 0.001 ≤ z ≤ 0.03, 0.05 ≤ x + x' ≤ 0.25, 0.001 ≤ y + z ≤ 0.03, wherein δ is a number which renders the composition of matter charge neutral. The compositions can be formed into sintered bodies suitable for use as solid electrolytes in devices including solid-state oxygen generators. Such sintered bodies have greater than 95% theoretical density at temperatures at or below 1600°C, and can be produced by a solid-state method.

9. 发明公开

EP1254862A2 Ceria based solid electrolytes 有权
标题翻译：三氧化铈enthaltende Festelektrolyte
公开(公告)号：EP1254862A2
公开(公告)日：2002-11-06
申请号：EP02009246.6
申请日：2002-04-26
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Cutler, Raymond Ashton , Richards, Robin Edward
IPC分类号： C01G23/00 , H01M8/12
CPC分类号： B01D53/326 , C01G23/002 , C01G23/006 , C01P2006/10 , H01M8/126 , Y02E60/525 , Y02P70/56
摘要： The present invention relates to compositions of matter represented by the general formula

Ln x Ln' x' A y Ti z Ce 1-x-x'-y-z O 2-δ

wherein Ln is selected from the group consisting of Sm, Gd, Y, and mixtures thereof; Ln' is selected from the group consisting of La, Pr, Nd, Pm, Eu, Tb, Dy, Ho, Er, Tm, Yb, Lu, A is selected from the group consisting of Mg, Ca, Sr and Ba, 0.05 ≤ x ≤ 0.25, 0 ≤ x' ≤ 0.25, 0 ≤ y ≤ 0.03, 0.001 ≤ z ≤ 0.03, 0.05 ≤ x + x' ≤ 0.25, 0.001 ≤ y + z ≤ 0.03, wherein δ is a number which renders the composition of matter charge neutral. The compositions can be formed into sintered bodies suitable for use as solid electrolytes in devices including solid-state oxygen generators. Such sintered bodies have greater than 95% theoretical density at temperatures at or below 1600°C, and can be produced by a solid-state method.
摘要翻译：本发明涉及由通式LnxLn'x'AyTizCe1-x-x'-y-zO2-delta表示的物质组合物，其中Ln选自Sm，Gd，Y及其混合物; Ln'选自La，Pr，Nd，Pm，Eu，Tb，Dy，Ho，Er，Tm，Yb，Lu，A选自Mg，Ca，Sr和Ba，0.05 ≤x≤0.25,0≤x≤0.0,0≤y≤0.03,0.001≤z≤0.03,0.05≤x+x≤0.25,0.001≤y+z≤0.03，其中δ是使组成的物质电荷中性。组合物可以形成为适合用作固体氧气发生器的装置中的固体电解质的烧结体。这种烧结体在等于或低于1600℃的温度下具有大于95％的理论密度，并且可以通过固态方法制备。

10. 发明授权

EP0834950B1 Planar solid electrolyte cell stack working as oxygen pump, with offset seals and biasing electrodes 失效
标题翻译：具有极化电极和偏置的密封件，工作作为氧泵扁平固体电解质型燃料电池
公开(公告)号：EP0834950B1
公开(公告)日：2000-01-26
申请号：EP97116357.1
申请日：1997-09-19
申请人： AIR PRODUCTS AND CHEMICALS, INC.
发明人： Adler, Stuart , Cutler, Raymond Ashton , Henderson, Brett Tamatea , Ludlow, Jimmy , Richards, Robin Edward , Taylor, Dale M. , Wilson, Merrill Anderson
IPC分类号： H01M8/24 , H01M8/12 , B01D53/32 , C03C10/00 , C04B35/20 , C04B35/443
CPC分类号： H01M8/0271 , B01D53/326 , B01D2257/104 , C01B13/0251 , C01B2210/0046 , C01B2210/0082 , C04B35/053

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