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51. 发明专利

JP2006249442A α-OLEFIN-CONJUGATED DIENE COPOLYMER 有权
标题翻译： α-烯烃共聚二烯共聚物
公开(公告)号：JP2006249442A
公开(公告)日：2006-09-21
申请号：JP2006135482
申请日：2006-05-15
申请人： Mitsui Chemicals Inc , 三井化学株式会社
发明人： FUJITA TERUNORI , DOI YASUSHI , MITANI MAKOTO , MATSUI NARIKAZU , SAITO JUNJI , NITAHARA MASATOSHI , SUGI KIYOAKI , MAKIO HARUYUKI , TSUTSUI TOSHIYUKI
IPC分类号： C08F210/00 , C08F4/64 , C08F236/04
摘要： PROBLEM TO BE SOLVED: To provide an olefin polymerization catalyst exhibiting excellent polymerization activities, to provide a process for olefin polymerization using the catalyst, to provide a new transition metal compound useful for the catalyst for olefin polymerization, and to provide an α-olefin-conjugated diene copolymer having specific properties. SOLUTION: The olefin polymerization catalyst comprises (A) a transition metal compound of formula (I) or (II), and (B) an organometallic compound, an organoaluminum oxy compound or an ionizing ionic compound. The new transition metal compound is a compound of formula (I), wherein M is a group 4 or 5 transition metal; m is an integer of 1 to 3; R 1 is a hydrocarbon or the like; R 2 to R 5 are each H, a halogen, a hydrocarbon or the like; R 6 is a halogen, a hydrocarbon or the like; n is a number satisfying a valence of M; and X is a halogen, a hydrocarbon or the like. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：为了提供显示出优异聚合活性的烯烃聚合催化剂，提供使用该催化剂进行烯烃聚合的方法，提供用于烯烃聚合催化剂的新的过渡金属化合物，并提供α 具有特定性质的α-烯烃 - 共轭二烯共聚物。解决方案：烯烃聚合催化剂包含（A）式（I）或（II）的过渡金属化合物和（B）有机金属化合物，有机铝氧化合物或离子化离子化合物。新的过渡金属化合物是式（I）化合物，其中M是4或5族过渡金属; m为1〜3的整数。 R 1是烃或类似物; R 2 至R 5各自为H，卤素，烃等; R 6是卤素，烃等; n是满足M价的数; X是卤素，烃类等。版权所有（C）2006，JPO＆NCIPI

52. 发明专利

JP2006199975A Olefin polymerization catalyst and method for polymerizing olefin in the presence of the catalyst 有权
标题翻译： OLEFIN聚合催化剂和在催化剂存在下聚合烯烃的方法
公开(公告)号：JP2006199975A
公开(公告)日：2006-08-03
申请号：JP2006126005
申请日：2006-04-28
申请人： Mitsui Chemicals Inc , 三井化学株式会社
发明人： NAKAYAMA YASUSHI , KAWAKITA KAZUMITSU , MAKIO HARUYUKI , KOJO SHINICHI
IPC分类号： C08F4/654
摘要： PROBLEM TO BE SOLVED: To provide an olefin polymerization catalyst which can (co)polymerize an olefin in high polymerization activity, and to provide a method for polymerizing an olefin in the presence of the catalyst.
SOLUTION: This olefin polymerization catalyst comprises (A) a solid titanium catalyst component produced by bringing a liquid magnesium compound into contact with a liquid titanium compound in the presence of a fluorene ring-having diether compound represented by the general formula (i), (wherein R
a and R
b are each a 1 to 6C alkyl; X and Y are each a 1 to 6C alkyl or a halogen atom; 0≤m≤4; and 0≤n≤4), (B) an organic metal compound component containing a metal selected from the group 1 to the group III in the periodic table, and (C) an electron donor.
COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：待解决的问题：提供能够（共）聚合高聚合活性的烯烃的烯烃聚合催化剂，并提供在催化剂存在下使烯烃聚合的方法。解决方案：该烯烃聚合催化剂包含（A）在通式（i）表示的含芴环的二醚化合物存在下使液态镁化合物与液体钛化合物接触而制备的固体钛催化剂组分），（其中R“SP”a 和R b 各自为1至6个烷基; X和Y各自为1至6个烷基或卤素原子;0≤m≤ 4;0≤n≤4），（B）含有选自元素周期表中第1族至第III族的金属的有机金属化合物组分和（C）电子给体。版权所有（C）2006，JPO＆NCIPI

53. 发明专利

JP2003342326A Olefin copolymer bearing reactive group and its manufacturing method 有权
标题翻译： OLEFIN共聚物轴承反应组及其制造方法
公开(公告)号：JP2003342326A
公开(公告)日：2003-12-03
申请号：JP2002151534
申请日：2002-05-24
申请人： Mitsui Chemicals Inc , 三井化学株式会社
发明人： MAKIO HARUYUKI , TAKAGI YUKIHIRO , FUJITA TERUNORI
IPC分类号： C08F4/64 , C08F4/70 , C08F210/02 , C08F212/02
摘要： PROBLEM TO BE SOLVED: To provide a reactive low-molecular weight polyethylene copolymer bearing both a reactive group and an aromatic group expected to be useful as a compatibilizer, a resin modifier and the like, and a method for efficiently manufacturing the reactive low-molecular weight polyethylene copolymer under mild polymerization conditions. SOLUTION: The ethylene-based polymer is represented by the formula (wherein T 1 and T 2 are each a hydrogen atom, a group selected from an alkyl group and an alkenyl group and T 1 and T 2 may form a ring together; Y is a functional group having a double bond; Z is an aromatic group; and a, b, c and d are each a number of at least 0 that satisfy the weight average molecular weight of the polymer of at most 20,000), has a reactive group (Y) at least at one end of the main chain and an aromatic group (Z) and substituting groups (T 1 , T 2 ) in the side chain, and has a weight-average molecular weight of at most 20,000. The polymer is manufactured using a catalyst comprising a specific transition metal compound. COPYRIGHT: (C)2004,JPO
摘要翻译：要解决的问题：提供一种具有预期可用作增容剂的反应性基团和芳族基团的反应性低分子量聚乙烯共聚物，树脂改性剂等，以及有效制造反应性的方法低分子量聚乙烯共聚物。解决方案：基于乙烯的聚合物由式（其中T 1 和T 2 表示为氢原子，选自烷基和链烯基和T 1 和T 2 可以一起形成环; Y是具有双键的官能团; Z是芳基; a，b， c和d各自为至少为0，满足聚合物的重均分子量为至多20,000），在主链的至少一端具有反应性基团（Y）和芳族基团（Z）并且在侧链中代替组（T 1 ，T 2 ），并且具有至多20,000的重均分子量。使用包含特定过渡金属化合物的催化剂制造聚合物。版权所有（C）2004，JPO

54. 发明专利

JP2000136208A POLYMERIZATION CATALYST FOR OLEFIN AND PRODUCTION OF CATALYST AND OLEFIN POLYMER 失效
公开(公告)号：JP2000136208A
公开(公告)日：2000-05-16
申请号：JP31140198
申请日：1998-10-30
申请人： MITSUI CHEMICALS INC
发明人： MAKIO HARUYUKI , TSUTSUI TOSHIYUKI
IPC分类号： C08F4/64 , C08F4/605 , C08F4/6592 , C08F10/00
摘要： PROBLEM TO BE SOLVED: To obtain the subject catalyst capable of efficiently producing a granular olefin polymer having a high bulk density and a narrow particle size distribution by pre-polymerizing a specific monomer in the presence of a porous carrier and a specific compound, etc., in a specific solvent. SOLUTION: This catalyst for polymerizing an olefin is obtained by pre- polymerizing (A) a monomer having a polymerizable double bond in the presence of (B) a porous carrier, (C) a transition metal compound, (D) an organic boron compound and/or (E) an organoaluminum compound in (F) a medium in which the ingredient C does not dissolve. As the ingredient A, an α-olefin, a polar group-containing compound, a vinyl compound, a polyene compound, etc., are cited. As the ingredient B, a carrier, etc., in which a polymer is filled in pores, is preferably used. As the ingredient C, a compound, etc., containing a transition metal of the 4th group of the periodic table, is preferably used. As the ingredient F, a fluorine-containing organic compound, etc., are cited.

55. 发明专利

JPH10316710A OLEFIN POLYMERIZATION CATALYST AND PROCESS FOR POLYMERIZING OLEFIN 失效
公开(公告)号：JPH10316710A
公开(公告)日：1998-12-02
申请号：JP12948097
申请日：1997-05-20
申请人： MITSUI CHEMICALS INC
发明人： MAKIO HARUYUKI , DOI YASUSHI , FUJITA TERUNORI
IPC分类号： C08F4/64 , C08F10/00
摘要： PROBLEM TO BE SOLVED: To obtain an olefin polymerization catalyst which has excellent olefin polymerization activity and can give a polyolefin having excellent properties by including a transition metal compound (e.g. titanium compound), an organometallic compound, an organoaluminumoxy compound and a compound forming an ion pair with the transition metal compound. SOLUTION: The transition metal compound is represented by the formula (wherein M is a transition metal of group 3-11 in the periodic table, especially desirably titanium; R to R are each hydrogen, a halogen, a hydrocarbon group, an organosilyl, an amido, nitrile or the like, provided that not all of them can be hydrogen atoms; m is a number satisfying the valence of M; X is hydrogen, a halogen, a 1-20 C hydrocarbon group, an oxygenic group or the like; and when a plurality of Xs are present, they,may form a ring) and is desirably one in which the dianion of a structure derived by the removal of the metal has an energy difference of 9.00 or below, particularly 8.00 or below between the maximum occupied orbit and the minimum occupied orbit as measured by the MOPAC VERSION 6.00 Hamiltonian PM3 method.

56. 发明公开

EP2450361A4 ORGANOMETALLIC COMPOUNDS AND PROCESS FOR PREPARATION THEREOF 有权
标题翻译： VERFAHREN ZU IHRER HERSTELLUNG有机玻璃
公开(公告)号：EP2450361A4
公开(公告)日：2013-12-18
申请号：EP10794168
申请日：2010-06-30
申请人： MITSUI CHEMICALS INC
发明人： OCHIAI TAKASHI , MAKIO HARUYUKI
IPC分类号： C07F3/06 , C07F3/02 , C07F5/00 , C07F5/06 , C08F2/38
CPC分类号： C07F3/06 , C07F7/184 , C08F10/00 , C08F2/01
摘要： It is an object of the present invention to provide a novel organometallic compound functioning usefully as a chain transfer agent and the like in polymerization reaction of a double-bond containing compound. The present invention provides an organometallic compound represented by the following general formula (1) and a production method thereof. (in the general formula (1), M is a magnesium atom, a zinc atom, an Al-R 11 group, or a Ga-R 11 group; R 1 and R 10 are each independently a hydrocarbon group having 1 to 20 carbon atoms, or R 1 and R 10 may be united with each other to form a divalent connecting group (R 101 ) having 4 or more carbon atoms and thus form a ring; R 2 to R 9 are each independently a hydrogen atom, or a hydrocarbon group having 1 to 20 carbon atoms; Q 1 and Q 3 are each independently a divalent hydrocarbon group; Q 2 is a divalent connecting group containing a linkage by a heteroatom excluding carbon; h, j, k, m, and p are each independently 0 or 1; n is an integer of 0 to 10; and r is an integer of 0 to 1000.
摘要翻译：本发明的目的是提供一种在含双键键合的化合物的聚合反应中可用作链转移剂等的新的有机金属化合物。本发明提供由以下通式（1）表示的有机金属化合物及其制备方法。（通式（1）中，M为镁原子，锌原子，Al-R 11基或Ga-R 11基; R 1和R 10各自独立地为碳原子数1〜20的烃基原子或R 1和R 10可以彼此结合形成具有4个或更多个碳原子并因此形成环的二价连接基团（R 101）; R 2至R 9各自独立地为氢原子或具有1至20个碳原子的烃基; Q 1和Q 3各自独立地为二价烃基; Q 2为包含不含碳的杂原子的键连的二价连接基团; h，j，k，m和p各自为独立地为0或1; n为0〜10的整数，r为0〜1000的整数。

57. 发明公开

EP1666507A4 POLYOLEFIN FUNCTIONAL AT EACH END 有权
标题翻译：两端功能化聚烯烃
公开(公告)号：EP1666507A4
公开(公告)日：2008-07-30
申请号：EP04772741
申请日：2004-08-27
申请人： MITSUI CHEMICALS INC
发明人： MAKIO HARUYUKI , FUJITA TERUNORI
IPC分类号： C08F8/00 , C08F4/64 , C08F10/00
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A polyolefin which is functional at each end and which is represented by the following general formula (I) and has a molecular-weight distribution (Mw/Mn) as determined by gel permeation chromatography (GPC) of 1.0 to 1.5. It is useful in various applications. X-P-Y (I) (In the formula (I), X and Y may be the same or different and each is a group containing at least one element selected among oxygen, sulfur, nitrogen, phosphorus, and halogens; and P represents a chain consisting mainly of units of an olefin constituted of carbon atoms and hydrogen atoms only, provided that X and Y are bonded respectively to the two ends of P.)

58. 发明公开

EP3000785A4 METAL OXIDE POROUS PARTICLES, METHOD FOR PRODUCING SAME, AND USE OF SAME 有权
标题翻译： PORÖSEMETALLOXIDPARTIKEL，VERFAHREN ZUR HERSTELLUNG DAVON UND VERWENDUNG DAVON
公开(公告)号：EP3000785A4
公开(公告)日：2017-01-18
申请号：EP14801195
申请日：2014-05-14
申请人： MITSUI CHEMICALS INC
发明人： NAKAYAMA NORIO , WANG HONGBO , MAKIO HARUYUKI
IPC分类号： C01B37/00 , C01B13/32 , C08K7/24 , C08K7/26 , C08L101/00 , C09D7/12 , C09D11/00 , C09D201/00
CPC分类号： A61K9/14 , C01B13/32 , C01B33/12 , C01B37/02 , C01P2004/04 , C01P2004/32 , C01P2004/45 , C01P2004/52 , C01P2004/62 , C01P2004/64 , C01P2006/12 , C01P2006/16 , C01P2006/17 , C08K7/24 , C08K7/26 , C08L101/00 , C09D7/40 , C09D11/00 , C09D11/037 , C09D201/00 , F16L59/028
摘要： Provided are porous metal oxide particles, in which 50 % mean particle size by volume is equal to or larger than 50 nm and equal to or smaller than 300 nm, ratio of 90 % mean particle size by volume to 50 % mean particle size by volume (D90/D50) is equal to or lower than 2.0, the particles have mesopores having a pore size determined by BJH method of equal to or larger than 5 nm and equal to or smaller than 30 nm, and the structure of the pores is a three-dimensional cubic phase structure.
摘要翻译：提供的是多孔金属氧化物颗粒，其中平均粒径为50％的平均粒径等于或大于50nm且等于或小于300nm，平均粒径为90体积％至平均粒径的50％（D90 / D50）等于或低于2.0，颗粒具有通过BJH方法确定的孔径等于或大于5nm且等于或小于30nm的孔径，并且孔的结构为三维立方相结构。

59. 发明公开

EP1666506A4 POLYOLEFIN FUNCTIONAL AT ONE END 有权
标题翻译：在末端功能化聚烯烃
公开(公告)号：EP1666506A4
公开(公告)日：2008-08-06
申请号：EP04772740
申请日：2004-08-27
申请人： MITSUI CHEMICALS INC
发明人： MAKIO HARUYUKI , FUJITA TERUNORI
IPC分类号： C08F8/00 , C08F4/64 , C08F10/00
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A polyolefin which is functional at one end and which is represented by the following general formula (I) and has a molecular-weight distribution (Mw/Mn) as determined by gel permeation chromatography (GPC) of 1.0 to 1.5. It is useful in various applications. P-X (I) (In the formula (I), X is a group containing at least one element selected among oxygen, sulfur, nitrogen, phosphorus, and halogens; and P represents a polymer chain consisting mainly of units of an olefin constituted of carbon atoms and hydrogen atoms only, provided that X is bonded to an end of P.)

60. 发明公开

EP2871216A4 POLYMER PARTICLES AND USE THEREOF 审中-公开
标题翻译： POLYMERPARTIKEL UND ANWENDUNG DAVON
公开(公告)号：EP2871216A4
公开(公告)日：2016-03-02
申请号：EP13813625
申请日：2013-06-28
申请人： MITSUI CHEMICALS INC
发明人： NAKAYAMA NORIO , MAKIO HARUYUKI , TAKAHASHI KATSUYUKI
IPC分类号： C08L101/02 , C08F8/08 , C08F8/32 , C08F10/02 , C08J3/12 , C08K3/08 , C08K3/22 , C08K5/00 , C08K5/07 , C08K5/1545 , C08K5/42 , C08K5/56 , C09K3/00 , C09K9/02 , C09K11/06 , G01K11/20
CPC分类号： C09K11/025 , C08F8/32 , C08K9/10 , C09D5/26 , C09D11/037 , C09D11/50 , C09K9/02 , C09K11/06 , C09K2211/1011 , C09K2211/1018 , C09K2211/14 , C09K2211/182 , C09K2211/185 , G01K11/20 , G02B5/23 , Y10T428/2982 , C08F8/08 , C08F10/02

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