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1. 发明申请

WO2008122636A3 STEAM OR WATER TREATMENT OF A CATALYST PRECURSOR IN ORDER TO OBTAIN AN EGG SHELL FT CATALYST 审中-公开
标题翻译：催化剂前驱体的蒸汽或水处理在订购EGG壳体FT催化剂
公开(公告)号：WO2008122636A3
公开(公告)日：2009-01-15
申请号：PCT/EP2008054185
申请日：2008-04-08
申请人： SHELL INT RESEARCH , CALIS HANS PETER ALEXANDER , REYNHOUT MARINUS JOHANNES , VERBIST GUY LODE MAGDA MARIA
发明人： CALIS HANS PETER ALEXANDER , REYNHOUT MARINUS JOHANNES , VERBIST GUY LODE MAGDA MARIA
IPC分类号： B01J21/00 , B01J21/04 , B01J21/08 , B01J21/12 , B01J21/20 , B01J23/745 , B01J23/75 , B01J23/755 , B01J23/94 , B01J35/00 , B01J37/06 , B01J38/48 , C07C1/04 , C10G2/00
CPC分类号： B01J37/06 , B01J21/063 , B01J23/74 , B01J23/75 , B01J23/8892 , B01J23/94 , B01J35/0093 , B01J37/0009 , B01J37/10 , B01J37/14 , B01J37/18 , C10G2/33 , C10G2/332
摘要： process for preparing a Fischer-Tropsch catalyst comprising the steps of a) providing a particle comprising a support and having a catalytically active metal homogenously distributed therein, whereby at least 50 wt% of the catalytically active metal is present as divalent oxide or divalent hydroxide; b) treating the particle with a water vapour comprising gas having a relative humidity of at least 80% or with liquid water for at least two hours; and c) drying the catalyst particle.
摘要翻译：制备费 - 托催化剂的方法包括以下步骤：a）提供包含载体和均匀分布在其中的催化活性金属的颗粒，由此至少50wt％的催化活性金属以二价氧化物或二价氢氧化物存在; b）用包含相对湿度至少为80％的气体或液体水的水蒸气处理颗粒至少2小时; 和c）干燥催化剂颗粒。

2. 发明申请

WO2008087149A1 CATALYST, CATALYST PRECURSOR, CATALYST CARRIER, PREPARATION AND USE OF THEREOF IN FISCHER-TROPSCH SYNTHESIS 审中-公开
标题翻译：催化剂，催化剂前体，催化剂载体，其在FISCHER-TROPSCH合成中的制备和使用
公开(公告)号：WO2008087149A1
公开(公告)日：2008-07-24
申请号：PCT/EP2008/050418
申请日：2008-01-16
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , CALIS, Hans Peter Alexander , VERBIST, Guy Lode Magda Maria
发明人： CALIS, Hans Peter Alexander , VERBIST, Guy Lode Magda Maria
IPC分类号： B01J35/02 , B01J23/75 , B01J23/889 , B01J37/00 , C10G2/00 , B01J23/74 , B01J23/40 , C10G47/02
CPC分类号： B01J35/026 , B01J21/06 , B01J21/063 , B01J23/40 , B01J23/74 , B01J23/745 , B01J23/75 , B01J23/8472 , B01J23/8892 , B01J37/0009 , C10G2/332 , C10G47/02 , Y10T428/2982
摘要： A catalyst, catalyst precursor, or catalyst carrier formed as an elongated shaped particle having a cross section comprising three protrusions each extending from and attached to a central position. The central position is aligned along the longitudinal axis of the particle. The cross-section of the particle occupies the space encompassed by the outer edges of six outer circles around a central circle, each of the six outer circles contacting two neighbouring outer circles, the particle occupying three alternating outer circles equidistant to the central circle and the six interstitial regions, the particle not occupying the three remaining outer circles which are between the alternating occupied outer circles. The ratio of the diameter of the central circle to the diameter of the outer occupied circle is more than 1, and the ratio of the diameter of the outer unoccupied circle to the diameter of the outer occupied circle is more than (1). The ratio of the diameter of the outer unoccupied circle to the diameter of the outer occupied circle is more than the ratio of the diameter of the central circle to the diameter of the outer occupied circle.
摘要翻译：形成为细长形状的颗粒的催化剂，催化剂前体或催化剂载体，其具有包括从中心位置延伸并连接到中心位置的三个突起的横截面。中心位置沿着颗粒的纵向轴线排列。颗粒的横截面占据围绕中心圆的六个外圆的外边缘包围的空间，六个外圆中的每一个与两个相邻的外圆接触，颗粒占据与中心圆等距的三个交替的外圆，并且六个间隙区域，颗粒不占据交替占据的外圆之间的三个剩余的外圆。中心圆的直径与外部占有圆的直径之比大于1，外部空心圆的直径与外部占有圆的直径之比大于（1）。外部未占空心圆的直径与外部占有圆的直径的比率大于中心圆的直径与外部占有圆的直径的比率。

3. 发明申请

WO2004002927A1 PROCESS FOR THE PREPARATION OF HYDROCARBONS 审中-公开
标题翻译：制备油料的方法
公开(公告)号：WO2004002927A1
公开(公告)日：2004-01-08
申请号：PCT/EP2003/006449
申请日：2003-06-18
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , CALIS, Hans, Peter, Alexander , GROENEVELD, Michiel, Jan , VERBIST, Guy, Lode, Magda, Maria
发明人： CALIS, Hans, Peter, Alexander , GROENEVELD, Michiel, Jan , VERBIST, Guy, Lode, Magda, Maria
IPC分类号： C07C1/04
CPC分类号： C10G2/32
摘要： The invention concerns a process for the preparation of hydrocarbons and generation of heat of carbon monoxide and hydrogen in the presence of a catalyst at elevated temperature and pressure in at least two stages which comprises: (i) introducing a gas comprising carbon monoxide and hydrogen into a first reactor section comprising catalyst and introducing cooling fluidum into this first reactor section; (ii) allowing a part of the carbon monoxide to react catalytically in the first reactor section to hydrocarbons and water, at least part of the reaction heat being absorbed directly by the cooling fluidum; (iii) withdrawing from the reactor section a stream consisting of the reaction product comprising the hydrocarbons, water, unconverted feed and cooling fluidum; (iv) cooling down at least a part of the withdrawn stream comprising cooling fluidum to generate heat; (v) optionally removing water from the withdrawn stream; (vi) repeating at least once steps i-v with the stream obtained in step v in further reactor section(s). The invention further relates to a reactor suitable for carrying out the above process.
摘要翻译：本发明涉及在至少两个阶段的高温和高压下在催化剂存在下制备碳氢化合物和产生一氧化碳和氢气的方法，包括：（i）将包含一氧化碳和氢气的气体引入第一反应器部分，包括催化剂并将冷却流体引入到该第一反应器部分中; （ii）允许一部分一氧化碳在第一反应器部分中催化反应成烃和水，至少部分反应热被冷却流体直接吸收; （iii）从反应器部分抽出由包含烃，水，未转化的进料和冷却流体的反应产物组成的料流; （iv）冷却至少部分包括冷却流体的排出物流以产生热量; （v）任选地从排出的流中除去水; （vi）用另外的反应器部分中的步骤v中获得的流重复至少一次步骤i-v。本发明还涉及一种适于实施上述方法的反应器。

4. 发明申请

WO1998006495A1 METHOD FOR PREPARING A COMPOSITE CATALYST 审中-公开
标题翻译：制备复合催化剂的方法
公开(公告)号：WO1998006495A1
公开(公告)日：1998-02-19
申请号：PCT/NL1997000461
申请日：1997-08-11
申请人： TECHNISCHE UNIVERSITEIT DELFT , VAN DER PUIL, Nelleke , CALIS, Hans, Peter, Alexander , OUDSHOORN, Otto, Leonard , JANSEN, Jacobus, Cornelis , VAN BEKKUM, Herman
发明人： TECHNISCHE UNIVERSITEIT DELFT
IPC分类号： B01J37/02
CPC分类号： B01J37/0246 , B01J2229/60
摘要： The invention relates to the preparation of composite catalysts consisting of a support material and a molecular sieve crystal phase that is present on the surface of the support material. The molecular sieve crystals can, as desired, be provided both on the inside and on the outside of a porous support material. With the method according to the invention a faster preparation of a composite with a higher crystal load and a better accessibility of the individual zeolite crystals can be realized. Further, the invention relates to the use of template on a support material for inducing in situ nucleation.
摘要翻译：本发明涉及由载体材料和存在于载体材料表面上的分子筛结晶相组成的复合催化剂的制备。根据需要，分子筛晶体可以在多孔载体材料的内侧和外侧上提供。利用根据本发明的方法，可以实现具有较高晶体负载和单个沸石晶体更好可接近性的复合材料的更快制备。此外，本发明涉及在载体材料上用于诱导原位成核的模板的用途。

5. 发明申请

WO1994009902A1 CATALYST SYSTEM OF THE STRUCTURED TYPE 审中-公开
标题翻译：结构型催化剂体系
公开(公告)号：WO1994009902A1
公开(公告)日：1994-05-11
申请号：PCT/NL1993000234
申请日：1993-11-05
申请人： TECHNISCHE UNIVERSITEIT DELFT , JANSEN, Jacobus, Cornelis , LEGEIN, Colette, Henriette , CALIS, Hans, Peter, Alexander , VAN BEKKUM, Herman , GERRITSEN, Albert, Willem , VAN DEN BLEEK, Cornelis, Maria
发明人： TECHNISCHE UNIVERSITEIT DELFT
IPC分类号： B01J37/02
CPC分类号： B01D53/8628 , B01J29/46 , B01J37/0246 , B01J2229/66
摘要： The invention relates to a catalyst system of the structured type, in which a structured support is covered with a layer of molecular sieve crystals and/or modifications thereof. These crystals have substantially the same orientation relative to the support surface. The invention further relates to a reactor in which this catalyst system is incorporated. Finally, the invention relates to a method for the selective reduction of nitrogen oxides utilizing a compound comprising a NH group, in which the catalyst system according to the invention is used.
摘要翻译：本发明涉及一种结构化型催化剂体系，其中结构化载体被一层分子筛晶体覆盖和/或其修饰。这些晶体相对于支撑表面具有基本相同的取向。本发明还涉及其中结合有该催化剂体系的反应器。最后，本发明涉及利用包含NH基团的化合物选择还原氮氧化物的方法，其中使用了本发明的催化剂体系。

6. 发明申请

WO2009077294A9 CATALYST WITH SUPPORT STRUCTURE 审中-公开
公开(公告)号：WO2009077294A9
公开(公告)日：2009-06-25
申请号：PCT/EP2008/066104
申请日：2008-11-25
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , BEZEMER, Gerrit Leendert , CALIS, Hans Peter Alexander , DOGTEROM, Ronald Jan
发明人： BEZEMER, Gerrit Leendert , CALIS, Hans Peter Alexander , DOGTEROM, Ronald Jan
IPC分类号： B01J19/32 , C23C2/40 , B01J21/06 , B01J23/75 , C10G47/12
摘要： The present invention relates to a catalyst carrier, catalyst and catalyst precursor comprising a refractory metal oxide and support structure comprising a wire gauze having between 100 2 to 600 2 openings per inch 2 , and having a wire thickness in the range of 20 micrometer to 110 micrometer. The volume of the support structure is less than 50% of the volume of the catalyst carrier and at least 70% of said openings are filled with the refractory metal oxide.

7. 发明申请

WO2009077294A3 CATALYST WITH ACTIVE METAL COMPONENT SUPPORTED ON A METAL OXIDE COVERED SUPPORT CONSISTING OF METALLIC GAUZE 审中-公开
公开(公告)号：WO2009077294A3
公开(公告)日：2009-06-25
申请号：PCT/EP2008/066104
申请日：2008-11-25
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , BEZEMER, Gerrit Leendert , CALIS, Hans Peter Alexander , DOGTEROM, Ronald Jan
发明人： BEZEMER, Gerrit Leendert , CALIS, Hans Peter Alexander , DOGTEROM, Ronald Jan
IPC分类号： B01J19/32 , C23C2/40 , B01J21/06 , B01J23/75 , C10G47/12
摘要： The present invention relates to a catalyst carrier, catalyst and catalyst precursor comprising a refractory metal oxide and support structure comprising a wire gauze having between 100 2 to 600 2 openings per inch 2 , and having a wire thickness in the range of 20 micrometer to 110 micrometer. The volume of the support structure is less than 50% of the volume of the catalyst carrier and at least 70% of said openings are filled with the refractory metal oxide.

8. 发明申请

WO2009077294A2 CATALYST WITH SUPPORT STRUCTURE 审中-公开
标题翻译：催化剂与支持结构
公开(公告)号：WO2009077294A2
公开(公告)日：2009-06-25
申请号：PCT/EP2008/066104
申请日：2008-11-25
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , BEZEMER, Gerrit Leendert , CALIS, Hans Peter Alexander , DOGTEROM, Ronald Jan
发明人： BEZEMER, Gerrit Leendert , CALIS, Hans Peter Alexander , DOGTEROM, Ronald Jan
IPC分类号： B01J19/32 , C23C2/40 , B01J21/06 , B01J23/75 , C10G47/12
CPC分类号： B01J23/75 , B01J8/06 , B01J19/30 , B01J19/32 , B01J23/56 , B01J23/8892 , B01J35/06 , B01J37/0232 , B01J2219/30215 , B01J2219/30408 , B01J2219/30416 , B01J2219/30475 , B01J2219/312 , B01J2219/32286 , B01J2219/32408 , B01J2219/32425 , B01J2219/32466 , C10G2/332 , C10G47/14
摘要： The present invention relates to a catalyst carrier, catalyst and catalyst precursor comprising a refractory metal oxide and support structure comprising a wire gauze having between 100 2 to 600 2 openings per inch 2 , and having a wire thickness in the range of 20 micrometer to 110 micrometer. The volume of the support structure is less than 50% of the volume of the catalyst carrier and at least 70% of said openings are filled with the refractory metal oxide.
摘要翻译：本发明涉及包含难熔金属氧化物和载体结构的催化剂载体，催化剂和催化剂前体，所述载体，载体结构包含具有每平方英寸1002至6002个开口2并且具有20微米至110微米范围内的金属丝厚度的金属丝网。载体结构的体积小于催化剂载体体积的50％，并且至少70％的所述开口填充有难熔金属氧化物。

9. 发明申请

WO2003045547A3 COMPOSITION A BASE D'UNE FERRIERITE ET SON UTILISATION DANS UN PROCEDE DE TRAITEMENT DE GAZ POUR LA REDUCTION DES EMISSIONS DES OXYDES D'AZOTE 审中-公开
公开(公告)号：WO2003045547A3
公开(公告)日：2003-06-05
申请号：PCT/FR2002/004019
申请日：2002-11-22
申请人： ATOFINA RESEARCH , PEUGEOT CITROEN AUTOMOBILE S.A. , RHODIA ELECTRONICS AND CATALYSIS , TECHNISCHE UNIVERSITEIT DELFT , UNIVERSITE LIBRE DE BRUXELLES , BLANCHARD, Gilbert , VAN DEN BLEEK, Cor , CALIS, Hans, Peter , KRUSE, Norbert , NOIROT, Rémi , TACHON, Denis , SEIJGER, Germaine
发明人： BLANCHARD, Gilbert , VAN DEN BLEEK, Cor , CALIS, Hans, Peter , KRUSE, Norbert , NOIROT, Rémi , TACHON, Denis , SEIJGER, Germaine
IPC分类号： B01J29/65
摘要： L'invention concerne des compositions catalytiques comprenant une zéolite ainsi que des procédés pour la réduction d'oxydes d'azote (NO x ) utilisant ces compositions catalytiques. Les compositions catalytiques de l'invention comprennent une zéolite du type ferrriétite (FER), laquelle a subi un échange d'ions avec une terre rare choisie parmi le cérium, le praséodyme, le samarium, le terbium, l'europium et l'ytterbium, cette zéolite pouvant être en particulier du Ce-H-FER. Ces compositions sont très actives dans la réduction catalytique sélective de NO x même si la réaction est réalisée en présence d'eau et de composés soufrés.

10. 发明申请

WO2003045547A2 COMPOSITION A BASE D'UNE FERRIERITE ET SON UTILISATION DANS UN PROCEDE DE TRAITEMENT DE GAZ POUR LA REDUCTION DES EMISSIONS DES OXYDES D'AZOTE 审中-公开
标题翻译：基于氟化物的组合物及其在减少氮氧化物排放的气体处理方法中的应用
公开(公告)号：WO2003045547A2
公开(公告)日：2003-06-05
申请号：PCT/FR2002/004019
申请日：2002-11-22
申请人： ATOFINA RESEARCH , PEUGEOT CITROEN AUTOMOBILE S.A. , RHODIA ELECTRONICS AND CATALYSIS , TECHNISCHE UNIVERSITEIT DELFT , UNIVERSITE LIBRE DE BRUXELLES , BLANCHARD, Gilbert , VAN DEN BLEEK, Cor , CALIS, Hans, Peter , KRUSE, Norbert , NOIROT, Rémi , TACHON, Denis , SEIJGER, Germaine
发明人： BLANCHARD, Gilbert , VAN DEN BLEEK, Cor , CALIS, Hans, Peter , KRUSE, Norbert , NOIROT, Rémi , TACHON, Denis , SEIJGER, Germaine
IPC分类号： B01J29/06
CPC分类号： B01J29/67 , B01D53/8628 , B01D53/9418 , B01D2251/206 , B01D2255/1021 , B01D2255/104 , B01D2255/2063 , B01D2255/2065 , B01D2255/20715 , B01D2255/20761 , B01D2255/20784 , B01D2255/50 , B01D2258/012 , B01J29/655 , B01J35/0006
摘要： L'invention concerne des compositions catalytiques comprenant une zéolite ainsi que des procédés pour la réduction d'oxydes d'azote (NO x ) utilisant ces compositions catalytiques. Les compositions catalytiques de l'invention comprennent une zéolite du type ferrriétite (FER), laquelle a subi un échange d'ions avec une terre rare choisie parmi le cérium, le praséodyme, le samarium, le terbium, l'europium et l'ytterbium, cette zéolite pouvant être en particulier du Ce-H-FER. Ces compositions sont très actives dans la réduction catalytique sélective de NO x même si la réaction est réalisée en présence d'eau et de composés soufrés.
摘要翻译：本发明涉及包含沸石的催化组合物和使用所述催化组合物还原氮氧化物（NOx）的方法。本发明的催化组合物包括已经与选自铈，镨，钐，铽，铕和镱的稀土进行离子交换的镁碱沸石型沸石（FER），所述沸石特别是Ce-H -fER。即使在水和硫化合物的存在下产生反应，所述组合物在选择性催化NOx还原中也非常活跃。

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