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1. 发明授权

US08859717B2 Nitrogen-containing fused ring compound, nitrogen-containing fused ring polymer, organic thin film, and organic thin film element 有权
标题翻译：含氮稠环化合物，含氮稠环聚合物，有机薄膜和有机薄膜元素
公开(公告)号：US08859717B2
公开(公告)日：2014-10-14
申请号：US13582246
申请日：2011-03-03
申请人： Yutaka Ie , Masashi Ueta , Yoshio Aso , Masato Ueda
发明人： Yutaka Ie , Masashi Ueta , Yoshio Aso , Masato Ueda
IPC分类号： C08G75/00 , C07D513/14 , C07D513/04 , H01L51/00 , H01L51/05
CPC分类号： H01L51/0036 , C07D513/04 , C07D513/14 , H01L51/0541 , H01L51/0545 , Y02E10/549
摘要： Nitrogen-containing fused ring compound having at least one structural unit selected from the group consisting of a structural unit represented by the formula (1-1) and a structural unit represented by the formula (1-2).
摘要翻译：具有选自由式（1-1）表示的结构单元和式（1-2）表示的结构单元的至少一种结构单元的含氮稠环化合物。

2. 发明申请

US20120091437A1 POLYMER, ORGANIC THIN FILM COMPRISING THE POLYMER, AND ORGANIC THIN-FILM ELEMENT INCLUDING SAME 审中-公开
标题翻译：聚合物，包含聚合物的有机薄膜和包括其中的有机薄膜元件
公开(公告)号：US20120091437A1
公开(公告)日：2012-04-19
申请号：US13255681
申请日：2010-03-08
申请人： Yutaka Ie , Atsuki Yoshimura , Yoshio Aso , Masato Ueda
发明人： Yutaka Ie , Atsuki Yoshimura , Yoshio Aso , Masato Ueda
IPC分类号： H01L51/10 , C07D409/14 , C09D147/00 , C07D333/78 , C08F128/06 , C08F14/18
CPC分类号： H01L51/004 , C08G61/04 , C08G2261/149 , C08G2261/15 , C08G2261/419 , C08G2261/92 , H01L51/0068 , H01L51/0074 , H01L51/0541 , H01L51/0545 , H01L51/0558 , Y02E10/549
摘要： An object of the present invention is to provide a polymer having a low LUMO, a high charge transport property, and further high solubility in a solvent. The present invention provides a polymer having a repeating unit represented by the formula (I): wherein Ar0 means an aromatic ring that may have a substituent or substituents, or a heterocycle that may have a substituent or substituents, and X1 and X2 are the same or different and each mean an oxygen atom or a sulfur atom.
摘要翻译：本发明的目的是提供具有低LUMO，高电荷转移性和在溶剂中进一步高溶解度的聚合物。本发明提供具有式（I）表示的重复单元的聚合物：其中Ar0表示可以具有取代基的芳环或可具有取代基的杂环，X1和X2相同或不同，并且各自表示氧原子或硫原子。

3. 发明申请

US20120056168A1 FLUOROPOLYMER AND THIN ORGANIC FILM COMPRISING SAME 审中-公开
标题翻译：氟聚合物和含有薄膜的有机薄膜
公开(公告)号：US20120056168A1
公开(公告)日：2012-03-08
申请号：US13255669
申请日：2010-03-08
申请人： Yutaka Ie , Masashi Nitani , Yoshio Aso , Masato Ueda
发明人： Yutaka Ie , Masashi Nitani , Yoshio Aso , Masato Ueda
IPC分类号： H01L51/30 , C08G75/06
CPC分类号： H01L51/0036 , C08G61/126 , C08G2261/1428 , C08G2261/146 , C08G2261/512 , C08G2261/92 , C09B69/109 , H01L51/0545 , Y02E10/549
摘要： An object of the invention is to provide a fluorine-containing polymer that is superior in both stability against doping of oxygen and solubility in an organic solvent. The invention provides a fluorine-containing polymer including a structure represented by formula (I) in a repeating unit. wherein R1 and R2 are the same or different and each mean a hydrogen atom, a halogen atom, or a monovalent group.
摘要翻译：本发明的目的是提供一种在掺入氧气的稳定性和在有机溶剂中的溶解度方面优异的含氟聚合物。本发明提供了包含由式（I）表示的结构的含氟聚合物的重复单元。其中R1和R2相同或不同，均为氢原子，卤素原子或一价基团。

4. 发明申请

US20120049174A1 CONJUGATED COMPOUND, AND ORGANIC THIN FILM AND ORGANIC THIN FILM ELEMENT EACH COMPRISING SAME 审中-公开
标题翻译：共轭化合物，有机薄膜和有机薄膜元件
公开(公告)号：US20120049174A1
公开(公告)日：2012-03-01
申请号：US13255373
申请日：2010-03-10
申请人： Yutaka Ie , Makoto Okabe , Yoshio Aso , Masato Ueda
发明人： Yutaka Ie , Makoto Okabe , Yoshio Aso , Masato Ueda
IPC分类号： H01L51/30 , C07D409/10 , C07D495/04 , C07D409/14 , C07D333/78
CPC分类号： H01L51/0068 , C07D333/78 , C07D495/04 , C07D495/14 , C09B3/78 , C09B23/0058 , C09B23/04 , C09B57/00 , C09B57/001 , H01L51/0036 , H01L51/0051 , H01L51/0074 , H01L51/008 , H01L51/0541 , Y02E10/549
摘要： A conjugated compound having a group represented by formula (I) and/or formula (II). [In the formulas, Ar represents an optionally substituted trivalent aromatic hydrocarbon or optionally substituted trivalent heterocyclic group, and A represents hydrogen, a halogen atom or a monovalent group. When multiple A groups are present they may be the same or different, and at least one A represents an electron-withdrawing group. Ar′ represents an optionally substituted C6 or greater divalent aromatic hydrocarbon or optionally substituted C4 or greater divalent heterocyclic group, and R1 and R2 are the same or different and each represents hydrogen, a halogen atom or a monovalent group, while A′ represents hydrogen, a halogen atom or a monovalent group. When multiple A′ groups are present they may be the same or different, and at least one A′ represents an electron-withdrawing group.]
摘要翻译：具有由式（I）和/或式（II）表示的基团的共轭化合物。 [式中，Ar表示任意取代的3价芳香族烃或任意取代的3价杂环基，A表示氢原子，卤原子或1价基团。当存在多个A基团时，它们可以相同或不同，并且至少一个A表示吸电子基团。 Ar'表示任选取代的C 6以上的二价芳香族烃或任选取代的C 4以上的2价杂环基，R 1和R 2相同或不同，分别表示氢原子，卤素原子或一价基团，A'表示氢原子，卤素原子或一价基团。当存在多个A'基团时，它们可以相同或不同，并且至少一个A'表示吸电子基团。

5. 发明授权

US08008336B2 Condensation compound between fluorinated cyclopentane ring and aromatic ring, and process for producing the same 失效
标题翻译：氟化环戊烷环和芳环之间的缩合化合物及其制备方法
公开(公告)号：US08008336B2
公开(公告)日：2011-08-30
申请号：US11885913
申请日：2006-03-02
申请人： Yutaka Ie , Yoshio Aso
发明人： Yutaka Ie , Yoshio Aso
IPC分类号： A61K31/409 , C07D495/22
CPC分类号： C07D495/20 , C07D333/78 , H01L51/0036
摘要： A condensation compound of a fluorinated cyclopentane ring and an aromatic ring, which is useful, for example, for electronic materials, and a process for producing the same are provided. For instance, according to Scheme 1 below, a compound (68) containing a condensed structure formed of a hexafluorocyclopentane ring and an aromatic ring is synthesized. The aromatic ring is not limited to a thiophene ring but can be any ring and any substituent can be used. Thus a compound containing a condensed ring structure formed of a hexafluorocyclopentane ring and an aromatic ring, particularly, for instance, a thiophene ring, which was impossible to produce conventionally, can be produced easily with high yield. The compound of the present invention is particularly suitable to be applied to, for example, electronic materials or semiconductors. When it is polymerized and thereby the π-electronic conjugation is extended, it also is expected to be applied to, for example, n-type organic semiconductors and molecular wires that are indispensable for developing molecular electronics elements.
摘要翻译：提供氟化环戊烷环和芳环的缩合化合物，其可用于例如电子材料，以及其制备方法。例如，根据下述方案1，合成含有由六氟环戊烷环和芳香环形成的稠合结构的化合物（68）。芳环不限于噻吩环，而是可以是任何环，并且可以使用任何取代基。因此，可以容易地以高产率制备含有由六氟环戊烷环和芳环形成的稠环结构的化合物，特别是例如噻吩环，这是不可能制备的。本发明的化合物特别适用于例如电子材料或半导体。当其被聚合并由此延长了电子共轭时，也可以应用于例如用于开发分子电子元件不可或缺的n型有机半导体和分子线。

6. 发明授权

US07932347B2 Polymer comprising unit comprising fluorocyclopentane ring fused with aromatic ring and organic thin film and organic thin film element both comprising the same 失效
标题翻译：包含与芳环稠合的氟环戊烷环和有机薄膜的聚合物，其均包含它们
公开(公告)号：US07932347B2
公开(公告)日：2011-04-26
申请号：US12066006
申请日：2006-08-28
申请人： Yutaka Ie , Yoshio Aso , Yoshikazu Umemoto , Masato Ueda
发明人： Yutaka Ie , Yoshio Aso , Yoshikazu Umemoto , Masato Ueda
IPC分类号： C08G75/00
CPC分类号： H01L51/0036 , C07D333/78 , C08G61/12 , C08G61/126 , C08G2261/146 , C08G2261/3223 , C08G2261/414 , H01L51/0035 , H01L51/0039 , H01L51/0043 , H01L51/0068 , H01L51/0541 , H01L51/0545 , H01L51/4206 , Y02E10/549
摘要： A polymer comprising a repeating unit represented by the following general formula (I). (In the formula, Ar1 represents a divalent aromatic hydrocarbon or divalent heterocyclic group, X1, Y1, X2 and Y2 each independently represent a fluorine atom or alkylthio group, and X1 and Y1 and X2 and Y2 may together form a carbonyl or thiocarbonyl group with their bonding carbon atom.)
摘要翻译：一种包含由以下通式（I）表示的重复单元的聚合物。（式中，Ar 1表示二价芳香族烃或二价杂环基，X 1，Y 1，X 2，Y 2各自独立地表示氟原子或烷硫基，X 1，Y 1，X 2和Y 2可以一起形成羰基或硫代羰基，它们的键合碳原子）

7. 发明申请

US20100301314A1 CONJUGATED COMPOUND, NITROGENATED CONDENSED-RING COMPOUND, NITROGENATED CONDENSED-RING POLYMER, ORGANIC THIN FILM, AND ORGANIC THIN FILM ELEMENT 失效
标题翻译：连结化合物，氮化聚合环化合物，氮化聚合物聚合物，有机薄膜和有机薄膜元件
公开(公告)号：US20100301314A1
公开(公告)日：2010-12-02
申请号：US12745481
申请日：2008-11-27
申请人： Yoshio Aso , Yutaka Ie , Makoto Okabe , Masashi Nitani , Masato Ueda
发明人： Yoshio Aso , Yutaka Ie , Makoto Okabe , Masashi Nitani , Masato Ueda
IPC分类号： H01L51/30 , C07D513/04 , C07D513/20 , C07D411/14
CPC分类号： H01L51/0069 , C07D277/60 , C07D333/22 , C07D333/78 , C07D409/14 , C07D417/14 , C09B3/78 , C09B57/00 , C09B57/001 , H01L51/0036 , H01L51/0558 , Y02E10/549
摘要： According to the first invention group there are provided conjugated compounds having two or more groups represented by the following formula (I) or the following formula (II): wherein one of Ar and Ar′ represents a C6 or greater divalent aromatic hydrocarbon group and the other represents a C4 or greater divalent heterocyclic group, wherein the groups each may have a substituent, with the proviso that the groups as a whole contain no fluorine atoms, R1 and R2 each independently represent a hydrogen atom, a halogen atom or a monovalent group, and Ar″ represents a trivalent aromatic hydrocarbon or trivalent heterocyclic group; when the conjugated compound has two or more groups represented by formula (I), the portion excluding these groups contain no fluorine atoms.According to the second group of the present invention there are provided nitrogen-containing fused-ring compounds represented by the following formula (α-I): in formula (α-I), R21 and R22 each independently represent a hydrogen atom, a halogen atom or an optionally substituted monovalent group, and Z21 and Z22 each independently represent any one of the groups represented by the following formulas (α-i)-(α-ix); wherein R23, R24, R25 and R26 each independently represent a hydrogen atom, a halogen atom or a monovalent group, and R23 and R24 may bond together to form a ring, the left side and the right side of the group represented by formula (α-viii) may be interchanged.
摘要翻译：根据第一发明组，提供具有两个以上由下式（I）或下式（II）表示的基团的共轭化合物：其中Ar和Ar'中的一个表示C6以上的二价芳香族烃基，其它表示C4以上的二价杂环基，其中各基团可以具有取代基，条件是基团整体上不含氟原子，R 1和R 2各自独立地表示氢原子，卤素原子或一价基团，Ar“表示三价芳香族烃或三价杂环基; 当共轭化合物具有两个以上由式（I）表示的基团时，不包括这些基团的部分不含氟原子。根据本发明的第二组，提供由下式（α-I）表示的含氮稠环化合物：在式（α-I）中，R 21和R 22各自独立地表示氢原子，卤素原子或任选取代的一价基团，Z 21和Z 22各自独立地表示由下式（α-i） - （α-ix）表示的基团中的任一个。其中R 23，R 24，R 25和R 26各自独立地表示氢原子，卤素原子或一价基团，R 23和R 24可以键合在一起形成环，式（α）表示的基团的左侧和右侧 -viii）可以互换。

8. 发明授权

US5185204A Agglomerate of whiskers or short fibers 失效
标题翻译：织物或短纤维
公开(公告)号：US5185204A
公开(公告)日：1993-02-09
申请号：US539626
申请日：1990-06-18
申请人： Tadao Shimizu , Yoshio Aso , Hidefumi Konnai
发明人： Tadao Shimizu , Yoshio Aso , Hidefumi Konnai
IPC分类号： C04B14/38 , C04B18/02 , C08K7/02 , C30B29/62
CPC分类号： C08K7/02 , C04B18/02 , Y10S428/903 , Y10T428/29 , Y10T428/2982
摘要： Whiskers having a diameter of 0.1-10 .mu.m and a length of 5-200 .mu.m are pelletized and granulated into agglomerates which have a size of 0.1-10 mm and a bulk density of 0.2-1.0 kg/liter.To pelletize, powders of whiskers are moistened with water while mixing to form primary aggregates. Then, the powders and the primary aggregates are subjected to a rolling movement to cause the primary aggregates to grow into secondary aggregates having desired size distribution. Finally, the secondary aggregates are dried to obtain pelletized or granulated agglomerates of whiskers.Handling of whiskers is facilitated because the agglomerates are less bulky and less likely to fly up in the air. When blended into molding materials for fiber reinforcement, however, the agglomerates are readily disintegrated back into separated individual fibers to provide homogeneous dispersion.

9. 发明申请

US20130324685A1 NITROGEN-CONTAINING CONDENSED RING COMPOUND, NITROGEN-CONTAINING CONDENSED RING POLYMER, ORGANIC THIN FILM, AND ORGANIC THIN FILM ELEMENT 有权
标题翻译：含氮聚合环化合物，含氮聚合环聚合物，有机薄膜和有机薄膜元件
公开(公告)号：US20130324685A1
公开(公告)日：2013-12-05
申请号：US13982410
申请日：2012-01-30
申请人： Yoshio Aso , Yutaka Ie , Masashi Ueta , Masato Ueda
发明人： Yoshio Aso , Yutaka Ie , Masashi Ueta , Masato Ueda
IPC分类号： H01L51/00
CPC分类号： H01L51/0071 , C07D513/04 , C07D513/14 , C08G61/123 , C08G61/126 , C08G2261/124 , C08G2261/3142 , C08G2261/3223 , C08G2261/3243 , C08G2261/3246 , C08G2261/3327 , C08G2261/3328 , C08G2261/414 , C08G2261/514 , H01L51/0036 , H01L51/0043 , H01L51/0541 , H01L51/0545 , Y02E10/549
摘要： It is an object of the present invention to provide a nitrogen-containing condensed ring compound, which can be used as an organic n-type semiconductor having an excellent electron transport property and which is also excellent in terms of solubility in an organic solvent. The nitrogen-containing condensed ring compound of the present invention has a structural unit represented by the following formula (1-1) or formula (1-2): wherein Ar1 represents an aromatic ring; one of Y1 and Y2 represents a single bond, and the other represents —C(R11)(R12)— or —C(═X1)—; one of Y3 and Y4 represents a single bond, and the other represents —C(R21)(R22)— or —C(═X2)—, and one of Y1 to Y4 represents —C(R11)(R12)— or —C(R21)(R22)—; at least one of W1 and W2 represents —N═; and Z1 and Z2 each represent any one of the groups represented by the formula (i) to the formula (ix).
摘要翻译：本发明的目的是提供一种含氮稠环化合物，其可以用作具有优异的电子传输性质的有机n型半导体，并且在有机溶剂中的溶解性也优异。本发明的含氮缩环化合物具有由下式（1-1）或式（1-2）表示的结构单元：其中Ar 1表示芳环; Y1和Y2之一表示单键，另一个表示-C（R 11）（R 12） - 或-C（= X 1） - ; Y 3和Y 4之一表示单键，另一个表示-C（R 21）（R 22） - 或-C（= X 2） - ，Y 1至Y 4中的一个表示-C（R 11）（R 12） - 或 - C（R 21）（R 22） - ; W1和W2中的至少一个表示-N =; 并且Z 1和Z 2各自表示由式（i）至式（ix）表示的基团中的任何一个。

10. 发明授权

US08378338B2 Conjugated compound, nitrogenated condensed-ring compound, nitrogenated condensed-ring polymer, organic thin film, and organic thin film element 失效
标题翻译：共轭化合物，氮化稠环化合物，氮化缩合环聚合物，有机薄膜和有机薄膜元件
公开(公告)号：US08378338B2
公开(公告)日：2013-02-19
申请号：US12745481
申请日：2008-11-27
申请人： Yoshio Aso , Yutaka Ie , Makoto Okabe , Masashi Nitani , Masato Ueda
发明人： Yoshio Aso , Yutaka Ie , Makoto Okabe , Masashi Nitani , Masato Ueda
IPC分类号： H01L29/08
CPC分类号： H01L51/0069 , C07D277/60 , C07D333/22 , C07D333/78 , C07D409/14 , C07D417/14 , C09B3/78 , C09B57/00 , C09B57/001 , H01L51/0036 , H01L51/0558 , Y02E10/549
摘要： According to the first invention group there are provided conjugated compounds having two or more groups represented by the following formula (I) or the following formula (II): wherein one of Ar and Ar′ represents a C6 or greater divalent aromatic hydrocarbon group and the other represents a C4 or greater divalent heterocyclic group, wherein the groups each may have a substituent, with the proviso that the groups as a whole contain no fluorine atoms, R1 and R2 each independently represent a hydrogen atom, a halogen atom or a monovalent group, and Ar″ represents a trivalent aromatic hydrocarbon or trivalent heterocyclic group; when the conjugated compound has two or more groups represented by formula (I), the portion excluding these groups contain no fluorine atoms. According to the second group of the present invention there are provided nitrogen-containing fused-ring compounds represented by the following formula (α-I): in formula (α-I), R21 and R22 each independently represent a hydrogen atom, a halogen atom or an optionally substituted monovalent group, and Z21 and Z22 each independently represent any one of the groups represented by the following formulas (α-i)-(α-ix); wherein R23, R24, R25 and R26 each independently represent a hydrogen atom, a halogen atom or a monovalent group, and R23 and R24 may bond together to form a ring, the left side and the right side of the group represented by formula (α-viii) may be interchanged.
摘要翻译：根据第一发明组，提供具有两个以上由下式（I）或下式（II）表示的基团的共轭化合物：其中Ar和Ar'中的一个表示C6以上的二价芳香族烃基，其它表示C4以上的二价杂环基，其中各基团可以具有取代基，条件是基团整体上不含氟原子，R 1和R 2各自独立地表示氢原子，卤素原子或一价基团，Ar“表示三价芳香族烃或三价杂环基; 当共轭化合物具有两个以上由式（I）表示的基团时，不包括这些基团的部分不含氟原子。根据本发明的第二组，提供由下式（α-I）表示的含氮稠环化合物：在式（α-I）中，R 21和R 22各自独立地表示氢原子，卤素原子或任选取代的一价基团，Z 21和Z 22各自独立地表示由下式（α-i） - （α-ix）表示的基团中的任一个。其中R 23，R 24，R 25和R 26各自独立地表示氢原子，卤素原子或一价基团，R 23和R 24可以键合在一起形成环，式（α）表示的基团的左侧和右侧 -viii）可以互换。

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