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1. 发明申请

US20090280318A1 OLEFIN POLYMER, COMPOSITION THEREOF AND ADHESIVE RESIN COMPRISING THE COMPOSITION 审中-公开
标题翻译： OLEFIN聚合物，其组合物和包含组合物的粘合树脂
公开(公告)号：US20090280318A1
公开(公告)日：2009-11-12
申请号：US12096655
申请日：2006-12-08
申请人： Tomoaki Matsugi , Junji Saito , Hideyuki Kaneko , Norio Kashiwa , Shin-ichi Kojoh , Takayuki Onogi , Motoaki Isokawa , Seiji Ota , Shigeyuki Yasui
发明人： Tomoaki Matsugi , Junji Saito , Hideyuki Kaneko , Norio Kashiwa , Shin-ichi Kojoh , Takayuki Onogi , Motoaki Isokawa , Seiji Ota , Shigeyuki Yasui
IPC分类号： B32B27/32 , C08F8/00 , C09J131/02
CPC分类号： C08L53/00 , C08F8/00 , C08F8/08 , C08F8/12 , C08F8/18 , C08F8/20 , C08F8/42 , C08F255/00 , C08F255/02 , C08F293/00 , C08F293/005 , C08F2810/50 , C08L23/0846 , C08L23/0884 , C08L23/0892 , C08L51/06 , C08L2205/02 , C08L2666/02 , C08L2666/14 , C09J123/02 , C09J123/0846 , C09J151/06 , C09J153/00 , Y10T428/263 , C08L2666/06 , C08F210/02 , C08F110/06 , C08F255/023 , C08F110/14 , C08F210/12
摘要： Provided is a new adhesive polyolefin resin composition, containing 1 to 100% by weight of a high polymer structure, that has good heat resistance and excellent adhesion performance to polyolefins and various polar materials, wherein a polyolefin segment (A) is bonded with an addition polymer segment (B) of a non-olefinic vinyl monomer and a reactive group is introduced into the addition polymer segment (B) and an adhesive or dispersion obtained therefrom.
摘要翻译：提供了一种新的粘合剂聚烯烃树脂组合物，其含有1至100重量％的高聚物结构，其具有良好的耐热性和对聚烯烃和各种极性材料的优异粘合性能，其中聚烯烃链段（A）与添加剂将非烯烃类乙烯基单体和反应性基团的聚合物链段（B）导入到加成聚合物链段（B）中，并由其获得粘合剂或分散体。

2. 发明授权

US5962615A Ethylene polymer 失效
标题翻译：乙烯聚合物
公开(公告)号：US5962615A
公开(公告)日：1999-10-05
申请号：US597472
申请日：1996-02-02
申请人： Shin-ichi Kojoh , Mamoru Kioka
发明人： Shin-ichi Kojoh , Mamoru Kioka
IPC分类号： C08F4/658 , C08F4/651 , C08F4/655 , C08F8/00 , C08F10/02 , C08F110/02
CPC分类号： C08F10/02 , C08F110/02 , Y10S526/904
摘要： An ethylene polymer having small values of Mw/Mn and Mz/Mw, a small proportion of long-chain branches, a high melt tension and a high swell ratio produced by using a solid titanium catalyst component obtained by initially bring a solid titanium composition which is obtained by the contact of a solid magnesium aluminum composite containing magnesium, halogen, aluminum, and an alkoxy group of 6 or more carbon atoms and/or alcohol of 6 of more carbon atom with a tetravalent titanium compound into contact with an organometallic compound, and then bringing the resulting product into contact with oxygen. The ethylene polymer is excellent in moldability, and the molded article obtained therefrom is excellent in rigidity and impact resistance and free from poor appearance.
摘要翻译：通过使用固体钛催化剂组分制得的具有Mw / Mn和Mz / Mw值小的乙烯聚合物，小分支的长支链，高熔体张力和高溶胀比，其通过首先得到固体钛组合物，通过将含有6个以上碳原子的碳原子数6以上的碳原子数为6以上的烷氧基的固体镁铝复合体与4价钛化合物接触而与有机金属化合物接触而获得，然后使得到的产物与氧接触。乙烯聚合物的成型性优异，由此得到的成型体的刚性和耐冲击性优异，外观不良。

3. 发明授权

US6054542A Ethylene polymer and process for preparing the same 失效
标题翻译：乙烯聚合物及其制备方法
公开(公告)号：US6054542A
公开(公告)日：2000-04-25
申请号：US927289
申请日：1997-09-11
申请人： Shin-ichi Kojoh , Mamoru Kioka
发明人： Shin-ichi Kojoh , Mamoru Kioka
IPC分类号： C08F10/02 , C08F110/02
CPC分类号： C08F10/02 , C08F110/02
摘要： An ethylene polymer having small values of Mw/Mn and Mz/Mw, a small proportion of long-chain branches, a high melt tension and a high swell ratio and a process for preparing the same by polymerizing ethylene in the presence of an ethylene polymerization catalyst comprising a solid titanium catalyst component containing titanium, magnesium, halogen and a compound having at least two ether linkages present through plural atoms with an organometallic compound catalyst component.
摘要翻译：具有小Mw / Mn和Mz / Mw值的小乙烯聚合物，长链支链的一小部分，高熔体张力和高溶胀比的乙烯聚合物及其在乙烯聚合存在下聚合乙烯的方法催化剂包含含有钛，镁，卤素的固体钛催化剂组分和通过多个原子与有机金属化合物催化剂组分存在至少两个醚键的化合物。

4. 发明授权

US07795347B2 Multi-branched polymer, process for producing the same, and applications thereof 有权
标题翻译：多支化聚合物，其制备方法及其应用
公开(公告)号：US07795347B2
公开(公告)日：2010-09-14
申请号：US10797144
申请日：2004-03-11
申请人： Hideyuki Kaneko , Tomoaki Matsugi , Shin-Ichi Kojoh , Shingo Matsuo , Nobuo Kawahara , Norio Kashiwa
发明人： Hideyuki Kaneko , Tomoaki Matsugi , Shin-Ichi Kojoh , Shingo Matsuo , Nobuo Kawahara , Norio Kashiwa
IPC分类号： C08F10/00 , C08F255/00 , C08F293/00 , C08F295/00
CPC分类号： C08F290/042
摘要： A group of polymers comprising a plurality of polyolefin chains and polar polymer chains and having a multi-branched structure such as a block structure, a graft structure and a star-shaped structure is produced efficiently by polymerizing or reacting a combination of various polar monomers and their polymers i.e. polar polymer chains by using a functional group-containing polyolefin as a macroinitiator, a macromonomer or a reactive polymer. The resulting multi-branched polymer has a specific shape such as a block structure, a graft structure or a star-shaped structure, and has properties of both the polyolefin and polar polymer, thus exhibiting useful performance in various uses in films and compatibilizing agents as a novel polyolefin-based polymer.
摘要翻译：通过聚合或反应各种极性单体和各种极性单体的组合，有效地制备了包含多个聚烯烃链和极性聚合物链并具有多支链结构的一组聚合物，例如嵌段结构，接枝结构和星形结构，它们的聚合物即通过使用含官能团的聚烯烃作为大分子引发剂，大分子单体或反应性聚合物的极性聚合物链。得到的多支链聚合物具有块状结构，接枝结构或星形结构等特定形状，具有聚烯烃和极性聚合物两者的性质，因此在膜和相容剂的各种用途中表现出有用的性能，如一种新型聚烯烃基聚合物。

5. 发明授权

US5731393A Ethylene polymer, process for preparing the same, solid titanium catalyst component for ethylene polymerization and ethylene polymerization catalyst 失效
标题翻译：乙烯聚合物，其制备方法，用于乙烯聚合的固体钛催化剂组分和乙烯聚合催化剂
公开(公告)号：US5731393A
公开(公告)日：1998-03-24
申请号：US835563
申请日：1997-04-09
申请人： Shin-ichi Kojoh , Mamoru Kioka
发明人： Shin-ichi Kojoh , Mamoru Kioka
IPC分类号： C08F4/654 , C08F4/60 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16
CPC分类号： C08F10/02 , C08F110/02 , C08F210/16
摘要： An ethylene polymer having small values of Mw/Mn and Mz/Mw, a small proportion of long-chain branches and a high swell ratio and a process for preparing the polymer are disclosed. A solid titanium catalyst component obtained by initially contacting a solid titanium composite containing titanium, magnesium, halogen and a compound having at least two ether linkages present through plural atoms with an organometallic compound and then contacting the resulting product with oxygen is further disclosed. An ethylene polymerization catalyst comprising the above catalyst component and an organometallic compound catalyst component is furthermore disclosed. The ethylene polymer is excellent in moldability, and from this polymer, a molded article which is excellent in rigidity and impact resistance and free from poor appearance can be obtained. By the use of the ethylene polymerization catalyst, an ethylene polymer having excellent properties as mentioned above can be obtained.
摘要翻译：公开了具有小的Mw / Mn值和Mz / Mw值，小分子量的长支链和高溶胀比的乙烯聚合物和制备该聚合物的方法。通过将含有钛，镁，卤素的固体钛复合物和具有至少两个通过多个原子存在的醚键的化合物与有机金属化合物接触然后使所得产物与氧接触而获得的固体钛催化剂组分进一步公开。还公开了包含上述催化剂组分和有机金属化合物催化剂组分的乙烯聚合催化剂。乙烯聚合物的成型性优异，从该聚合物可以获得刚性和耐冲击性优异且外观差的成型品。通过使用乙烯聚合催化剂，可以得到如上所述具有优异性能的乙烯聚合物。

6. 发明授权

US6080828A Polymerization catalyst and process for preparing an ethylene polymer 失效
标题翻译：聚合催化剂和制备乙烯聚合物的方法
公开(公告)号：US6080828A
公开(公告)日：2000-06-27
申请号：US310918
申请日：1999-05-13
申请人： Shin-ichi Kojoh , Mamoru Kioka
发明人： Shin-ichi Kojoh , Mamoru Kioka
IPC分类号： C08F4/658 , C08F4/651 , C08F4/655 , C08F8/00 , C08F10/02 , C08F110/02
CPC分类号： C08F10/02 , C08F110/02 , Y10S526/904
摘要： An ethylene polymer having small values of Mw/Mn and Mz/Mw, a small proportion of long-chain branches, a high melt tension and a high swell ratio, and a process for preparing the ethylene polymer are disclosed. A solid titanium catalyst component obtained by initially bringing a solid titanium composite which is obtained by the contact of a solid magnesium aluminum composite containing magnesium, halogen, aluminum, and an alkoxy group of 6 or more carbon atoms and/or alcohol of 6 or more carbon atoms with a tetravalent titanium compound into contact with an organometallic compound, and then bringing the resulting product into contact with oxygen is further disclosed. An ethylene polymerization catalyst comprising the above catalyst component and an organometallic compound catalyst component is furthermore disclosed. Therefore, the ethylene polymer is excellent in moldability, and a molded article obtained therefrom is excellent in rigidity and impact resistance and free from poor appearance.
摘要翻译：公开了具有小的Mw / Mn值和Mz / Mw值，小分支长支链，高熔体张力和高溶胀比的乙烯聚合物，以及制备乙烯聚合物的方法。一种固体钛催化剂组分，其通过首先将含有6个或更多个碳原子和/或6个或更多个碳原子的烷基的固体镁铝复合物与含有镁，卤素，铝的固体镁铝复合物接触而获得的固体钛复合物碳原子与四价钛化合物与有机金属化合物接触，然后使所得产物与氧接触。还公开了包含上述催化剂组分和有机金属化合物催化剂组分的乙烯聚合催化剂。因此，乙烯聚合物的成型性优异，其得到的成型体的刚性和耐冲击性优异，外观不良。

7. 发明申请

US20070190333A1 Polyolefin-based molded product coated with polar polymer, method for producing the same, and uses of the same 审中-公开
标题翻译：涂布有极性聚合物的聚烯烃类成型体，其制造方法及其用途
公开(公告)号：US20070190333A1
公开(公告)日：2007-08-16
申请号：US11491894
申请日：2006-07-25
申请人： Tomoaki Matsugi , Shin-ichi Kojoh , Nobuo Kawahara , Shingo Matsuo , Hideyuki Kaneko , Takayuki Onogi , Junji Saito , Norio Kashiwa
发明人： Tomoaki Matsugi , Shin-ichi Kojoh , Nobuo Kawahara , Shingo Matsuo , Hideyuki Kaneko , Takayuki Onogi , Junji Saito , Norio Kashiwa
IPC分类号： B32B27/36 , B32B27/32 , B32B15/08 , B32B17/10
CPC分类号： B32B27/08 , B32B15/08 , B32B17/10 , B32B27/306 , B32B27/308 , B32B27/32 , B32B27/325 , B32B2255/10 , B32B2255/26 , B32B2307/306 , B32B2307/7242 , B32B2307/728 , B32B2457/00 , C08J7/047 , C08J2323/06 , C08J2467/00 , Y10T428/31536 , Y10T428/31645 , Y10T428/31692 , Y10T428/31797 , Y10T428/31938
摘要： A polyolefin-based molded product having excellent printability, coatability, heat resistance, impact resistance, hydrophilicity or hydrophobicity, or exhibiting excellent performance such as the performance of adhesion with metal, plastics, paper and the like, that is, a polyolefin-based molded product which is coated with a polar segment layer through covalent bonding, without impairing the properties of the polyolefin base material and without substantial delamination at the interface, based on a novel conception that a polyolefin molded product has a structure of being coated with polar polymer segments at the surface, and a vinylic monomer or a small-membered cyclic compound is polymerized on the surface; and a method for producing the same are provided. A polyolefin-based molded product having a polar polymer (B) coated on the surface of a polyolefin molded product (A), characterized by having a structure in which the polar polymer (B) is bound to the surface of the polyolefin molded product (A) through covalent bonding, and a method for producing the same are provided.
摘要翻译：具有优异的可印刷性，涂布性，耐热性，耐冲击性，亲水性或疏水性，或具有优异性能的聚烯烃基成型体，例如与金属，塑料，纸等的粘合性能，即聚烯烃基成型基于聚烯烃模制产品具有涂覆有极性聚合物链段的结构的新概念，通过共价键合涂覆极性链段的产品，而不损害聚烯烃基材的性能并且在界面处没有显着的分层在表面上聚合有乙烯基单体或小元环状化合物; 并提供其制造方法。在聚烯烃成型体（A）的表面上涂布极性聚合物（B）的聚烯烃类成型体，其特征在于，具有极性聚合物（B）与聚烯烃成型体的表面（B A）通过共价键合，提供其制造方法。

8. 发明授权

US07067587B2 Polyolefin macromonomer, graft polymer obtained from the polyolefin macromonomer, and use thereof 有权
标题翻译：聚烯烃大分子单体，由聚烯烃大分子单体得到的接枝聚合物及其用途
公开(公告)号：US07067587B2
公开(公告)日：2006-06-27
申请号：US10650919
申请日：2003-08-29
申请人： Hideyuki Kaneko , Shin-ichi Kojoh , Nobuo Kawahara , Shingo Matsuo , Tomoaki Matsugi , Junji Saito , Sadahiko Matsuura , Kazuhisa Miyazaki , Norio Kashiwa
发明人： Hideyuki Kaneko , Shin-ichi Kojoh , Nobuo Kawahara , Shingo Matsuo , Tomoaki Matsugi , Junji Saito , Sadahiko Matsuura , Kazuhisa Miyazaki , Norio Kashiwa
IPC分类号： C08F4/42 , C08F110/06 , C08F297/06 , C08G63/91
CPC分类号： C08G18/6204 , C08F290/042 , C08F299/00
摘要： A novel graft polymer useful in various uses that has a polyolefin backbone having polyolefin segments excellent in moldability can be obtained by homopolymerizing a novel polyolefin macromonomer or polymerizing the novel polyolefin macromonomer in the coexistence of other olefins depending on need, wherein the macromonomer has at the terminal of its polyolefin chain a vinyl group whose α-position may be substituted, and the macromonomer can be efficiently obtained by a method, for example, successively carrying out i) a step of producing a polyolefin having a hydroxyl group at the terminal of the polyolefin chain and ii) a step of converting the terminal hydroxyl group of the polyolefin in chain into an acryloyl group, a methacryloyl group or a styryl group.
摘要翻译：可以通过均聚聚合新型聚烯烃大分子单体或根据需要在其它烯烃共聚下聚合新型聚烯烃大分子单体而获得具有聚烯烃主链的聚烯烃主链，其聚烯烃主链具有聚烯烃链段优异的各种用途，其中大分子单体在其聚烯烃链的末端是其α-位可被取代的乙烯基，并且可以通过例如依次进行的方法有效地获得大分子单体：i）制备在末端具有羟基的聚烯烃的步骤聚烯烃链和ii）将链中的聚烯烃的末端羟基转化为丙烯酰基，甲基丙烯酰基或苯乙烯基的步骤。

9. 发明授权

US07022763B2 Branched olefin copolymer, process for producing the same, and use thereof 有权
标题翻译：支链烯烃共聚物，其制备方法及其用途
公开(公告)号：US07022763B2
公开(公告)日：2006-04-04
申请号：US10681181
申请日：2003-10-09
申请人： Tomoaki Matsugi , Nobuo Kawahara , Hideyuki Kaneko , Shingo Matsuo , Shin-ichi Kojoh , Norio Kashiwa
发明人： Tomoaki Matsugi , Nobuo Kawahara , Hideyuki Kaneko , Shingo Matsuo , Shin-ichi Kojoh , Norio Kashiwa
IPC分类号： C08L51/08 , C08G63/91
CPC分类号： C09J151/06 , C08F8/00 , C08F8/12 , C08F8/18 , C08F8/30 , C08F255/00 , C08F290/00 , C08F291/00 , C08F293/005 , C08F2800/10 , C08F2810/50 , C08L23/26 , C08L51/06 , C08L53/00 , C08L2666/02 , C09D151/06 , C09D153/00 , C09J153/00 , C08F10/00 , C08F255/02 , C08F8/14 , C08F210/02
摘要： A branched olefin copolymer demonstrating excellent performance in various uses, comprising a building block (A) represented by formula (1) below and a building block (B) represented by formula (2) below, obtained by e.g. a method which involves sequentially conducting (step 1) a step of synthesizing a polar group-containing olefin copolymer (Q) containing at least one functional group (G) selected from a hydroxyl group, a carboxylic acid group, an ester group, an amino group, an epoxy group, a silanol group and an acid anhydride group, (step 2) a step of converting the functional group (G) into a group having an ability to initiate radical polymerization, and (Step 3) a step of installing a polymer segment (Z) by radical polymerization of a monomer essentially comprising carbon-carbon double bond-containing compound (R) containing at least one selected from an oxygen atom, a nitrogen atom, a halogen atom and an aryl group;
摘要翻译：在各种用途中表现出优异性能的支链烯烃共聚物，其包含由下式（1）表示的结构单元（A）和由下式（2）表示的结构单元（B））。涉及顺序地进行（步骤1）合成含有至少一个选自羟基，羧酸基，酯基，氨基的官能团（G）的含极性基团的烯烃共聚物（Q）的步骤基团，环氧基，硅烷醇基和酸酐基团（步骤2）将官能团（G）转化为具有引发自由基聚合能力的基团的步骤，（步骤3）将聚合物链段（Z），其通过基本上包含含有选自氧原子，氮原子，卤素原子和芳基中的至少一种的含碳 - 碳双键的化合物（R）的单体的自由基聚合;

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