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    • 9. 发明授权
    • Zeolite catalyst activity enhancement by aluminum phosphate and
phosphorus
    • 沸石催化剂活性提高磷酸铝和磷
    • US6080303A
    • 2000-06-27
    • US38649
    • 1998-03-11
    • Guang CaoLuc R. M. MartensJeffrey L. WhiteTan-Jen ChenMatu J. Shah
    • Guang CaoLuc R. M. MartensJeffrey L. WhiteTan-Jen ChenMatu J. Shah
    • B01J29/84B01J27/16B01J29/06C10G11/05C10G11/18
    • C10G11/05B01J27/16B01J29/06
    • The present invention provides a process for improving the catalytic activity of small and medium pore acidic zeolite catalyst which comprises the steps of treating a zeolite with a phosphorus compound to form a phosphorus treated zeolite and combining the phosphorus treated zeolite with AlPO.sub.4. Optionally the phosphorus treated zeolite is calcined. The step of combining the zeolite with AlPO.sub.4 may optionally be followed by steaming the combined catalyst. Examples of useful phosphorus containing compounds useful in treating the zeolite include phosphoric acid, ammonium mono or dihydrogen phosphate, organic phosphites, and organophosphines. Preferably the phosphorus containing compound is an ammonium acid phosphate. An additional alternate embodiment provides a process for increasing the hydrothermal stability of a zeolite catalyst which comprises first treating a zeolite with a phosphorus containing compound then blending with AlPO.sub.4. The catalyst of the invention may be combined with other catalysts or used alone. The invention may be used in a process for cracking hydrocarbons which comprises contacting a hydrocarbon feedstock with a catalyst prepared as described above.
    • 本发明提供了改善中孔酸性沸石催化剂的催化活性的方法,其包括用磷化合物处理沸石以形成磷处理的沸石并将磷处理的沸石与AlPO 4组合的步骤。 任选地,将经磷处理的沸石煅烧。 将沸石与AlPO 4组合的步骤可以任选地随后蒸合组合的催化剂。 可用于处理沸石的含磷化合物的实例包括磷酸,磷酸一铵或二磷酸酯,有机亚磷酸酯和有机膦。 含磷化合物优选为磷酸铵。 另外的替代实施方案提供了一种提高沸石催化剂的水热稳定性的方法,其包括首先用含磷化合物处理沸石,然后与AlPO 4共混。 本发明的催化剂可与其它催化剂组合使用或单独使用。 本发明可用于裂解烃的方法,其包括使烃原料与如上所述制备的催化剂接触。