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1. 发明授权

US07388103B2 Cyclopentane carboxylate compounds, process and intermediates for preparing the same and use thereof 有权
标题翻译：环戊烷羧酸酯化合物，其制备方法和中间体及其应用
公开(公告)号：US07388103B2
公开(公告)日：2008-06-17
申请号：US11258919
申请日：2005-10-27
申请人： Lunjia Xie , Hongbin Du , Zhibiao Hu , Tianyi Zhang , Siyuan Zhao , Xinsheng Wang
发明人： Lunjia Xie , Hongbin Du , Zhibiao Hu , Tianyi Zhang , Siyuan Zhao , Xinsheng Wang
IPC分类号： C07C69/74
CPC分类号： C07C67/31 , C07C67/14 , C07C67/343 , C07C69/757 , C07C2601/08 , C08F10/00 , C08F110/06 , C08F4/6545 , C08F4/651 , C08F2500/15 , C08F2500/12
摘要： The present invention discloses cyclopentane carboxylate compounds. The 1-hydrocarbyl-2-acyloxy-cyclopentane carboxylates according to the invention have a general formula (I): wherein groups R1, R2 and R3, which are identical or different, are independently selected from the group consisting of linear or branched C1-C20alkyl, C3-C20cycloalkyl, C6-C20aryl, C7-C20alkaryl and C7-C20aralkyl. The present invention also discloses a process as well as intermediate compounds for preparing the compounds of formula (I), and use of the compounds (I) as electron donor in the preparation of catalysts for propylene polymerization.
摘要翻译：本发明公开了环戊烷羧酸酯化合物。根据本发明的1-烃基-2-酰氧基 - 环戊烷羧酸盐具有通式（I）：其中基团R 1，R 2和R 3 其相同或不同，独立地选自直链或支链C 1 -C 20烷基，C 3〜 C 20 -C 20环烷基，C 6 -C 20芳基，C 7 -C 20 烷芳基和C 7 -C 20芳烷基。本发明还公开了一种制备式（I）化合物的中间体化合物和用于制备丙烯聚合催化剂的化合物（I）作为电子给体的方法。

2. 发明申请

US20060094843A1 Cyclopentane carboxylate compounds, process and intermediates for preparing the same and use thereof 有权
标题翻译：环戊烷羧酸酯化合物，其制备方法和中间体及其应用
公开(公告)号：US20060094843A1
公开(公告)日：2006-05-04
申请号：US11258919
申请日：2005-10-27
申请人： Lunjia Xie , Hongbin Du , Zhibiao Hu , Tianyi Zhang , Siyuan Zhao , Xinsheng Wang
发明人： Lunjia Xie , Hongbin Du , Zhibiao Hu , Tianyi Zhang , Siyuan Zhao , Xinsheng Wang
IPC分类号： C07C69/74 , C08F2/00
CPC分类号： C07C67/31 , C07C67/14 , C07C67/343 , C07C69/757 , C07C2601/08 , C08F10/00 , C08F110/06 , C08F4/6545 , C08F4/651 , C08F2500/15 , C08F2500/12
摘要： The present invention discloses cyclopentane carboxylate compounds. The 1-hydrocarbyl-2-acyloxy-cyclopentane carboxylates according to the invention have a general formula (I): wherein groups R1, R2 and R3, which are identical or different, are independently selected from the group consisting of linear or branched C1-C20alkyl, C3-C20cycloalkyl, C6-C20aryl, C7-C20alkaryl and C7-C20aralkyl. The present invention also discloses a process as well as intermediate compounds for preparing the compounds of formula (I), and use of the compounds (I) as electron donor in the preparation of catalysts for propylene polymerization.
摘要翻译：本发明公开了环戊烷羧酸酯化合物。根据本发明的1-烃基-2-酰氧基 - 环戊烷羧酸盐具有通式（I）：其中基团R 1，R 2和R 3 其相同或不同，独立地选自直链或支链C 1 -C 20烷基，C 3〜 C 20 -C 20环烷基，C 6 -C 20芳基，C 7 -C 20 烷芳基和C 7 -C 20芳烷基。本发明还公开了一种制备式（I）化合物的中间体化合物和用于制备丙烯聚合催化剂的化合物（I）作为电子给体的方法。

3. 发明授权

US06822109B2 Silicon ether compound, a method for the preparation thereof and use thereof 有权
标题翻译：硅醚化合物，其制备方法和用途
公开(公告)号：US06822109B2
公开(公告)日：2004-11-23
申请号：US10620508
申请日：2003-07-16
申请人： Lunjia Xie , Mingzhi Gao , Tianyi Li , Siyuan Zhao , Mingsen Zhang , Changjiang Wu
发明人： Lunjia Xie , Mingzhi Gao , Tianyi Li , Siyuan Zhao , Mingsen Zhang , Changjiang Wu
IPC分类号： C07F704
CPC分类号： C08F10/00 , C07F7/1804 , C08F110/06 , C08F4/6465 , C08F2500/15 , C08F2500/12
摘要： The present invention relates to a silicon ether compound having general formula (I): wherein, R and R1-R10 groups, which may be Identical or different, represent hydrogen, halogen, C1-C20 linear or branched alkyl, C3-C20 cycloalkyl, C8-C20 aryl, C7-C20 alkaryl or C7-C20 aralkyl group, and two or more R groups can be linked to form saturated or unsaturated condensed ring structure which is optionally substituted by a group having the same meanings with that of R1, R and R1-R10 groups optionally contain one or more hetero-atoms replacing carbon atom, hydrogen atom or the both, said heteroatom is selected from the group consisting of nitrogen, oxygen, sulfur, silicon, phosphorus and halogen atom, and A represents carbon atom or silicon atom. The present invention also relates to a method for the preparation of the silicon ether compounds of general formula (I) and a process for polymerization of olefins.
摘要翻译：本发明涉及具有通式（I）的硅醚化合物：其中，R和R 1 -R 10基团可以相同或不同，表示氢，卤素，C 1 -C 20直链或支链烷基，C 3 -C 20环烷基， C8-C20芳基，C7-C20烷芳基或C7-C20芳烷基，并且两个或更多个R基团可连接形成饱和或不饱和稠环结构，其任选被具有与R 1，R 并且R 1 -R 10基团任选地含有一个或多个取代碳原子，氢原子或二者的杂原子，所述杂原子选自氮，氧，硫，硅，磷和卤素原子，A表示碳原子或硅原子。本发明还涉及制备通式（I）的硅醚化合物的方法和烯烃聚合方法。

4. 发明申请

US20130324682A1 SOLID CATALYST COMPONENT AND CATALYST FOR OLEFIN POLYMERIZATION 有权
标题翻译：用于烯烃聚合的固体催化剂组分和催化剂
公开(公告)号：US20130324682A1
公开(公告)日：2013-12-05
申请号：US13980359
申请日：2012-01-19
申请人： Zhong TAN , Lunjia Xie , Xiudong Xu , Yu Tian , Qilong Zhou , Zaixing Feng , Li'an Yan , Siyuan Zhao , Jinhua Yu , Zhufang Sun , Fengkui Li , Shanshan Yin , Weiwei Song
发明人： Zhong TAN , Lunjia Xie , Xiudong Xu , Yu Tian , Qilong Zhou , Zaixing Feng , Li'an Yan , Siyuan Zhao , Jinhua Yu , Zhufang Sun , Fengkui Li , Shanshan Yin , Weiwei Song
IPC分类号： C08F110/06
CPC分类号： C08F110/06 , C08F10/06 , C08F4/651 , C08F2500/04 , C08F2500/12 , C08F2500/15 , C08F4/6548
摘要： Disclosed is a solid catalyst component for olefin polymerization. The catalyst component comprises a dialkoxy magnesium carrier, a titanium compound, and a product from an internal electron donor reacting in an inert solvent. Said internal electron donor compound comprises a 2,3-di-non-linear-alkyl-2-cyano succinic acid diester compound as presented in formula I: as in formula I, R1 and R2 radicals are independently chosen from linear or branched C1-C4 alkyl groups; R is chosen from C3-C6 iso-alkyl, sec-alkyl, or cycloalkyl groups. Also disclosed is another solid catalyst component. The catalyst component comprises a dialkoxy magnesium carrier, a titanium compound, and a product from an internal electron donor reacting in an inert solvent. In addition to a 2,3-di-non-linear-alkyl-2-cyano succinic acid diester compound as presented in formula I, the internal electron donor compound can also comprise 2-isopropyl-2-(3-methylbutyl)-1,3-dimethoxy propane and/or a carboxylic ester compound. Also disclosed is a catalyst containing the solid catalyst component. The catalyst is used for olefin polymerization, particularly propylene polymerization, and is relatively active during polymerization. The obtained polymer has the advantages of wide molecular weight distribution, high molecular bulk density, good hydrogen regulation sensitivity, good stereospecificity, good particle shape, and small fine powder content.
摘要翻译：公开了用于烯烃聚合的固体催化剂组分。催化剂组分包括二烷氧基镁载体，钛化合物和在惰性溶剂中反应的内电子给体的产物。所述内电子给体化合物包含式I所示的2,3-二 - 非线性 - 烷基-2-氰基琥珀酸二酯化合物：如式I所示，R 1和R 2基团独立地选自直链或支链C1- C4烷基; R选自C 3 -C 6异烷基，仲烷基或环烷基。还公开了另一种固体催化剂组分。催化剂组分包括二烷氧基镁载体，钛化合物和在惰性溶剂中反应的内电子给体的产物。除了式I所示的2,3-二 - 非线性 - 烷基-2-氰基琥珀酸二酯化合物之外，内电子给体化合物还可以包含2-异丙基-2-（3-甲基丁基）-1 ，3-二甲氧基丙烷和/或羧酸酯化合物。还公开了含有固体催化剂组分的催化剂。该催化剂用于烯烃聚合，特别是丙烯聚合，并且在聚合期间相对有活性。得到的聚合物具有分子量分布宽，分子体积密度高，调节灵敏度好，立体定向性好，粒子形状好，细粉含量低的优点。

5. 发明授权

US09376513B2 Solid catalyst component and catalyst for olefin polymerization 有权
标题翻译：固体催化剂组分和烯烃聚合催化剂
公开(公告)号：US09376513B2
公开(公告)日：2016-06-28
申请号：US13980359
申请日：2012-01-19
申请人： Zhong Tan , Lunjia Xie , Xiudong Xu , Yu Tian , Qilong Zhou , Zaixing Feng , Li'an Yan , Siyuan Zhao , Jinhua Yu , Zhufang Sun , Fengkui Li , Shanshan Yin , Weiwei Song
发明人： Zhong Tan , Lunjia Xie , Xiudong Xu , Yu Tian , Qilong Zhou , Zaixing Feng , Li'an Yan , Siyuan Zhao , Jinhua Yu , Zhufang Sun , Fengkui Li , Shanshan Yin , Weiwei Song
IPC分类号： C08F110/06 , C08F10/06
CPC分类号： C08F110/06 , C08F10/06 , C08F4/651 , C08F2500/04 , C08F2500/12 , C08F2500/15 , C08F4/6548
摘要： Disclosed is a solid catalyst component for olefin polymerization. The catalyst component comprises a dialkoxy magnesium carrier, a titanium compound, and a product from an internal electron donor reacting in an inert solvent. The internal electron donor compound comprises a 2,3-di-non-linear-alkyl-2-cyano succinic acid diester compound as presented in formula I.
摘要翻译：公开了用于烯烃聚合的固体催化剂组分。催化剂组分包括二烷氧基镁载体，钛化合物和在惰性溶剂中反应的内电子给体的产物。内给电子体化合物包含式I所示的2,3-二 - 非直链烷基-2-氰基琥珀酸二酯化合物。

6. 发明授权

US08669392B2 Process for preparing 2,3-di-non-straight-alkyl-2-cyanosuccinic acid diesters 有权
标题翻译：制备2,3-二 - 非直链烷基-2-氰基琥珀酸二酯的方法
公开(公告)号：US08669392B2
公开(公告)日：2014-03-11
申请号：US13202282
申请日：2010-02-12
申请人： Lunjia Xie , Yu Tian , Zaixing Feng , Siyuan Zhao , Yu Kang , Zhufang Sun
发明人： Lunjia Xie , Yu Tian , Zaixing Feng , Siyuan Zhao , Yu Kang , Zhufang Sun
IPC分类号： C07C253/30 , C07C67/32 , C07C51/38
CPC分类号： C07C253/30 , C07C51/09 , C07C67/08 , C07C255/22 , C07C55/02 , C07C69/34
摘要： A process for preparing 2,3-di(non-linear-alkyl)-2-cyanosuccinate compounds, especially 2,3-diisopropyl-2-cyanosuccinate compounds, and processes for preparing 2,3-di(non-linear-alkyl)succinic acids and esters thereof by using the 2,3-di-non-linear propyl-2-cyanosuccinate compounds as intermediates are disclosed.
摘要翻译：制备2,3-二（非线性烷基）-2-氰基琥珀酸盐化合物，特别是2,3-二异丙基-2-氰基琥珀酸盐化合物的方法，以及2,3-二（非直链烷基）公开了通过使用2,3-二 - 非线性丙基-2-氰基琥珀酸盐化合物作为中间体的琥珀酸及其酯。

7. 发明申请

US20110040051A1 CATALYST COMPONENT FOR OLEFIN POLYMERIZATION AND A CATALYST COMPRISING THE SAME 有权
标题翻译：用于烯烃聚合的催化剂组分和包含其的催化剂
公开(公告)号：US20110040051A1
公开(公告)日：2011-02-17
申请号：US12856175
申请日：2010-08-13
申请人： Lunjia XIE , Yongtai Ling , Yu Tian , Zaixing Feng , Siyuan Zhao , Qing Hu , Zhufang Sun , Yu Kang
发明人： Lunjia XIE , Yongtai Ling , Yu Tian , Zaixing Feng , Siyuan Zhao , Qing Hu , Zhufang Sun , Yu Kang
IPC分类号： C08F4/16 , B01J31/04 , C08F4/602
CPC分类号： C08F10/06 , B01J27/135 , B01J27/138 , B01J31/0201 , B01J31/0255 , B01J31/0272 , B01J31/143 , B01J31/38 , C08F110/06 , C08F4/651 , C08F2500/15 , C08F2500/12 , C08F2500/04
摘要： A catalyst component for olefin polymerization comprising an α-cyanosuccinate compound as an internal electron donor, a catalyst comprising the catalyst component, and use of the catalyst in olefin polymerization. When used in propylene polymerization, the catalyst can exhibit good catalytic activity and good hydrogen response, and the resulting polymer can have a good isotacticity and a good molecular weight distribution.
摘要翻译：一种用于烯烃聚合的催化剂组分，其包含作为内部电子给体的α-氰基琥珀酸盐化合物，包含催化剂组分的催化剂，以及烯烃聚合中催化剂的用途。当用于丙烯聚合时，该催化剂可表现出良好的催化活性和良好的氢响应，所得聚合物可具有良好的全同立构规整度和良好的分子量分布。

8. 发明授权

US07399812B2 Silicon ether compounds and a method for the preparation thereof 有权
标题翻译：硅醚化合物及其制备方法
公开(公告)号：US07399812B2
公开(公告)日：2008-07-15
申请号：US11059581
申请日：2005-02-16
申请人： Lunjia Xie , Mingzhi Gao , Siyuan Zhao , Jing Ma , Zhufang Sun , Haitao Liu , Tianyi Li , Mingsen Zhang , Changjiang Wu
发明人： Lunjia Xie , Mingzhi Gao , Siyuan Zhao , Jing Ma , Zhufang Sun , Haitao Liu , Tianyi Li , Mingsen Zhang , Changjiang Wu
IPC分类号： C08F4/42
CPC分类号： C08F10/00 , C07F7/1804 , C08F110/06 , C08F4/6545 , C08F4/6465 , C08F4/651 , C08F2500/12 , C08F2500/15
摘要： The present invention relates to silicon ether compounds having a general formula (I), a method for the preparation thereof and use thereof as a component of catalysts for polymerization of olefins. In particular, in propylene polymerization, catalyst systems comprising the silicon ether compounds as external electron donor component exhibit good hydrogen response, and can be used to prepare polymer having high isotacticity at high yield. wherein R1-R10 groups are as defined in the description.
摘要翻译：本发明涉及具有通式（I）的硅醚化合物，其制备方法及其作为烯烃聚合催化剂组分的用途。特别地，在丙烯聚合中，包含作为外电子给体组分的硅醚化合物的催化剂体系表现出良好的氢响应，并且可以用于以高产率制备具有高全同立构规整度的聚合物。其中R 1 -R 10基团如说明书中所定义。

9. 发明授权

US08541333B2 Catalyst component for olefin polymerization and a catalyst comprising the same 有权
标题翻译：用于烯烃聚合的催化剂组分和包含其的催化剂
公开(公告)号：US08541333B2
公开(公告)日：2013-09-24
申请号：US12856175
申请日：2010-08-13
申请人： Lunjia Xie , Yongtai Ling , Yu Tian , Zaixing Feng , Siyuan Zhao , Qing Hu , Zhufang Sun , Yu Kang
发明人： Lunjia Xie , Yongtai Ling , Yu Tian , Zaixing Feng , Siyuan Zhao , Qing Hu , Zhufang Sun , Yu Kang
IPC分类号： B01J31/00 , C08F4/02 , C08F4/44 , C08F4/06 , C08F2/00 , C08F4/00
CPC分类号： C08F10/06 , B01J27/135 , B01J27/138 , B01J31/0201 , B01J31/0255 , B01J31/0272 , B01J31/143 , B01J31/38 , C08F110/06 , C08F4/651 , C08F2500/15 , C08F2500/12 , C08F2500/04
摘要： A catalyst component for olefin polymerization comprising an α-cyanosuccinate compound as an internal electron donor, a catalyst comprising the catalyst component, and use of the catalyst in olefin polymerization. When used in propylene polymerization, the catalyst can exhibit good catalytic activity and good hydrogen response, and the resulting polymer can have a good isotacticity and a good molecular weight distribution.
摘要翻译：一种用于烯烃聚合的催化剂组分，其包含作为内部电子给体的α-氰基琥珀酸盐化合物，包含催化剂组分的催化剂，以及在烯烃聚合中使用该催化剂。当用于丙烯聚合时，该催化剂可表现出良好的催化活性和良好的氢响应，所得聚合物可具有良好的全同立构规整度和良好的分子量分布。

10. 发明申请

US20120046490A1 PROCESS FOR PREPARING 2,3-DI-NON-STRAIGHT-ALKYL-2-CYANOSUCCINIC ACID DIESTERS 有权
标题翻译：制备2,3-二 - 非直链烷基-2-氰基脂肪酸乳液的方法
公开(公告)号：US20120046490A1
公开(公告)日：2012-02-23
申请号：US13202282
申请日：2010-02-12
申请人： Lunjia Xie , Yu Tian , Zaixing Feng , Siyuan Zhao , Yu Kang , Zhufang Sun
发明人： Lunjia Xie , Yu Tian , Zaixing Feng , Siyuan Zhao , Yu Kang , Zhufang Sun
IPC分类号： C07C253/30 , C07C67/32 , C07C51/38
CPC分类号： C07C253/30 , C07C51/09 , C07C67/08 , C07C255/22 , C07C55/02 , C07C69/34
摘要： A process for preparing 2,3-di(non-linear-alkyl)-2-cyanosuccinate compounds, especially 2,3-diisopropyl-2-cyanosuccinate compounds, and processes for preparing 2,3-di(non-linear-alkyl)succinic acids and esters thereof by using the 2,3-di-non-linear propyl-2-cyanosuccinate compounds as intermediates are disclosed.
摘要翻译：制备2,3-二（非线性烷基）-2-氰基琥珀酸盐化合物，特别是2,3-二异丙基-2-氰基琥珀酸盐化合物的方法，以及2,3-二（非直链烷基）公开了通过使用2,3-二 - 非线性丙基-2-氰基琥珀酸盐化合物作为中间体的琥珀酸及其酯。

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