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41. 发明授权

US5043508A Process for preparing long chain alkyl aromatic compounds 失效
标题翻译：制备长链烷基芳族化合物的方法
公开(公告)号：US5043508A
公开(公告)日：1991-08-27
申请号：US483690
申请日：1990-02-23
申请人： Brent A. Aufdembrink , Charles T. Kresge , Quang N. Le , Joosup Shim , Stephen S. Wong
发明人： Brent A. Aufdembrink , Charles T. Kresge , Quang N. Le , Joosup Shim , Stephen S. Wong
IPC分类号： B01J21/06 , B01J21/16 , B01J23/04 , B01J27/053 , B01J29/04 , C07B61/00 , C07C2/66 , C07C15/02 , C07C15/107 , C10M105/06
CPC分类号： B01J29/049 , C07C2/66 , C10M105/06 , C07C2521/06 , C07C2523/04 , C10M2203/06
摘要： Relatively long chain alkyl aromatic compounds are prepared by alkylating an alkylatable aromatic compound with a relatively long chain alkylating agent under alkylation reaction conditions in the presence of a layered material as an alkylation catalyst. The layered material contains titanate in the layers and oxide pillars separating the layers. The layers also contain vacancies and/or metals incorporated therein. The degree of alkylation is a function of the interplanar d-spacing of the pillared material, which is, in turn a function of the chain length of the swelling agent used to prepare the layered material.
摘要翻译：通过在烷基化反应条件下，在作为烷基化催化剂的层状材料存在下，用相对长链烷基化剂烷基化可烷基化芳族化合物来制备相对长链烷基芳族化合物。层状材料在层中含有钛酸盐和分离层的氧化物柱。这些层还含有掺入其中的空位和/或金属。烷基化程度是柱状材料的面间距d的函数，其又是用于制备层状材料的溶胀剂的链长度的函数。

42. 发明授权

US4956517A Dehydrogenation process utilizing a pillared layered silicate plus a base metal or noble metal 失效
标题翻译：使用柱状层状硅酸盐加贱金属或贵金属的脱氢方法
公开(公告)号：US4956517A
公开(公告)日：1990-09-11
申请号：US459215
申请日：1989-12-29
申请人： Ivy D. Johnson , Pochen Chu , Charles T. Kresge
发明人： Ivy D. Johnson , Pochen Chu , Charles T. Kresge
IPC分类号： C07C5/32 , C07C5/333
CPC分类号： C07C5/325 , C07C5/3337
摘要： There is provided a process for the dehydrogenation of saturated hydrocarbons having from 2 to 5 carbon atoms. The feed is contacted with a catalyst which includes a base metal or noble metal which is incorporated into or onto a pillared layered silicate. A preferred pillared layered silicate is kenyaite containing interspathic silica, and a preferred base metal or noble metal is chromium.
摘要翻译：提供了具有2至5个碳原子的饱和烃脱氢的方法。进料与催化剂接触，催化剂包括引入到柱状层状硅酸盐中或其上的贱金属或贵金属。优选的柱状层状硅酸盐是含有间隙二氧化硅的肯尼亚，优选的贱金属或贵金属是铬。

43. 发明授权

US4899011A Xylene isomerization process to exhaustively convert ethylbenzene and non-aromatics 失效
标题翻译：二甲苯异构化方法彻底转化乙苯和非芳族化合物
公开(公告)号：US4899011A
公开(公告)日：1990-02-06
申请号：US819072
申请日：1986-01-15
申请人： Yung F. Chu , Charles T. Kresge , Rene B. LaPierre
发明人： Yung F. Chu , Charles T. Kresge , Rene B. LaPierre
IPC分类号： B01J29/00 , B01J29/40 , B01J29/70 , C07B61/00 , C07C1/00 , C07C5/27 , C07C15/08 , C07C67/00
CPC分类号： C07C5/2724 , Y02P20/52
摘要： A new xylene isomerization process which is capable of converting ethylbenzene and non-aromatic exhaustively while selectively converting xylenes to thermal equilibrium in mixed EB/xylene feeds is proposed. The new process employs a two component catalyst system; each of the components contains a strong hydrogenation metal and a zeolite. The zeolite of each of the two components differs from the other in its selectivity for xylene isomerization and its capacity to deethylete ethylbenzene. That selectivity for xylene isomerization is described by xylene diffusion properties of the zeolite. In one embodiment of the invention, ZSM-5 of greater than 1 micron crystal size and an alpha value of greater than 100 in a first component and ZSM-5 of less than 1 micron crystal size and an alpha of less than 100 in a second catalyst component satisfy the diffusion properties which allow for the exhaustive conversion of ethyl benzene and non-aromatics and the selectivity for xylene isomerization of typical xylene isomerization feeds. In a preferred embodiment, the feed is cascaded over the first component and then the aforementioned second component.
摘要翻译：提出了一种新的二甲苯异构化方法，其能够在选择性地将二甲苯转化为混合的EB /二甲苯进料中的热平衡的同时彻底转化乙苯和非芳族。新工艺采用双组分催化剂体系; 每种组分含有强氢化金属和沸石。两种组分中的每一种的沸石在二甲苯异构化的选择性及其对乙酸乙酯的能力方面彼此不同。对二甲苯异构化的选择性由沸石的二甲苯扩散性质描述。在本发明的一个实施方案中，大于1微米晶体尺寸的ZSM-5和第一组分中的大于100的α值和小于1微米晶体尺寸的ZSM-5和在一秒钟内小于100的α 催化剂组分满足允许乙苯和非芳族化合物的彻底转化以及典型的二甲苯异构化进料的二甲苯异构化的选择性的扩散性质。在优选实施方式中，进料在第一组分上然后上述第二组分级联。

44. 发明授权

US4493764A Separately supported polymetallic reforming catalyst 失效
标题翻译：单独支撑的多金属重整催化剂
公开(公告)号：US4493764A
公开(公告)日：1985-01-15
申请号：US618791
申请日：1984-06-08
申请人： Charles T. Kresge , Sowmithri Krishnamurthy , William D. McHale
发明人： Charles T. Kresge , Sowmithri Krishnamurthy , William D. McHale
IPC分类号： B01J23/656 , C10G35/09 , C10G35/06
CPC分类号： C10G35/09 , B01J23/6565
摘要： There is provided, in accordance with the present invention, a catalyst composition made up of a mixture of two components, one component comprising a minor proportion of platinum and rhenium on a support and the second component comprising a minor proportion of iridium and rhenium on a separate support. A process for reforming a charge stock, such as naphtha, utilizing such catalyst is also provided.
摘要翻译：根据本发明，提供了由两种组分的混合物组成的催化剂组合物，一种在载体上包含少量铂和铼的组分，第二组分包含少量的铱和铼单独支持。还提供了利用这种催化剂重整电荷原料如石脑油的方法。

45. 发明授权

US06447741B1 Thermally stable, high surface area, modified mesoporous aluminophosphate material 有权
标题翻译：热稳定，高表面积，改性介孔磷酸铝材料
公开(公告)号：US06447741B1
公开(公告)日：2002-09-10
申请号：US09468451
申请日：1999-12-21
申请人： Arthur W. Chester , Frederick E. Daugherty , Charles T. Kresge , Hye-Kyung C. Timken , James C. Vartuli
发明人： Arthur W. Chester , Frederick E. Daugherty , Charles T. Kresge , Hye-Kyung C. Timken , James C. Vartuli
IPC分类号： C01B2536
CPC分类号： B01J35/1061 , B01J27/16 , B01J27/1804 , B01J27/1853 , B01J27/187 , B01J29/084 , B01J35/0006 , B01J35/10 , B01J35/1019 , B01J35/108 , B01J37/03 , B01J2229/42 , C10G11/02 , C10G2400/02 , Y10S423/30
摘要： A mesoporous aluminophosphate material includes a solid aluminophosphate composition modified with at least one element selected from zirconium, cerium, lanthanum, manganese, cobalt, zinc, and vanadium. This mesoporous aluminophosphate material has a specific surface area of at least 100 m2/g, an average pore size less than or equal to 100 Å, and a pore size distribution such that at least 50% of the pores have a pore diameter less than 100 Å. The material can be used as a support for a catalytic cracking catalyst. Additionally, a method for making such a mesoporous aluminophosphate material is disclosed. The method, which preferably avoids use of organic reagents or solvents, includes providing an aqueous solution containing an inorganic phosphorus component; an inorganic aluminum containing component; and an inorganic modifying component containing at least one element selected from zirconium, cerium, lanthanum, manganese, cobalt, zinc, and vanadium. A solid mesoporous aluminophosphate material is formed in the solution by adjusting the pH of the solution to the range of 7 to 12 and is then recovered.
摘要翻译：介孔磷酸铝材料包括用至少一种选自锆，铈，镧，锰，钴，锌和钒的元素改性的固体磷酸铝组合物。该介孔磷酸铝材料的比表面积为至少100m 2 / g，平均孔径小于或等于100，孔径分布使孔至少50％的孔径小于100 一个。该材料可用作催化裂化催化剂的载体。另外，公开了制造这种中孔磷酸铝材料的方法。优选避免使用有机试剂或溶剂的方法包括提供含有无机磷组分的水溶液; 无机含铝组分; 和含有选自锆，铈，镧，锰，钴，锌和钒中的至少一种元素的无机改性成分。通过将溶液的pH调节至7至12的范围，在溶液中形成固体介孔磷酸铝材料，然后回收。

46. 发明授权

US6124232A Method for preparing an acidic solid oxide 失效
标题翻译：制备酸性固体氧化物的方法
公开(公告)号：US6124232A
公开(公告)日：2000-09-26
申请号：US357503
申请日：1998-07-20
申请人： Clarence D. Chang , Charles T. Kresge , Jose G. Santiesteban , James C. Vartuli
发明人： Clarence D. Chang , Charles T. Kresge , Jose G. Santiesteban , James C. Vartuli
IPC分类号： B01J21/06 , B01J23/00 , B01J23/30 , B01J23/888 , B01J37/03 , B01J37/06 , B01J37/10
CPC分类号： B01J21/06 , B01J21/066 , B01J23/002 , B01J23/30 , B01J23/888 , B01J37/03 , B01J37/06 , B01J37/10 , B01J2523/00
摘要： There is provided a method for preparing an acidic solid oxide having a reduced particle density, where the acidic solid oxide comprises a Group IVB metal oxide modified with an anion or oxyanion of a Group VIB metal. An example of this acidic solid oxide is zirconia modified with tungstate. The acidic solid oxide having a reduced particle density is prepared by coprecipitating the Group IVB metal oxide along with the anion or oxyanion of the Group VIB metal in the presence of a salt. This acidic solid oxide is particularly effective as a paraffin isomerization catalyst.
摘要翻译：提供了一种制备具有降低的颗粒密度的酸性固体氧化物的方法，其中酸性固体氧化物包括用VIB族金属的阴离子或氧阴离子改性的IVB族金属氧化物。这种酸性固体氧化物的实例是用钨酸盐改性的氧化锆。具有降低的颗粒密度的酸性固体氧化物通过在盐的存在下与第ⅥB族金属的阴离子或氧阴离子一起共沉淀而制备。该酸性固体氧化物作为石蜡异构化催化剂是特别有效的。

47. 发明授权

US5583276A Process for producing low aromatic diesel fuel with high cetane index 失效
标题翻译：具有高十六烷指数的低芳烃柴油的生产工艺
公开(公告)号：US5583276A
公开(公告)日：1996-12-10
申请号：US442549
申请日：1995-05-16
申请人： Stuart D. Hellring , Charles T. Kresge , David O. Marler , Ernest W. Valyocsik
发明人： Stuart D. Hellring , Charles T. Kresge , David O. Marler , Ernest W. Valyocsik
IPC分类号： B01J29/04 , B01J29/70 , C01B39/12 , C01B39/46 , C01B39/48 , C07C2/58
CPC分类号： C01B39/12 , B01J29/04 , C01B39/48 , C07C2/58 , C07C2529/70
摘要： A process for converting at least one olefin and at least one isoparaffin to a diesel fuel blending component comprising the steps of contacting the olefin and the isoparaffin with a catalyst comprising MCM-58 to provide a diesel fuel. Process conditions can be varied to favor the formation of gasoline, distillate, lube range products or mixtures thereof.
摘要翻译：一种将至少一种烯烃和至少一种异链烷烃转化为柴油燃料共混组分的方法，包括使烯烃和异链烷烃与包含MCM-58的催化剂接触以提供柴油燃料的步骤。工艺条件可以变化以有利于形成汽油，馏出物，润滑剂产品或其混合物。

48. 发明授权

US5510309A Method for preparing a modified solid oxide 失效
标题翻译：制备改性固体氧化物的方法
公开(公告)号：US5510309A
公开(公告)日：1996-04-23
申请号：US236073
申请日：1994-05-02
申请人： Clarence D. Chang , Charles T. Kresge , Jose G. Santiesteban , James C. Vartuli
发明人： Clarence D. Chang , Charles T. Kresge , Jose G. Santiesteban , James C. Vartuli
IPC分类号： B01J23/30 , B01J21/06 , B01J23/882 , B01J23/888 , B01J37/03 , B01J37/08 , C07B61/00 , C07C2/58 , C07C5/27 , C07C9/14 , C10G50/00
CPC分类号： B01J23/30 , B01J23/882 , B01J23/888 , C07C2/58 , C07C5/2772 , C10G50/00 , B01J37/03 , C07C2521/06 , C07C2523/30
摘要： There is provided a method for preparing an acidic solid comprising a Group IVB metal oxide modified with an oxyanion of a Group VIB metal. An example of this acidic solid is zirconia, modified with tungstate. This modified solid oxide may be used as a catalyst, for example, to isomerize C.sub.4 to C.sub.8 paraffins. The modified solid oxide is prepared by co-precipitating the Group IVB metal oxide along with the oxyanion of the Group VIB metal.
摘要翻译：提供了一种制备酸性固体的方法，该酸性固体包含用VIB族金属的氧阴离子改性的ⅣB族金属氧化物。这种酸性固体的一个例子是用钨酸盐改性的氧化锆。该改性的固体氧化物可以用作催化剂，例如使C4至C8链烷烃异构化。通过将IVB族金属氧化物与VIB族金属的氧阴离子共沉淀来制备改性的固体氧化物。

49. 发明授权

US5364999A Organic conversion with a catalyst comprising a crystalline pillared oxide material 失效
标题翻译：用包含结晶柱状氧化物材料的催化剂进行有机转化
公开(公告)号：US5364999A
公开(公告)日：1994-11-15
申请号：US28440
申请日：1993-03-09
申请人： Charles T. Kresge , Wieslaw J. Roth , Kenneth G. Simmons , James C. Vartuli
发明人： Charles T. Kresge , Wieslaw J. Roth , Kenneth G. Simmons , James C. Vartuli
IPC分类号： B01J20/18 , B01J29/04 , C01B33/44 , C01B39/02 , C07C1/24 , C07C2/12 , C07C2/00 , C07C4/00 , C07C5/00
CPC分类号： B01J29/049 , C01B39/026
摘要： There is provided a process for converting organic compounds using a catalyst comprising a pillared, layered crystalline oxide material. This material may be prepared by intercepting a swellable layered oxide before calcination. The intercepted material is swollen and pillared. If the material is not intercepted in this manner, it is transformed into a zeolite by calcination. The pillared material may have a large degree of catalytic activity, and it may have rather porous layers.
摘要翻译：提供了使用包含柱状层状结晶氧化物材料的催化剂转化有机化合物的方法。该材料可以通过在煅烧之前截取可溶胀的层状氧化物来制备。被拦截的材料肿胀和支柱。如果不以这种方式截留材料，则通过煅烧将其转变成沸石。柱状材料可能具有大的催化活性，并且它可能具有相当多孔的层。

50. 发明授权

US5304363A Porous materials 失效
标题翻译：多孔材料
公开(公告)号：US5304363A
公开(公告)日：1994-04-19
申请号：US907941
申请日：1992-07-02
申请人： Jeffrey S. Beck , Charles T. Kresge , Sharon B. McCullen , Wieslaw J. Roth , James C. Vartuli
发明人： Jeffrey S. Beck , Charles T. Kresge , Sharon B. McCullen , Wieslaw J. Roth , James C. Vartuli
IPC分类号： B01D53/86 , B01J20/02 , B01J29/03 , B01J29/04 , B01J29/40 , B01J29/70 , B01J29/82 , B01J29/83 , B01J29/85 , C01B37/00 , C01B37/02 , C01B37/08 , C01B39/00 , C10G11/05 , C10G47/16 , C01B33/26
CPC分类号： C10G47/16 , B01D53/8628 , B01J20/041 , B01J20/06 , B01J20/08 , B01J20/103 , B01J20/3078 , B01J29/0308 , B01J29/041 , B01J29/40 , B01J29/70 , B01J29/82 , B01J29/83 , B01J29/85 , C01B37/00 , C01B37/02 , C01B37/08 , C01B39/00 , C10G11/05 , B01J2229/26 , B01J2229/32 , B01J2229/34 , B01J2229/36 , B01J2229/40 , B01J2229/42
摘要： There is provided a porous material. A process for preparing this material involves adding an amphiphilic compound to the reaction mixture for preparing a crystalline oxide. The amphiphilic compound may be a quaternary ammonium cationic surfactant. These surfactants may be in the form of lamellar liquid crystals, and may function as templates for the formation of the present mesoporous oxide materials.
摘要翻译：提供多孔材料。制备该材料的方法包括向反应混合物中加入两亲性化合物以制备结晶氧化物。两亲性化合物可以是季铵阳离子表面活性剂。这些表面活性剂可以是层状液晶的形式，并且可以用作形成本中介氧化物材料的模板。

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