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1. 发明授权

US09200207B2 Methods of producing liquid hydrocarbon fuels from solid plastic wastes 有权
标题翻译：从固体塑料废物生产液体烃燃料的方法
公开(公告)号：US09200207B2
公开(公告)日：2015-12-01
申请号：US13484359
申请日：2012-05-31
申请人： Cunping Huang , Amit Gujar , Marianne Rodgers
发明人： Cunping Huang , Amit Gujar , Marianne Rodgers
IPC分类号： C10B57/04 , C10G1/10 , C10G1/00 , C10B53/07 , C10L5/40
CPC分类号： C10G1/10 , C10B53/07 , C10G1/002 , C10G2300/1003 , C10G2400/02 , C10G2400/04 , C10L5/406
摘要： A method of producing liquid hydrocarbon fuels for solid waste plastic by reacting the waste plastic with a metal hydride and a supported catalyst which is mixed and then gasified to produce liquid hydrocarbons is described.
摘要翻译：描述了通过使废塑料与金属氢化物和负载的催化剂反应生产液体烃燃料用于固体废塑料的方法，该催化剂混合然后气化以产生液体烃。

2. 发明申请

US20090188164A1 METHOD AND SYSTEM FOR HYDROGEN SULFIDE REMOVAL 审中-公开
标题翻译：硫化氢去除方法与系统
公开(公告)号：US20090188164A1
公开(公告)日：2009-07-30
申请号：US12359858
申请日：2009-01-26
申请人： CUNPING HUANG , FRANKLYN SMITH , CLOVIS A. LINKOUS , KARTHIKEYAN RAMASAMY , ALI T. RAISSI , NAZIM MURADOV
发明人： CUNPING HUANG , FRANKLYN SMITH , CLOVIS A. LINKOUS , KARTHIKEYAN RAMASAMY , ALI T. RAISSI , NAZIM MURADOV
IPC分类号： C10L3/10 , B01J8/00
CPC分类号： C10L3/10 , B01D53/52 , B01D53/965 , B01D2257/304 , C01B17/05 , C10L3/102
摘要： A method and system for hydrogen sulfide removal from a sour gas mixture including hydrogen sulfide includes providing an aqueous solution comprising a transition metal oxide, sulfide or carbonate compound, wherein a transition metal of the transition metal oxide is at a first valence and has at least one reduction state from the first valence. The sour gas mixture is reacted with the transition metal compound and the aqueous solution in a reactor, wherein sulfide from the hydrogen sulfide is oxidized to form elemental sulfur and the transition metal is reduced to form a reduced state transition metal compound. An electrochemical redox reaction is performed including the reduced state transition metal compound to regenerate the transition metal compound in an electrolyzer comprising an anode, a cathode, and an electrolyte membrane between the anode and cathode, wherein an oxygen including gas is added to the cathode during the electrochemical redox reaction. The transition metal compound that is regenerated in the electrochemical redox reaction is then returned to the reactor for the reacting.
摘要翻译：从包含硫化氢的酸性气体混合物中除去硫化氢的方法和系统包括提供包含过渡金属氧化物，硫化物或碳酸盐化合物的水溶液，其中过渡金属氧化物的过渡金属处于第一化合价并且至少具有一个还原状态从第一价。酸性气体混合物与反应器中的过渡金属化合物和水溶液反应，其中来自硫化氢的硫化物被氧化以形成元素硫，并且过渡金属被还原以形成还原态过渡金属化合物。进行电化学氧化还原反应，包括还原态过渡金属化合物，以在包括阳极和阴极之间的阳极，阴极和电解质膜的电解槽中再生过渡金属化合物，其中在阴极中加入包含气体的氧气电化学氧化还原反应。然后在电化学氧化还原反应中再生的过渡金属化合物返回反应器进行反应。

3. 发明授权

US08691068B1 Solar metal sulfate-ammonia based thermochemical water splitting cycle for hydrogen production 有权
标题翻译：用于氢气生产的太阳能金属硫酸铵 - 氨基热化学水分解循环
公开(公告)号：US08691068B1
公开(公告)日：2014-04-08
申请号：US12267569
申请日：2008-11-08
申请人： Cunping Huang , Ali T-Raissi , Nazim Muradov
发明人： Cunping Huang , Ali T-Raissi , Nazim Muradov
IPC分类号： C25B1/02 , C01C1/246 , C01B17/50 , C25B1/00
CPC分类号： C25B1/003 , C01B3/06 , C01B13/0203 , C01B17/504 , C25B1/02 , Y02E60/368
摘要： Two classes of hybrid/thermochemical water splitting processes for the production of hydrogen and oxygen have been proposed based on (1) metal sulfate-ammonia cycles (2) metal pyrosulfate-ammonia cycles. Methods and systems for a metal sulfate MSO4—NH3 cycle for producing H2 and O2 from a closed system including feeding an aqueous (NH3)4SO3 solution into a photoctalytic reactor to oxidize the aqueous (NH3)4SO3 into aqueous (NH3)2SO4 and reduce water to hydrogen, mixing the resulting aqueous (NH3)2SO4 with metal oxide (e.g. ZnO) to form a slurry, heating the slurry of aqueous (NH4)2SO4 and ZnO(s) in the low temperature reactor to produce a gaseous mixture of NH3 and H2O and solid ZnSO4(s), heating solid ZnSO4 at a high temperature reactor to produce a gaseous mixture of SO2 and O2 and solid product ZnO, mixing the gaseous mixture of SO2 and O2 with an NH3 and H2O stream in an absorber to form aqueous (NH4)2SO3 solution and separate O2 for aqueous solution, recycling the resultant solution back to the photoreactor and sending ZnO to mix with aqueous (NH4)2SO4 solution to close the water splitting cycle wherein gaseous H2 and O2 are the only products output from the closed ZnSO4—NH3 cycle.
摘要翻译：已经提出了基于（1）金属硫酸盐 - 氨循环（2）金属硫酸氢铵 - 氨循环的两类用于生产氢和氧的混合/热化学水分解方法。用于从封闭系统生产H 2和O 2的金属硫酸盐MSO4-NH3循环的方法和系统，包括将（NH 3）4 SO 3水溶液进料到光催化反应器中，以将（NH 3）4 SO 3水溶液氧化成NH 3水溶液并减少水将氢（NH 3）2 SO 4与金属氧化物（例如ZnO）混合以形成浆料，在低温反应器中加热（NH 4）2 SO 4水溶液和ZnO的浆液以产生NH 3和 H 2 O和固体ZnSO 4，在高温反应器中加热固体ZnSO 4以产生SO 2和O 2的气体混合物和固体产物ZnO，将SO 2和O 2的气体混合物与NH 3和H 2 O流混合在吸收器中以形成水溶液（NH4）2SO3溶液和分离的O 2用于水溶液，将所得溶液再循环回光反应器，并将ZnO与（NH 4）2 SO 4水溶液混合以封闭水分解循环，其中气体H 2和O 2是从封闭的ZnSO4-NH3c ycle。

4. 发明授权

US08647497B2 Method and system for hydrogen sulfide removal 有权
标题翻译：硫化氢去除方法和系统
公开(公告)号：US08647497B2
公开(公告)日：2014-02-11
申请号：US13352016
申请日：2012-01-17
申请人： Cunping Huang , Franklyn Smith , Clovis A. Linkous , Karthikeyan Ramasamy , Ali T. Raissi , Nazim Muradov
发明人： Cunping Huang , Franklyn Smith , Clovis A. Linkous , Karthikeyan Ramasamy , Ali T. Raissi , Nazim Muradov
IPC分类号： C01B17/05 , B01D53/52
CPC分类号： B01D53/52 , B01D53/965 , B01D2257/304 , C01B17/05 , C10L3/10 , C10L3/102
摘要： A system for hydrogen sulfide removal from a sour gas mixture including hydrogen sulfide. The sour gas mixture is reacted with a transition metal compound in a scrubber. Sulfide from the hydrogen sulfide is oxidized to form elemental sulfur and the transition metal is reduced to form a reduced state transition metal compound. An electrochemical redox reaction is performed including the reduced state transition metal compound to regenerate the transition metal compound in an electrolyzer including a power source. During the electrochemical redox reaction a voltage from the power source applied to the electrolyzer is controlled to regenerate the transition metal compound at a rate sufficient to match a flow rate of hydrogen sulfide into the scrubber or maintain a predetermined maximum hydrogen sulfide level out from the scrubber. The transition metal compound regenerated is returned to the scrubber for the reacting.
摘要翻译：从包含硫化氢的酸性气体混合物中除去硫化氢的系统。酸性气体混合物与洗涤器中的过渡金属化合物反应。来自硫化氢的硫化物被氧化形成元素硫并且过渡金属被还原以形成还原态的过渡金属化合物。进行电化学氧化还原反应，包括还原态过渡金属化合物以在包括电源的电解器中再生过渡金属化合物。在电化学氧化还原反应期间，控制施加到电解器的电源的电压，以使硫化氢流入洗涤器中或将洗涤器中保持预定最大硫化氢水平的速率重新生成过渡金属化合物。再生过渡金属化合物返回洗涤器进行反应。

5. 发明申请

US20120148465A1 METHOD AND SYSTEM FOR HYDROGEN SULFIDE REMOVAL 有权
标题翻译：硫化氢去除方法与系统
公开(公告)号：US20120148465A1
公开(公告)日：2012-06-14
申请号：US13352016
申请日：2012-01-17
申请人： CUNPING HUANG , FRANKLYN SMITH , CLOVIS A. LINKOUS , KARTHIKEYAN RAMASAMY , ALI T. RAISSI , NAZIM MURADOV
发明人： CUNPING HUANG , FRANKLYN SMITH , CLOVIS A. LINKOUS , KARTHIKEYAN RAMASAMY , ALI T. RAISSI , NAZIM MURADOV
IPC分类号： B01D53/52 , C01B17/05
CPC分类号： B01D53/52 , B01D53/965 , B01D2257/304 , C01B17/05 , C10L3/10 , C10L3/102
摘要： A system for hydrogen sulfide removal from a sour gas mixture including hydrogen sulfide. The sour gas mixture is reacted with a transition metal compound in a scrubber. Sulfide from the hydrogen sulfide is oxidized to form elemental sulfur and the transition metal is reduced to form a reduced state transition metal compound. An electrochemical redox reaction is performed including the reduced state transition metal compound to regenerate the transition metal compound in an electrolyzer including a power source. During the electrochemical redox reaction a voltage from the power source applied to the electrolyzer is controlled to regenerate the transition metal compound at a rate sufficient to match a flow rate of hydrogen sulfide into the scrubber or maintain a predetermined maximum hydrogen sulfide level out from the scrubber. The transition metal compound regenerated is returned to the scrubber for the reacting.
摘要翻译：从包含硫化氢的酸性气体混合物中除去硫化氢的系统。酸性气体混合物与洗涤器中的过渡金属化合物反应。来自硫化氢的硫化物被氧化形成元素硫并且过渡金属被还原以形成还原态的过渡金属化合物。进行电化学氧化还原反应，包括还原态过渡金属化合物以在包括电源的电解器中再生过渡金属化合物。在电化学氧化还原反应期间，控制施加到电解器的电源的电压，以使硫化氢流入洗涤器中或将洗涤器中保持预定最大硫化氢水平的速率重新生成过渡金属化合物。再生过渡金属化合物返回洗涤器进行反应。

6. 发明授权

US07332146B1 Method for zero emission liquid hydrogen production from methane and landfill gas 有权
标题翻译：从甲烷和填埋气中零排放液氢生产方法
公开(公告)号：US07332146B1
公开(公告)日：2008-02-19
申请号：US11148778
申请日：2005-06-08
申请人： Cunping Huang , Nazim Muradov , Ali T. Raissi
发明人： Cunping Huang , Nazim Muradov , Ali T. Raissi
IPC分类号： C01B3/02 , C01B3/22 , C01B3/24 , C01B3/26 , C01B31/20
CPC分类号： C01B3/506 , C01B32/50 , C01B2203/0233 , C01B2203/025 , C01B2203/0266 , C01B2203/0283 , C01B2203/046 , C01B2203/047 , C01B2203/0475 , C01B2203/049 , C01B2203/0495 , C01B2203/0844 , C01B2203/1241 , C01B2203/141 , C01B2203/142 , C01B2203/148 , F25J3/0209 , F25J3/0223 , F25J3/0233 , F25J3/0252 , F25J3/0257 , F25J3/0261 , F25J3/0266 , F25J3/061 , F25J3/0625 , F25J3/0635 , F25J3/0655 , F25J3/0665 , F25J3/067 , F25J2200/74 , F25J2210/66 , F25J2215/04 , F25J2220/02 , F25J2245/02 , F25J2260/20 , F25J2260/30 , F25J2270/90 , Y02C10/12 , Y02P20/152
摘要： Processes, methods, systems and devices for zero emission liquid hydrogen production directly from a variety of methane sources, such as natural gas and landfill gas, are disclosed. Five embodiments of plant designs for liquid hydrogen production are presented. The embodiments combine hydrogen production and liquefaction into a single process to produce liquid hydrogen directly via methane containing gases; thus, eliminating the conventional technology of pressure swing adsorption process for gas mixture separation. The innovative process can be applied to produce high purity liquid hydrogen with no carbon dioxide emission to the atmosphere; and can also co-produce highly pure solid carbon and liquid carbon dioxide as by-products for industrial application. The invention has provided advantages over conventional approaches that result in up to approximately 85% of first low efficiencies and approximately 56% of second law efficiency, up to approximately 100% of hydrogen and methane recovery, and a very high purity of liquid hydrogen (99.9999%).
摘要翻译：公开了直接来自各种甲烷源（例如天然气和填埋气体）的用于零排放液态氢生产的方法，方法，系统和装置。介绍了液态氢生产工厂设计的五个实施例。这些实施例将氢气生产和液化组合成单一工艺，直接通过含甲烷气体产生液态氢; 因此，消除了用于气体混合物分离的变压吸附过程的常规技术。创新的工艺可以应用于生产高纯度液态氢，没有二氧化碳排放到大气中; 并且还可以共同生产高纯度固体碳和液态二氧化碳作为工业应用的副产物。本发明提供了优于常规方法的优点，其导致高达约85％的第一低效率和约56％的第二定律效率，高达约100％的氢气和甲烷回收率以及非常高的液态氢纯度（99.9999 ％）。

7. 发明授权

US09263756B1 Electrochemical method for the removal of PPM levels of carbon monoxide from hydrogen for a fuel cell 有权
标题翻译：用于从燃料电池的氢气中去除一氧化碳的PPM水平的电化学方法
公开(公告)号：US09263756B1
公开(公告)日：2016-02-16
申请号：US11732794
申请日：2007-04-04
申请人： Cunping Huang , Ruichun Jiang , Mohamed Elbaccouch , Nazim Muradov , James M. Fenton
发明人： Cunping Huang , Ruichun Jiang , Mohamed Elbaccouch , Nazim Muradov , James M. Fenton
IPC分类号： H01M8/06 , H01M8/10 , H01M8/04
CPC分类号： H01M8/0668 , C25B1/00 , C25B1/02 , C25B15/08 , H01M8/04126 , H01M8/0662 , H01M8/0675 , H01M8/1018 , H01M16/00 , H01M2008/1095
摘要： An electrochemical water gas shift system for removing low level carbon monoxide from hydrogen stream. The system including an electrolyzer having a porous anode for absorbing carbon monoxide from a hydrogen stream as a feed stream for a polymer electrolyte membrane fuel cell for generating an electrical energy, a small portion of electricity generated by the fuel cell is applied to the electrolyzer to convert carbon monoxide adsorbed in the porous anode to carbon dioxide and hydrogen via an electrochemical gas shift reaction without oxygen or air input. In an embodiment, the system includes a first electrolyzer operating as a CO adsorber and a second electrolyzer connected in parallel with the first electrolyzer operating as a CO remover. Two electrolyzers can be operated alternatively as CO adsorber and CO remover.
摘要翻译：一种用于从氢气流中去除低浓度一氧化碳的电化学水煤气变换系统。该系统包括具有用于从氢气流吸收一氧化碳的多孔阳极的电解器，作为用于产生电能的聚合物电解质膜燃料电池的进料流，将由燃料电池产生的小部分电力施加到电解器通过无氧或空气输入的电化学气体转换反应将吸附在多孔阳极中的一氧化碳转化为二氧化碳和氢气。在一个实施例中，系统包括作为CO吸附器操作的第一电解器和与作为CO去除器操作的第一电解器并联连接的第二电解器。可以使用两个电解槽作为CO吸附剂和CO去除剂。

8. 发明申请

US20120310023A1 Methods of Producing Liquid Hydrocarbon Fuels from Solid Plastic Wastes 有权
标题翻译：固体塑料废料生产液体烃燃料的方法
公开(公告)号：US20120310023A1
公开(公告)日：2012-12-06
申请号：US13484359
申请日：2012-05-31
申请人： Cunping Huang , Amit Gujar , Marianne Rodgers
发明人： Cunping Huang , Amit Gujar , Marianne Rodgers
IPC分类号： C10G1/02
CPC分类号： C10G1/10 , C10B53/07 , C10G1/002 , C10G2300/1003 , C10G2400/02 , C10G2400/04 , C10L5/406
摘要： Embodiments of the present disclosure provide methods of producing high quality liquid fuels from solid plastic waste, high quality liquid fuels, and the like.
摘要翻译：本公开的实施方案提供了从固体塑料废物，高质量液体燃料等生产高质量液体燃料的方法。

9. 发明授权

US08207081B1 Nanocomposite for photocatalytic Hydrogen production and method for its preparation 有权
标题翻译：纳米复合材料用于光催化氢生产及其制备方法
公开(公告)号：US08207081B1
公开(公告)日：2012-06-26
申请号：US12715759
申请日：2010-03-02
申请人： Cunping Huang , Weifeng Yao , Nazim Muradov , Ali Raissi
发明人： Cunping Huang , Weifeng Yao , Nazim Muradov , Ali Raissi
IPC分类号： B01J27/047 , B01J27/043 , B01J27/045 , B01J23/00
CPC分类号： B01J23/6522 , B01J23/40 , B01J23/60 , B01J35/0013 , B01J35/004 , B01J37/0219 , B01J37/0221 , B01J37/035 , B01J37/16
摘要： A novel M—Pd—Cr2O3 (M═Pt, Ru, Rh, Os, Au and Ag) nanocomposite cocatalysts and its preparation method. The cocatalysts loaded on CdS photocatalyst enhances the photocatalytic activities toward H2 evolution from aqueous solutions (NH4)2SO3, a regenerable electron donor, under sunlight radiation. An embodiment provides a new and facile method and system for the preparation of M—Pd—Cr2O3 nanocomposite cocatalysts at room temperature. Pd—Cr2O3 loaded CdS photocatalyst has higher hydrogen evolution activity than that of a plain Pd metal loaded CdS and its performance is comparable to that of Pt/CdS photocatalyst. Formation of a Pd—Cr2O3 composite with reduced size of nanoparticles results in an increase in the photocatalyst activity for H2 evolution.
摘要翻译：一种新型的M-Pd-Cr2O3（M = Pt，Ru，Rh，Os，Au和Ag）纳米复合助催化剂及其制备方法。负载在CdS光催化剂上的助催化剂增强了在阳光辐射下从水溶液（NH4）2SO3（可再生电子给体）中向H2逸出的光催化活性。一个实施例提供了一种用于在室温下制备M-Pd-Cr2O3纳米复合助催化剂的新颖且简便的方法和系统。 Pd-Cr2O3负载的CdS光催化剂具有比平坦Pd金属负载的CdS更高的析氢活性，其性能与Pt / CdS光催化剂相当。形成具有减小尺寸的纳米颗粒的Pd-Cr2O3复合物导致用于H 2析出的光催化剂活性的增加。

10. 发明申请

US20080289951A1 Thermochemical Cycle for Production of Hydrogen and/or Oxygen Via Water Splitting Processes 审中-公开
标题翻译：通过水分离工艺生产氢和/或氧的热化学循环
公开(公告)号：US20080289951A1
公开(公告)日：2008-11-27
申请号：US12092674
申请日：2006-06-27
申请人： Cunping Huang , Ali Tabatabaie-Raissi , Nazim Muradov
发明人： Cunping Huang , Ali Tabatabaie-Raissi , Nazim Muradov
IPC分类号： C01B17/44 , C01B3/54 , C01B13/02 , C01B3/08
CPC分类号： C01B3/042 , C01B3/06 , C01B13/0207 , Y02E60/364 , Y02P20/134
摘要： A method for the production of hydrogen via thermochemical water splitting includes the steps of providing an ammonium sulfite compound, dissolving the ammonium sulfite in water, and oxidizing the aqueous ammonium sulfite solution, wherein hydrogen is produced as a water reduction product associated with the oxidation. If purified air is used instead for the oxidation of aqueous ammonium sulfite solution, the method produces oxygen from the purified air. In a preferred embodiment of the invention, the oxidation is a photooxidation. Light for the photoxidation can be provide by a direct light source, such as solar energy, or indirectly from conversion of electrical energy to light, such as using a UV or visible light lamp. Electrical energy can be provided by a variety of sources, including low cost sources comprising wind driven, water driven (hydroelectric), or nuclear power.
摘要翻译：通过热化学水分解生产氢气的方法包括提供亚硫酸铵化合物，将亚硫酸铵溶解在水中并氧化亚硫酸氢铵水溶液的步骤，其中产生氢作为与氧化相关的减水产物。如果使用净化空气来代替亚硫酸铵水溶液的氧化，则该方法从净化空气中产生氧气。在本发明的优选实施方案中，氧化是光氧化反应。用于光氧化的光可以通过诸如太阳能的直接光源提供，或者可以间接地将电能转换成光，例如使用UV或可见光灯。电能可以由各种来源提供，包括包括风力驱动，水驱（水力发电）或核能的低成本来源。

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