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1. 发明授权

US09267037B2 Silicone composite particles, making method, and cosmetic composition 有权
标题翻译：有机硅复合颗粒，制作方法和化妆品组成
公开(公告)号：US09267037B2
公开(公告)日：2016-02-23
申请号：US12943166
申请日：2010-11-10
申请人： Yoshinori Inokuchi , Ryuichi Inaba
发明人： Yoshinori Inokuchi , Ryuichi Inaba
IPC分类号： A61K8/58 , C08L83/04 , A61K8/19 , A61K8/27 , A61K8/29 , A61K8/891 , A61Q15/00 , A61Q17/00 , A61Q17/04 , C08J3/12 , C08G77/12 , C08G77/20
CPC分类号： C08L83/04 , A61K8/19 , A61K8/27 , A61K8/29 , A61K8/891 , A61K2800/412 , A61K2800/413 , A61Q15/00 , A61Q17/005 , A61Q17/04 , C08G77/12 , C08G77/20 , C08J3/12 , C08J3/128 , C08J2383/04 , C08L83/00
摘要： Silicone composite particles are provided in which silicone elastomer spherical particles having a volume average particle size of 0.1-100 μm are coated with an organosilsesquioxane-based silicone resin containing inorganic nano-particles having a volume average particle size of up to 100 nm. The silicone composite particles are compounded in a cosmetic composition to exert a UV screening effect or bactericidal property inherent to inorganic nano-particles and to impart a pleasant feel on use. A preparing method and a cosmetic composition are also provided.
摘要翻译：提供了一种硅酮复合颗粒，其中体积平均粒度为0.1-100μm的硅氧烷弹性体球形颗粒用含有体积平均粒度高达100nm的无机纳米颗粒的有机倍半硅氧烷基硅树脂涂覆。将有机硅复合颗粒复合在化妆品组合物中以发挥无机纳米颗粒固有的紫外线屏蔽效果或杀菌性能，并赋予使用愉悦感。还提供了制备方法和化妆品组合物。

2. 发明授权

US08389118B2 Cosmetic 有权
标题翻译：化妆品
公开(公告)号：US08389118B2
公开(公告)日：2013-03-05
申请号：US12693865
申请日：2010-01-26
申请人： Yoshinori Inokuchi , Ryuichi Inaba , Ryuji Horiguchi
发明人： Yoshinori Inokuchi , Ryuichi Inaba , Ryuji Horiguchi
IPC分类号： B32B5/16
CPC分类号： A61Q1/12 , A61K8/046 , A61K8/585 , A61K8/895 , A61K2800/412 , A61K2800/614 , A61Q1/02 , A61Q1/06 , A61Q1/10 , A61Q3/02 , A61Q15/00 , A61Q17/04 , A61Q19/00 , C08G77/12 , C08G77/20 , C08L83/04 , Y10T428/2991 , Y10T428/2996 , Y10T428/2998
摘要： Provided is a cosmetic including silicone microparticles, in which the silicone microparticles include 100 parts by mass of silicone elastomer spherical microparticles having a volume average particle diameter within a range from 0.1 to 100 μm, and 0.5 to 25 parts by mass of a polyorganosilsesquioxane that coats a surface of the silicone elastomer spherical microparticles, and the silicone elastomer is capable of absorbing not less than 30 parts by mass of at least one oily substance selected from the group consisting of sebum, hydrocarbon oils and ester oils per 100 parts by mass of the silicone elastomer. Even if containing an unctuous agent, the cosmetic exhibits favorable feelings upon use, with no spreading difficulties, stickiness, greasiness, oily film feeling, or the like, and is also capable of suppressing problems caused by sebum, namely, changes in the makeup cosmetic properties of the cosmetic, changes in the color of the cosmetic, increased shine, and the like.
摘要翻译：本发明提供一种含有硅微粒的化妆品，其中，硅氧烷微粒包括100质量份体积平均粒径在0.1〜100μm范围内的硅氧烷弹性体球形微粒，以及0.5〜25质量份涂布的聚有机倍半硅氧烷有机硅弹性体球形微粒的表面，并且硅氧烷弹性体每100质量份能够吸收不少于30质量份的选自皮脂，烃油和酯油的至少一种油性物质有机硅弹性体。即使含有挥发性物质，化妆品在使用时表现出良好的感觉，没有传播困难，粘性，油脂，油膜感觉等，并且还能够抑制由皮脂引起的问题，即化妆化妆品的变化化妆品的性质，化妆品的颜色的变化，增加的光泽等。

3. 发明申请

US20100112074A1 SILICONE MICROPARTICLES COMPRISING SILICONE ELASTOMER SPHERICAL MICROPARTICLES COATED WITH POLYORGANOSILSESQUIOXANE, AND METHOD OF PRODUCING SAME 有权
标题翻译：含有聚硅氧烷硅氧烷的硅氧烷弹性体微球的硅氧烷微球及其生产方法
公开(公告)号：US20100112074A1
公开(公告)日：2010-05-06
申请号：US12609429
申请日：2009-10-30
申请人： Yoshinori INOKUCHI , Ryuji Horiguchi
发明人： Yoshinori INOKUCHI , Ryuji Horiguchi
IPC分类号： A61K8/89
CPC分类号： C08J7/047 , A61K8/11 , A61K8/891 , A61K2800/412 , A61Q19/00 , C08J2383/10 , C08J2483/00 , Y10T428/2991 , Y10T428/2996 , Y10T428/2998
摘要： Provided are silicone microparticles including 100 parts by mass of silicone elastomer spherical microparticles having a volume average particle diameter within a range from 0.1 to 100 μm, and 0.5 to 25 parts by mass of a polyorganosilsesquioxane that coats the surface of the silicone elastomer spherical microparticles, in which the silicone elastomer is capable of absorbing not less than 200 parts by mass of a polymethylsiloxane having a viscosity at 25° C. of not more than 10 mm2/s per 100 parts by mass of the silicone elastomer. These silicone microparticles are capable of absorbing a large amount of the above types of polymethylsiloxanes, which represent low-viscosity silicones, and can therefore suppress the greasiness, stickiness, and oily film feeling of cosmetic materials containing this type of polymethylsiloxane. The silicone microparticles can be produced by hydrolyzing and condensing an organotrialkoxysilane in a water medium, in the presence of the above silicone elastomer spherical microparticles and an alkaline material, thereby coating the surface of the silicone elastomer spherical microparticles with a polyorganosilsesquioxane.
摘要翻译：提供了包含100质量份体积平均粒径在0.1〜100μm范围内的硅氧烷弹性体球形微粒和涂覆有机硅弹性体球形微粒表面的聚有机倍半硅氧烷0.5〜25质量份的有机硅微粒，其中有机硅弹性体能够吸收不少于200质量份的在25℃下的粘度为每100质量份硅氧烷弹性体不大于10mm 2 / s的聚甲基硅氧烷。这些硅氧烷微粒能够吸收大量上述类型的代表低粘度硅氧烷的聚甲基硅氧烷，因此可以抑制含有这种聚甲基硅氧烷的化妆品的油性，粘性和油性感觉。有机硅微粒可以通过在水介质中，在上述硅氧烷弹性体球形微粒和碱性物质的存在下水解和缩合有机三烷氧基硅烷来制备，从而用聚有机倍半硅氧烷涂覆硅氧烷弹性体球形微粒的表面。

4. 发明申请

US20100112023A1 SILICONE MICROPARTICLES COMPRISING SILICONE ELASTOMER SPHERICAL MICROPARTICLES COATED WITH POLYORGANOSILSESQUIOXANE, AND METHOD OF PRODUCING SAME 有权
标题翻译：含有聚硅氧烷硅氧烷的硅氧烷弹性体微球的硅氧烷微球及其生产方法
公开(公告)号：US20100112023A1
公开(公告)日：2010-05-06
申请号：US12609524
申请日：2009-10-30
申请人： Yoshinori INOKUCHI , Ryuji Horiguchi
发明人： Yoshinori INOKUCHI , Ryuji Horiguchi
IPC分类号： A61K8/02 , A61K31/74 , A61Q19/10
CPC分类号： C08J7/047 , A61K8/11 , A61K8/891 , A61K2800/412 , A61Q19/00 , C08J2383/10 , C08J2483/00
摘要： Provided are silicone microparticles including 100 parts by mass of silicone elastomer spherical microparticles having a volume average particle diameter within a range from 0.1 to 100 μm, and 0.5 to 25 parts by mass of a polyorganosilsesquioxane that coats the surface of the silicone elastomer spherical microparticles, in which the silicone elastomer is capable of absorbing not less than 30 parts by mass of at least one oily substance selected from the group consisting of sebum, hydrocarbon oils and ester oils per 100 parts by mass of the silicone elastomer. These silicone microparticles are capable of absorbing a large amount of the above oily substances, are able to ameliorate various problems caused by sebum such as changes in cosmetic make-up properties, changes in the color of cosmetic materials and increased shininess of cosmetic materials, and are also able to suppress the greasiness, stickiness, and oily film feeling of cosmetic materials containing at least one of liquid oils composed of hydrocarbon oils and ester oils. The silicone microparticles can be produced by hydrolyzing and condensing an organotrialkoxysilane in a water medium, in the presence of the above silicone elastomer spherical microparticles and an alkaline material, thereby coating the surface of the silicone elastomer spherical microparticles with a polyorganosilsesquioxane.
摘要翻译：提供了包含100质量份体积平均粒径在0.1〜100μm范围内的硅氧烷弹性体球形微粒和涂覆有机硅弹性体球形微粒表面的聚有机倍半硅氧烷0.5〜25质量份的有机硅微粒，其中所述硅氧烷弹性体能够相对于每100质量份硅氧烷弹性体吸收不少于30质量份的选自皮脂，烃油和酯油的至少一种油性物质。这些硅氧烷微粒能够吸收大量的上述油性物质，能够改善由皮脂引起的各种问题，例如化妆品化妆品的变化，化妆品的颜色变化和化妆品的光泽增加，以及也能够抑制含有由烃油和酯油组成的液体油中的至少一种的化妆品的油性，粘性和油性感觉。有机硅微粒可以通过在水介质中，在上述硅氧烷弹性体球形微粒和碱性物质的存在下水解和缩合有机三烷氧基硅烷来制备，从而用聚有机倍半硅氧烷涂覆硅氧烷弹性体球形微粒的表面。

5. 发明申请

US20070059538A1 Coating agent 有权
标题翻译：涂层剂
公开(公告)号：US20070059538A1
公开(公告)日：2007-03-15
申请号：US11515709
申请日：2006-09-05
申请人： Yoshinori Inokuchi
发明人： Yoshinori Inokuchi
IPC分类号： B32B27/40 , C08L83/00 , C08L75/04 , C08G77/00
CPC分类号： C09D183/04 , C09D175/04 , C09D183/08 , Y10T428/31551 , Y10T428/31663 , C08L83/00 , C08L2666/14
摘要： An object of the present invention is to provide a coating agent capable of giving a coating film having excellent adhesion to the base surface, and exhibiting excellent releasability with good surface lubricity. The coating agent comprises a water-base resin composition containing the following components A and B: component A: a curable silicone composition composed of: component (A-1): an organopolysiloxane in which a group selected from among a hydroxyl group and groups represented by the formula R1O— (where R1 is a monovalent hydrocarbon group having 1 to 6 carbon atoms), and a group represented by the following formula (1): are bonded to the same silicon atom at two or more terminals of the polysiloxane chain, component (A-2): an alkoxy silane compound or a partial hydrolysis-condensation product thereof, and component (A-3): a condensation catalyst in an amount of 0 to 10 mass parts per 100 mass parts of the total amount of the components (A-1) and (A-2); and component B: a polyurethane resin.
摘要翻译：本发明的目的是提供一种能够赋予与基材表面优异的粘合性的涂膜的涂布剂，并具有良好的脱模性和良好的表面润滑性。涂层剂包含含有以下组分A和B的水性基础树脂组合物：组分A：由以下组分组成的可固化有机硅组合物：组分（A-1）：其中选自羟基和表示的基团的有机聚硅氧烷由式R 0 O-（其中R 1是具有1至6个碳原子的一价烃基）和由下式（1）表示的基团：（A-2）：烷氧基硅烷化合物或其部分水解缩合产物和组分（A-3）：在聚硅氧烷链的两个或多个末端的相同硅原子上键合：（A-1）和（A-2）的总量为100质量份为0〜10质量份。和组分B：聚氨酯树脂。

6. 发明申请

US20060222870A1 Coating composition for rubber 有权
标题翻译：橡胶涂料组合物
公开(公告)号：US20060222870A1
公开(公告)日：2006-10-05
申请号：US11396463
申请日：2006-04-04
申请人： Yoshinori Inokuchi
发明人： Yoshinori Inokuchi
IPC分类号： B32B25/00 , C08L83/04 , C08L75/04 , C08G77/00
CPC分类号： C09D183/08 , C08K3/24 , C08K5/5425 , C08L75/04 , C08L83/04 , C09D175/16 , Y10T428/31663 , C08L2666/14 , C08L2666/34 , C08L2666/44 , C08L2666/20
摘要： The invention provides a coating composition for rubbers which forms a coating film having excellent adhesion to the rubber surface as well as excellent wear resistance and surface lubricity. The composition is an aqueous resin composition containing 100 parts by weight of the component (A), 10 to 100 parts by weight of the component (B) and 5 to 150 parts by weight of the component (C): wherein the component (A) is a curable silicone composition consisting of (A-1) which is an organopolysiloxane in which a group selected from the group consisting of a hydroxyl group and groups represented by the formula R1O— (R1 is a monovalent hydrocarbon group), and a group represented by the formula (1), below are bonded to each of at least two terminal silicon atoms of a polysiloxane chain: (A-2) which is an alkoxysilane and, optionally, (A-3) which is a metal compound as a condensation catalyst; component (B) which is a polyurethane resin; and component (C) which is an organic resin fine powder having a melting point of 150° C. or higher and an average particle diameter of 0.5 to 50 μm.
摘要翻译：本发明提供一种用于橡胶的涂料组合物，其形成对橡胶表面具有优异粘附性以及优异的耐磨性和表面润滑性的涂膜。该组合物是含有100重量份组分（A），10至100重量份组分（B）和5至150重量份组分（C）的水性树脂组合物：其中组分（A ）是由（A-1）组成的可固化的有机硅组合物，其为有机聚硅氧烷，其中选自羟基和由式R 0表示的基团的基团O- SUP 1是一价烃基），由下式（1）表示的基团与聚硅氧烷链的至少两个末端硅原子键合：（A-2），其为烷氧基硅烷和任选的作为缩合催化剂的金属化合物的（A-3）作为聚氨酯树脂的组分（B）; 和作为熔点为150℃以上，平均粒径为0.5〜50μm的有机树脂细粉末的成分（C）。

7. 发明授权

US06376078B1 Spherical fine particles of silicone resin 失效
标题翻译：硅树脂的球形细颗粒
公开(公告)号：US06376078B1
公开(公告)日：2002-04-23
申请号：US09584964
申请日：2000-06-02
申请人： Yoshinori Inokuchi
发明人： Yoshinori Inokuchi
IPC分类号： B32B516
CPC分类号： C08J3/12 , C08J3/126 , C08J2383/04 , Y10T428/2991 , Y10T428/2995 , Y10T428/2998
摘要： Disclosed are spherical particles of a polyorganosilsesquioxane resin have a unique optical properties when each particle has a core-cladding composite structure consisting of a core portion of, for example, a polymethylsilsesquioxane resin and a cladding layer of, for example, a polyphenylsilsesquioxane resin having refractive indices differing by at least 0.02, the diameter of the core portion being in a specified range relative to the diameter of the whole particle. Such particles of a core-cladding structure can be prepared by conducting the hydrolysis-condensation reaction of organotrialkoxysilanes, e.g., methyl trimethoxysilane and phenyl trimethoxysilane, in two successive steps by using different silane compounds or by using silane mixtures of different mixing proportion in the first and second step reactions.
摘要翻译：公开了聚有机倍半硅氧烷树脂的球形颗粒，当每个颗粒具有由例如聚甲基倍半硅氧烷树脂的芯部分组成的芯包层复合结构和例如具有折射率的聚苯基倍半硅氧烷树脂的包覆层时具有独特的光学性质指数至少为0.02，芯部的直径相对于整个颗粒的直径在特定范围内。芯包层结构的这种颗粒可以通过使用不同的硅烷化合物或通过使用不同混合比例的硅烷混合物在第一个步骤中连续两步进行有机三烷氧基硅烷例如甲基三甲氧基硅烷和苯基三甲氧基硅烷的水解缩合反应来制备和第二步反应。

8. 发明授权

US5871761A Method for the preparation of improved water-base toiletry composition 失效
标题翻译：制备改进的水基化妆品组合物的方法
公开(公告)号：US5871761A
公开(公告)日：1999-02-16
申请号：US928671
申请日：1997-09-12
申请人： Satoshi Kuwata , Morizo Nakazato , Yoshinori Inokuchi
发明人： Satoshi Kuwata , Morizo Nakazato , Yoshinori Inokuchi
IPC分类号： A61K8/04 , A61K8/891 , A61K8/892 , A61K8/895 , A61Q5/00 , A61Q5/02 , A61Q19/00 , A61K6/00 , A61K7/00 , A61K7/06
CPC分类号： A61Q19/00 , A61K8/025 , A61K8/891 , A61K8/895 , A61K2800/412 , A61K2800/81 , A61Q5/00 , A61Q5/02
摘要： Proposed is a reliable method for the preparation of a water-base hair-care or skin-care toiletry preparation capable of imparting the hair or skin of the user with excellent touch feeling of smoothness and sleekness. The method comprises (a) preparing an aqueous dispersion of globular particles of a cured silicone rubber having a specified average particle diameter by the in situ crosslinking hydrosilation reaction in liquid droplets of a vinyl group-containing dimethylpolysiloxane and an organohydrogenpolysiloxane in combination in the presence of a surface active agent and (b) admixing a base mixture consisting of the principal ingredients of a water-base toiletry composition with a specified amount of the aqueous dispersion of the cured silicone rubber particles.
摘要翻译：提出了一种制备能够赋予使用者的头发或皮肤的优异的平滑度和光滑感的水性护发或护肤化妆品制剂的可靠方法。该方法包括：（a）通过在含乙烯基的二甲基聚硅氧烷和有机氢聚硅氧烷的液滴中的原位交联氢化硅烷化合物，在具有特定平均粒径的固化硅橡胶的存在下，表面活性剂和（b）将由水性盥洗用组合物的主要成分组成的碱性混合物与规定量的固化的硅橡胶粒子的水分散液混合。

9. 发明授权

US5149748A Process of preparing surface-modified polymethylsilsesquioxane spherical fine particles 失效
标题翻译：表面改性聚甲基硅氧烷球形细颗粒的制备方法
公开(公告)号：US5149748A
公开(公告)日：1992-09-22
申请号：US450822
申请日：1989-12-14
申请人： Takaaki Shimizu , Toshihiro Okon , Toshio Ohba , Yoshinori Inokuchi
发明人： Takaaki Shimizu , Toshihiro Okon , Toshio Ohba , Yoshinori Inokuchi
IPC分类号： C08G77/06 , C08J3/12
CPC分类号： C08J3/12 , C08G77/06 , C08J2383/04 , Y10T428/2998 , Y10T428/31663
摘要： The surface-modified polymethylsilsesquioxane spherical fine particles of this invention comprise polymethylsilsesquioxane spherical fine particles serving as nuclei, and at least one member of an alkyl group having two or more carbon atoms, an alkenyl group, a phenyl group, an epoxy group, an acryloxy group and an amino group is bonded to the surface of a particle. They are prepared by a process comprising the step of carrying out reaction in an aqueous suspension of polymethylsilsesquioxane fine particles in the presence of an alkali catalyst. The surface-modified spherical fine particles can have various organic groups on their surfaces, and are used in various fields such as rubbers, plastics, coating materials, inks, and cosmetics, depending on the types of the organic groups.

10. 发明授权

US09023473B2 Silicone microparticle and method for producing the same 有权
标题翻译：硅微粒及其制造方法
公开(公告)号：US09023473B2
公开(公告)日：2015-05-05
申请号：US13564336
申请日：2012-08-01
申请人： Yoshinori Inokuchi , Ryuji Horiguchi
发明人： Yoshinori Inokuchi , Ryuji Horiguchi
IPC分类号： B32B27/08 , B05D7/02 , C08L83/04 , A61Q19/00 , A61K8/02 , C08G77/04 , C08G77/12 , C08G77/20 , C08L39/00
CPC分类号： C08L83/04 , A61K8/025 , A61K2800/10 , A61K2800/412 , A61K2800/624 , A61K2800/654 , A61Q19/00 , C08G77/045 , C08G77/12 , C08G77/20 , C08L39/00 , C08L2205/18 , Y10T428/2989 , C08L83/00
摘要： The present invention provides a silicone microparticle, wherein the silicone microparticle comprises 100 parts by mass of a silicone elastomer spherical microparticle having volume-average particle diameter of 0.1 to 100 μm and 0.5 to 25 parts by mass of a polyorganosilsesquioxane to cover surface of the silicone elastomer spherical microparticle, wherein the polyorganosilsesquioxane has a shape of granule with the size thereof being 60 nm or less. There can be provided a silicone microparticle having low agglomerating tendency and excellent dispersibility even if rubber hardness of a silicone elastomer microparticle is low and a particle diameter thereof is small.
摘要翻译：本发明提供一种硅氧烷微粒，其中，硅氧烷微粒包含100质量份体积平均粒径为0.1〜100μm的有机硅弹性体球形微粒和0.5〜25质量份的覆盖硅氧烷的表面的聚有机倍半硅氧烷弹性体球形微粒，其中聚有机倍半硅氧烷具有尺寸为60nm以下的颗粒形状。即使硅酮弹性体微粒的橡胶硬度低，粒径小，也可以提供聚集性低，分散性优异的硅酮微粒。

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