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1. 发明申请

US20120270726A1 CATALYTIC COMPOSITION AND PROCESS FOR THE TRANSALKYLATION OF AROMATIC HYDROCARBONS 有权
标题翻译：催化组合物和芳烃转化反应的方法
公开(公告)号：US20120270726A1
公开(公告)日：2012-10-25
申请号：US13454595
申请日：2012-04-24
申请人： Elena Bencini , Gianni Girotti
发明人： Elena Bencini , Gianni Girotti
IPC分类号： B01J29/08 , B01J29/70
CPC分类号： C10G29/205 , B01J29/06 , B01J29/084 , B01J29/70 , B01J29/7007 , B01J35/002 , B01J35/0026 , B01J35/10 , B01J35/1042 , B01J35/108 , B01J37/0009 , B01J2229/42 , C07C6/126 , C10G2300/1092 , C10G2300/1096 , C10G2300/301 , C10G2300/4018 , C10G2400/30 , Y02P20/52 , C07C15/085 , C07C15/073
摘要： A catalytic composition for transalkylation of aromatic hydrocarbons which contains a zeolite and an inorganic binder and has an extra-zeolitic porosity higher than or equal to 0.7 cc/g for a fraction of pores of which at least 30% have a diameter greater than 100 nanometers. A catalytic composition having a crushing strength not lower than 1.7 kg/mm and an apparent density not higher than 0.5 g/cc. A process for transalkylating polyalkylated aromatic hydrocarbons using a catalytic composition.
摘要翻译：含有沸石和无机粘合剂并具有高于或等于0.7cc / g的超沸石孔隙率的芳族烃的烷基转移的催化组合物，其中至少30％的直径大于100纳米的孔的一部分。具有不低于1.7kg / mm的破碎强度和不高于0.5g / cc的表观密度的催化组合物。使用催化组合物使多烷基化芳烃烷基转移的方法。

2. 发明授权

US06924247B2 Method for the separation of zeolites 有权
标题翻译：沸石分离方法
公开(公告)号：US06924247B2
公开(公告)日：2005-08-02
申请号：US10014853
申请日：2001-12-14
申请人： Angela Carati , Giannino Pazzuconi , Carlo Perego , Oscar Cappellazzo , Gianni Girotti
发明人： Angela Carati , Giannino Pazzuconi , Carlo Perego , Oscar Cappellazzo , Gianni Girotti
IPC分类号： B01J20/18 , B01J20/30 , B01J29/70 , C01B39/02 , B01J29/06
CPC分类号： B01J29/06 , B01J29/7007 , B01J29/7034 , C01B39/026
摘要： The object of the present invention relates to a simple, rapid and inexpensive process for effecting solid-liquid separations in the case of zeolites, also having small crystals. This process, which is particularly useful for the recovery of zeolite crystals in suspension in the crystallization water, comprises treating this suspension of crystals with an acid or one of its precursors and subjecting the resulting mixture to filtration or decanting.According to a particular aspect of the invention, the crystalline phase is separated in a mixture with oxides which can be used as ligands. Said oxides can be generated by the reagents of the zeolite preparation reagent mixture, not transformed into crystalline phase during the synthesis hydrothermal treatment, or they can be added to the suspension of crystals before the separation treatment, or again they can be generated by precursors suitably added to the crystallization slurry.
摘要翻译：本发明的目的涉及在具有小晶体的沸石的情况下实现固液分离的简单，快速和便宜的方法。对于在结晶水中悬浮的沸石晶体的回收特别有用的该方法包括用酸或其前体之一处理该晶体悬浮液，并将所得混合物过滤或倾析。根据本发明的特定方面，结晶相与可用作配体的氧化物以混合物分离。所述氧化物可以通过沸石制备试剂混合物的试剂产生，在合成水热处理期间不转化为结晶相，或者可以在分离处理之前加入到晶体悬浮液中，或者再次由前体合成生成加入到结晶浆料中。

3. 发明申请

US20100331576A1 PROCESS FOR THE PREPARATION OF TS-1 ZEOLITES 有权
标题翻译：制备TS-1沸石的方法
公开(公告)号：US20100331576A1
公开(公告)日：2010-12-30
申请号：US12808080
申请日：2008-12-03
申请人： Angela Carati , Donatella Berti , Roberto Millini , Franco Rivetti , Angela Maria Mantegazza , Gianni Girotti
发明人： Angela Carati , Donatella Berti , Roberto Millini , Franco Rivetti , Angela Maria Mantegazza , Gianni Girotti
IPC分类号： C07C249/04 , C01B39/02 , B01J29/06
CPC分类号： B01J29/89 , B01J35/023 , C01B37/005 , C01B39/085 , C07C249/04 , C07C251/44
摘要： The invention relates to a new process which allows the preparation of TS-1 zeolites in a pure phase and with a crystallinity higher than 95%, operating at reduced reaction volumes, and obtaining high productivities and extremely high crystallization yields. The particular crystalline form of the TS-1 zeolite thus prepared, is also described.
摘要翻译：本发明涉及一种新方法，其允许在纯相中制备TS-1沸石并且结晶度高于95％，在降低的反应体积下操作，并且获得高生产率和极高的结晶产率。还描述了如此制备的TS-1沸石的特定结晶形式。

4. 发明授权

US07812204B2 Process for the production of 2,6-dimethylnaphthalene 有权
标题翻译：生产2,6-二甲基萘的方法
公开(公告)号：US07812204B2
公开(公告)日：2010-10-12
申请号：US11576412
申请日：2005-11-30
申请人： Gianni Girotti , Franco Rivetti , Renzo Bignazzi
发明人： Gianni Girotti , Franco Rivetti , Renzo Bignazzi
IPC分类号： C07C5/27 , C07C6/12 , C07C2/64
CPC分类号： C07C5/2737 , C07C6/12 , C07C6/126 , C07C2529/70 , Y02P20/582 , C07C15/24
摘要： The invention relates to a multi-step chemical transformation process for the production of 2,6-dimethylnaphthalene starting from one or more naphthalene hydrocarbons or hydrocarbon blends containing the same, one or more benzene hydrocarbons and, optionally, a methylating agent reacted in the presence of a catalyst containing a zeolite belonging to the MTW structural group, where hydrogen is fed in at least one of the steps.
摘要翻译：本发明涉及从一种或多种萘烃或含有它们的烃共混物，一种或多种苯烃和任选的甲基化剂在存在下反应的生产2,6-二甲基萘的多步化学转化方法的含有属于MTW结构基团的沸石的催化剂，其中在至少一个步骤中进料氢。

5. 发明申请

US20070265480A1 Process for the Production of 2,6-Dimethylnaphthalene 有权
标题翻译： 2,6-二甲基萘的制备方法
公开(公告)号：US20070265480A1
公开(公告)日：2007-11-15
申请号：US11576412
申请日：2005-11-30
申请人： Gianni Girotti , Franco Rivetti , Renzo Bignazzi
发明人： Gianni Girotti , Franco Rivetti , Renzo Bignazzi
IPC分类号： C07C15/24
CPC分类号： C07C5/2737 , C07C6/12 , C07C6/126 , C07C2529/70 , Y02P20/582 , C07C15/24
摘要： The invention relates to a multi-step chemical transformation process for the production of 2,6-dimethylnaphthalene starting from one or more naphthalene hydrocarbons or hydrocarbon blends containing the same, one or more benzene hydrocarbons and, optionally, a methylating agent reacted in the presence of a catalyst containing a zeolite belonging to the MTW structural group, where hydrogen is fed in at least one of the steps.
摘要翻译：本发明涉及从一种或多种萘烃或含有它们的烃共混物，一种或多种苯烃和任选的甲基化剂在存在下反应的生产2,6-二甲基萘的多步化学转化方法的含有属于MTW结构基团的沸石的催化剂，其中在至少一个步骤中进料氢。

6. 发明申请

US20060258893A1 Catalytic composition and process for the transalkylation of aromatic hdrocarbons 有权
标题翻译：催化组合物和芳族羟基烷基转移的方法
公开(公告)号：US20060258893A1
公开(公告)日：2006-11-16
申请号：US10538641
申请日：2003-12-15
申请人： Elena Bencini , Gianni Girotti
发明人： Elena Bencini , Gianni Girotti
IPC分类号： C07C15/12 , B01J29/06 , B01J29/08
CPC分类号： C10G29/205 , B01J29/06 , B01J29/084 , B01J29/70 , B01J29/7007 , B01J35/002 , B01J35/0026 , B01J35/10 , B01J35/1042 , B01J35/108 , B01J37/0009 , B01J2229/42 , C07C6/126 , C10G2300/1092 , C10G2300/1096 , C10G2300/301 , C10G2300/4018 , C10G2400/30 , Y02P20/52 , C07C15/085 , C07C15/073
摘要： A catalytic composition is described for the transalkylation of aromatic hydrocarbons comprising a zeolite and an inorganic binder, characterized by an extra-zeolitic porosity, i.e. the porosity obtained by adding the mesoporosity and the macroporosity fractions present in the catalytic composition, higher than or equal to 0.7 cc/g, which is such as to consist for a fraction of at least 30% of pores having a diameter greater than 100 nanometers. These catalytic compositions have a crushing strength not lower than 1.7 kg/mm and an apparent density not higher than 0.5 g/cc. A process is also described for the transalkylation of polyalkylated aromatic hydrocarbons which uses these catalytic compositions.
摘要翻译：描述了一种催化组合物用于包含沸石和无机粘合剂的芳族烃的烷基转移，其特征在于沸石外孔隙率，即通过加入存在于催化剂组合物中的介孔度和大孔度组分得到的孔隙率，高于或等于 0.7cc / g，其为至少30％直径大于100纳米的孔的一部分。这些催化剂组合物的破碎强度不低于1.7kg / mm 2，表观密度不高于0.5g / cc。还描述了使用这些催化组合物的多烷基化芳烃的烷基转移的方法。

7. 发明授权

US09358531B2 Process for the preparation of TS-1 zeolites 有权
标题翻译：制备TS-1沸石的方法
公开(公告)号：US09358531B2
公开(公告)日：2016-06-07
申请号：US12808080
申请日：2008-12-03
申请人： Angela Carati , Donatella Berti , Roberto Millini , Franco Rivetti , Maria Angela Mantegazza , Gianni Girotti
发明人： Angela Carati , Donatella Berti , Roberto Millini , Franco Rivetti , Maria Angela Mantegazza , Gianni Girotti
IPC分类号： C01B39/08 , C01B37/00 , B01J29/89 , B01J35/02 , C07C249/04
CPC分类号： B01J29/89 , B01J35/023 , C01B37/005 , C01B39/085 , C07C249/04 , C07C251/44
摘要： The invention relates to a new process which allows the preparation of TS-1 zeolites in a pure phase and with a crystallinity higher than 95%, operating at reduced reaction volumes, and obtaining high productivities and extremely high crystallization yields. The particular crystalline form of the TS-1 zeolite thus prepared, is also described.
摘要翻译：本发明涉及一种新方法，其允许在纯相中制备TS-1沸石并且结晶度高于95％，在降低的反应体积下操作，并且获得高生产率和极高的结晶产率。还描述了如此制备的TS-1沸石的特定结晶形式。

8. 发明授权

US07524788B2 Process for the alkylation of aromatic compounds 有权
标题翻译：芳族化合物的烷基化方法
公开(公告)号：US07524788B2
公开(公告)日：2009-04-28
申请号：US10499345
申请日：2002-12-18
申请人： Gianni Girotti , Franco Rivetti , Stefano Ramello
发明人： Gianni Girotti , Franco Rivetti , Stefano Ramello
IPC分类号： B01J29/06
CPC分类号： C07C37/08 , B01J23/72 , B01J23/80 , B01J23/868 , B01J23/8892 , B01J29/072 , B01J29/7615 , B01J29/7815 , B01J35/0006 , C07C2/867 , C07C2523/06 , C07C2523/34 , C07C2523/72 , Y02P20/52 , C07C15/085 , C07C39/04
摘要： Process for preparing alkylated aromatic compounds which comprises reacting an aromatic compound with a ketone and hydrogen in the presence of a catalytic composition comprising a solid acid material and copper. A preferred aspect is to use a catalytic composition also containing one or more elements selected from elements of groups IIIA, IVA, IIIB, IVB, VB, VIB, VIIB, group VIII limited to Fe, Ru and Os, and of the series of lanthanides. A particularly preferred aspect is to use a catalytic composition containing one or more elements selected from elements of groups IIIA and VIB.
摘要翻译：制备烷基化芳族化合物的方法，其包括在包含固体酸物质和铜的催化剂组合物存在下使芳族化合物与酮和氢反应。优选的方面是使用还含有选自IIIA，IVA，IIIB，IVB，VB，VIB，VIIB族VIII族元素的元素的一种或多种元素的催化剂组合物，其限于Fe，Ru和Os，以及一系列镧系元素。特别优选的方面是使用含有选自IIIA族和VIB族元素的一种或多种元素的催化组合物。

9. 发明申请

US20070276173A1 Catalyst and Process for the Preparation of Alkylated Aromatic Hydrocarbons 有权
标题翻译：用于制备烷基化芳族烃的催化剂和方法
公开(公告)号：US20070276173A1
公开(公告)日：2007-11-29
申请号：US11630390
申请日：2005-06-21
申请人： Guido Spano' , Stefano Ramello , Gianni Girotti , Franco Rivetti , Angela Carati
发明人： Guido Spano' , Stefano Ramello , Gianni Girotti , Franco Rivetti , Angela Carati
IPC分类号： C07C6/12 , B01J29/70 , C10G29/20 , C07C2/66
CPC分类号： C10G29/205 , C10G45/64 , C10G2300/1092 , C10G2300/1096 , C10G2400/30
摘要： The present invention relates to a new zeolite having a beta-type crystalline structure, characterized by a distribution of the Lewis acid sites and Brønsted acid sites corresponding to a molar ratio [Lewis sites] [Brønsted sites] equal to or higher than 1.5. This new zeolite is useful in preparation processes of alkylated aromatic hydrocarbons through the alkylation and/or transalkylation of aromatic compounds. The preparation method of the new zeolite is also object of the present invention.
摘要翻译：本发明涉及具有β型结晶结构的新沸石，其特征在于路易斯酸位点和布朗斯台德酸位点的分布对应于等于或高于1.5的摩尔比[路易斯位点] [Brnnsted位点]。这种新沸石可用于通过芳族化合物的烷基化和/或烷基转移来制备烷基化芳烃的方法。新沸石的制备方法也是本发明的目的。

10. 发明授权

US06642172B1 Extruded catalyst based on silica/alumina gel 失效
标题翻译：基于二氧化硅/氧化铝凝胶的挤出催化剂
公开(公告)号：US06642172B1
公开(公告)日：2003-11-04
申请号：US08377829
申请日：1995-01-25
申请人： Carlo Perego , Gianluca Bassi , Gianni Girotti
发明人： Carlo Perego , Gianluca Bassi , Gianni Girotti
IPC分类号： B01J2112
CPC分类号： C07C2/10 , B01J21/12 , B01J37/0009 , B01J37/033 , C07C2521/12
摘要： A catalyst in the form of extruded bodies is disclosed, which consists of an inert binding agent and a catalytically active phase of a silica/alumina gel. The catalyst is particularly active in acid-catalysed reactions.
摘要翻译：公开了一种挤出体形式的催化剂，其由惰性粘合剂和二氧化硅/氧化铝凝胶的催化活性相组成。催化剂在酸催化反应中特别活跃。

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