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1. 发明授权

US07465778B2 Silante terminated polyurethane 有权
标题翻译： Silante封端聚氨酯
公开(公告)号：US07465778B2
公开(公告)日：2008-12-16
申请号：US10741871
申请日：2003-12-19
申请人： Richard R. Roesler , Derek L. Crawford
发明人： Richard R. Roesler , Derek L. Crawford
IPC分类号： B05D3/02 , B32B7/12 , C08G18/08 , C08G18/28 , C08G77/04 , C08J3/00 , C08K3/20 , C08L75/00 , C08L83/00 , C08L83/04 , C09J4/00 , C09J101/00 , C09J201/00
CPC分类号： C08G18/3893 , C08G18/283 , C08G18/8064 , C08G18/809 , C08G2190/00 , C08L75/04 , C09J5/06 , C09J2475/00 , Y10T428/31551 , Y10T428/31591
摘要： A curable, alkoxysilane-functional polyether urethane composition formed by combining a) a first silane terminated polyurethane prepared by reacting i) a mono-functional compounds with ii) an isocyanate component containing two isocyanate groups, the reaction product reacted with iii) a compound containing an isocyanate-reactive group and one or more reactive silane groups to form a moisture-curable, alkoxysilane-functional polyether urethane; and b) a second silane terminated polyurethane prepared by reacting i) an alkyl monofunctional alcohol, amine, and/or thiol, with ii) an isocyanate component containing two isocyanate groups, the reaction product reacted with iii) a compound containing an isocyanate-reactive group and one more reactive silane groups. The urethane composition can be used in coating, sealant and/or adhesive compositions. The coating compositions are used to form a coated substrate. The sealant and/or adhesive compositions are used in a method of joining a first adherend and a second adherend to form a bonded assembly.
摘要翻译：通过组合a）通过使i）单官能化合物与ii）含有两个异氰酸酯基团的异氰酸酯组分反应制备的第一种硅烷封端的聚氨酯形成的可固化的烷氧基硅烷官能的聚氨酯组合物，所述反应产物与iii）含有异氰酸酯反应性基团和一个或多个反应性硅烷基团以形成可湿气固化的烷氧基硅烷官能的聚醚聚氨酯; 和b）通过使i）烷基单官能醇，胺和/或硫醇与ii）含有两个异氰酸酯基团的异氰酸酯组分反应制备的第二个硅烷封端的聚氨酯，所述反应产物与iii）含有异氰酸酯反应性的化合物基团和一个以上反应性硅烷基团。聚氨酯组合物可用于涂料，密封剂和/或粘合剂组合物中。涂料组合物用于形成涂布的基材。密封剂和/或粘合剂组合物用于接合第一被粘物和第二被粘物以形成接合组件的方法。

2. 发明授权

US06833423B2 Moisture-curable, polyether urethanes with reactive silane groups and their use as sealants, adhesives and coatings 有权
标题翻译：具有反应性硅烷基团的水分固化型聚醚聚氨酯及其作为密封剂，粘合剂和涂料的用途
公开(公告)号：US06833423B2
公开(公告)日：2004-12-21
申请号：US10690954
申请日：2003-10-22
申请人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
发明人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
IPC分类号： C08G7724
CPC分类号： C08G18/3893 , C08G18/0885 , C08G18/10 , C08G18/283 , C08G18/3821 , C08G18/4866 , C08G18/718 , C08G2190/00 , C09J175/04 , C09K3/1021 , C08G18/289
摘要： A moisture curable, alkoxysilane-functional polyether urethanes containing a) 20 to 90% by weight, of a polyether urethane containing two or more reactive silane groups and polyether segments having a number average molecular weight (Mn) of at least 3000 and a degree of unsaturation of less than 0.04 milliequivalents/g, where the sum of Mn of the polyether segments averages 6000 to 20,000, and the reactive silane groups are incorporated by reaction of an isocyanate-reactive group with a compound of formula OCN—Y—Si—(X)3 (I) b) 10 to 80% by weight, of a polyether urethane containing one reactive silane group and one or more polyether segments having Mn of 1000 to 15,000, where the reactive silane groups are incorporated by the reaction of an isocyanate group with a compound of formula
摘要翻译：含有a）20〜90重量％的含有两个以上反应性硅烷基团的聚醚型聚氨酯和数均分子量（Mn）为3000以上且不饱和度的聚醚链段的湿气固化型烷氧基硅烷官能团聚氨酯小于0.04毫当量/克，其中聚醚片段的Mn的平均值为6000至20,000，并且反应性硅烷基团通过异氰酸酯反应性基团与公式的化合物的反应引入）10至80重量％含有一个反应性硅烷基团和一个或多个Mn为1000至15,000的聚醚链段的聚醚型聚氨酯，其中反应性硅烷基团通过异氰酸酯基与式

3. 发明授权

US07309753B2 Process for the preparation of moisture-curable, polyether urethanes with terminal cyclic urea reactive silane groups 有权
标题翻译：用于制备具有末端环状脲反应性硅烷基团的可湿气固化的聚醚型聚氨酯的方法
公开(公告)号：US07309753B2
公开(公告)日：2007-12-18
申请号：US10539218
申请日：2003-12-05
申请人： Richard R. Roesler , Derek L. Crawford
发明人： Richard R. Roesler , Derek L. Crawford
IPC分类号： C08G18/28 , C08G18/48 , C08G18/71 , C08G18/83
CPC分类号： C09J175/04 , C08G18/12 , C08G18/283 , C08G18/4866 , C08G77/38 , C08G2190/00 , C08L83/06 , C09D175/04 , C08G18/289 , C08L83/00
摘要： A process for preparing a moisture-curable, polyether urethane containing terminal cyclic urea/reactive silane groups by reacting at an NCO:OH equivalent ratio of 1.5:1 to 2.5:1 a) a hydroxyl component containing i) a polyether containing two hydroxyl groups and one or more polyether segments, wherein the polyether segments have a number average molecular weight of at least 3000 and a degree of unsaturation of less than 0.04 milliequivalents/g, and ii) a polyether containing one hydroxyl group and one or more polyether segments having a number average molecular weight of 1000 to 15,000, with b) an isocyanate component containing i) a compound containing two isocyanate groups, and ii) a compound containing one isocyanate group, and subsequently reacting this reaction product at an equivalent ratio of isocyanate groups to isocyanate-reactive groups of 0.8:1 to 1.1:1 with c) a compound containing an aspartate group and a reactive silane group to form an intermediate polyether urethane containing terminal non-cyclic urea/reactive silane groups and converting the non-cyclic urea groups to cyclic urea groups by reacting the intermediate polyether urethane.
摘要翻译：通过以1.5：1至2.5：1的NCO:OH当量比反应制备具有末端环状脲/反应性硅烷基团的可湿气固化的聚醚型氨基甲酸酯的方法a）含有i）含有两个羟基的聚醚的羟基组分和一个或多个聚醚链段，其中聚醚链段的数均分子量至少为3000，不饱和度小于0.04毫当量/ g，和ii）含有一个羟基的聚醚和一个或多个聚醚链段，数均分子量为1000至15,000，其中b）异氰酸酯组分，其含有i）含有两个异氰酸酯基团的化合物，和ii）含有一个异氰酸酯基团的化合物，随后使该反应产物以异氰酸酯基团的当量比与异氰酸酯反应性基团为0.8:1至1.1:1，c）含有天冬氨酸基团和反应性硅烷基团的化合物以形成中间体聚醚聚氨酯树脂通过使中间聚醚聚氨酯反应，将末端非环状尿素/反应性硅烷基团转化为环状脲基团，形成环状脲基。

4. 发明授权

US06844413B2 Moisture-curable, polyether urethanes with reactive silane groups and their use as sealants, adhesives and coatings 有权
标题翻译：具有反应性硅烷基团的水分固化型聚醚聚氨酯及其作为密封剂，粘合剂和涂料的用途
公开(公告)号：US06844413B2
公开(公告)日：2005-01-18
申请号：US10690956
申请日：2003-10-22
申请人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
发明人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
IPC分类号： C08G18/08 , C08G18/10 , C08G18/28 , C08G18/38 , C08G18/48 , C09D175/04 , C09J175/04 , C08G77/26
CPC分类号： C08G18/3893 , C08G18/0885 , C08G18/10 , C08G18/283 , C08G18/289 , C08G18/3821 , C08G18/4866 , C08G2190/00 , C09J175/04
摘要： A moisture-curable, alkoxysilane-functional polyether urethanes containing a) 20 to 90% by weight, of a polyether urethane containing two or more reactive silane groups and one or more polyether segments, where the polyether segments have a number average molecular weight (Mn) of at least 3000 and a degree of unsaturation of less than 0.04 milliequivalents/g, and the sum of Mn of all of the polyether segments per molecule averages 6000 to 20,000, and the reactive silane groups are incorporated by the reaction of an isocyanate group with a compound of formula H2N—Y—Si—(X)3 (I) b) 10 to 80% by weight, of a polyether urethane containing one reactive silane group and one or more polyether segments having Mn of 1000 to 15,000, where the reactive silane groups are incorporated by the reaction of an isocyanate group with a compound of formula
摘要翻译：含有20〜90重量％的含有两个以上反应性硅烷基团和一个以上聚醚链段的聚醚型聚氨酯的水分固化性烷氧基硅烷官能团聚氨酯，其中聚醚链段的数均分子量（Mn）至少3000，不饱和度小于0.04毫当量/ g，每个分子中所有聚醚链段的Mn的总和平均为6000至20,000，反应性硅烷基团通过异氰酸酯基团与一种化合物）10-80重量％的含有一个反应性硅烷基团的聚醚聚氨酯和一个或多个Mn为1000-15,000的聚醚链段，其中反应性硅烷基团通过异氰酸酯基团与式的化合物

5. 发明申请

US20090030146A1 Polyurethane dispersions for sealants 审中-公开
标题翻译：聚氨酯分散体用于密封剂
公开(公告)号：US20090030146A1
公开(公告)日：2009-01-29
申请号：US11880747
申请日：2007-07-24
申请人： Yuliya Berezkin , Peter D. Schmitt , Lyubov K. Gindin , Dinesh Pethiyagoda , Derek L. Crawford
发明人： Yuliya Berezkin , Peter D. Schmitt , Lyubov K. Gindin , Dinesh Pethiyagoda , Derek L. Crawford
IPC分类号： C08G18/08 , C08L75/08
CPC分类号： C09K3/1021 , C08G18/0823 , C08G18/12 , C08G18/348 , C08G18/36 , C08G18/4018 , C08G18/4277 , C08G18/4812 , C08G18/4829 , C08G18/6659 , C08G18/6696 , C08G18/722 , C08G2190/00 , C09D175/08 , C08G18/3228
摘要： An isocyanate-terminated prepolymer having an isocyanate group content of about 2 to 7% by weight is provided. The prepolymer comprises the reaction product of a) at least one polyether diol having a number average molecular weight of 3000 to 5000; b) at least one active-hydrogen containing material having a number average molecular weight of 200 to 700 and containing two or three hydroxyl groups and optionally one carboxy group; c) at least one hydroxyalkane carboxylic acid having a number average molecular weight of less than about 200; d) optionally, a polyether monol having a number average molecular weight between 400-3,000; e) optionally, a polyether triol having a number average molecular weight of 3,000 to 9,000; and f) an aliphatic and/or cycloaliphatic diisocyanate.
摘要翻译：提供异氰酸酯封端的预聚物，其异氰酸酯基含量为约2至7重量％。预聚物包含a）至少一种数均分子量为3000-5000的聚醚二醇的反应产物; b）至少一种数均分子量为200至700并含有两个或三个羟基和任选一个羧基的含活性氢的材料; c）至少一种数均分子量小于约200的羟基烷烃羧酸; d）任选地，数均分子量在400-3,000之间的聚醚单醇; e）任选地，数均分子量为3,000至9,000的聚醚三醇; 和f）脂族和/或脂环族二异氰酸酯。

6. 发明授权

US06998459B2 Polyether urethanes containing one reactive silane group and their use in moisture-curable polyether urethanes 有权
标题翻译：含有一个反应性硅烷基团的聚醚氨基甲酸酯及其在可湿气固化的聚氨酯中的用途
公开(公告)号：US06998459B2
公开(公告)日：2006-02-14
申请号：US10690931
申请日：2003-10-22
申请人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
发明人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
IPC分类号： C08G77/26
CPC分类号： C09J175/08 , C08G18/0885 , C08G18/10 , C08G18/283 , C08G18/289 , C08G18/3821 , C08G18/4825 , C08G18/718 , C08G18/755 , C08G18/778 , C08G2190/00
摘要： The present invention relates to a polyether urethane containing one reactive silane group and one or more polyether segments having a number average molecular weight of 1000 to 15,000, wherein the reactive silane groups are incorporated by the reaction of an isocyanate group with a compound corresponding to the formula wherein X represents identical or different organic groups which are inert to isocyanate groups below 100° C., provided that at least two of these groups are alkoxy or acyloxy groups, Y represents a linear or branched alkylene group containing 1 to 8 carbon atoms and R1 represents an organic group which is inert to isocyanate groups at a temperature of 100° C. or less.
摘要翻译：本发明涉及含有一个反应性硅烷基团和一个或多个数均分子量为1000至15,000的聚醚链段的聚醚型聚氨酯，其中反应性硅烷基团通过异氰酸酯基团与对应于形成

7. 发明授权

US06887964B2 Moisture-curable, polyether urethanes with reactive silane groups and their use as sealants, adhesives and coatings 有权
标题翻译：具有反应性硅烷基团的水分固化型聚醚聚氨酯及其作为密封剂，粘合剂和涂料的用途
公开(公告)号：US06887964B2
公开(公告)日：2005-05-03
申请号：US10690955
申请日：2003-10-22
申请人： Kurt C. Frisch , Derek L. Crawford , Richard R. Roesler , Karen M. Henderson , Michael D. Strohecker
发明人： Kurt C. Frisch , Derek L. Crawford , Richard R. Roesler , Karen M. Henderson , Michael D. Strohecker
IPC分类号： C08G18/10 , C08G18/12 , C08G18/28 , C08G18/38 , C08G18/48 , C08G18/71 , C08G65/336 , C08L71/02 , C09D175/04 , C09J175/04 , C09J175/12 , C08G77/26
CPC分类号： C08G18/718 , C08G18/10 , C08G18/12 , C08G18/283 , C08G18/289 , C08G18/3893 , C08G18/4866 , C08G65/336 , C08G2190/00 , C08L71/02 , C09D175/04 , C09J175/04 , C09J175/12 , Y10S528/901 , C08G18/307
摘要： A moisture-curable, alkoxysilane-functional polyether urethanes containing a) 20 to 90% by weight, based on the weight of a) and b), of a polyether urethane containing two or more reactive silane groups and one or more polyether segments, wherein the polyether segments have a number average molecular weight of at least 3000 and a degree of unsaturation of less than 0.04 milliequivalents/g, provided that the sum of the number average molecular weights of all of the polyether segments per molecule averages 6000 to 20,000, and wherein the reactive silane groups are incorporated as the reaction product of an isocyanate group with a compound corresponding to the formula b) 10 to 80% by weight, based on the weight of a) and b), of a polyether urethane containing one reactive silane group and one or more polyether segments having a number average molecular weight of 1000 to 15,000.
摘要翻译：含有a）基于a）和b）重量的20-90％重量的含有两个或更多个反应性硅烷基团和一个或多个聚醚链段的聚醚聚氨酯的湿固化型烷氧基硅烷官能聚醚聚氨酯，其中聚醚片段的数均分子量至少为3000，不饱和度小于0.04毫当量/克，条件是每个分子中所有聚醚链段的数均分子量之和平均为6000至20,000，而其中反应性硅烷基团作为异氰酸酯基团与对应于式b）的化合物的反应产物引入含有一个反应性硅烷的聚醚聚氨酯的基于a）和b）的重量为10至80重量％基团和一个或多个数均分子量为1000至15,000的聚醚链段。

8. 发明授权

US07115696B2 Moisture-curable, polyether urethanes with reactive silane groups and their use as sealants, adhesives and coatings 有权
公开(公告)号：US07115696B2
公开(公告)日：2006-10-03
申请号：US10690751
申请日：2003-10-22
申请人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
发明人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Dinesh Pethiyagoda , Karsten Danielmeier
IPC分类号： C08G77/24
CPC分类号： C09J175/08 , C08G18/10 , C08G18/283 , C08G18/4866 , C08G2190/00 , C08G18/289
摘要： A moisture-curable, alkoxysilane-functional polyether urethanes containing a) 20 to 90% by weight, of a polyether urethane containing two or more reactive silane groups and one or more polyether segments, where the polyether segments have a number average molecular weight (Mn) of at least 3000 and a degree of unsaturation of less than 0.04 milliequivalents/g, and the sum of Mn of all of the polyether segments per molecule averages 6000 to 20,000, and the reactive silane groups are incorporated by the reaction of an isocyanate group with a compound of formula and b) 10 to 80% by weight, of a polyether urethane containing one reactive silane group and one or more polyether segments having Mn of 1000 to 15,000.

9. 发明授权

US06809170B2 Moisture-curable, polyether urethanes with reactive silane groups and their use as sealants, adhesive and coatings 失效
标题翻译：具有反应性硅烷基团的水分固化型聚醚聚氨酯及其作为密封剂，粘合剂和涂料的用途
公开(公告)号：US06809170B2
公开(公告)日：2004-10-26
申请号：US10690953
申请日：2003-10-22
申请人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Karsten Danielmeier , Dinesh Pethiyagoda , Gerhard Ruttmann
发明人： Richard R. Roesler , Derek L. Crawford , Kurt C. Frisch , Karsten Danielmeier , Dinesh Pethiyagoda , Gerhard Ruttmann
IPC分类号： C08G7726
CPC分类号： C08G18/4866 , C08G18/0885 , C08G18/283 , C08G18/289 , C08G18/4825 , C08G2190/00
摘要： Preparation of moisture-curable, alkoxysilane-functional polyether urethanes by reacting at an NCO:OH equivalent ratio of 1.5:1 to 2.5:1 a) a hydroxyl component containing i) 20 to 100 wt. %, of a polyether diol and other polyether segments, where the polyether segments have Mn of at least 3000 and degree of unsaturation of less than 0.04 meq/g, where the sum of Mn of polyether segments per molecule averages 6000 to 20,000, and ii) 0 to 80 wt. % of a polyether monool and other polyether segments having Mn of 1000 to 15,000, with b) an isocyanate component containing i) 20 to 100 wt. % of a diisocyanate, and ii) 0 to 80 wt. % of a monoisocyanate, forming an isocyanate-containing reaction product reacted at an equivalent ratio of 0.8:1 to 1.1:1 with c) a compound containing an isocyanate-reactive group and reactive silane groups where at least 10 mole % is a compound of formula

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