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71. 发明授权

US07009014B2 Process for the polymerization olefins 失效
标题翻译：烯烃聚合方法
公开(公告)号：US07009014B2
公开(公告)日：2006-03-07
申请号：US10009738
申请日：2001-06-29
申请人： Yasuhiko Suzuki , Tomoaki Matsugi , Yukihiro Takagi , Yasunori Yoshida , Junji Saito , Shigekazu Matsui , Yoshihisa Inoue , Terunori Fujita
发明人： Yasuhiko Suzuki , Tomoaki Matsugi , Yukihiro Takagi , Yasunori Yoshida , Junji Saito , Shigekazu Matsui , Yoshihisa Inoue , Terunori Fujita
IPC分类号： C08F4/44
CPC分类号： C08F10/02 , C08F110/02 , C08F210/16 , C08F4/64048 , C08F2500/17 , C08F210/08 , C08F210/14
摘要： A process for polymerizing an olefin is capable of polymerizing an olefin with excellent polymerization activity, and comprises polymerizing or copolymerizing an olefin at a polymerization reaction temperature of 50 to 200° C. in the presence of a catalyst comprising a transition metal compound (A) represented by the following formula (I), a compound (B-1) having a reduction ability which reacts with the transition metal compound (A) to convert an imine structure moiety to a metal amide structure, and a compound (B-2) which reacts with the transition metal compound (A) to form an ion pair; wherein M is a transition metal atom of Groups 3 to 11 of the periodic table; m is an integer of 1 to 6; Y is O, S, Se, or —C(R7)—; R1 to R7 may be the same or different, and are each a hydrogen atom, a halogen atom, a hydrocarbon group, an oxgen-containing group, a nitrogen-containing group and the like; n is a number satisfying a valence of M; and X is a hydrogen atom, a halogen atom, a hydrocarbon group and the like.
摘要翻译：聚合烯烃的方法能够聚合具有优异聚合活性的烯烃，并且包括在包含过渡金属化合物（A）的催化剂的存在下，在50至200℃的聚合反应温度下聚合或共聚烯烃，由下式（I）表示的具有与过渡金属化合物（A）反应以将亚胺结构部分转化为金属酰胺结构的还原能力的化合物（B-1）和化合物（B-2）其与过渡金属化合物（A）反应形成离子对; 其中M是周期表第3〜11族的过渡金属原子; m为1〜6的整数。 Y是O，S，Se或-C（R 7） - ; R 1至R 7可以相同或不同，并且各自为氢原子，卤素原子，烃基，含氧基团，含氮基团，含有基团等; n是满足M价的数; X是氢原子，卤原子，烃基等。

72. 发明授权

US06444603B1 CATALYST COMPONENT FOR ETHYLENICALLY UNSATURATED MONOMER POLYMERIZATION, CATALYST FOR ETHYLENICALLY UNSATURATED MONOMER POLYMERIZATION, AND PROCESS FOR ETHYLENICALLY UNSATURATED MONOMER POLYMERIZATION USING SAID CATALYST 有权
标题翻译：用于乙烯不饱和单体聚合的催化剂组分，用于乙烯单体不饱和单体聚合的催化剂，以及使用所述催化剂进行乙烯单体不饱和单体聚合的方法
公开(公告)号：US06444603B1
公开(公告)日：2002-09-03
申请号：US09216481
申请日：1998-12-21
申请人： Yasushi Tohi , Haruyuki Makio , Terunori Fujita , Toshiyuki Tsutsui
发明人： Yasushi Tohi , Haruyuki Makio , Terunori Fujita , Toshiyuki Tsutsui
IPC分类号： B01J3100
CPC分类号： C08F10/00 , C08F4/65927 , C08F110/02 , C08F4/64072 , C08F4/65912 , C08F2500/17 , C08F4/64048 , C08F4/64079 , C08F4/64186 , C08F4/64068 , C08F4/7006 , C08F4/7027
摘要： The invention relates to a catalyst component which can provide, in combination with a transition metal compound, a catalyst for ethylenically unsaturated monomer polymerization, a catalyst comprising the catalyst component and a transition metal compound, and a process for ethylenically unsaturated monomer polymerization using the catalyst. The catalyst component comprises a compound obtained by the reaction of, in any order, (i) a compound comprising a metal of Group 13 of the periodic table; (ii) a compound capable of reacting with the compound (i) to be bonded to two or more of the Group 13 metal; (iii) a compound capable of reacting the compound (i); and optionally (iv) a hydrocarbon compound or the like.
摘要翻译：本发明涉及一种催化剂组分，其可与过渡金属化合物，烯键式不饱和单体聚合催化剂，含催化剂组分和过渡金属化合物的催化剂和使用该催化剂的烯键式不饱和单体聚合方法。催化剂组分包括通过以任何顺序反应获得的化合物，（i）包含周期表第13族金属的化合物; （ii）能够与要与第13族金属中的两种以上结合的化合物（i）反应的化合物; （iii）能够使化合物（i）反应的化合物; 和（iv）烃化合物等。

73. 发明授权

US06369177B1 Catalyst for olefin polymerization and method of polymerizing olefin 失效
标题翻译：用于烯烃聚合的催化剂和烯烃聚合方法
公开(公告)号：US06369177B1
公开(公告)日：2002-04-09
申请号：US09485792
申请日：2000-02-15
申请人： Yasushi Tohi , Shigekazu Matsui , Terunori Fujita
发明人： Yasushi Tohi , Shigekazu Matsui , Terunori Fujita
IPC分类号： C08F444
CPC分类号： C08F10/00 , C08F10/02 , C08F4/7042
摘要： The present invention is intended to provide an olefin polymerization catalyst exhibiting excellent olefin polymerization activity and capable of producing polyolefins of excellent properties and to provide a process for olefin polymerization using this catalyst. The olefin polymerization catalyst comprises a transition metal imine compound (A) represented by the following formula (I-a) or (I-b) and at least one compound (B) selected from an organometallic compound (B-1), an organoaluminum oxy-compound (B-2) and a compound (B-3) which reacts with the transition metal imine compound (A) to form an ion pair; wherein M is a transition metal atom of Group 8 to Group 11 of the periodic table; R1 to R4 are each a hydrogen atom, a hydrocarbon group or the like; R5 and R6 are each a hydrocarbon group or the like; R1 and R5, R2 and R6, R1 and R3, or R2 and R4 may be bonded to each other to form a ring; m is an integer of 0 to 2; n is 0 or 2; A is an atom of Group 13 to Group 16 of the periodic table; E is a substituent group having carbon or the like; p is a number satisfying a valence of M; X is a halogen atom or the like; and Y is an atom of Group 15 of the periodic table.
摘要翻译：本发明旨在提供一种表现出优异的烯烃聚合活性且能够生产出优异性能的聚烯烃并提供使用该催化剂的烯烃聚合方法的烯烃聚合催化剂。烯烃聚合催化剂包含由下式（Ia）或（Ib）表示的过渡金属亚胺化合物（A）和至少一种选自有机金属化合物（B-1），有机铝氧化合物（B-1） B-2）和与过渡金属亚胺化合物（A）反应形成离子对的化合物（B-3）;其中M是周期表第8族至第11族的过渡金属原子; R 1〜R 4各自为氢原子，烃基等; R5和R6各自为烃基等; R1和R5，R2和R6，R1和R3，或R2和R4可以彼此键合形成环; m为0〜2的整数; n为0或2; A是周期表第13至16组的原子; E是具有碳等的取代基; p是满足M价的数; X是卤素原子等; Y是周期表第15族的原子。

74. 发明授权

US06303727B1 Linear triene compound and copolymer 失效
标题翻译：线性三烯化合物和共聚物
公开(公告)号：US06303727B1
公开(公告)日：2001-10-16
申请号：US09320838
申请日：1999-05-26
申请人： Ken Maeda , Masaaki Yasuda , Terunori Fujita , Keiji Okada , Makoto Kamimura , Kazuyuki Takimoto , Hidetatsu Murakami , Masaaki Kawasaki , Keiji Watanabe
发明人： Ken Maeda , Masaaki Yasuda , Terunori Fujita , Keiji Okada , Makoto Kamimura , Kazuyuki Takimoto , Hidetatsu Murakami , Masaaki Kawasaki , Keiji Watanabe
IPC分类号： C08F13600
CPC分类号： C08F236/22 , C07C2/04 , C07C11/21 , C07C2527/24 , C07C2531/14
摘要： A novel and useful linear triene compound represented by the following formula (1) is co-polymerized with an &agr;-olefin to obtain an ethylenically unsaturated copolymer which is superior in weather-ability, heat resitance and fastness to ozone, together with superior scorch stability and vulcanizability at high velocity in which R1, R2, R3, R4, R5 and R6 stand each, independently of each other, for hydrogen atom or an alkyl having 1-3 carbon atoms, R7 represents an alkyl having 1-3 carbon atoms and n is an integer of 0-5, with the proviso that each of R4s or of R5s may be identical with or different from each other, respectively, when n is 2 or greater.
摘要翻译：由下式（1）表示的新型有用的线性三烯化合物与α-烯烃共聚，得到耐候性，耐热性和耐臭氧性优异的烯属不饱和共聚物，以及优异的焦烧稳定性和R 1，R 2，R 3，R 4，R 5和R 6各自独立地表示氢原子或具有1-3个碳原子的烷基的高速度下的硫化性，R7表示具有1-3个碳原子的烷基，n表示是0-5的整数，条件是当n为2或更大时，R 4或R 5中的每一个可以分别彼此相同或不同。

75. 发明授权

US06291718B1 Process for preparing hydroperoxides 有权
标题翻译：制备氢过氧化物的方法
公开(公告)号：US06291718B1
公开(公告)日：2001-09-18
申请号：US09254176
申请日：1999-03-02
申请人： Shigekazu Matsui , Hiroshi Kuroda , Nobuya Hirokane , Haruyuki Makio , Toshihiro Takai , Koji Kato , Terunori Fujita , Makoto Kamimura
发明人： Shigekazu Matsui , Hiroshi Kuroda , Nobuya Hirokane , Haruyuki Makio , Toshihiro Takai , Koji Kato , Terunori Fujita , Makoto Kamimura
IPC分类号： C07C40700
CPC分类号： C07C407/00 , C07C409/10
摘要： A process for preparing hydroperoxides which comprises oxidizing hydrocarbon by a gas containing oxygen in the presence of a specific compound and converting them selectively to corresponding hydroperoxides. The specific compound is the compound that can capture radicals. The preferable example may be a compound selected from radicals of oxygen, nitrogen, phosphorus, sulfur, carbon or silicon or a compound that forms radicals of these in the reaction system. The present invention can be applied to oxidation of hydrocarbons including arylalkylhydrocarbons such as cumene, m-diisopropylbenzene, p-diisopropylbenzene, 1,3,5-triisopropylbenzene, isopropylnaphthalene, diisopropylnaphthalene, isopropylbiphenyl, diisopropylbiphenyl, etc.
摘要翻译：一种制备氢过氧化物的方法，其包括在特定化合物存在下通过含氧气体氧化烃，并将它们选择性地转化成相应的氢过氧化物。具体化合物是可以捕获自由基的化合物。优选的实例可以是选自氧，氮，磷，硫，碳或硅的基团的化合物或在反应体系中形成这些基团的化合物。本发明可应用于包括芳基烷基烃如枯烯，间二异丙基苯，对二异丙基苯，1,3,5-三异丙基苯，异丙基萘，二异丙基萘，异丙基联苯，二异丙基联苯等烃类的氧化。

76. 发明授权

US06255419B1 Olefin polymerization catalyst and process for producing olefin polymers 失效
标题翻译：烯烃聚合催化剂和烯烃聚合物的制备方法
公开(公告)号：US06255419B1
公开(公告)日：2001-07-03
申请号：US09169930
申请日：1998-10-07
申请人： Junichi Imuta , Junji Saito , Kenji Sugimura , Terunori Fujita
发明人： Junichi Imuta , Junji Saito , Kenji Sugimura , Terunori Fujita
IPC分类号： C08F444
CPC分类号： C08F12/04 , C08F10/00 , C08F110/02 , C08F110/06 , C08F110/14 , C08F210/02 , C08F210/06 , C08F210/08 , C08F210/16 , C08F4/62 , C08F2500/17 , C08F212/08 , C08F232/00 , C08F210/14 , C08F4/64072
摘要： The present invention provides olefin polymerization catalysts which can produce olefin polymers with excellent polymerization activity and an olefin polymerization method using the catalyst, wherein the catalyst comprises a transition metal amide compound represented by general formula (I) below: where M1 is Ti, etc.; R1 is alkyl, (substituted) phenyl, etc.; R2 is C(R5)2C(R6)mC(R5)2— or —C(R5)2—X1—C(R5)2— (X1 representing a silicon-containing group, etc., and R5 and R6 representing hydrocarbon groups, etc.); and R3 is a hydrocarbon group or halogen, etc.; and at least one compound selected from among organoaluminum oxy-compounds, ionizing ionic compounds and organometallic compounds.
摘要翻译：本发明提供了可以制备具有优异聚合活性的烯烃聚合物和使用该催化剂的烯烃聚合方法的烯烃聚合催化剂，其中催化剂包含由以下通式（I）表示的过渡金属酰胺化合物：其中M1是Ti等。 ; R1是烷基，（取代的）苯基等; R2是C（R5）2C（R6）mC（R5）2-或-C（R5）2-X1-C（R5）2-（X1代表含硅基团等，R5和R6代表烃团体等）; R3为烃基或卤素等; 和至少一种选自有机铝氧化合物，离子化离子化合物和有机金属化合物的化合物。

77. 发明授权

US5723640A Transition metal compound having indenyl-containing metallocene 失效
标题翻译：具有含茚基茂金属的过渡金属化合物
公开(公告)号：US5723640A
公开(公告)日：1998-03-03
申请号：US622592
申请日：1996-03-26
申请人： Daisuke Fukuoka , Takashi Tashiro , Koji Kawaai , Junji Saito , Takashi Ueda , Yoshihisa Kiso , Junichi Imuta , Terunori Fujita , Masatoshi Nitabaru , Masayasu Yoshida
发明人： Daisuke Fukuoka , Takashi Tashiro , Koji Kawaai , Junji Saito , Takashi Ueda , Yoshihisa Kiso , Junichi Imuta , Terunori Fujita , Masatoshi Nitabaru , Masayasu Yoshida
IPC分类号： C07C45/46 , C07C49/67 , C07C49/697 , C07F17/00 , C08F4/60 , C08F4/602 , C08F4/619 , C08F4/6192 , C08F4/64 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06 , C08F210/16 , C07F7/08
CPC分类号： C08F210/16 , C07C45/46 , C07C49/67 , C07C49/697 , C07F17/00 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06 , C08F4/61912 , C08F4/61927 , C08F4/65908 , C08F4/65912 , C08F4/65916 , C08F4/65927 , Y10S526/904 , Y10S526/943
摘要： The novel transition metal compound of the invention is represented by the following formula (I): ##STR1## wherein M is a transition metal; R.sup.1 is a hydrocarbon group of 2 to 6 carbon atoms, R.sup.2 is an aryl group of 6 to 16 carbon atoms; X.sup.1 and X.sup.2 are each a halogen atom or the like; and Y is a divalent hydrocarbon group, a divalent silicon-containing group or the like. An olefin polymerization catalyst component of the present invention comprises the aforementioned transition metal compound.
摘要翻译：本发明的新型过渡金属化合物由下式（I）表示：是2至6个碳原子的烃基，R 2是6至16个碳原子的芳基; X1和X2各自为卤素原子等; Y为二价烃基，二价含硅基团等。本发明的烯烃聚合催化剂组分包含上述过渡金属化合物。

78. 发明授权

US4582944A Process for producing hydroxydiphenyl ethers 失效
标题翻译：生产羟基二苯醚的方法
公开(公告)号：US4582944A
公开(公告)日：1986-04-15
申请号：US606611
申请日：1984-05-03
申请人： Katsuo Taniguchi , Hideo Nakamura , Terunori Fujita
发明人： Katsuo Taniguchi , Hideo Nakamura , Terunori Fujita
IPC分类号： B01J27/00 , B01J27/12 , C07B61/00 , C07C41/00 , C07C41/09 , C07C43/295 , C07C67/00
CPC分类号： C07C41/09
摘要： A process for producing a hydroxydiphenyl ether, which comprises reacting at least one hydroquinone compound with itself or with a monohydric phenol compound in the presence of a catalyst composed essentially of a synthetic mica in which at least 10 mole % of cation-exchangeable interlayer cations are made up of a metal ion other than alkali metal ions, and/or a proton.
摘要翻译：一种生产羟基二苯醚的方法，其包括使至少一种氢醌化合物与其自身或与一元酚化合物在催化剂存在下反应，所述催化剂基本上由合成云母组成，其中至少10摩尔％的可阳离子交换的层间阳离子是由除金属离子以外的金属离子和/或质子组成。

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