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1. 发明授权

US5834523A Substituted .alpha.,.beta.,.beta.-trifluorostyrene-based composite membranes 失效
标题翻译：取代的α，β，β-三氟苯乙烯基复合膜
公开(公告)号：US5834523A
公开(公告)日：1998-11-10
申请号：US583638
申请日：1996-01-05
申请人： Alfred E. Steck , Charles Stone
发明人： Alfred E. Steck , Charles Stone
IPC分类号： B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , B32B27/30 , C08F8/00 , C08F12/30 , C08F14/18 , C08F212/14 , C08J5/22 , G01N27/40 , G01N27/407 , H01B1/06 , H01M2/16 , H01M8/02 , H01M8/10
CPC分类号： C08J5/2281 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C08F12/30 , C08F14/185 , C08F212/14 , C08F8/12 , C08J5/225 , G01N27/40 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , H01M8/106 , H01M8/1081 , C08J2323/06 , C08J2327/18 , Y02P70/56
摘要： A composite membrane is provided in which a porous substrate is impregnated with a polymeric composition comprising various combinations of .alpha.,.beta.,.beta.-trifluorostyrene, substituted .alpha.,.beta.,.beta.-trifluorostyrene and ethylene-based monomeric units. Where the polymeric composition includes ion-exchange moieties, the resultant composite membranes are useful in electrochemical applications, particularly as membrane electrolytes in electrochemical fuel cells.
摘要翻译：提供了复合膜，其中多孔基材浸渍有包含α，β，β-三氟苯乙烯，取代的α，β，β-三氟苯乙烯和基于乙烯的单体单元的各种组合的聚合物组合物。当聚合物组合物包括离子交换部分时，所得到的复合膜可用于电化学应用中，特别是作为电化学燃料电池中的膜电解质。

2. 发明授权

US06723758B2 Graft polymeric membranes and ion-exchange membranes formed therefrom 失效
标题翻译：由其形成的接枝聚合物膜和离子交换膜
公开(公告)号：US06723758B2
公开(公告)日：2004-04-20
申请号：US09934176
申请日：2001-08-21
申请人： Charles Stone , Alfred E. Steck , Biswajit Choudhury
发明人： Charles Stone , Alfred E. Steck , Biswajit Choudhury
IPC分类号： C08J522
CPC分类号： B01D67/0093 , B01D71/28 , B01D71/32 , B01D71/36 , B01D71/82 , B01D2323/38 , C08F255/02 , C08F255/023 , C08F259/08 , C08F291/00 , C08F291/18 , C08J5/225 , C08J7/16 , C08J2327/12 , H01M8/1023 , H01M8/1039 , H01M8/1072 , H01M8/1088 , Y02P70/56
摘要： Graft polymeric membranes and methods for making graft polymeric membranes have one or more trifluorovinyl aromatic monomers that are radiation graft polymerized to a polymeric base film. The membranes comprise a polymeric base film to which has been graft polymerized substituted &agr;,&agr;,&bgr;-trifluorostyrene and/or &agr;,&agr;,&bgr;-trifluorovinylnaphthylene monomers, which are activated towards graft polymerization. As ion-exchange membranes, the membranes are suitable for use in electrode apparatus, including membrane electrode assemblies in, for example, fuel cells. The membranes can also be crosslinked.
摘要翻译：接枝聚合物膜和用于制备接枝聚合物膜的方法具有一个或多个被辐射接枝聚合成聚合物基膜的三氟乙烯基芳族单体。膜包含已被接枝聚合的取代的α，α，β-三氟苯乙烯和/或α，α，β-三氟乙烯基萘基单体的聚合物基膜，其被接枝聚合而被活化。作为离子交换膜，该膜适用于电极装置，包括例如燃料电池中的膜电极组件。膜也可以交联。

3. 发明授权

US06258861B1 &agr;,&bgr;,&bgr;-trifluorostyrene-based composite membranes 失效
标题翻译： α，β，β-三氟苯乙烯基复合膜
公开(公告)号：US06258861B1
公开(公告)日：2001-07-10
申请号：US09441181
申请日：1999-11-15
申请人： Alfred E. Steck , Charles Stone
发明人： Alfred E. Steck , Charles Stone
IPC分类号： C08J522
CPC分类号： C08J5/2281 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C08F8/12 , C08F12/30 , C08F14/185 , C08F212/14 , C08J5/225 , C08J2323/06 , C08J2327/18 , G01N27/40 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , H01M8/106 , H01M8/1081 , Y02P70/56
摘要： A composite membrane is provided in which a porous substrate is impregnated with a polymeric composition comprising various combinations of &agr;, &bgr;, &bgr;-trifluorostyrene, substituted &agr;, &bgr;, &bgr;-trifluorostyrene and ethylene-based monomeric units. Where the polymeric composition includes ion-exchange moieties, the resultant composite membranes are useful in electrochemical applications, particularly as membrane electrolytes in electrochemical fuel cells.
摘要翻译：提供了复合膜，其中多孔基材浸渍有包含α，β，β-三氟苯乙烯，取代的α，β，β-三氟苯乙烯和基于乙烯的单体单元的各种组合的聚合物组合物。当聚合物组合物包括离子交换部分时，所得到的复合膜可用于电化学应用中，特别是作为电化学燃料电池中的膜电解质。

4. 发明授权

US5498639A Trifluorostyrene and substituted trifluorostyrene copolymeric ion-exchange membranes 失效
标题翻译：三氟苯乙烯和取代的三氟苯乙烯共聚物离子交换膜
公开(公告)号：US5498639A
公开(公告)日：1996-03-12
申请号：US442206
申请日：1995-05-16
申请人： Jinzhu Wei , Charles Stone , Alfred E. Steck
发明人： Jinzhu Wei , Charles Stone , Alfred E. Steck
IPC分类号： B01D61/42 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C07C309/86 , C08F8/00 , C08F12/30 , C08F14/18 , C08F212/14 , C08F214/18 , C08J5/22 , C08L27/12 , G01N27/40 , G01N27/407 , H01M2/16 , H01M8/02 , H01M8/10
CPC分类号： B01D71/76 , B01D69/02 , B01D69/12 , C07C309/86 , C08F12/30 , C08F14/185 , C08F212/14 , C08F8/34 , C08J5/225 , G01N27/40 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , B01D71/28 , B01D71/32 , C08F2800/20 , C08J2327/12 , C08J5/2237
摘要： Polymeric compositions are derived from copolymers of .alpha.,.beta., .beta.-trifluorostyrene with a variety of substituted .alpha.,.beta.,.beta.-trifluorostyrenes. These compositions are suitable for use as membranes, particularly as ion-exchange membranes, and most particularly as solid polymer electrolytes in electrochemical applications, such as, for example, electrochemical fuel cells.
摘要翻译：聚合物组合物衍生自α，β，β-三氟苯乙烯与各种取代的α，β，β-三氟苯乙烯的共聚物。这些组合物适合用作膜，特别是用作离子交换膜，特别是作为电化学应用中的固体聚合物电解质，例如电化学燃料电池。

5. 发明授权

US5464700A Gasketed membrane electrode assembly for electrochemical fuel cells 失效
标题翻译：用于电化学燃料电池的垫片膜电极组件
公开(公告)号：US5464700A
公开(公告)日：1995-11-07
申请号：US225519
申请日：1994-04-11
申请人： Alfred E. Steck , Jinzhu Wei
发明人： Alfred E. Steck , Jinzhu Wei
IPC分类号： C25B9/00 , H01M8/02 , H01M8/10
CPC分类号： C25B9/00 , H01M8/0273 , H01M8/1007 , H01M2300/0082
摘要： A gasketed membrane electrode assembly for electrochemical fuel cells employs gasketing material at the periphery of the ion exchange membrane, rather than the membrane itself, as a gasket. The gasketing material may be formed from an elastomeric material suitable for cold bonding or bonding by heat and pressure. A nonhydrophilic thermoplastic elastomer is the preferred gasketing material. The gasketed membrane electrode assembly provides a seal between the electrically conductive separator plates that is more effective and economical than assemblies employing the membrane itself as the gasketing material. In an alternative embodiment, a gasketed membrane assembly for use in the humidification portion of a fuel cell employs gasketing material at the periphery of a water permeable membrane.
摘要翻译：用于电化学燃料电池的垫圈膜电极组件在离子交换膜的周边采用衬垫材料，而不是膜本身作为衬垫。衬垫材料可以由适合于通过热和压力进行冷粘合或粘合的弹性体材料形成。非亲水性热塑性弹性体是优选的衬垫材料。垫圈膜电极组件提供了导电隔板之间的密封，其比使用膜本身作为衬垫材料的组件更有效和经济。在替代实施例中，用于燃料电池的加湿部分的垫圈膜组件在透水膜的周边采用衬垫材料。

6. 发明授权

US06359019B1 Graft polymeric membranes and ion-exchange membranes formed therefrom 失效
标题翻译：由其形成的接枝聚合物膜和离子交换膜
公开(公告)号：US06359019B1
公开(公告)日：2002-03-19
申请号：US08967960
申请日：1997-11-12
申请人： Charles Stone , Alfred E. Steck
发明人： Charles Stone , Alfred E. Steck
IPC分类号： C08J522
CPC分类号： C08J7/16 , C08F255/02 , C08F255/023 , C08F259/08 , C08F291/00 , C08F291/18 , C08J5/2237 , C08J2323/06 , C08J2327/18 , H01M8/1023 , H01M8/1039 , H01M8/1067 , H01M8/1072 , H01M8/1088 , Y02P70/56
摘要： Graft polymeric membranes in which one or more trifluorovinyl aromatic monomers are radiation graft polymerized to a preformed polymeric base film are provided, as well as ion-exchange membranes prepared therefrom. Preferred monomers include substituted &agr;, &bgr;, &bgr;-trifluorostyrenes and trifluorovinyl naphthalenes which are activated towards the grafting reaction or facilitate the introduction of more than one ion-exchange group per monomer unit in the grafted chains. The ion-exchange membranes are useful in dialysis applications, and particularly in electrochemical applications, for example as membrane electrolytes in electrochemical fuel cells and electrolyzers.
摘要翻译：提供其中一个或多个三氟乙烯基芳族单体被辐射接枝聚合成预制的聚合物基膜的接枝聚合物膜以及由其制备的离子交换膜。优选的单体包括被取代的α，β，β-三氟苯乙烯和三氟乙烯基萘，其被接触反应活化或促进每个单体单元在接枝链中引入多于一个离子交换基团。离子交换膜可用于透析应用，特别是在电化学应用中，例如作为电化学燃料电池和电解器中的膜电解质。

7. 发明授权

US5985942A .alpha., .beta., .beta.-trifluorostyrene-based composite membranes 失效
标题翻译： α，β，β-三氟苯乙烯基复合膜
公开(公告)号：US5985942A
公开(公告)日：1999-11-16
申请号：US186449
申请日：1998-11-05
申请人： Alfred E. Steck , Charles Stone
发明人： Alfred E. Steck , Charles Stone
IPC分类号： B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , B32B27/30 , C08F8/00 , C08F12/30 , C08F14/18 , C08F212/14 , C08J5/22 , G01N27/40 , G01N27/407 , H01B1/06 , H01M2/16 , H01M8/02 , H01M8/10
CPC分类号： C08J5/2281 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C08F12/30 , C08F14/185 , C08F212/14 , C08F8/12 , C08J5/225 , G01N27/40 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , H01M8/106 , H01M8/1081 , C08J2323/06 , C08J2327/18 , Y02P70/56
摘要： A composite membrane is provided in which a porous substrate is impregnated with a polymeric composition comprising various combinations of .alpha.,.beta.,.beta.-trifluorostyrene, substituted .alpha.,.beta.,.beta.-trifluorostyrene and ethylene-based monomeric units. Where the polymeric composition includes ion-exchange moieties, the resultant composite membranes are useful in electrochemical applications, particularly as membrane electrolytes in electrochemical fuel cells.
摘要翻译：提供了复合膜，其中多孔基材浸渍有包含α，β，β-三氟苯乙烯，取代的α，β，β-三氟苯乙烯和基于乙烯的单体单元的各种组合的聚合物组合物。当聚合物组合物包括离子交换部分时，所得到的复合膜可用于电化学应用中，特别是作为电化学燃料电池中的膜电解质。

8. 发明授权

US5773480A Trifluorostyrene and substituted trifluorostyrene copolymeric compositions and ion-exchange membranes formed therefrom 失效
公开(公告)号：US5773480A
公开(公告)日：1998-06-30
申请号：US768615
申请日：1996-12-18
申请人： Charles Stone , Alfred E. Steck , Jinzhu Wei
发明人： Charles Stone , Alfred E. Steck , Jinzhu Wei
IPC分类号： B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C08F8/00 , C08F12/30 , C08F14/18 , C08F212/14 , C08J5/22 , G01N27/40 , G01N27/407 , H01M2/16 , H01M8/10
CPC分类号： C08J5/2237 , B01D69/02 , B01D69/12 , B01D71/76 , C08F12/30 , C08F14/185 , C08F212/14 , C08F8/34 , G01N27/40 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , B01D71/32 , C08F2800/20 , C08J2327/12
摘要： Polymeric compositions are derived from copolymers of .alpha.,.beta.,.beta.-trifluorostyrene with a variety of substituted .alpha.,.beta.,.beta.-trifluorostyrenes. These compositions are suitable for use as membranes, particularly as ion-exchange membranes, and most particularly as solid polymer electrolytes in electrochemical applications, such as, for example, electrochemical fuel cells.

9. 发明授权

US5602185A Substituted trifluorostyrene compositions 失效
标题翻译：取代的三氟苯乙烯组合物
公开(公告)号：US5602185A
公开(公告)日：1997-02-11
申请号：US480098
申请日：1995-06-06
申请人： Charles Stone , Alfred E. Steck , Robert D. Lousenberg
发明人： Charles Stone , Alfred E. Steck , Robert D. Lousenberg
IPC分类号： B01D61/42 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C07C309/86 , C08F8/00 , C08F12/30 , C08F14/18 , C08F114/18 , C08F212/14 , C08F214/18 , C08J5/22 , C08L27/12 , G01N27/40 , G01N27/407 , H01M2/16 , H01M8/02 , H01M8/10
CPC分类号： G01N27/40 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C07C309/86 , C08F12/30 , C08F14/185 , C08F212/14 , C08F8/12 , C08J5/225 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , C08F2800/10 , C08F2800/20 , C08J2327/12
摘要： Sulfonyl fluoride substituted .alpha.,.beta.,.beta.-trifluorostyrene monomers are disclosed. The monomers are incorporated into polymeric compositions which are conveniently hydrolyzed to produce polymeric compositions which include ion-exchange moieties. The resulting compositions which include ion-exchange moieties are particularly suitable for use as solid polymer electrolytes in electrochemical applications, such as, for example, electrochemical fuel cells.
摘要翻译：公开了磺酰氟取代的α，β，β-三氟苯乙烯单体。将单体引入聚合物组合物中，其中方便地水解以产生包括离子交换部分的聚合物组合物。包括离子交换部分的所得组合物特别适合用作电化学应用中的固体聚合物电解质，例如电化学燃料电池。

10. 发明授权

US5422411A Trifluorostyrene and substituted trifluorostyrene copolymeric compositions and ion-exchange membranes formed therefrom 失效
标题翻译：三氟苯乙烯和取代的三氟苯乙烯共聚物组合物和由其形成的离子交换膜
公开(公告)号：US5422411A
公开(公告)日：1995-06-06
申请号：US124924
申请日：1993-09-21
申请人： Jinzhu Wei , Charles Stone , Alfred E. Steck
发明人： Jinzhu Wei , Charles Stone , Alfred E. Steck
IPC分类号： B01D61/42 , B01D69/02 , B01D69/12 , B01D71/28 , B01D71/32 , C07C309/86 , C08F8/00 , C08F12/30 , C08F14/18 , C08F212/14 , C08F214/18 , C08J5/22 , C08L27/12 , G01N27/40 , G01N27/407 , H01M2/16 , H01M8/02 , H01M8/10
CPC分类号： B01D71/76 , B01D69/02 , B01D69/12 , C07C309/86 , C08F12/30 , C08F14/185 , C08F212/14 , C08F8/34 , C08J5/225 , G01N27/40 , G01N27/4073 , G01N27/4074 , H01M2/1653 , H01M8/1023 , H01M8/1039 , B01D71/28 , B01D71/32 , C08F2800/20 , C08J2327/12 , C08J5/2237
摘要： Polymeric compositions are derived from copolymers of .alpha.,.beta.,.beta.-trifluorostyrene with a variety of substituted .alpha.,.beta.,.beta.-trifluorostyrenes. These compositions are suitable for use as membranes, particularly as ion-exchange membranes, and most particularly as solid polymer electrolytes in electrochemical applications, such as, for example, electrochemical fuel cells.
摘要翻译：聚合物组合物衍生自α，β，β-三氟苯乙烯与各种取代的α，β，β-三氟苯乙烯的共聚物。这些组合物适合用作膜，特别是用作离子交换膜，特别是作为电化学应用中的固体聚合物电解质，例如电化学燃料电池。

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