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51. 发明专利

JP2010280974A Gas diffusion electrode and method of manufacturing the same 有权
标题翻译：气体扩散电极及其制造方法
公开(公告)号：JP2010280974A
公开(公告)日：2010-12-16
申请号：JP2009136659
申请日：2009-06-05
申请人： Permelec Electrode Ltd , Tokyo Institute Of Technology , ペルメレック電極株式会社 , 国立大学法人東京工業大学
发明人： OSAKA TAKEO , FERDOUSI BEGUM NADIRA , OKAJIMA TAKEYOSHI , SUZUKI TOMOHISA , NISHIKI YOSHINORI
IPC分类号： C25B11/06 , C25B11/03 , C25B11/08
摘要： PROBLEM TO BE SOLVED: To provide a gas diffusion electrode being more inexpensive and having higher electrode activity than a platinum group metal or a metal oxide, prevented from the deterioration of the electrode and capable of attaining the stabilization of an electrochemical system and the longer life of the electrode.
SOLUTION: The gas diffusion electrode has a co-catalyst layer containing a metal such as tantalum and/or the metal oxide and formed on the surface of a main catalyst particle of a platinum group or the like formed on the surface of a conductive base material. The activity of the co-catalyst layer synergistically is increased by forming the co-catalyst layer on the surface of the main catalyst particle.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：为了提供比铂族金属或金属氧化物更便宜并且具有更高的电极活性的气体扩散电极，防止了电极的劣化并且能够实现电化学系统的稳定化，电极寿命更长。解决方案：气体扩散电极具有包含诸如钽和/或金属氧化物的金属的助催化剂层，并且形成在形成在表面上的铂族等的主催化剂颗粒的表面上导电基材。通过在主催化剂颗粒的表面上形成助催化剂层，协同催化剂层的活性增加。版权所有（C）2011，JPO＆INPIT

52. 发明专利

JP2010174358A Anode for electrolysis and method for electrolytically synthesizing fluorine-containing substance using the anode for electrolysis 审中-公开
标题翻译：用于电解的阳极和使用阳离子电解的含氟化合物的电解合成方法
公开(公告)号：JP2010174358A
公开(公告)日：2010-08-12
申请号：JP2009021157
申请日：2009-02-02
申请人： Permelec Electrode Ltd , ペルメレック電極株式会社
发明人： TASAKA AKIMASA , UNO MASAHARU , NISHIKI YOSHINORI , FURUTA TSUNETO
IPC分类号： C25B11/12 , C25B1/24
CPC分类号： C25B11/12 , C25B1/245 , C25B11/0405
摘要： PROBLEM TO BE SOLVED: To provide an anode material for electrolysis, which is free from the occurrence of an anode effect in electrolysis with an electrolytic bath containing hydrofluoric acid, does not remarkably produce sludge due to the dissolution of an electrode, is capable of suppressing the production of CF 4 and capable of stably continuing electrolysis without causing the breakdown of the electrode. SOLUTION: At least part of a conductive material substrate whose surface is made of glassy carbon is coated with a conductive diamond film. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：为了提供一种电解用负极材料，其不含在含有氢氟酸的电解浴中的电解中产生阳极效应，不会由于电极的溶解而显着地产生污泥，是能够抑制CF 4 的生产，并能够稳定地继续电解而不引起电极的破坏。解决方案：其表面由玻璃碳制成的导电材料基材的至少一部分涂覆有导电金刚石膜。版权所有（C）2010，JPO＆INPIT

53. 发明专利

JP2009138262A Membrane-electrode assembly, electrolysis cell using the same, electrolyzed water spraying device, and sterilization method 有权
标题翻译：膜电极组件，使用其的电解质电池，电解水喷雾装置和灭菌方法
公开(公告)号：JP2009138262A
公开(公告)日：2009-06-25
申请号：JP2008266158
申请日：2008-10-15
申请人： Institute Of National Colleges Of Technology Japan , Permelec Electrode Ltd , ペルメレック電極株式会社 , 独立行政法人国立高等専門学校機構
发明人： KITAORI NORIYUKI , SEKIDO KOTA , SHIBATA TOMOYASU , SUZUKI TOMOHISA , TANAKA MASASHI , FURUTA TSUNETO , NISHIKI YOSHINORI
IPC分类号： C25B9/00 , A61L2/22 , C02F1/46 , C25B1/13
CPC分类号： C02F2201/003
摘要： PROBLEM TO BE SOLVED: To provide a membrane-electrode assembly and an electrolysis cell for producing an electrolyzed water which has an electrolytic product such as ozone dissolved therein in higher concentration than before; a device for spouting the electrolyzed water obtained by using them; and a miniaturized spray device particularly for spraying the obtained electrolyzed water in a mist state. SOLUTION: This membrane-electrode assembly has: a rod-shaped anode 7; a tubular diaphragm 8 installed in the periphery of the anode 7; a wire-shaped cathode 9 which is installed in the periphery of the diaphragm 8 and is used for fixing the diaphragm 8 to the anode 7; and an anode chamber 10 thereby formed in between the diaphragm 8 and the anode 7, which forms a passage for a gas and a liquid therein. By adequately selecting each member, the concentration of electrolyte species in the electrolyzed water can be set at a desired value. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：解决方案：提供一种膜电极组件和用于生产电解水的电解池，该电解水具有比以前更高浓度的溶解有臭氧的电解产物的电解水; 用于喷射通过使用它们获得的电解水的装置; 以及特别用于雾化所得到的电解水的小型喷雾装置。解决方案：该膜 - 电极组件具有：杆状阳极7; 安装在阳极7的周围的管状隔膜8; 线状阴极9，其安装在隔膜8的周围，用于将隔膜8固定到阳极7; 以及由此形成在隔膜8和阳极7之间的阳极室10，其在其中形成气体和液体的通道。通过适当地选择每个构件，可以将电解水中的电解质种类的浓度设定为期望值。版权所有（C）2009，JPO＆INPIT

54. 发明专利

JP2008127631A Oxygen-gas diffusion cathode for use in brine electrolysis 有权
标题翻译：氧气扩散阴极在电泳中的应用
公开(公告)号：JP2008127631A
公开(公告)日：2008-06-05
申请号：JP2006314216
申请日：2006-11-21
申请人： Permelec Electrode Ltd , ペルメレック電極株式会社
发明人： YAMADA YUJI , IZAWA YUKI , NISHIKI YOSHINORI
IPC分类号： C25B11/08 , C25B1/02 , C25B9/00 , C25B11/03 , C25B11/12
CPC分类号： C25B11/035 , C25B11/0494 , C25B11/12
摘要： PROBLEM TO BE SOLVED: To provide a superior gas diffusion cathode which has long time stability and lowers cell voltage compared to a conventional electrode so as to enable the industrial production of gases through brine electrolysis in which the cathode is exposed to a harsh electrolysis environment.
SOLUTION: The oxygen-gas diffusion cathode 1 for use in the brine electrolysis has a catalyst layer 2 comprising silver and palladium formed so as to cover a porous and electroconductive substrate 3 made from silver, a hydrophobic material and a carbon material. Thus, formed structure makes the catalyst layer 2 including silver and palladium decrease overvoltage by lowering electric resistance and improving catalytic activity, and makes the electroconductive substrate 3 provide superior gas supply properties because of its porosity and improved electroconductivity. Accordingly, the cathode can decrease the overvoltage, reduce the resistance component, improve durability, and can be used for the brine electrolysis of which the electrolysis condition is harsh among electrolysis reactions.
COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：要解决的问题：提供与常规电极相比具有长时间稳定性和降低电池电压的优异气体扩散阴极，以便能够通过盐水电解工业生产气体，其中阴极暴露于苛刻电解环境。解决方案：用于盐水电解的氧气扩散阴极1具有包含银和钯形成的催化剂层2，以覆盖由银，疏水材料和碳材料制成的多孔导电基材3。因此，形成结构使得包含银和钯的催化剂层2通过降低电阻和改善催化活性而降低过电压，并且由于其孔隙率和改善的导电性，导电基板3提供优异的气体供应性能。因此，阴极可以降低过电压，降低电阻成分，提高耐久性，并且可以用于电解反应中电解条件恶劣的盐水电解。版权所有（C）2008，JPO＆INPIT

55. 发明专利

JP2007242433A Electrode catalyst for electrochemical reaction, manufacturing method of the same, and electrochemical electrode having the same 审中-公开
标题翻译：电化学反应用电极催化剂及其制造方法及其电化学电极
公开(公告)号：JP2007242433A
公开(公告)日：2007-09-20
申请号：JP2006063586
申请日：2006-03-09
申请人： Permelec Electrode Ltd , Shinshu Univ , ペルメレック電極株式会社 , 国立大学法人信州大学
发明人： TAKASU YOSHIO , MURAKAMI YASUSHI , SUGIMOTO WATARU , YAMADA YUJI , UNO MASAHARU , NISHIKI YOSHINORI , FURUTA TSUNETO
IPC分类号： H01M4/86 , H01M4/88 , H01M8/10
CPC分类号： H01M4/90 , C25B1/34 , C25B11/0478 , H01M4/8605 , H01M4/9083 , H01M4/92 , H01M4/926 , H01M2008/1095
摘要： PROBLEM TO BE SOLVED: To provide an electrode catalyst for an electrochemical reaction for a fuel cell or brine electrolysis and the like which is stabilized in catalyst activity more than a conventional diamond electrode.
SOLUTION: This electrode catalyst for an electrochemical reaction is formed out of conductive diamond particles each formed by supporting a carbon reactive catalyst metal to pores formed on its surface. The catalyst can be used as an oxygen electrode 2 or a hydrogen electrode 3 of a fuel cell, or as a gas diffusion negative electrode of a brine electrolysis bath. The metal catalyst supported in the pores is high in stability of the catalyst (aggregation suppression, come-off prevention as compared with a metal catalyst supported to a particle surface), can achieve high activity and a long life by a small amount of metal, and can reduce usage of an expensive metal.
COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供一种用于燃料电池或盐水电解等的电化学反应的电极催化剂，其比传统的金刚石电极更能稳定催化剂活性。解决方案：用于电化学反应的电极催化剂由导电金刚石颗粒形成，每个导电金刚石颗粒通过将碳反应性催化剂金属担载在其表面上形成的孔而形成。催化剂可以用作燃料电池的氧电极2或氢电极3，也可以用作盐水电解槽的气体扩散负极。负载在孔中的金属催化剂在催化剂的稳定性方面（凝聚抑制，与负载于颗粒表面的金属催化剂相比的脱离防止）可以通过少量的金属实现高活性和长寿命，并且可以减少贵金属的使用。版权所有（C）2007，JPO＆INPIT

56. 发明专利

JP2006193768A Cathode for hydrogen generation 有权
标题翻译：氢生成阴极
公开(公告)号：JP2006193768A
公开(公告)日：2006-07-27
申请号：JP2005004921
申请日：2005-01-12
申请人： Permelec Electrode Ltd , ペルメレック電極株式会社
发明人： NARA MIWAKO , NAKANO YUSUKE , NISHIKI YOSHINORI , FURUTA TSUNETO , SHIMIZU HIDETO , HIRAO KAZUHIRO
IPC分类号： C25B11/06 , C25B11/04
摘要： PROBLEM TO BE SOLVED: To provide a cathode for hydrogen generation in which electrode activity is high, and which has long term stability compared with the conventional one.
SOLUTION: The cathode for hydrogen generation is obtained by forming a catalyst layer on a cathode substrate. The catalyst layer comprises metals of cerium, platinum and ruthenium, the metal oxides or hydroxides thereof in the ranges of 0
摘要翻译：要解决的问题：提供电极活性高的氢气生成用阴极，与现有技术相比长期稳定。解决方案：通过在阴极基板上形成催化剂层来获得产生氢气的阴极。催化剂层包括铈，铂和钌的金属，其金属氧化物或氢氧化物的含量范围为0

57. 发明专利

JP2005166500A Manufacturing method of porous electrode for electrochemistry 有权
标题翻译：电化学多孔电极的制备方法
公开(公告)号：JP2005166500A
公开(公告)日：2005-06-23
申请号：JP2003404871
申请日：2003-12-03
申请人： Permelec Electrode Ltd , ペルメレック電極株式会社
发明人： KASUGA TAKESHI , UNO MASAHARU , NISHIKI YOSHINORI , FURUTA TSUNETO
IPC分类号： H01M4/88
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a manufacturing method of a porous electrode for electrolysis carrying a catalyst only on the surface of the porous electrode without carrying the catalyst inside pores on the inside of the porous electrode and usable as an electrode substrate or a current collector. SOLUTION: At least the substrate surface side space of pores is sealed with a sealant 6 by covering a porous substrate surface 1 having pores 2 with a sealant solution, a catalyst layer is formed on the substrate surface, and the sealant is eluted and removed. Penetration of an electrode catalyst into the pores is substantially prevented, and the porous electrode for electrochemistry in which the electrode catalyst is present only on the surface can be obtained. COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：提供一种用于仅在多孔电极的表面上承载催化剂的电解多孔电极的制造方法，而不在多孔电极的内部的孔内携带催化剂并可用作电极基板或集电器。解决方案：通过用密封剂溶液覆盖具有孔2的多孔基材表面1，在密封剂6上至少密封孔的基板表面侧空间，在基板表面上形成催化剂层，并且密封剂被洗脱并删除。基本上可以防止电极催化剂渗透到孔中，并且可以获得电极催化剂仅存在于表面上的用于电化学的多孔电极。版权所有（C）2005，JPO＆NCIPI

58. 发明专利

JP2004332108A Diamond electrode for electrolysis 有权
公开(公告)号：JP2004332108A
公开(公告)日：2004-11-25
申请号：JP2004105766
申请日：2004-03-31
申请人： Permelec Electrode Ltd , Toyo Tanso Kk , ペルメレック電極株式会社 , 東洋炭素株式会社
发明人： HOSONUMA MASASHI , NARA MIWAKO , UNO MASAHARU , NISHIKI YOSHINORI , FURUTA TSUNETO , KUROSU TATEO , FUKUNAGA OSAMU , TOJO TETSURO
IPC分类号： B01J21/18 , C01B31/06 , C23C16/27 , C25B11/06
摘要： PROBLEM TO BE SOLVED: To provide a diamond electrode having a lower service life by combining the conventional diamond electrode having a relatively short service life with the other components.
SOLUTION: The diamond electrode for electrolysis comprises an electrode base material 11 in which at least the surface consists of Magneli phase titanium oxide and electrically conductive diamond 12 supported on the electrode as an electrode catalyst, and titanium oxide powder 13 according to necessary. The Magneli phase titanium oxide does not form a stable oxide layer on the surface of the base material, and attains the improvement of its electrical conductivity.
COPYRIGHT: (C)2005,JPO&NCIPI

59. 发明专利

JP2004068127A Electrode for electrolysis, method for manufacturing the same, and electrolytic cell having this electrode for electrolysis 审中-公开
公开(公告)号：JP2004068127A
公开(公告)日：2004-03-04
申请号：JP2002232389
申请日：2002-08-09
申请人： Permelec Electrode Ltd , ペルメレック電極株式会社
发明人： IWAKURA CHIAKI , INOUE HIROSHI , FURUKAWA NAOHARU , NOHARA SHINJI , FURUTA TSUNETO , NISHIKI YOSHINORI , KOIZUMI MEGUMI
IPC分类号： C25B11/08 , C25B11/03
摘要： PROBLEM TO BE SOLVED: To provide an electrode which can drastically improve current efficiency and can rapidly perform a desired reaction, a method for manufacturing the same, and an electrolytic cell using this electrode.
SOLUTION: The electrode 5 for electrolysis is obtained by three-dimensionally forming a hydrogen occlusion material 3 which is an electrode active material on the surface of an electrode base material 1. Atomic hydrogen which is occluded into the hydrogen occlusion material and has high activity is usable as a hydrogenation source and the hydrogen occlusion material has a three-dimensional structure and has an immense increase of its surface area. The current efficiency of the target hydrogenation reaction etc., is improved by the synergistic effects of both.
COPYRIGHT: (C)2004,JPO

60. 发明专利

JP2003073873A Electrolytic fluorination method for organic ether compound 有权
标题翻译：有机醚化合物的电解荧光法
公开(公告)号：JP2003073873A
公开(公告)日：2003-03-12
申请号：JP2001264220
申请日：2001-08-31
申请人： Permelec Electrode Ltd , ペルメレック電極株式会社
发明人： FUCHIGAMI TOSHIO , ISHIKAWA HIDEKI , HASEGAWA MASARU , NISHIKI YOSHINORI , FURUTA TSUNETO
IPC分类号： C07D319/12 , C07C41/22 , C07C43/12 , C07D307/18 , C25B3/08
摘要： PROBLEM TO BE SOLVED: To provide an easier method for performing a fluorination reaction of an organic ether compound, by solving such problems that a conventional organic electrolytic reaction with the use of a solvent, often generates by- products, and causes not only reduction in a yield and selectivity coefficient, but also trouble in isolation of an aimed product.
SOLUTION: This method is characterized by using an electrolytic solution comprising the organic ether compound and a molten salt containing fluorine, to perform the fluorination reaction of the organic ether compound, without using a dedicated solvent. The method is economic and practical, because of thus using no dedicated solvent, further generates little by-product, and obviates an inconvenience associated with the by-product.
COPYRIGHT: (C)2003,JPO
摘要翻译：要解决的问题：为了提供进行有机醚化合物的氟化反应的更容易的方法，通过解决常规的使用溶剂的有机电解反应常常产生副产物的问题，并且不仅导致产率和选择性系数，也是分离目标产品的麻烦。解决方案：该方法的特征在于使用包含有机醚化合物的电解液和含氟的熔融盐，以不使用专用溶剂进行有机醚化合物的氟化反应。该方法是经济实用的，因为不使用专用溶剂，进一步产生副产物，并避免与副产物相关的不便。

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