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81. 发明授权

US06200704B1 High capacity/high discharge rate rechargeable positive electrode 有权
标题翻译：高容量/高放电倍率的可充电正极
公开(公告)号：US06200704B1
公开(公告)日：2001-03-13
申请号：US09145484
申请日：1998-09-01
申请人： Bruce D. Katz , Lutgard C. De Jonghe , May-Ying Chu , Steven J. Visco
发明人： Bruce D. Katz , Lutgard C. De Jonghe , May-Ying Chu , Steven J. Visco
IPC分类号： H01M458
CPC分类号： H01M4/02 , H01M4/362 , H01M4/581 , H01M4/5815 , H01M4/625 , H01M10/0436 , H01M10/052 , H01M2004/028
摘要： Disclosed is a positive electrode that has a low equivalent weight and high cell voltage and consequently a high specific energy, and a high discharge rate pulse capability. Also disclosed are methods for fabricating active-sulfur-based composite electrodes, and battery cells incorporating such electrodes. The batteries of this invention are preferably rechargeable and operate at high sulfur utilization over many cycles. Positive electrodes according to the present invention are composed of at least two electrochemically active materials: an “active-sulfur” material, and a second electrochemically active material having a higher discharge rate than the active-sulfur component. The active-sulfur component is also oxidizing with respect to the higher discharge rate material. In operation, the active-sulfur component of the positive electrode discharges to satisfy power demands below its maximum discharge rate. The high discharge rate (but relatively low capacity) material is discharged to satisfy power demands that exceed the active-sulfur's discharge rate. The high discharge rate material in the positive electrode may be effectively recharged (or “regenerated”) chemically by oxidation by the active-sulfur material during a “resting” phase, that is, when the power demands on a battery cell in which the cathode is incorporated are low enough that they may be met without exceeding the maximum discharge rate of the active-sulfur component of the positive electrode.
摘要翻译：公开了具有低当量和高电池电压并因此具有高比能量和高放电率脉冲能力的正电极。还公开了制造活性硫基复合电极的方法以及包含这种电极的电池单体。本发明的电池优选是可充电的并且在多个循环中以高硫利用运行。根据本发明的正电极由至少两种电化学活性材料：“活性硫”材料和具有比活性硫组分更高的放电率的第二电化学活性材料组成。相对于较高的排出速率的材料，活性硫成分也是氧化的。在操作中，正极的活性硫成分排出以满足低于其最大放电率的功率需求。高放电率（但容量相对较小）的材料排放满足超过活性硫排放速率的电力需求。正极中的高放电率材料可以通过在“静止”阶段期间被活性硫材料氧化而化学地再充电（或“再生”），即当电力需要电池单元时，其中阴极并不足够超过正极的活性硫成分的最大排出速度，所以能够满足这些要求。

82. 依法登记的发明

USH1946H1 Tertiary polyamines as additives to lithium-ion cell electrolytes to provide lithium-ion cell having improved properties 有权
公开(公告)号：USH1946H1
公开(公告)日：2001-03-06
申请号：US09345550
申请日：1999-06-30
申请人： Donald L. Foster , Wishvender K. Behl , Jeffery B. Wolfenstine
发明人： Donald L. Foster , Wishvender K. Behl , Jeffery B. Wolfenstine
IPC分类号： H01M458
摘要： A secondary, lithium-ion electrochemical cell having improved properties and a method for providing a secondary, lithium-ion electrochemical cell having the same. Specifically, the invention relates to a method for reducing and/or preventing the exfoliation of the graphitic carbonaceous electrode of a lithium-ion cell, wherein the exfoliation is caused by the intercalation of electrolyte solvent along with lithium ion into the graphitic carbonaceous electrode. This method is accomplished by adding one or more chelating polyamines to the electrolyte solution of the lithium-ion cell. The novel method and the improved lithium-ion cell are claimed herein.

83. 发明授权

US06187477B1 Lithium secondary battery and cathode composition therefor 有权
标题翻译：锂二次电池及其阴极组成
公开(公告)号：US06187477B1
公开(公告)日：2001-02-13
申请号：US09163012
申请日：1998-09-30
申请人： Isao Watanabe , Hiroshi Horiuchi , Kensuke Yoshida , Tsutomu Miyashita , Tamotsu Yamamoto , Masami Tsutsumi
发明人： Isao Watanabe , Hiroshi Horiuchi , Kensuke Yoshida , Tsutomu Miyashita , Tamotsu Yamamoto , Masami Tsutsumi
IPC分类号： H01M458
CPC分类号： H01M10/05 , H01M4/62 , H01M4/621 , H01M10/4235
摘要： A lithium secondary battery includes a cathode which can be dischargeably charged with lithium ions, an anode made of lithium metal, a lithium alloy or any other anode material which can be releasably doped with lithium ions, and an electrolyte which allows migration of lithium ions between both electrodes. The cathode contains a halogen compound which releases halogen atoms, halogen ions or a reactive halogen-containing substance for reacting with the anode, thereby deactivating the anode to prevent excessive heat generation before oxygen released from the cathode due to a temperature rise reacts with the anode.
摘要翻译：锂二次电池包括可以放电地充有锂离子的阴极，由锂金属制成的阳极，锂合金或可以可释放地掺杂有锂离子的任何其它阳极材料，以及允许锂离子之间迁移的电解质两个电极。阴极含有卤素原子的卤素化合物，卤素离子或与阳极反应的反应性含卤物质，从而使阳极失活以防止由于温度升高与阳极反应而从阴极释放的氧之间产生过多的热量。

84. 发明授权

US06174624B1 Positive-electrode active material for alkaline secondary battery and an alkaline secondary battery 有权
标题翻译：碱性二次电池用正极活性物质和碱性二次电池
公开(公告)号：US06174624B1
公开(公告)日：2001-01-16
申请号：US09267399
申请日：1999-03-15
申请人： Mutsumi Yano , Mitsunori Tokuda , Mitsuzou Nogami , Shin Fujitani , Koji Nishio
发明人： Mutsumi Yano , Mitsunori Tokuda , Mitsuzou Nogami , Shin Fujitani , Koji Nishio
IPC分类号： H01M458
CPC分类号： H01M6/085 , H01M4/364 , H01M4/48 , H01M4/50 , H01M4/52 , H01M10/283
摘要： A positive-electrode active material for alkaline secondary battery according to the invention has an &agr;-Ni(OH)2 crystal structure which incorporates therein manganese and a trivalent metal other than manganese.
摘要翻译：根据本发明的碱性二次电池用正极活性物质具有含有锰和锰以外的三价金属的α-Ni（OH）2结晶结构。

85. 发明授权

US06171726B2 Active electrode composition with nonfilbrillating binder 有权
标题翻译：活性电极组合物与无刷玻璃粘合剂
公开(公告)号：US06171726B2
公开(公告)日：2001-01-09
申请号：US09221676
申请日：1998-12-24
申请人： Benjamin Reichman , William Mays , Michael A. Fetcenko
发明人： Benjamin Reichman , William Mays , Michael A. Fetcenko
IPC分类号： H01M458
CPC分类号： H01M4/0416 , H01M4/04 , H01M4/0402 , H01M4/0404 , H01M4/043 , H01M4/0471 , H01M4/242 , H01M4/621 , H01M4/623 , H01M10/345 , Y10S420/90
摘要： An active composition for an electrode of an electrochemical cell. The active composition comprises an electrode material, and a nonfibrillating polymeric binder. The polymeric binder may comprise a fluoradditive. Also disclosed in an electrode and an electrochemical cell comprising the active composition.
摘要翻译：一种用于电化学电池的电极的活性组合物。活性组合物包含电极材料和非原纤化聚合物粘合剂。聚合物粘合剂可以包含氟加成物。还公开在包含活性组合物的电极和电化学电池中。

86. 发明授权

US06821676B2 Metal hydride battery material with high storage capacity 失效
标题翻译：金属氢化物电池材料具有高存储容量
公开(公告)号：US06821676B2
公开(公告)日：2004-11-23
申请号：US09995457
申请日：2001-11-27
申请人： Martin Ouwerkerk , Anna-Maria Janner , Petrus Henricus Laurentius Notten
发明人： Martin Ouwerkerk , Anna-Maria Janner , Petrus Henricus Laurentius Notten
IPC分类号： H01M458
CPC分类号： C22C23/06 , C01B3/0031 , C01B3/0047 , C22C28/00 , C22C30/00 , H01M4/383 , Y02E60/327 , Y10S420/90
摘要： A hydrogen storage material has a magnesium-containing intermetallic compound which can form a hydride with hydrogen. The intermetallic compound has an alloy of magnesium and a trivalent metal selected from the group of Sc, Y, La and the rare earth elements. The hydrogen storage material can further have a catalytically active material.
摘要翻译：储氢材料具有可与氢形成氢化物的含镁金属间化合物。金属间化合物具有镁和选自Sc，Y，La和稀土元素的三价金属的合金。储氢材料还可以具有催化活性材料。

87. 发明授权

US06818351B2 Mixed cathode active material for lithium secondary battery 失效
标题翻译：锂二次电池混合阴极活性材料
公开(公告)号：US06818351B2
公开(公告)日：2004-11-16
申请号：US10079590
申请日：2002-02-22
申请人： Takuya Sunagawa , Masatoshi Takahashi , Yoshikumi Miyamoto
发明人： Takuya Sunagawa , Masatoshi Takahashi , Yoshikumi Miyamoto
IPC分类号： H01M458
CPC分类号： H01M4/131 , C01G45/1242 , C01G51/54 , C01G53/54 , C01P2002/32 , C01P2002/54 , C01P2004/54 , C01P2006/10 , C01P2006/40 , H01M4/364 , H01M4/485 , H01M4/505 , H01M4/525 , H01M10/0525 , H01M2300/0037
摘要： A lithium secondary battery having improved load characteristics such as high rate discharge properties is obtained by using a mixed cathode active material comprising a mixture of lithium-containing manganese oxide having a spinel type crystal structure and lithium-containing cobalt oxide, wherein the cathode collector retains mixed cathode active material in such a manner that the mixing ratio of lithium cobaltate X thereof should fall in a range of 0.1≦X≦0.9, that the bulk density Y (g/cm3) of the cathode mixed agent should be confined in a range satisfying the relation of 0.5X+2.7≦Y≦0.6X+3.3, and that the mean particle diameter of spinel type lithium manganate should be greater than the mean particle diameter of lithium cobaltate.
摘要翻译：通过使用包含具有尖晶石型晶体结构的含锂锰氧化物和含锂钴氧化物的混合物的混合阴极活性材料，获得具有诸如高倍率放电性能的改善的负载特性的锂二次电池，其中阴极集电体保持混合阴极活性物质，使得其钴酸锂的混合比例应该落在0.1 <= X <= 0.9的范围内，阴极混合剂的体积密度Y（g / cm 3）应该被限制在满足0.5X + 2.7 <= Y <= 0.6X + 3.3的关系的范围内，并且尖晶石型锰酸锂的平均粒径应大于钴酸锂的平均粒径。

88. 发明授权

US06818349B2 Positive active material for rechargeable lithium-sulfur batteries and method of preparing same 失效
标题翻译：可充电锂硫电池正极活性物质及其制备方法
公开(公告)号：US06818349B2
公开(公告)日：2004-11-16
申请号：US10157158
申请日：2002-05-30
申请人： Su-Suk Choi , Ho-Jin Kweon , Jun-Won Suh , Jea-Woan Lee , Ji-Seong Han
发明人： Su-Suk Choi , Ho-Jin Kweon , Jun-Won Suh , Jea-Woan Lee , Ji-Seong Han
IPC分类号： H01M458
CPC分类号： H01M10/052 , H01M4/0402 , H01M4/0438 , H01M4/044 , H01M4/0442 , H01M4/045 , H01M4/0492 , H01M4/0497 , H01M4/136 , H01M4/366 , H01M4/581 , H01M4/5815 , H01M4/62
摘要： A positive active material for a rechargeable lithium-sulfur battery includes a core of a sulfur compound and a surface-passivation layer formed on the core. The surface-passivation layer is made of a coating-element-included compound selected from the group consisting of a coating-element-included hydroxide, a coating-element-included oxyhydroxide, a coating-element-included oxycarbonate, a coating-element-included hydroxycarbonate, a mixture thereof.
摘要翻译：用于可再充电的锂 - 硫电池的正极活性材料包括硫化合物的芯和形成在芯上的表面钝化层。表面钝化层由选自含有涂覆元素的氢氧化物，包括涂覆元素的羟基氢氧化物，含涂覆元素的含氧碳酸酯，涂覆元素的氧化物，包括羟基碳酸酯，其混合物。

89. 发明授权

US06794086B2 Thermally protective salt material for thermal spraying of electrode materials 失效
标题翻译：用于热喷涂电极材料的耐热盐材料
公开(公告)号：US06794086B2
公开(公告)日：2004-09-21
申请号：US09795696
申请日：2001-02-28
申请人： Jinxiang Dai , Ronald A. Guidotti , Tongsan D. Xiao , David E. Reisner
发明人： Jinxiang Dai , Ronald A. Guidotti , Tongsan D. Xiao , David E. Reisner
IPC分类号： H01M458
CPC分类号： H01M6/36 , C23C4/04 , C23C4/11 , H01M4/08
摘要： A method for the manufacture of an electrode for an energy storage or conversion device comprises thermally spraying a feedstock mixture comprising an effective quantity of a source of a thermally protective salt and an active material or active material precursor onto a substrate to produce a film of the active material and salt. The film can have a thickness of about 1 to about 1000 microns. In a particularly advantageous feature, the active materials which ordinarily decompose or are unavailable at the high temperatures used during thermal spray processes, such as metal chalcogenides such as pyrite, CoS2, WS2, Ni(OH)2, MnO2, and the like may be thermally sprayed to form an electrode when the feedstock mixture employs an effective amount of a source of the thermally protective salt coating. The active material feedstock may comprise microstructured or nanostructured materials, which after thermal spray results in electrodes having microstructured or nanostructured active materials, respectively.
摘要翻译：一种用于制造用于能量储存或转化装置的电极的方法包括将包含有效量的热保护盐源和活性材料或活性材料前体的原料混合物热喷涂到基底上以产生活性物质和盐。该膜可以具有约1至约1000微米的厚度。在特别有利的特征中，通常在热喷涂过程中使用的高温下分解或不可用的活性材料，例如金属硫族化物如黄铁矿，CoS 2，WS 2 ，当原料混合物使用有效量的耐热盐涂层源时，Ni（OH）2，MnO 2等可以被热喷涂以形成电极。活性材料原料可以包含微结构或纳米结构材料，其在热喷涂后分别导致具有微结构或纳米结构的活性材料的电极。

90. 发明授权

US06780541B2 Carbon electrode coated with porous metal film, its fabrication method and lithium secondary battery using the same 有权
标题翻译：涂有多孔金属膜的碳电极，其制造方法和使用其的锂二次电池
公开(公告)号：US06780541B2
公开(公告)日：2004-08-24
申请号：US09932940
申请日：2001-08-21
申请人： Kyung-Suk Yun , Byung-Won Cho , Won-Il Cho , Hyung-Sun Kim , Un-Seok Kim , Sang-Cheol Nam , Young-Soo Yoon
发明人： Kyung-Suk Yun , Byung-Won Cho , Won-Il Cho , Hyung-Sun Kim , Un-Seok Kim , Sang-Cheol Nam , Young-Soo Yoon
IPC分类号： H01M458
CPC分类号： H01M4/04 , H01M4/0402 , H01M4/0421 , H01M4/0426 , H01M4/485 , H01M4/505 , H01M4/525 , H01M4/587 , Y10T428/31678
摘要： A method for fabricating carbon electrode coated with a porous metal film includes the steps of: positioning a roll of carbon material within a vacuum chamber; winding the carbon material off the roll at a certain speed, winding the carbon material on a different roll while coating a porous metal to a thickness of a few Å˜a few &mgr;m on the carbon material between the two rolls from a metal evaporation source; and stabilizing the thusly coated carbon material under a vacuum. The coated porous metal film is of Li, Al, Sn, Bi, Si, Sb, Ni, Cu, Ti, V, Cr, Mn, Fe, Co, Zn, Mo, W, Ag, Au, Pt, Ru, Ir, In or their alloys. Since the stable film is formed on the surface of the carbon material, when the thusly coated carbon material is use for forming a cathode electrode of a secondary battery, the reversibility and high rate charging and discharging characteristics of the carbon electrode can be improved. In addition, when a lithium-ion secondary battery is fabricated using the carbon electrode coated with lithium or a lithium alloy, the capacity degradation due to the irreversible capacity of the conventional carbon electrode appearing at the initial state of charging can be prevented, so that the capacity can be increased.
摘要翻译：涂覆有多孔金属膜的碳电极的制造方法包括以下步骤：将碳材料卷定位在真空室内; 以一定的速度将碳材料从轧辊上卷绕，将碳材料卷绕在不同的辊上，同时在来自金属蒸发源的两个辊之间的碳材料上涂覆几微米厚度的多孔金属; 并在真空下稳定如此涂覆的碳材料。涂层多孔金属膜为Li，Al，Sn，Bi，Si，Sb，Ni，Cu，Ti，V，Cr，Mn，Fe，Co，Zn，Mo，W，Ag，Au，Pt，Ru，Ir ，In或它们的合金。由于在碳材料的表面上形成稳定的膜，所以当这样涂覆的碳材料用于形成二次电池的阴极时，可以提高碳电极的可逆性和高速充放电特性。此外，当使用涂覆有锂或锂合金的碳电极制造锂离子二次电池时，可以防止由于在初始充电状态下出现的常规碳电极的不可逆容量导致的容量降低，使得可以增加容量。

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