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21. 发明授权

US07220349B2 Process for the production of middle distillates by two-step hydroisomerisation and hydrocracking of feeds from the Fischer-Tropsch process 有权
标题翻译：通过费 - 托方法的进料的两步加氢异构化和加氢裂化生产中间馏分的方法
公开(公告)号：US07220349B2
公开(公告)日：2007-05-22
申请号：US10189759
申请日：2002-07-08
申请人： Eric Benazzi , Christophe Gueret
发明人： Eric Benazzi , Christophe Gueret
IPC分类号： C10G65/12
CPC分类号： C10G65/12 , C10G2300/1022 , C10G2300/301 , C10G2300/4081 , C10G2400/06 , C10G2400/08
摘要： The invention concerns a process for producing middle distillates from an effluent produced by a Fischer-Tropsch unit, comprising optional fractionation to obtain at least one heavy fraction with an initial boiling point in the range 120-200° C., said heavy fraction or said effluent optionally being hydrotreated, then bringing it into contact with a first amorphous hydrocracking/hydroisomerization catalyst that contains at least one noble group VIII metal, the effluent obtained is distilled, then the residual fraction boiling above the middle distillates and/or a portion of the middle distillates is brought into contact with a second amorphous hydrocracking/hydroisomerization catalyst containing at least one noble group VIII metal. The invention also concerns a unit.
摘要翻译：本发明涉及从由费 - 托单元产生的流出物中生产中间馏分的方法，该方法包括任选的分馏以获得至少一种初馏点在120-200℃范围内的重馏分，所述重馏分或所述流出物任选地进行加氢处理，然后使其与含有至少一种贵金属VIII族金属的第一无定形加氢裂化/加氢异构化催化剂接触，将所得流出物蒸馏，然后在中间馏分沸腾的残余馏分和/或部分使中间馏分与含有至少一种贵金属VIII族金属的第二无定形加氢裂化/加氢异构化催化剂接触。本发明还涉及一个单元。

22. 发明授权

US07156978B2 Process for the production of middle distillates by hydroisomerisation and hydrocracking of two fractions from feeds originating from the fischer-tropsch process 有权
$Process for the production of middle distillates by hydroisomerisation and hydrocracking of two fractions from feeds originating from the fischer-tropsch process$
标题翻译：通过加氢异构化和加氢裂化来自费 - 托方法的原料的两种馏分生产中间馏分的方法
公开(公告)号：US07156978B2
公开(公告)日：2007-01-02
申请号：US10189793
申请日：2002-07-08
申请人： Eric Benazzi , Christophe Gueret
发明人： Eric Benazzi , Christophe Gueret
IPC分类号： C10G49/02 , C10G47/02 , C10G69/14
CPC分类号： C10G65/00 , C10G45/62 , C10G47/14 , C10G65/14 , C10G69/14 , C10G2300/1022 , C10G2300/301 , C10G2300/4018 , C10G2300/4081 , C10G2400/04 , C10G2400/06 , C10G2400/08 , Y10S208/95
摘要： A system comprising: a paraffin feed produced by the Fischer-Tropsch process is fractionable into at least three fractions: an intermediate fraction boiling between T1 and T2, T1 being in the range 120–200° C. and T2 being more than 300° C. and less than 410° C., a light fraction boiling below it and a heavy fraction boiling above it; at least a portion of the intermediate fraction is hydrotreated then at least a portion thereof is passed over an amorphous hydroisomerisation/hydrocracking catalyst; the heavy fraction is passed over an amorphous hydroisomerisation/hydrocracking catalyst with a conversion of 370° C.+ products into 370° C.− products of more than 80% by weight; the hydrocracked/hydroisomerised fractions are distilled to obtain middle distillates (kerosine, gas oil).
摘要翻译：一种系统，包括：通过费 - 托法生产的链烷烃进料可分馏成至少三个馏分：在T 1和T 2之间沸腾的中间馏分，T 1在120-200℃范围内，T 2更多低于300℃，低于410℃，在其下方沸腾的轻馏分和在其上沸腾的重馏分; 将至少一部分中间馏分进行加氢处理，然后将其至少一部分通过无定形加氢异构化/加氢裂化催化剂; 将重馏分通过无定形加氢异构化/加氢裂化催化剂，转化率为370℃+产物至370℃，产率大于80％; 将加氢裂化/加氢异构化馏分蒸馏得到中间馏分（煤油，瓦斯油）。

23. 发明授权

US07404890B2 Process for the production of middle distillates by hydroisomerisation and hydrocracking feeds from the Fischer-Tropsch process 有权
标题翻译：通过费 - 托工艺的加氢异构化和加氢裂化原料生产中间馏分的方法
公开(公告)号：US07404890B2
公开(公告)日：2008-07-29
申请号：US10189738
申请日：2002-07-08
申请人： Eric Benazzi , Christophe Gueret
发明人： Eric Benazzi , Christophe Gueret
IPC分类号： C10G47/00 , C10G45/58
CPC分类号： C10G65/12 , C10G45/62 , C10G47/14 , C10G2300/1022 , C10G2300/301 , C10G2300/4081 , C10G2400/06 , C10G2400/08
摘要： The invention concerns a process and apparatus wherein the paraffin effluent from the Fischer-Tropsch process is separated into a heavy fraction with an initial boiling point of 120-200° C., said heavy fraction then optionally being hydrotreated then brought into contact with an amorphous hydroisomerization/hydrocracking catalyst that converts at least 80% by weight of the 370° C.+ products into products with a boiling point of less than 370° C. After distilling the hydrocracked fraction obtained to separate middle distillates, the residual heavy fraction is recycled.
摘要翻译：本发明涉及一种方法和设备，其中将来自费 - 托法的石蜡流出物分离成初馏点为120-200℃的重馏分，然后任选加氢处理然后使其与非晶态物质接触加氢异构化/加氢裂化催化剂，其将370℃+产物的至少80重量％转化成沸点小于370℃的产物。蒸馏得到的加氢裂化馏分分离中间馏分后，将残余重馏分循环。

24. 发明授权

US06583330B1 Catalysts containing heteropolyanions usable in processes for conversion of paraffins 失效
标题翻译：含有可用于石蜡转化方法的杂多阴离子的催化剂
公开(公告)号：US06583330B1
公开(公告)日：2003-06-24
申请号：US09604055
申请日：2000-06-26
申请人： Christine Travers , Maryline Delage , Eric Benazzi , Jean-François Joly
发明人： Christine Travers , Maryline Delage , Eric Benazzi , Jean-François Joly
IPC分类号： C07C258
CPC分类号： B01J21/066 , B01J27/188 , C07C2/58 , C07C5/2791 , C07C2521/06 , C07C2523/44 , C07C2523/46 , C07C2523/755 , C07C2523/88 , C07C2523/888 , C07C2527/18 , C07C9/00
摘要： New catalysts that contain heteropolyanions of the 12-tungstophosphoric acid or the 12-tungstomolybdic acid, and, for some of these, at least one metal of group VIII, and that are deposited on substrates that develop a specific surface area and a high pore volume, such as zirconium oxide (ZrO2), silicas, silica-aluminas or aluminas, are used in particular in isomerization of paraffinic fractions that contain in large part n-paraffins that have, for example, 4 to 8 carbon atoms per molecule and in aliphatic alkylation of isoparaffins (for example isobutane and/or isopentane) by at least one olefin that comprises, for example, 2 to 6 carbon atoms per molecule (C2 to C6).
摘要翻译：含有12-钨磷酸或12-钨钼酸杂多糖的新型催化剂，以及其中一些这些至少一种第VIII族金属，并且沉积在形成比表面积和高孔体积的基材上，例如氧化锆（ZrO 2），二氧化硅，二氧化硅 - 氧化铝或氧化铝，特别是用于大部分含有例如每分子4至8个碳原子的正链烷烃和脂族的链烷烃级分的异构化通过至少一种包含例如每分子2至6个碳原子（C 2至C 6）的烯烃烷基化异链烷烃（例如异丁烷和/或异戊烷）。

25. 发明授权

US06558647B2 Microporous and mesoporous silicoaluminate solid, process for preparation, use as a catalyst and for hydrocarbon conversion 有权
标题翻译：微孔和介孔硅铝酸盐固体，制备方法，用作催化剂和烃转化
公开(公告)号：US06558647B2
公开(公告)日：2003-05-06
申请号：US09736048
申请日：2000-12-14
申请人： Sylvie Lacombe , David Marseault , Philippe Caullet , Henri Kessler , Eric Benazzi , Alexandre Jouve
发明人： Sylvie Lacombe , David Marseault , Philippe Caullet , Henri Kessler , Eric Benazzi , Alexandre Jouve
IPC分类号： C01B3904
CPC分类号： B01J29/005 , B01J29/0308 , B01J29/041 , B01J29/7007 , B01J29/7415 , B01J2229/42 , C01B39/023 , C10G47/20 , Y10S423/27
摘要： The invention relates to an acidic silicoaluminate solid that has a microporous zeolitic phase that is characterized by at least one infrared band between 400-1600 cm−1, an organized mesoporosity that is characterized by the presence of at least one X-diffraction line between 20-100 Å, a silica/alumina molar ratio of between 5-250 and an acidity that is measured by infrared analysis via an area of the band at about 1545 cm−1 at least equal to 50 g of dry solid. The invention also relates to a process for the preparation of the solid, a substrate that consists of solid and at least one matrix, and a catalyst that comprises said solid. The catalyst can be used for the conversion of hydrocarbons and in particular hydrocracking.
摘要翻译：本发明涉及一种酸性硅铝酸盐固体，其具有微孔沸石相，其特征在于至少一个在400-1600cm -1之间的红外波段，有组织的介孔密度，其特征在于存在至少一个X射线在20 -100埃，二氧化硅/氧化铝摩尔比在5-250之间，并且通过红外分析通过在约1545cm -1至少等于50g干固体的带的面积测量的酸度。本发明还涉及制备固体的方法，由固体和至少一种基质组成的底物和包含所述固体的催化剂。催化剂可用于转化烃，特别是加氢裂化。

26. 发明授权

US06524470B1 Catalyst comprising beta zeolite and promoter element for hydrocracking 失效
标题翻译：包含β沸石和加氢裂化促进剂元素的催化剂
公开(公告)号：US06524470B1
公开(公告)日：2003-02-25
申请号：US09305290
申请日：1999-05-05
申请人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
发明人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
IPC分类号： B01J2976
CPC分类号： C10G47/20 , B01J29/7615 , B01J29/7815 , B01J2229/16 , B01J2229/26 , B01J2229/42 , C10G47/16
摘要： A catalyst comprising, in weight % with respect to the total catalyst weight 0.1% to 60% (expressed as the % by weight of oxide) of at least one hydro-dehydrogenating metal selected from the group formed by group VIB and VIII metals; 0.1% to 99% of at least one amorphous or low crystallinity porous matrix; 0.1% to 99.7% of beta zeolite; 0.1% to 20% (expressed as the % by weight of oxide) of at least one promoter element selected from the group formed by boron, silicon and phosphorous; 0 to 20% of at least one halogen; 0 to 20% (expressed as the % by weight of oxide) of at least one group VIIB element, the catalyst being especially useful for cracking hydrocarbon feeds.
摘要翻译：一种催化剂，其以相对于总催化剂重量％计含有选自由VIB族和VIII族金属形成的基团的至少一种加氢脱氢金属的0.1％至60％（以氧化物重量计） 0.1％至99％的至少一种无定形或低结晶度多孔基体; 0.1％至99.7％的β沸石; 至少一种选自硼，硅和磷形成的助催化剂元素的0.1％至20％（表示为氧化物的重量％）; 0至20％的至少一种卤素; 0至20％（表示为氧化物的重量％）的至少一种VIIB族元素，该催化剂特别适用于裂化烃进料。

27. 发明授权

US06491809B1 Synthetic oil with a high viscosity number and a low pour point 有权
标题翻译：具有高粘度数和低倾点的合成油
公开(公告)号：US06491809B1
公开(公告)日：2002-12-10
申请号：US09671294
申请日：2000-09-27
申请人： Patrick Briot , Alain Forestiere , Serge Gautier , Eric Benazzi , Leon Lew
发明人： Patrick Briot , Alain Forestiere , Serge Gautier , Eric Benazzi , Leon Lew
IPC分类号： C10M10506
CPC分类号： C10M105/02 , C10M105/06
摘要： Synthetic oil that contains wholly or partly of dialkylbenzenes and/or partially or totally hydrogenated dialkylbenzenes. The synthetic oil according to the invention can also be used as an oil base or oil base additive and comprises at least one dialkylbenzene and/or at least one partially or totally hydrogenated dialkylbenzene and meets the general chemical formula: R1—A—R2 in which R1 and R2 represent alkyl groups and A is a benzene core and/or a cyclohexane core and/or a cyclohexene core and/or a cyclohexadiene core and is characterized in that it contains between 1 and 20% by weight or ortho isomers and in that at least one of the alkyl groups is attached for the most part to group A by carbon 2 of the aliphatic chain. The two alkyl groups are preferably attached for the most part to group A by carbon 2 of the aliphatic chain.
摘要翻译：含有全部或部分二烷基苯和/或部分或完全氢化的二烷基苯的合成油。根据本发明的合成油还可以用作油基或油基添加剂，并且包含至少一种二烷基苯和/或至少一种部分或全部氢化的二烷基苯，并且满足以下通式：其中R 1和R 2表示烷基基团和A是苯核心和/或环己烷核心和/或环己烯核心和/或环己二烯核心，其特征在于其含有1至20重量％或邻位异构体，并且其中至少一个烷基通过脂族链的碳2大部分连接到基团A上。两个烷基优选通过脂族链的碳2连接到大部分为基团A。

28. 发明授权

US06402936B1 Catalyst that comprises a partially amorphous Y zeolite, an element of group VB and its use in hydroconversion and hydrorefining of hydrocarbon petroleum feedstocks 有权
标题翻译：包含部分无定形Y沸石，VB族元素及其在烃类石油原料加氢转化和加氢精制中的应用的催化剂
公开(公告)号：US06402936B1
公开(公告)日：2002-06-11
申请号：US09572971
申请日：2000-05-18
申请人： Eric Benazzi , Jean-Marie Deves , Slavik Kasztelan
发明人： Eric Benazzi , Jean-Marie Deves , Slavik Kasztelan
IPC分类号： C01G1718
CPC分类号： C10G47/16 , B01J29/166 , C10G45/12
摘要： The invention relates to a catalyst that contains at least one partially amorphous Y zeolite, at least one metal of group VB, preferably niobium, at least one amorphous or poorly crystallized matrix, optionally at least one metal that is selected from group VIB and group VIII, optionally at least one element that is selected from the group that is formed by P, B, and Si, and optionally at least one element of group VIIA. The invention also relates to the use of this catalyst in hydrocracking and hydrorefining of hydrocarbon feedstocks.
摘要翻译：本发明涉及含有至少一种部分无定形Y沸石，至少一种VB族金属，优选铌，至少一种无定形或不完全结晶的基质，任选至少一种选自VIB族和VIII族的金属的催化剂，可选地至少一种选自由P，B和Si形成的基团以及任选的至少一种VIIA族元素的元素。本发明还涉及该催化剂在烃原料的加氢裂化和加氢精制中的用途。

29. 发明授权

US06306286B1 IM-5 phosphorus zeolite, catalytic composition, its preparation and its use in catalytic cracking 有权
标题翻译： IM-5磷沸石，催化剂组成，其制备及其在催化裂化中的应用
公开(公告)号：US06306286B1
公开(公告)日：2001-10-23
申请号：US09569303
申请日：2000-05-11
申请人： Samuel Mignard , Avelino Corma Canos , Joaquin Martinez Triguero , Eric Benazzi , Sylvie Lacombe , Gil Mabilon
发明人： Samuel Mignard , Avelino Corma Canos , Joaquin Martinez Triguero , Eric Benazzi , Sylvie Lacombe , Gil Mabilon
IPC分类号： C01G1105
CPC分类号： C10G11/05 , B01J29/005 , B01J29/084 , B01J29/70 , B01J29/85 , B01J2229/183 , B01J2229/26 , B01J2229/30 , B01J2229/36 , B01J2229/42 , C01B39/026 , C10G2400/20
摘要： An IM-5 zeolite that is modified by adding phosphorus that is optionally dealuminified, preferably in aluminosilicic form, and that contains at most 10% by weight of phosphorus, a composition that contains it, its processes for preparation and its application to catalytic cracking of hydrocarbon feedstocks are described.
摘要翻译：通过添加任选脱磷的铝，优选以铝硅酸盐形式，并且含有至多10重量％的磷的磷，含有它的组合物，其制备方法及其在催化裂化中的应用而改性的IM-5沸石描述了烃原料。

30. 发明授权

US06171474B2 Zeolite Y catalyst containing silicon useful for hydrocracking 有权
标题翻译：含有可用于加氢裂化的硅的沸石Y催化剂
公开(公告)号：US06171474B2
公开(公告)日：2001-01-09
申请号：US09305288
申请日：1999-05-05
申请人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
发明人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
IPC分类号： C01G4700
CPC分类号： B01J29/08 , B01J2229/16 , B01J2229/22 , C10G47/20
摘要： Useful for example, for the hydrocracking of hydrocarbons is a catalyst comprising a matrix, at least one Y zeolite which is dealuminated and has a lattice parameter in the range 2.424 nm to 2.455 nm, a global SiO2/Al2O3 mole ratio is more than 8, the quantity of alkaline-earth metal cations or alkali metal cations and/or rare earth metal cations is such that the atomic ratio (n×Mn+)/Al is less than 0.8, the specific surface area, determined using the BET method, is more than 400 m2/g, and the water adsorption capacity is more than 6% by weight for P/P0 =0.2 at 25° C., said catalyst also comprising silicon deposited on the catalyst.
摘要翻译：对于例如烃的加氢裂解是有用的催化剂，它是一种催化剂，它包括一个基体，至少一个Y脱铝的Y沸石，其晶格参数在2.424 nm到2.455 nm之间，全球的SiO2 / Al2O3摩尔比大于8，碱土金属阳离子或碱金属阳离子和/或稀土金属阳离子的数量使得原子比（nxMn +）/ Al小于0.8，使用BET法测定的比表面积大于400 m2 / g，在25℃时P / P0 = 0.2，水吸附量大于6重量％，所述催化剂还含有沉积在催化剂上的硅。

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