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1. 发明授权

US5110866A Thermoplastic polyester resin composition having improved impact resistance 失效
标题翻译：具有改善抗冲击性的热塑性聚酯树脂组合物
公开(公告)号：US5110866A
公开(公告)日：1992-05-05
申请号：US493599
申请日：1990-03-05
申请人： Masafumi Hongo , Hideyuki Shigemitsu
发明人： Masafumi Hongo , Hideyuki Shigemitsu
IPC分类号： C08L51/04 , C08L51/06 , C08L67/00 , C08L67/02 , C08L69/00 , C08L71/12
CPC分类号： C08L51/04 , C08L67/02 , C08L71/123 , C08L67/00 , C08L69/00
摘要： A thermoplastic polyester resin composition having an improved impact resistance is disclosed. This composition is comprised of (A) 30 to 70 weight parts of a polyester resin composed mainly of a polyalkylene terphthalate, (B) 5 to 28 weight parts of a polycarbonate resin, (C) 5 to 35 weight parts of a graft copolymer obtained by graft-polymerizing a monomer selected from aromatic vinyl monomers and methacrylic acid ester monomers in the presence of a rubbery polymer, and (D) 10 to 45 weight parts of a polyphenylene ether resin, which further comprises (E) 2 to 20 weight parts, per 100 weight parts of the resin composition comprising the components (A) through (D), of a copolymer having a main chain of a polyolefin copolymerized with glycidyl methacrylate and a side chain of a styrene polymer, in which the content of glycidyl methacrylate in the polyolefin copolymerized with glycidyl methacrylate is 5 to 30 weight %.

2. 发明授权

US07488775B2 Graft copolymer and thermoplastic resin composition 有权
标题翻译：接枝共聚物和热塑性树脂组合物
公开(公告)号：US07488775B2
公开(公告)日：2009-02-10
申请号：US10450720
申请日：2001-12-21
申请人： Yoshihiro Nakai , Hideyuki Shigemitsu
发明人： Yoshihiro Nakai , Hideyuki Shigemitsu
IPC分类号： C08L51/00
CPC分类号： C08L51/04 , C08F265/04 , C08F291/02 , C08L33/04 , C08L33/066 , C08L33/20 , C08L51/003 , C08L51/085 , C08L2666/24 , C08L2666/02 , C08L2666/04
摘要： A thermoplastic resin composition comprising 10 to 98 parts by weight of a graft polymer (1A) containing a rubber-like polymer (1G) having a diene unit content of 50% by weight or less, 2 to 50 parts by weight of a hydroxyl group-containing acrylic copolymer (1B) and 0 to 80 parts by weight of other thermoplastic resin (1F), wherein the rubber-like polymer (1G) is at least one selected from the group consisting of a diene-based rubber, a polyorganosiloxane-based rubber and an olefin-based rubber; and, a graft copolymer (2A) obtained by grafting a vinyl-based polymer to a (meth)acrylate-based rubber-like polymer (2G) expansion-treated with an acid group-containing copolymer latex (2K) wherein the (meth)acrylate-based rubber-like polymer contains two or more poly-functional monomer units.
摘要翻译：一种热塑性树脂组合物，其包含10至98重量份的含有二烯单元含量为50重量％以下的橡胶状聚合物（1G）的接枝聚合物（1A），2〜50重量份的羟基丙烯酸共聚物（1B）和0〜80重量份的其他热塑性树脂（1F），其中，所述橡胶状聚合物（1G）为选自二烯系橡胶，聚有机硅氧烷 - 基于橡胶和烯烃的橡胶; 和通过用含酸基的共聚物胶乳（2K）进行膨胀处理的（甲基）丙烯酸酯类橡胶状聚合物（2G））接枝乙烯基系聚合物而得到的接枝共聚物（2A），其中，（甲基）丙烯酸酯系橡胶状聚合物含有2个以上的多官能单体单元。

3. 发明授权

US5049348A Method for producing thermoplastic resin compound 失效
标题翻译：热塑性树脂化合物的制造方法
公开(公告)号：US5049348A
公开(公告)日：1991-09-17
申请号：US413848
申请日：1989-09-28
申请人： Masafumi Hongo , Hideyuki Shigemitsu
发明人： Masafumi Hongo , Hideyuki Shigemitsu
IPC分类号： C08L67/00 , C08L67/02 , C08L69/00 , C08L71/12
CPC分类号： C08L71/123 , C08L67/02 , C08L67/00 , C08L69/00 , Y10S525/905
摘要： With the aim of preventing deterioration in properties of resins in the production of a thermoplastic resin compound by melting and kneading a polyester resin and a polyphenylene ether resin, a method for producing the thermoplastic resin compound comprising 30 to 70% by weight of a polyester resin (A) mainly comprising polyalkylene terephthalate and 70 to 30% by weight of a polyphenylene ether resin (B) mainly comprising polyphenylene ether comprises separately melting the component (A) and the component (B) and, after adjusting the ratio of viscosity (in poise) of the component (B) to that of the component (A) at a shear rate of 10.sup.3 (sec.sup.-1) to 10 or less, kneading the molten components (A) and (B) together.

4. 发明授权

US4755559A Thermoplastic resin composition of a polycarbonate and a vinyl aromatic-vinyl cyanide monomers/diene rubber graft copolymer 失效
标题翻译：聚碳酸酯和乙烯基芳族 - 乙烯基氰单体/二烯橡胶接枝共聚物的热塑性树脂组合物
公开(公告)号：US4755559A
公开(公告)日：1988-07-05
申请号：US806467
申请日：1985-12-09
申请人： Kazuo Kishida , Hiroshi Kawasaki , Hideyuki Shigemitsu
发明人： Kazuo Kishida , Hiroshi Kawasaki , Hideyuki Shigemitsu
IPC分类号： C08L51/00 , C08F279/02 , C08L7/00 , C08L21/00 , C08L25/00 , C08L25/12 , C08L33/00 , C08L33/02 , C08L51/02 , C08L51/04 , C08L55/02 , C08L69/00
CPC分类号： C08L51/04 , C08L25/12 , C08L55/02 , C08L69/00
摘要： A thermoplastic resin composition comrpising:(A) from 5 to 50 parts by weight of a graft copolymer obtained by graft polymerizing from 20 to less than 40 parts by weight of monomers comprising from 20 to 80% by weight of an .alpha.-alkyl aromatic vinyl monomer, from 3 to 40% by weight of an aromatic vinyl monomer containing no .alpha.-alkyl aromatic vinyl monomer, from 15 to 40% by weight of a vinyl cyanide monomer and from 0 to 35% by weight of a vinyl monomer copolymerizable with these monomers, to from more than 60 to 80 parts by weight of a diene rubber-like polymer, the total amount of the monomers and the rubber-like polymer being 100 parts by weight;(B) from 0 to 60 parts by weight of a copolymer obtained by polymerizing from 60 to 90% by weight of an aromatic vinyl monomer, from 10 to 40% by weight of a vinyl cyanide monomer and from 0 to 30% by weight of a vinyl monomer copolymerizable with these monomers; and(C) from 15 to 80 parts by weight of a polycarbonate resin;the total amount of components (A), (B) and (C) being 100 parts by weight. The composition is useful for making molded products.
摘要翻译：一种热塑性树脂组合物，其包括：（A）5至50重量份的接枝共聚物，所述接枝共聚物通过接枝聚合20至少于40重量份的包含20至80重量％的α-烷基芳族乙烯基单体，3至40重量％的不含α-烷基芳族乙烯基单体的芳族乙烯基单体，15至40重量％的乙烯基氰单体和0至35重量％可与其共聚的乙烯基单体单体，从多于60〜80重量份的二烯橡胶状聚合物，单体和橡胶状聚合物的总量为100重量份; （B）0至60重量份通过聚合60至90重量％的芳族乙烯基单体，10至40重量％的乙烯基氰单体和0至30重量％可与这些单体共聚的乙烯基单体; 和（C）15〜80重量份的聚碳酸酯树脂; 组分（A），（B）和（C）的总量为100重量份。该组合物可用于制备模塑产品。

5. 发明授权

US5284914A Thermoplastic polyester resin compound 失效
标题翻译：热塑性聚酯树脂复合物
公开(公告)号：US5284914A
公开(公告)日：1994-02-08
申请号：US692782
申请日：1991-04-26
申请人： Yutaka Toyooka , Masafumi Hongo , Hideyuki Shigemitsu
发明人： Yutaka Toyooka , Masafumi Hongo , Hideyuki Shigemitsu
IPC分类号： C08L67/02 , C08L51/04 , C08L67/03 , C08L69/00 , C08L71/12
CPC分类号： C08L67/02
摘要： A thermoplastic polyester resin composition characterized by comprising30-70% by weight of a polyester resin (A) constituted mainly of a polyalkylene terephthalate,5-35% by weight of a graft polymer (B) obtained by graft-polymerizing at least one selected from the group consisting of an aromatic vinyl monomer and a methacrylate monomer in the presence of a rubbery polymer, and10-45% by weight of a polyphenylene ether resin (C) andresulting from blending these polymers so that the content of said polyester resin (A) may be higher than that of said polyphenylene ether resin (C).
摘要翻译：一种热塑性聚酯树脂组合物，其特征在于包含30-70重量％的主要由聚对苯二甲酸亚烷基酯组成的聚酯树脂（A），5-35重量％的接枝聚合物（B），其通过接枝聚合至少一种选择的在橡胶状聚合物的存在下由芳香族乙烯基单体和甲基丙烯酸酯单体组成的组和10-45重量％的聚苯醚树脂（C）进行混合，由此将所述聚酯树脂的含量（A）可以高于所述聚苯醚树脂（C）。

6. 发明申请

US20100159134A1 RESIN COMPOSITION FOR DIRECT VAPOR DEPOSITION, MOLDED ARTICLES MADE BY USING THE SAME, AND SURFACE-METALLIZED LAMP HOUSING 有权
标题翻译：用于直接蒸发沉积的树脂组合物，使用它们的模塑制品和表面金属化的灯泡壳
公开(公告)号：US20100159134A1
公开(公告)日：2010-06-24
申请号：US12716646
申请日：2010-03-03
申请人： Yoshihiro NAKAI , Takahiro Ikebe , Keiji Obata , Hideyuki Shigemitsu
发明人： Yoshihiro NAKAI , Takahiro Ikebe , Keiji Obata , Hideyuki Shigemitsu
IPC分类号： C23C16/00
CPC分类号： C08L51/003 , C08L51/04 , C08L51/085 , Y10T428/31507 , Y10T428/31663
摘要： The direct vapor depositing resin composition of the present invention comprises at least one selected from the group consisting of (A-I): a graft copolymer obtained by graft-polymerizing one or more monomers or a monomer mixture to a complex rubber-like polymer (G) composed of a polyorganosiloxane and a (meth)acrylate-based polymer and (A-II): a graft copolymer obtained by graft-polymerizing one or more monomers or a monomer mixture including an alkyl (meth)acrylate as an essential component to a rubber-like polymer (R) in which the content of diene units is 30% by weight or less in 100% by weight of the whole rubber-like polymer. The direct vapor depositing resin composition of the present invention can provide a beautiful bright appearance after direct vapor deposition of a metal, further, has high level mechanical strengths such as impact strength and the like, and weather resistance, and is also excellent in hot plate welding property with a transparent resin such as PMMA resins, PC resins and the like.
摘要翻译：本发明的直接气相沉积树脂组合物包括选自（AI）中的至少一种：通过将一种或多种单体或单体混合物接枝聚合到复合橡胶状聚合物（G）而获得的接枝共聚物，由聚有机硅氧烷和（甲基）丙烯酸酯类聚合物组成的（A-II）：将一种或多种单体或包含（甲基）丙烯酸烷基酯作为必要成分的单体混合物接枝聚合得到的接枝共聚物，类聚合物（R），其中二烯单元的含量在全部橡胶状聚合物的100重量％中为30重量％以下。本发明的直接气相沉积树脂组合物可以在金属的直接气相沉积之后提供美观的外观，而且还具有诸如冲击强度等的高水平的机械强度和耐候性，并且在热板上也是优异的使用透明树脂如PMMA树脂，PC树脂等进行焊接。

7. 发明授权

US5346952A Blends of polyphenylene ether, aromatic vinyl resins and vinyl aromatic-vinyl heterocyclic monomer grafted butadiene based polymers 失效
标题翻译：聚苯醚，芳族乙烯基树脂和乙烯基芳族乙烯基杂环单体接枝丁二烯基聚合物的共混物
公开(公告)号：US5346952A
公开(公告)日：1994-09-13
申请号：US54838
申请日：1993-04-30
申请人： Masafumi Hongo , Hideki Yano , Hideyuki Shigemitsu
发明人： Masafumi Hongo , Hideki Yano , Hideyuki Shigemitsu
IPC分类号： C08L25/04 , C08L51/04 , C08L71/12 , C08L39/04
CPC分类号： C08L25/04 , C08L51/04 , C08L71/123 , C08L71/12 , Y10S525/905
摘要： Disclosed is a thermoplastic resin composition comprised of (A) 10-60 weight parts of a polyphenylene ether resin, (B) 20-70 weight parts of (b-1) an aromatic vinyl resin and/or (b-2) a copolymer of an aromatic vinyl monomer with a heterocyclic compound having a vinyl group and containing nitrogen as the hetero atom and (C) 10-60 weight parts of (c-1) a graft copolymer obtained by polymerizing an aromatic vinyl monomer, optionally with other vinyl monomer, in the presence of a butadiene type rubbery polymer or (c-2) a graft copolymer obtained by polymerizing an aromatic vinyl monomer and a heterocyclic compound having a vinyl group and containing nitrogen as the hereto atom, optionally with other ethylenically unsaturated compound, in the presence of a butadiene type rubbery polymer, wherein at least one of the components (B) and (C) is a polymer of the nitrogen-containing heterocyclic compound, and the total amount of the components (A), (B) and (C) is 100 parts by weight.
摘要翻译：公开了一种热塑性树脂组合物，其包含（A）10-60重量份聚苯醚树脂，（B）20-70重量份（b-1）芳族乙烯基树脂和/或（b-2）共聚物具有乙烯基并含有氮作为杂原子的杂环化合物的芳族乙烯基单体和（C）10-60重量份的（c-1）通过芳香族乙烯基单体聚合获得的接枝共聚物，任选地与其它乙烯基单体，在丁二烯型橡胶状聚合物的存在下，或（c-2）通过使芳族乙烯基单体和具有乙烯基并含有氮作为本发明原子的杂环化合物任选地与其它烯属不饱和化合物聚合而获得的接枝共聚物，在丁二烯型橡胶状聚合物的存在下，其中组分（B）和（C）中的至少一种是含氮杂环化合物的聚合物，以及组分（A），（B）和（C）为100重量份。

8. 发明授权

US4888388A Polycarbonate resin composition 失效
标题翻译：聚碳酸酯树脂组合物
公开(公告)号：US4888388A
公开(公告)日：1989-12-19
申请号：US246612
申请日：1988-09-20
申请人： Masafumi Hongo , Hideyuki Shigemitsu , Naoki Yamamoto , Akira Yanagase
发明人： Masafumi Hongo , Hideyuki Shigemitsu , Naoki Yamamoto , Akira Yanagase
IPC分类号： C08F285/00 , C08L69/00
CPC分类号： C08L69/00 , C08F285/00
摘要： A polycarbonate resin composition comprising a polycarbonate resin (A) or a mixture (A') of a polycarbonate resin with a saturated polyester resin and/or a polyester elastomer, and a compound rubber type graft copolymer (B) having at least one vinyl monomer graft-polymerized onto a compound rubber composed of from 10 to 90% by weight of a polyorganosiloxane rubber and from 10 to 90% by weight of a polyalkyl (meth)acrylate rubber in a total amount of 100% by weight in an inseparable interlocking fashion and having an average particle size of from 0.08 to 0.6 .mu.m, or a mixture (B') of such a compound rubber type graft copolymer (B) with a vinyl monomer, wherein component (B) or (B') is in an amount such that the compound rubber is from 0.5 to 60% by weight based on the entire resin composition.

9. 发明授权

US4764555A Thermoplastic resin composition 失效
标题翻译：热塑性树脂组合物
公开(公告)号：US4764555A
公开(公告)日：1988-08-16
申请号：US105728
申请日：1987-10-07
申请人： Hideyuki Shigemitsu , Masafumi Hongo , Yutaka Toyooka
发明人： Hideyuki Shigemitsu , Masafumi Hongo , Yutaka Toyooka
IPC分类号： C08L55/02 , C08L51/04 , C08L55/00 , C08L69/00
CPC分类号： C08L69/00
摘要： A thermoplastic resin composition comprising:(A) from 15 to 90 parts by weight of a polycarbonate resin;(B) from 10 to 85 parts by weight of a multi-stage graft copolymer obtained by graft polymerizing from 2 to 50 parts by weight of an acrylate monomer (b) as a monomer for the first stage graft polymerization, in the presence of from 15 to 80 parts by weight of a rubbery polymer (a) of which at least 50% by weight is constituted by butadiene units and then graft polymerizing from 18 to 83 parts by weight of vinyl monomers (c) comprising from 25 to 85% by weight of an aromatic vinyl monomer (i), from 15 to 40% by weight of a vinyl cyanide monomer (ii) and from 0 to 35% by weight of another vinyl monomer (iii) copolymerizable with these monomers, as monomers for the second stage or subsequent graft polymerization, the total amount of the monomers (i) to (iii) being 100% by weight, and the total amount of components (a) to (c) being 100 parts by weight; and(C) from 0 to 60 parts by weight of a polymer obtained by polymerizing at least one member selected from the group consisting of an aromatic vinyl monomer, a vinyl cyanide monomer and a methacrylate monomer;the total amount of components (A), (B) and (C) being 100 parts by weight.
摘要翻译：一种热塑性树脂组合物，其包含：（A）15〜90重量份的聚碳酸酯树脂; （B）10〜85重量份的多级接枝共聚物，其通过接枝聚合2〜50重量份作为第一阶段接枝聚合用单体的丙烯酸酯单体（b），在 15至80重量份的橡胶状聚合物（a），其中至少50重量％由丁二烯单元构成，然后接枝聚合18至83重量份的乙烯基单体（c），其包含25至85％的芳族乙烯基单体（i）的重量，15至40重量％的乙烯基氰单体（ii）和0至35重量％的可与这些单体共聚的乙烯基单体（iii）作为第二个单体阶段或随后的接枝聚合，单体（i）至（iii）的总量为100重量％，组分（a）至（c）的总量为100重量份; 和（C）0至60重量份通过聚合选自芳族乙烯基单体，乙烯基氰单体和甲基丙烯酸酯单体中的至少一种的聚合物获得的聚合物; 组分（A），（B）和（C）的总量为100重量份。

10. 发明授权

US07910028B2 Resin composition for direct vapor deposition, molded articles made by using the same, and surface-metallized lamp housing 有权
标题翻译：用于直接气相沉积的树脂组合物，使用该树脂组合物和表面金属化的灯壳体
公开(公告)号：US07910028B2
公开(公告)日：2011-03-22
申请号：US12716646
申请日：2010-03-03
申请人： Yoshihiro Nakai , Takahiro Ikebe , Keiji Obata , Hideyuki Shigemitsu
发明人： Yoshihiro Nakai , Takahiro Ikebe , Keiji Obata , Hideyuki Shigemitsu
IPC分类号： B29D11/00
CPC分类号： C08L51/003 , C08L51/04 , C08L51/085 , Y10T428/31507 , Y10T428/31663
摘要： The direct vapor depositing resin composition of the present invention comprises at least one selected from the group consisting of (A-I): a graft copolymer obtained by graft-polymerizing one or more monomers or a monomer mixture to a complex rubber-like polymer (G) composed of a polyorganosiloxane and a (meth)acrylate-based polymer and (A-II): a graft copolymer obtained by graft-polymerizing one or more monomers or a monomer mixture including an alkyl (meth)acrylate as an essential component to a rubber-like polymer (R) in which the content of diene units is 30% by weight or less in 100% by weight of the whole rubber-like polymer. The direct vapor depositing resin composition of the present invention can provide a beautiful bright appearance after direct vapor deposition of a metal, further, has high level mechanical strengths such as impact strength and the like, and weather resistance, and is also excellent in hot plate welding property with a transparent resin such as PMMA resins, PC resins and the like.
摘要翻译：本发明的直接气相沉积树脂组合物包括选自（AI）中的至少一种：通过将一种或多种单体或单体混合物接枝聚合到复合橡胶状聚合物（G）而获得的接枝共聚物，由聚有机硅氧烷和（甲基）丙烯酸酯类聚合物组成的（A-II）：将一种或多种单体或包含（甲基）丙烯酸烷基酯作为必要成分的单体混合物接枝聚合得到的接枝共聚物，类聚合物（R），其中二烯单元的含量在全部橡胶状聚合物的100重量％中为30重量％以下。本发明的直接气相沉积树脂组合物可以在金属的直接气相沉积之后提供美观的外观，而且还具有诸如冲击强度等的高水平的机械强度和耐候性，并且在热板上也是优异的使用透明树脂如PMMA树脂，PC树脂等进行焊接。

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