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61. 发明申请

US20130006029A1 HYDROTREATING PROCESS 有权
标题翻译：加氢过程
公开(公告)号：US20130006029A1
公开(公告)日：2013-01-03
申请号：US13575849
申请日：2011-02-21
申请人： Gabor Kiss , Iulian Nistor , John Zengel , Sabato Miseo , Roman Krycak , Teh C. Ho
发明人： Gabor Kiss , Iulian Nistor , John Zengel , Sabato Miseo , Roman Krycak , Teh C. Ho
IPC分类号： C07C1/32
CPC分类号： C10G49/24 , B01J38/56 , C10G45/02 , C10G45/08 , C10G2300/1055 , C10G2300/1096 , C10G2300/202 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2400/04
摘要： A process for hydrotreating a first aromatics- and sulfur-containing hydrocarbon feed using a fresh supported CoMo catalyst, includes treating the fresh catalyst under first hydrotreating conditions with a second hydrocarbon feed having a lower aromatics content than the first feed.
摘要翻译：使用新鲜负载的CoMo催化剂加氢处理第一芳烃和含硫烃进料的方法包括在第一加氢处理条件下用比第一进料芳烃含量低的第二烃进料处理新鲜催化剂。

62. 发明授权

US08067331B2 Bulk catalyst comprising nickel tungsten metal oxidic particles 有权
标题翻译：包含镍钨金属氧化物颗粒的散装催化剂
公开(公告)号：US08067331B2
公开(公告)日：2011-11-29
申请号：US12091322
申请日：2006-10-25
申请人： Sona Eijsbouts-Spickova , Robertus Gerardus Leliveld , Marinus Bruce Cerfontain , Frans L. Plantenga , Eelco Titus Carel Vogt , Jacobus Nicolaas Louwen , Stuart Leon Soled , Sabato Miseo , Kenneth L. Riley
发明人： Sona Eijsbouts-Spickova , Robertus Gerardus Leliveld , Marinus Bruce Cerfontain , Frans L. Plantenga , Eelco Titus Carel Vogt , Jacobus Nicolaas Louwen , Stuart Leon Soled , Sabato Miseo , Kenneth L. Riley
IPC分类号： C10G45/04
CPC分类号： B01J23/888 , B01J23/002 , B01J35/002 , B01J37/0009 , B01J37/03 , B01J37/10 , B01J37/20 , B01J2523/00 , C10G45/08 , C10G2300/202 , B01J2523/69 , B01J2523/847 , B01J2523/68 , B01J2523/56
摘要： The invention relates to a nickel tungsten bulk catalyst, to a process for the manufacture of said catalyst and to the use of said catalyst for the hydrotreatment, in particular the hydrodesulphurisation and hydrodenitrogenation of hydrocarbon feedstock. The catalyst comprises nickel tungsten metal oxidic particles obtainable by a process comprising forming a slurry of a first solid metal compound comprising Group VNI metal nickel and a second solid metal compound comprising Group VIB metal tungsten in a protic liquid, reacting the first and second solid metal compounds at elevated temperature whereby the first and second solid metal compounds remain at least partly in the solid state during the entire reaction to form the nickel tungsten oxidic bulk catalyst.
摘要翻译：本发明涉及镍钨体积催化剂，制备所述催化剂的方法以及所述催化剂用于加氢处理的用途，特别是烃原料的加氢脱硫和加氢脱氮。该催化剂包括可通过以下工艺获得的镍钨金属氧化物颗粒，所述方法包括在质子液体中形成包含VNI族金属镍的第一固体金属化合物和包含第VIB族金属钨的第二固体金属化合物的浆料，使第一和第二固体金属化合物在高温下由此第一和第二固体金属化合物在整个反应期间保持至少部分为固体状态以形成镍钨氧化物本体催化剂。

63. 发明申请

US20070082811A1 Method of preparing a hydrotreating catalyst on a support containing a rare earth metal 有权
标题翻译：在含有稀土金属的载体上制备加氢处理催化剂的方法
公开(公告)号：US20070082811A1
公开(公告)日：2007-04-12
申请号：US11238930
申请日：2005-09-29
申请人： Stuart Soled , Sabato Miseo , Joseph Baumgartner , Christine Kliewer , Jeffrey Elks
发明人： Stuart Soled , Sabato Miseo , Joseph Baumgartner , Christine Kliewer , Jeffrey Elks
IPC分类号： B01J23/00
CPC分类号： B01J23/8871 , B01J23/888 , B01J37/0203 , B01J37/0205 , B01J37/20
摘要： This invention relates to supported multi-metallic catalysts for use in the hydroprocessing of hydrocarbon feeds, as well as a method for preparing such catalysts. The catalysts are prepared from a catalyst precursor comprised of at least one Group VIII metal and a Group VI metal and an organic agent selected from the group consisting of amino alcohols and amino acids.
摘要翻译：本发明涉及用于烃进料加氢处理的负载型多金属催化剂，以及制备这种催化剂的方法。催化剂由至少一种VIII族金属和第Ⅵ族金属的催化剂前体和选自氨基醇和氨基酸的有机试剂制备。

64. 发明申请

US20060060502A1 Bulk bi-metallic catalysts made from precursors containing an organic agent 有权
公开(公告)号：US20060060502A1
公开(公告)日：2006-03-23
申请号：US11227726
申请日：2005-09-14
申请人： Stuart Soled , Sabato Miseo , Zhiguo Hou
发明人： Stuart Soled , Sabato Miseo , Zhiguo Hou
IPC分类号： C10G45/04 , C10G45/44 , C10G47/02 , C10G45/60 , C07C5/02 , B01J27/02 , B01J31/00 , B01J27/043
CPC分类号： B01J35/002 , B01J23/88 , B01J23/883 , B01J23/888 , B01J27/188 , B01J27/24 , B01J35/1014 , B01J35/1038 , B01J37/0018 , B01J37/03 , B01J37/20 , B01J37/28 , C10G45/08 , C10G45/38 , C10G45/50 , C10G45/60 , C10G47/02 , C10G49/04 , C10G49/08 , C10G65/02 , C10G65/12
摘要： Bulk bi-metallic catalysts for use in the hydroprocessing of hydrocarbon feeds, as well as a method for preparing such catalysts. The catalysts are prepared from a catalyst precursor containing an organic agent.

65. 发明授权

US5728644A Dispersed metal sulfide catalysts for hydroprocessing 失效
标题翻译：用于加氢处理的分散金属硫化物催化剂
公开(公告)号：US5728644A
公开(公告)日：1998-03-17
申请号：US524228
申请日：1995-09-05
申请人： Teh Chung Ho , Stuart Leon Soled , Sabato Miseo , Gary Brice Mc Vicker , Michel Daage , Viktor Buchholz
发明人： Teh Chung Ho , Stuart Leon Soled , Sabato Miseo , Gary Brice Mc Vicker , Michel Daage , Viktor Buchholz
IPC分类号： B01J31/22 , B01J23/887 , B01J23/889 , B01J27/051 , B01J37/08 , B01J37/20 , C07B35/02 , C10G45/46 , C10G45/50 , B01J27/047 , B01J23/63 , B01J31/00
CPC分类号： B01J37/086 , B01J23/887 , B01J23/8878 , B01J23/8892 , B01J27/051 , B01J37/20 , C10G45/46 , C10G45/50
摘要： The present invention is directed toward a catalyst composition comprising a catalyst prepared by a process comprising: (a) impregnating an oxide precursor selected from the group consisting of rare earth oxide precursors, yttria precursors and mixtures thereof, onto an inorganic refractory oxide support; (b) drying said support at a temperature of about 100.degree. to about 120.degree. C. followed by calcining said support at a temperature of about 400.degree. to about 600.degree. C.; and (c) compositing or depositing on said support of step (b), a catalyst precursor salt represented by (ML)(Mo.sub.y W.sub.1-y O.sub.4).sub.a wherein M comprises Cr and/or one or more divalent promoter metals selected from the group consisting of Mn, Fe, Co, Ni, Cu, Zn and mixtures thereof, wherein y is any value ranging from 0 to 1, and wherein L is one or more neutral, nitrogen-containing ligands at least one of which is a chelating polydentate ligand; a=1 when chromium is not one of the promoter metals and 0.5.ltoreq.a.ltoreq.3 when Cr is one of the promoter metals. (d) sulfiding said deposited or composited supports of step (c) with an excess amount of sulfur in the form of one or more sulfur bearing compounds and at a temperature of at least about 250.degree. C. to form catalysts. In a preferred embodiment, the process will further comprise decomposing the composited or deposited supports of step (c) in a nonoxidizing atmosphere at a temperature of at least about 250.degree. C. prior to said sulfiding step (d). In a second aspect of the invention there is provided an improved aromatics hydrogenation process.
摘要翻译：本发明涉及一种催化剂组合物，其包含通过以下方法制备的催化剂，所述催化剂包括：（a）将选自稀土氧化物前体，氧化钇前体及其混合物的氧化物前体浸渍到无机耐火氧化物载体上; （b）在约100至约120℃的温度下干燥所述载体，然后在约400至约600℃的温度下煅烧所述载体; 和（c）在步骤（b）的所述载体上合成或沉积由（ML）（MoyW1-yO4）a表示的催化剂前体盐，其中M包含Cr和/或一种或多种选自以下的二价助催化剂金属： Mn，Fe，Co，Ni，Cu，Zn及其混合物，其中y是0至1的任何值，并且其中L是一种或多种中性含氮配体，其中至少一种是螯合多齿配体; 当Cr不是助催化剂金属之一时，a = 1，当Cr是助催化剂金属之一时，a = 1。（d）用一种或多种带硫化合物形式的过量硫磺和至少约250℃的温度硫化所述步骤（c）的沉积或复合载体以形成催化剂。在优选的实施方案中，该方法还包括在所述硫化步骤（d）之前，在至少约250℃的温度下，在非氧化气氛中分解步骤（c）的复合或沉积的载体。在本发明的第二方面，提供了一种改进的芳族化合物氢化方法。

66. 发明授权

US4752600A Slurried CO hydrogenation catalysts 失效
标题翻译：浆化CO加氢催化剂
公开(公告)号：US4752600A
公开(公告)日：1988-06-21
申请号：US909788
申请日：1986-09-22
申请人： Rocco A. Fiato , Sabato Miseo
发明人： Rocco A. Fiato , Sabato Miseo
IPC分类号： B01J23/46 , C07C1/04 , B01J21/06
CPC分类号： B01J23/462 , C07C1/0445 , C07C2521/06 , C07C2523/46
摘要： A process for forming a catalyst composition produced by the steps of:(a) adding to a stirred reactor TiO.sub.2, a ruthenium carbonyl complex and an inert alkane hydrocarbon;(b) adding a gas mixture of N.sub.2 :CO to said slurry reactor;(c) adding a gas mixture of N.sub.2 :H.sub.2 to said slurry reactor; and(d) increasing the temperature of said slurry reactor from about 20.degree. C. to about 250.degree. C. and the pressure of said slurry reactor from about 1 to about 20 atm for about 2 to about 6 hours to cause the decomposition of said ruthenium carbonyl complex to form said slurry catalyst composition.
摘要翻译：一种形成催化剂组合物的方法，所述催化剂组合物通过以下步骤制备：（a）向搅拌的反应器中加入TiO 2，羰基钌羰基络合物和惰性烷烃; （b）向所述淤浆反应器中加入N 2 :CO的气体混合物; （c）将N 2：H 2的气体混合物加入到所述淤浆反应器中; 和（d）将所述淤浆反应器的温度从约20℃升至约250℃，所述淤浆反应器的压力从约1至约20大气压下加热约2至约6小时，以使所述钌羰基络合物以形成所述浆料催化剂组合物。

67. 发明授权

US4657885A Cerium promoted Fischer-Tropsch catalysts 失效
标题翻译：铈促进费 - 托催化剂
公开(公告)号：US4657885A
公开(公告)日：1987-04-14
申请号：US754004
申请日：1985-07-11
申请人： Rocco A. Fiato , Ronny Bar-Gadda , Sabato Miseo
发明人： Rocco A. Fiato , Ronny Bar-Gadda , Sabato Miseo
IPC分类号： B01J23/80 , B01J23/889 , C07C1/04 , B01J21/00 , B01J23/24
CPC分类号： C07C1/044 , B01J23/80 , B01J23/889 , C07C1/0445 , C07C2521/06 , C07C2523/04 , C07C2523/06 , C07C2523/10 , C07C2523/34 , C07C2523/745 , C07C2523/83 , C07C2523/889 , Y10S502/524
摘要： New Fischer-Tropsch catalysts containing a Lanthanide Group element, such as cerium, exhibit improved activity over conventional catalysts and exhibit a reversal in the olefin/paraffin ratio of low molecular weight hydrocarbons. The catalyst comprises:(a) a Group VIII metal oxide;(b) a Group IIB metal oxide;(c) a Group IVB and/or VIIB metal oxide;(d) a Group IA metal oxide; and,(e) a Lanthanide group metal oxide.
摘要翻译：含有镧系元素元素（如铈）的新的费 - 托催化剂显示出比常规催化剂更好的活性，并表现出低分子量烃的烯烃/石蜡比例的逆转。催化剂包括：（a）第Ⅷ族金属氧化物; （b）IIB族金属氧化物; （c）IVB族和/或VIIB族金属氧化物; （d）IA族金属氧化物; 和（e）镧系元素金属氧化物。

68. 发明授权

US08394263B2 Bulk catalyst comprising metal oxidic particles and a process for the manufacture thereof 有权
标题翻译：包含金属氧化物颗粒的散装催化剂及其制造方法
公开(公告)号：US08394263B2
公开(公告)日：2013-03-12
申请号：US12091327
申请日：2006-10-25
申请人： Sona Eijsbouts-Spickova , Robertus Gerardus Leliveld , Stuart Leon Soled , Sabato Miseo
发明人： Sona Eijsbouts-Spickova , Robertus Gerardus Leliveld , Stuart Leon Soled , Sabato Miseo
IPC分类号： B01J23/755
CPC分类号： B01J37/20 , B01J23/85 , B01J23/8885 , B01J35/002 , B01J35/1014 , B01J35/1019 , B01J35/1061 , B01J37/0009 , B01J37/0045 , B01J37/10 , C10G45/08 , C10G2300/202
摘要： The invention relates to a bulk catalyst having improved activity in hydrodesulphurization, in particular in relatively low Group VIII over Group VIB metal molar ratios. The bulk catalyst comprises metal oxidic particles comprising one or more Group VIB metals and one or more-Group VIII metals which metal oxidic particles are obtainable by a process comprising the steps of reacting the compounds comprising one or more Group VIB metals and compounds comprising one or more Group VIII metals in hydrothermal conditions at a reaction temperature above the boiling temperature of the protic liquid, preferably in an autoclave at a reaction pressure above atmospheric pressure and. The invention also relates to the corresponding sulphided catalyst, to a process for the manufacture of said bulk catalyst and to the use of said catalyst for the hydrotreatment, in particular the hydrodesulphurization and hydrodenitrogenation of hydrocarbon feedstock.
摘要翻译：本发明涉及具有改进的加氢脱硫活性的本体催化剂，特别是在VIB族金属摩尔比相对较低的第VIII族。本体催化剂包含包含一种或多种VIB族金属和一种或多种VIII族金属的金属氧化物颗粒，该金属氧化物颗粒可通过包括以下步骤的方法获得，所述方法包括使包含一种或多种VIB族金属的化合物与包含一种或多种反应温度高于质子液体沸点温度的水热条件下，优选在反应压力高于大气压的高压釜中。本发明还涉及相应的硫化催化剂，制备所述本体催化剂的方法以及所述催化剂用于加氢处理的用途，特别是烃原料的加氢脱硫和加氢脱氮。

69. 发明授权

US07288182B1 Hydroprocessing using bulk Group VIII/Group VIB catalysts 有权
标题翻译：使用本体VIII / VIB族催化剂进行加氢处理
公开(公告)号：US07288182B1
公开(公告)日：2007-10-30
申请号：US09869984
申请日：2000-01-14
申请人： Stuart Leon Soled , Sabato Miseo , Roman Krycak , Hilda B. Vroman , Teh Chung Ho , Kenneth Lloyd Riley
发明人： Stuart Leon Soled , Sabato Miseo , Roman Krycak , Hilda B. Vroman , Teh Chung Ho , Kenneth Lloyd Riley
IPC分类号： C10G73/02 , C10G11/00 , B01J29/70 , B01J23/00 , B01J23/70
CPC分类号： B01J23/002 , B01J23/85 , B01J23/88 , B01J23/883 , B01J23/8878 , B01J23/888 , B01J23/8885 , B01J37/03 , B01J37/082 , B01J2523/00 , C08F8/00 , C08F8/04 , C08F8/50 , C10G45/08 , C10G45/16 , C10G47/04 , C10G65/04 , C10G65/08 , C10G65/12 , C10G2400/10 , C10G2400/14 , C08F240/00 , B01J2523/68 , B01J2523/69 , B01J2523/847 , B01J2523/842 , B01J2523/67 , B01J2523/31 , B01J2523/41
摘要： A process for hydroprocessing petroleum and chemical feedstocks by use of a bulk multimetallic catalyst comprised of at least one Group VIII non-noble metal and at least one, preferably two Group VIB metal wherein the ratio of Group VIB metal to Group VIII metal is from about 10:1 to 1:10.
摘要翻译：通过使用由至少一种VIII族非贵金属和至少一种，优选两种VIB族金属组成的本体多金属催化剂加氢处理石油和化学原料的方法，其中VIB族金属与VIII族金属的比例为约 10：1到1:10。

70. 发明申请

US20060293544A1 Partially decomposed catalyst and hydrocarbon oxidation processes using the same 有权
标题翻译：部分分解的催化剂和烃氧化方法使用它们
公开(公告)号：US20060293544A1
公开(公告)日：2006-12-28
申请号：US11434717
申请日：2006-05-16
申请人： Jihad Dakka , Sabato Miseo , Stuart Soled , Jose Santiesteban , Joseph Baumgartner , Michiel Van Vliet , Roger Sheldon
发明人： Jihad Dakka , Sabato Miseo , Stuart Soled , Jose Santiesteban , Joseph Baumgartner , Michiel Van Vliet , Roger Sheldon
IPC分类号： C07C27/00
CPC分类号： B01J31/2243 , B01J23/76 , B01J2231/70 , B01J2531/16 , B01J2531/847 , C07C68/00 , C07C69/96
摘要： The present invention is related to a hydrocarbon oxidation process. The process comprises bringing one or more hydrocarbons into contact with a source of oxygen in the presence of a radical initiator and a catalyst. The catalyst comprises an organic metal complex located on a catalyst support, and is obtained by partial decomposition of the organic metal complex. For example, the process can be used to produce dimethyl carbonate from dimethoxy methane. The invention is also related to a partially decomposed catalyst that comprises a silica support and an organic metal complex, wherein at least 5% of the organic compound remains in the catalyst. The organic metal complex comprises an organic compound and a metal-based compound wherein the metal is selected from copper, nickel, and combinations thereof. The invention is also related to a process for manufacturing of a catalyst comprising mixing L-arginine, a Cu-based compound, water, and optionally another metal-based compound to form a solution; impregnating the solution onto a silica support to form a catalyst precursor; and partially decomposing the L-arginine to form the catalyst so that at least 5% of L-arginine remains in the catalyst.
摘要翻译：本发明涉及烃氧化方法。该方法包括在自由基引发剂和催化剂的存在下使一种或多种烃与氧源接触。催化剂包含位于催化剂载体上的有机金属络合物，并通过有机金属络合物的部分分解获得。例如，该方法可用于从二甲氧基甲烷生产碳酸二甲酯。本发明还涉及包含二氧化硅载体和有机金属络合物的部分分解的催化剂，其中至少5％的有机化合物保留在催化剂中。有机金属络合物包括有机化合物和金属基化合物，其中金属选自铜，镍及其组合。本发明还涉及制造催化剂的方法，其包括将L-精氨酸，Cu基化合物，水和任选的其它金属类化合物混合以形成溶液; 将溶液浸渍到二氧化硅载体上以形成催化剂前体; 并部分分解L-精氨酸以形成催化剂，使得至少5％的L-精氨酸保留在催化剂中。

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