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1. 发明授权

US5106558A Method for continuous preparation of polyethylene material having high strength and high modulus of elasticity 失效
标题翻译：连续制备具有高强度和高弹性模量的聚乙烯材料的方法
公开(公告)号：US5106558A
公开(公告)日：1992-04-21
申请号：US515706
申请日：1990-04-27
申请人： Keizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Keiji Jimbo , Kazuhiko Kurihara , Hiroshi Yazawa , Mihoko Okada
发明人： Keizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Keiji Jimbo , Kazuhiko Kurihara , Hiroshi Yazawa , Mihoko Okada
IPC分类号： B29C43/22 , B29C43/44 , B29C55/00 , B29C55/04 , B29C55/06 , B29C55/18 , B29C69/02 , B29K23/00 , B29L7/00 , C08F4/60 , C08F4/64 , C08F10/02 , C08J3/09 , C08J5/18
CPC分类号： C08J5/18 , B29C55/005 , B29C55/04 , B29C55/18 , C08J3/09 , B29K2023/06 , B29K2023/0683 , C08J2323/04
摘要： A method for the continuous preparation of a polyethylene having high strength and high modulus of elasticity is here disclosed which comprises the steps of mixing 100 parts by weight of an ultra-high-molecular-weight polyethylene powder having an intrinsic viscosity of 5 to 50 dl/g in decalin at 135.degree. C. with 2 to 50 parts by weight of a liquid organic compound having a boiling point higher than the melting point of the polyethylene, feeding the resulting mixture to between a pair of upper and lower endless belts facing each other, continuously compression-molding the mixture at a temperature less than the melting point of the mixture by pressing means disposed inside the endless belts, and rolling and then drawing the same.

2. 发明授权

US5693708A Colored stretched polyethylene material and process for producing the same 失效
标题翻译：彩色拉伸聚乙烯材料及其制造方法
公开(公告)号：US5693708A
公开(公告)日：1997-12-02
申请号：US433954
申请日：1995-05-04
申请人： Yoshimu Iwanami , Seizo Kobayashi , Takashi Mizoe , Osamu Otsu
发明人： Yoshimu Iwanami , Seizo Kobayashi , Takashi Mizoe , Osamu Otsu
IPC分类号： C08K3/00 , B29C43/00 , B29C43/22 , B29C55/00 , B29C55/02 , B29C55/06 , B29C55/18 , B29K23/00 , B29L7/00 , C08K5/00 , C08L23/00 , C08L23/06 , D02J1/22
CPC分类号： B29C43/24 , B29C43/003 , B29C43/22 , B29C43/228 , B29C55/005 , B29C55/06 , B29C55/18 , B29C2043/483 , B29K2023/0683 , B29K2105/0032
摘要： The present invention discloses a colored stretched polyethylene material which comprises an ultra-high-molecular-weight polyethylene having an intrinsic viscosity of 5-50 dl/g in decalin at 135.degree. C. and 0.001-50 parts by weight, per 100 parts by weight of the polyethylene, of a dye and/or a pigment and which has been stretched at a temperature lower than the melting point of the polyethylene, and a process for producing said polyethylene material. This colored stretched polyethylene material has a tensile modulus of 120 Gpa or more and a tensile strength of 1.5 GPa or more.
摘要翻译：本发明公开了一种着色的拉伸聚乙烯材料，其包含在135℃的十氢化萘中特性粘度为5-50dl / g的超高分子量聚乙烯和每100份的0.001-50重量份聚乙烯，染料和/或颜料的重量，并且在低于聚乙烯的熔点的温度下被拉伸，以及制造所述聚乙烯材料的方法。该着色拉伸聚乙烯材料的拉伸模量为120Gpa以上，拉伸强度为1.5GPa以上。

3. 发明授权

US5091133A Continuous production process of high-strength and high-modulus polyolefin material 失效
标题翻译：高强度和高模量聚烯烃材料的连续生产工艺
公开(公告)号：US5091133A
公开(公告)日：1992-02-25
申请号：US451788
申请日：1989-12-18
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami
IPC分类号： B29C43/22 , C08L23/06
CPC分类号： B29C43/003 , B29C43/228 , C08L23/06 , B29C2043/483 , B29K2033/00 , B29K2105/251
摘要： A high-strength and high-modulus polyolefin material can be continuously produced from a polyolefin in a powder form by feeding the polyolefin powder between a combination of endless belts disposed in an up-and-down opposing relation, compression-molding the polyolefin powder at a temperature lower than the melting point of the polyolefin powder by means of a pressing device while holding the polyolefin powder between the endless belts and conveying the same, and then rolling and stretching the resultant compression-molded polyolefin. The pressing device is constructed of pressing platens and corresponding sets of rollers, which are all accommodated within the respective endless belts. The rollers in each set are connected together, and the sets of rollers are arranged movably in an endless fashion between the respective platens and the endless belts associated therewith.

4. 发明授权

US4895903A Thermoplastic elastomer compositions 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US4895903A
公开(公告)日：1990-01-23
申请号：US185109
申请日：1988-04-22
申请人： Seizo Kobayashi , Katumi Usui , Takashi Mizoe
发明人： Seizo Kobayashi , Katumi Usui , Takashi Mizoe
IPC分类号： C08K5/13 , C08F210/16 , C08K3/10 , C08L23/00 , C08L23/08 , C08L23/10 , C08L23/14 , C08L23/16 , C09K3/10 , H01B3/44
CPC分类号： C08L23/16 , C08L2205/03 , C08L23/0815 , C08L23/14 , C08L2312/04
摘要： A thermoplastic elastomer composition prepared by crosslinking a composition comprising the following components (A), (B) and (C) by using a phenolic curing agent:(A) 30-70 parts by weight of an ethylene/.alpha.-olefin copolymer prepared by copolymerizing ethylene and an .alpha.-olefin having 3 to 12 carbon atoms in the presence of a catalyst comprising a solid component and an organoaluminum compound which solid component contains at least magnesium and titanium, said ethylene/.alpha.-olefin copolymer having the following properties (I) to (IV):______________________________________ (I) Melt index 0.01-100 g/10 min (II) Density 0.860-0.910 g/cm.sup.3 (III) Maximum peak temperature as measured according to a not lower than 100.degree. C. differential scanning calorimetry (DSC) (IV) Insolubles in boiling n-hexane not less than 10 wt. % ______________________________________ (B) 70-30 parts by weight of a propylene polymer; and(C) 70-150 parts by weight, based on 100 parts by weight of the components (A) and (B), of an ethylene/.alpha.-olefin/non-conjugated diene copolymer rubber.
摘要翻译：通过使用酚类固化剂将包含以下组分（A），（B）和（C）的组合物交联制备的热塑性弹性体组合物：（A）30-70重量份由乙烯/α-烯烃共聚物制备的乙烯/α-烯烃共聚物在包含固体组分和固体组分至少含有镁和钛的有机铝化合物的催化剂存在下，使乙烯和具有3至12个碳原子的α-烯烃共聚，所述乙烯/α-烯烃共聚物具有以下性质（I ）至（IV）： - （I）熔体指数0.01-100g / 10分钟 - （II）密度0.860-0.910g / cm 3 - （III）测量的最大峰 - 温度 - 不低于100℃ - 差示扫描量热法（DSC） - （IV）沸点正己烷中不溶于10重量％％ - （B）70-30重量份丙烯聚合物; 和（C）基于100重量份组分（A）和（B））的70-150重量份的乙烯/α-烯烃/非共轭二烯共聚物橡胶。

5. 发明授权

US4732940A Crosslinked resin compositions 失效
标题翻译：交联树脂组合物
公开(公告)号：US4732940A
公开(公告)日：1988-03-22
申请号：US808884
申请日：1985-12-13
申请人： Noboru Yamaoka , Kiyoyasu Tanabe , Katumi Usui , Takashi Mizoe , Kazuo Matsuura
发明人： Noboru Yamaoka , Kiyoyasu Tanabe , Katumi Usui , Takashi Mizoe , Kazuo Matsuura
IPC分类号： C08L23/00 , C08J3/24 , C08J3/28 , C08K5/14 , C08L7/00 , C08L21/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L23/14 , C08L23/16 , C08L51/00 , C08L51/02 , C08L53/00 , C08L77/00 , C08L101/00 , C08L23/26 , C08L23/18
CPC分类号： C08L23/0815 , C08L2205/02 , C08L2205/03 , C08L23/12 , C08L23/14 , C08L2312/00
摘要： A crosslinked resin composition obtained by crosslinking a composition comprising (A) 95-10 wt. % of a propylene polymer and (B) 5-90 wt. % of an ethylene/.alpha.-olefin copolymer having the following properties (I) to (iv) and prepared by copolymerizing ethylene with an .alpha.-olefin having 3 to 12 carbon atoms in the presence of a catalyst, said catalyst comprising a solid component and an organoaluminum compound, said solid component containing at least magnesium and titanium:______________________________________ (i) Melt index 0.01-100 g/10 min (ii) Density 0.860-0.910 g/cm.sup.3 (iii) Maximum peak temperature not lower than 100.degree. C. measured according to a differential scanning calorimetry (DSC) (iv) Insolubles in boiling not less than 10 wt. % n-hexane ______________________________________
摘要翻译：交联树脂组合物，其通过将包含（A）95-10重量％％的丙烯聚合物和（B）5-90重量％％的具有以下特性（I）至（iv）的乙烯/α-烯烃共聚物，并通过在催化剂存在下使乙烯与具有3至12个碳原子的α-烯烃共聚制备，所述催化剂包含固体组分和有机铝化合物，所述固体组分至少含有镁和钛： - （i）熔体指数0.01-100g / 10min - （ii）密度0.860-0.910g / cm 3 - （iii）最高峰温不低于100℃ C. - 根据差示扫描量热法（DSC）测量 - （iv）不溶于沸点不小于10wt。％ - 正己烷 -

6. 发明授权

US5445883A Laminate 失效
标题翻译：层压板
公开(公告)号：US5445883A
公开(公告)日：1995-08-29
申请号：US272629
申请日：1994-07-11
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Keizi Jimbo
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Keizi Jimbo
IPC分类号： B32B27/32 , C09J7/02
CPC分类号： B32B27/32 , Y10S428/91 , Y10T428/2878 , Y10T428/31913 , Y10T428/31928
摘要： An anisotropy-free laminate having much higher strength and stiffness as compared with conventional articles is here disclosed which can be prepared by laminating an orientated ultra-high-molecular-weight polyethylene onto an adhesive layer obtained by modifying an olefin polymer with an unsaturated carboxylic acid and/or its derivative at a temperature lower than the melting point of the orientated ultra-high-molecular-weight polyethylene. The anisotropy-free material having high strength and high stiffness of the present invention can be substituted for various materials such as metals, lumber and FRP, and is also lightweight and excellent in water resistance.
摘要翻译：这里公开了与常规制品相比具有高得多的强度和刚度的无向异性层压材料，其可以通过将取向的超高分子量聚乙烯层压到通过用不饱和羧酸改性烯烃聚合物获得的粘合剂层上来制备和/或其衍生物在低于取向的超高分子量聚乙烯的熔点的温度下进行。本发明的具有高强度和高硬度的各向异性材料可以代替金属，木材和FRP等各种材料，并且重量轻且耐水性优异。

7. 发明授权

US4722973A Thermoplastic elastomer composition 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US4722973A
公开(公告)日：1988-02-02
申请号：US847430
申请日：1986-04-02
申请人： Noboru Yamaoka , Kiyoyasu Tanabe , Katumi Usui , Takashi Mizoe , Kazuo Matsuura
发明人： Noboru Yamaoka , Kiyoyasu Tanabe , Katumi Usui , Takashi Mizoe , Kazuo Matsuura
IPC分类号： C08L23/16 , C08L23/18
CPC分类号： C08L23/16 , C08L23/0815 , C08L2312/00
摘要： This invention provides a thermoplastic elastomer composition obtained by blending (A) a hard segment comprising a low-density ethylene-.alpha.-olefin copolymer formed by copolymerizing ethylene with an .alpha.-olefin by the use of a specific catalyst and characterized by specifically defined properties and (B) a soft segment comprising an ethylene-.alpha.-olefin copolymer rubber, or obtained by partial cross-linking of the resulting blend.This elastomer composition has characteristic features such as high flexibility, good fluidity, excellent tensile properties, good thermal resistance and oil resistance and low permanent strain.
摘要翻译：本发明提供一种热塑性弹性体组合物，其通过将（A）包含通过使用特定催化剂将乙烯与α-烯烃共聚而形成的低密度乙烯-α-烯烃共聚物的硬链段并且特征在于具体限定的性质和（B）包含乙烯-α-烯烃共聚物橡胶的软链段，或通过所得共混物的部分交联获得。该弹性体组合物具有柔软性高，流动性好，拉伸性能优异，耐热性好，耐油性好，永久变形小的特征。

8. 发明授权

US5578373A Split polyethylene stretched material and process for producing the same 失效
标题翻译：分离聚乙烯拉伸材料及其制备方法
公开(公告)号：US5578373A
公开(公告)日：1996-11-26
申请号：US357089
申请日：1994-12-15
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Osamu Otsu , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Osamu Otsu , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa
IPC分类号： B29C43/22 , B29C55/18 , B29D28/00 , D02G1/02 , D02G3/00 , B29K43/48
CPC分类号： B30B5/067 , B29C43/228 , B29C43/48 , B29C55/18 , B29D28/00 , B29C2043/483 , B29K2023/0683 , B29L2028/00 , Y10S264/47 , Y10S428/901 , Y10T428/2913 , Y10T428/2925
摘要： The present invention provides a split polyethylene stretched material having a tensile strength of at least 0.7 GPa when twisted in the range of 50-500 times/m, which material is produced by subjecting a polyethylene having an intrinsic viscosity of 5-50 dl/g as measured at 135.degree. C. in decalin, i.e. an ultra-high-molecular-weight polyethylene to stretching and then subjecting the stretched polyethylene to splitting, as well as a process for producing said material. The split polyethylene stretched material according to the present invention has a large surface area and accordingly can be easily laminated to other materials, and has a high strength and flexibility.
摘要翻译：本发明提供了一种裂解聚乙烯拉伸材料，其在50-500次/ m的范围内扭曲时的拉伸强度至少为0.7GPa，该材料通过使特性粘度为5-50dl / g的聚乙烯如在135℃下在十氢化萘中测量的，即超高分子量聚乙烯，以拉伸然后使拉伸的聚乙烯分裂，以及制备所述材料的方法。根据本发明的分裂聚乙烯拉伸材料具有大的表面积，因此可以容易地层压到其它材料上，并且具有高强度和柔韧性。

9. 发明授权

US5200129A Process for continuous production of polyolefin material 失效
标题翻译：连续生产聚烯烃材料的工艺
公开(公告)号：US5200129A
公开(公告)日：1993-04-06
申请号：US687501
申请日：1991-04-19
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami
IPC分类号： B29C43/48 , B29C43/22 , B29C55/02 , B29C55/18 , B29K23/00 , B29L7/00
CPC分类号： B30B5/067 , B29C43/228 , B29C55/18 , B29C2043/483 , B29K2023/00
摘要： According to the present invention, a polyolefin sheet, film or fiber having a high strength and a high modulus can be continuously produced by:feeding an ultra-high-molecular-weight polyolefin powder between a pair of upper and lower endless belts opposed to each other,conveying the polyolefin powder between the endless belts under compression to compression-mold the polyolefin powder at a temperature lower than the melting point of the polyolefin powder, the compression being continuously and smoothly effected, via the endless belts, by a pressing means comprising two sets of rollers which are arranged at the back sides of the endless belts so that each one roller of the two roller sets faces each other and each of which rollers is rotatably supported at the shaft ends by a frame, and thenrolling and stretching the resultant compression-molded polyolefin in this order.

10. 发明授权

US5106555A Process for the continuous production of high-strength and high-modulus polyethylene material 失效
标题翻译：连续生产高强度和高模量聚乙烯材料的工艺
公开(公告)号：US5106555A
公开(公告)日：1992-04-21
申请号：US557654
申请日：1990-07-25
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa , Mihoko Okada
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa , Mihoko Okada
IPC分类号： B29C43/22 , B29C43/48 , B29C55/02 , B29C55/18 , B29K23/00
CPC分类号： B29C55/18 , B29C43/228 , B29C2043/483 , B29K2023/06
摘要： A process is provided for the continuous production of a high-strength and high-modulus polyethylene material having excellent properties. According to the process, powder composed of ultra-high-molecular-weight polyethylene powder as a principal component is subjected to compression molding, rolling and stretching. The polyethylene powder has an intrinsic viscosity of 5-50 dl/g as measured at 135.degree. C. in decalin. The compression molding is carried out by feeding the polyethylene powder between endless belts arranged in an opposing up-and-down relation, and conveying the polyethylene powder while holding the same between the endless belts and at the same time, continuously compression molding the polyethylene powder at a temperature lower than its melting point by a compressing means provided inside of the endless belts. In at least one of the compression molding step and rolling step, an olefin polymer having a molecular weight lower than the polyolefin polymer is concurrently processed.

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