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21. 发明授权

US06746793B1 Polymer electrolyte fuel cell 失效
标题翻译：聚合物电解质燃料电池
公开(公告)号：US06746793B1
公开(公告)日：2004-06-08
申请号：US09719664
申请日：2000-12-15
申请人： Hisaaki Gyoten , Eiichi Yasumoto , Kazuhito Hatoh , Makoto Uchida , Yasushi Sugawara , Teruhisa Kanbara , Junji Morita , Hideo Ohara , Kazufumi Nishida , Osamu Sakai , Yukiyoshi Ono , Yasuo Takebe
发明人： Hisaaki Gyoten , Eiichi Yasumoto , Kazuhito Hatoh , Makoto Uchida , Yasushi Sugawara , Teruhisa Kanbara , Junji Morita , Hideo Ohara , Kazufumi Nishida , Osamu Sakai , Yukiyoshi Ono , Yasuo Takebe
IPC分类号： H01M802
CPC分类号： H01M4/8642 , H01M4/8605 , H01M4/926 , H01M8/1004 , H01M2300/0082
摘要： The polymer electrolyte fuel cell of the present invention exhibits an excellent performance with an efficient electrode reaction; by providing a layer comprising an electroconductive fine particle between the catalytic reaction layer and the gas diffusion layer in the electrodes; by providing a hydrogen ion diffusion layer on at least either surface of the catalyst particle or the carrier, which carries the catalyst particle in the catalytic reaction layer; or by constituting the catalytic reaction layer with at least a catalyst comprising a hydrophilic carbon material with catalyst particles carried thereon and a water repellent carbon material.
摘要翻译：本发明的高分子电解质型燃料电池具有优异的电极反应性能，通过在催化反应层和电极中的气体扩散层之间提供包含导电细颗粒的层; 通过在催化剂颗粒或载体的至少任一个表面上提供氢离子扩散层，其在催化反应层中承载催化剂颗粒; 或者通过使至少包含亲水性碳材料的催化剂与承载有催化剂颗粒的催化反应层和防水性碳材料构成。

22. 发明授权

US06372373B1 Solid polymer electrolyte fuel cell and method for producing the same 失效
标题翻译：固体聚合物电解质燃料电池及其制造方法
公开(公告)号：US06372373B1
公开(公告)日：2002-04-16
申请号：US09292594
申请日：1999-04-16
申请人： Hisaaki Gyoten , Kazuhito Hatoh , Kazufumi Nishida , Hideo Ohara , Eiichi Yasumoto , Teruhisa Kanbara , Makoto Uchida , Yasushi Sugawara , Toshihiro Matsumoto , Kouji Nakagawa
发明人： Hisaaki Gyoten , Kazuhito Hatoh , Kazufumi Nishida , Hideo Ohara , Eiichi Yasumoto , Teruhisa Kanbara , Makoto Uchida , Yasushi Sugawara , Toshihiro Matsumoto , Kouji Nakagawa
IPC分类号： H01M208
CPC分类号： H01M8/2485 , H01M8/0206 , H01M8/0254 , H01M8/0258 , H01M8/0263 , H01M8/0267 , H01M8/0271 , H01M8/0276 , H01M8/028 , H01M8/0297 , H01M8/241 , H01M8/2415 , H01M2300/0082
摘要： A compact solid polymer electrolyte fuel cell having a simplified structure of a high mechanical strength and an improved gas-sealing property is disclosed. In the solid polymer electrolyte fuel cell of the present invention, gas-tight electrically insulating layers are provided on the flanks or the insides of the module of the above-mentioned laminated unit cells, thereby to give a gas-tightness between said electrode and separator.
摘要翻译：公开了一种具有机械强度高，气密性好的简化结构的紧凑型固体聚合物电解质燃料电池。在本发明的固体高分子电解质型燃料电池中，在上述层叠单元电池的组件的侧面或内侧设置气密性电绝缘层，从而在所述电极和分离器之间形成气密性。

23. 发明授权

US5866423A Measuring method of the specific surface area available for reaction of noble metal catalyst in the electrode of polymer electrolyte membrane fuel cell 失效
标题翻译：贵金属催化剂在聚合物电解质膜燃料电池电极中可用于反应的比表面积的测量方法
公开(公告)号：US5866423A
公开(公告)日：1999-02-02
申请号：US783577
申请日：1997-01-15
申请人： Yasushi Sugawara , Makoto Uchida , Yuko Fukuoka , Nobuo Eda
发明人： Yasushi Sugawara , Makoto Uchida , Yuko Fukuoka , Nobuo Eda
IPC分类号： G01N15/08 , B01J23/38 , B01J23/42 , H01M4/90 , H01M4/92 , H01M8/10
CPC分类号： H01M4/926 , H01M4/92 , H01M8/1004 , H01M2300/0082
摘要： A measuring method for determining the specific surface area available for reaction of a noble metal catalyst of an electrode for use in a polymer electrolyte membrane fuel cell. The method includes measuring the total specific surface area of the noble metal catalyst and the specific surface area of the noble metal catalyst mixed with a polymer electrolyte by detecting the adsorption amounts of carbon monoxide upon exposure to carbon monoxide after reduction in hydrogen, and subtracting the latter from the former. Also provided is an electrode material for use in a polymer electrolyte membrane fuel cell having excellent polarization characteristics by controlling the utilization of a noble metal catalyst determined from the total specific surface area and specific surface area available for reaction of the noble metal catalyst. The electrode material includes a noble metal catalyst powder and a polymer electrolyte, wherein the utilization ratio of the noble metal catalyst is at least 40% of the saturation value of the utilization of the noble metal catalyst powder.
摘要翻译：一种用于确定用于聚合物电解质膜燃料电池的电极的贵金属催化剂可用于反应的比表面积的测量方法。该方法包括通过检测在氢还原后暴露于一氧化碳时一氧化碳的吸附量，测量贵金属催化剂的总比表面积和与聚合物电解质混合的贵金属催化剂的比表面积，并减去后者来自前者。还提供了一种用于聚合物电解质膜燃料电池的电极材料，其通过控制由可用于贵金属催化剂的反应的总比表面积和比表面积确定的贵金属催化剂的利用而具有优异的极化特性。电极材料包括贵金属催化剂粉末和聚合物电解质，其中贵金属催化剂的利用率为贵金属催化剂粉末的利用饱和值的至少40％。

24. 发明申请

US20100136456A1 POLYMER ELECTROLYTE FUEL CELL AND FUEL CELL SEALING MEMBER FOR THE SAME 有权
标题翻译：聚合物电解质燃料电池和燃料电池密封组件
公开(公告)号：US20100136456A1
公开(公告)日：2010-06-03
申请号：US11917965
申请日：2006-07-10
申请人： Yasushi Sugawara , Takayuki Urata , Junji Morita , Soichi Shibata , Takahiro Umeda
发明人： Yasushi Sugawara , Takayuki Urata , Junji Morita , Soichi Shibata , Takahiro Umeda
IPC分类号： H01M8/10 , H01M2/08
CPC分类号： H01M8/0271 , H01M8/0258 , H01M8/026 , H01M8/0267 , H01M8/0276 , H01M8/1004 , H01M8/242
摘要： To provide a polymer electrolyte fuel cell in which a reaction gas can be utilized efficiently for an electrode reaction even when a gap is formed between an anode-side sealing member and the end face of an anode and between a cathode-side sealing member and the end face of a cathode, and sufficient power generation performance can be ensured with a simple constitution. At least one of the anode-side sealing member and the cathode-side sealing member of the fuel cell includes an annular body, and at least one deformable protruding portion provided on the inner surface of the annular body.
摘要翻译：为了提供一种聚合物电解质燃料电池，其中即使在阳极侧密封构件和阳极的端面之间以及阴极侧密封构件和阴极侧密封构件之间形成间隙的情况下，也可以有效地利用反应气体进行电极反应阴极的端面，能够以简单的结构确保足够的发电性能。燃料电池的阳极侧密封构件和阴极侧密封构件中的至少一个包括环形体，以及设置在环状体的内表面上的至少一个可变形突出部。

25. 发明申请

US20100028731A1 OPERATION METHOD OF FUEL CELL SYSTEM AND FUEL CELL SYSTEM 审中-公开
标题翻译：燃料电池系统和燃料电池系统的运行方法
公开(公告)号：US20100028731A1
公开(公告)日：2010-02-04
申请号：US12527348
申请日：2008-03-18
申请人： Yasushi Sugawara , Takayuki Urata , Takahiro Umeda , Soichi Shibata , Junji Morita
发明人： Yasushi Sugawara , Takayuki Urata , Takahiro Umeda , Soichi Shibata , Junji Morita
IPC分类号： H01M8/04
CPC分类号： H01M8/04302 , H01M8/0263 , H01M8/04126 , H01M8/04223 , H01M8/04225 , H01M8/2483 , H01M2008/1095
摘要： An operation method of a fuel cell system of the present invention has a water layer forming step in which before starting supply of at least one of the reducing agent and the oxidizing agent in a supply start operation of at least one of the reducing agent and the oxidizing agent, the water supplier supplies water to form a water layer so as to clog at least one of at least a portion of the reducing agent supply path which is located upstream of the reducing agent supply end in a flow direction of the reducing agent and at least a portion of the oxidizing agent supply path which is located upstream of the oxidizing agent supply end in a flow direction of the oxidizing agent.
摘要翻译：本发明的燃料电池系统的运转方法具有水层形成工序，其中在所述还原剂和所述氧化剂中的至少一种的还原剂和所述氧化剂的供给开始动作中开始供给之前，氧化剂，供水者供水以形成水层，以便阻止位于还原剂供应端的上游的至少一部分还原剂供应路径中的至少一部分在还原剂的流动方向上，以及所述氧化剂供给路径的至少一部分位于所述氧化剂供给端的上游侧的氧化剂的流动方向。

26. 发明申请

US20090047555A1 FUEL CELL SYSTEM 有权
标题翻译：燃油电池系统
公开(公告)号：US20090047555A1
公开(公告)日：2009-02-19
申请号：US12095829
申请日：2006-11-28
申请人： Yasushi Sugawara , Takayuki Urata , Takahiro Umeda , Akihiko Yoshida , Soichi Shibata , Junji Morita
发明人： Yasushi Sugawara , Takayuki Urata , Takahiro Umeda , Akihiko Yoshida , Soichi Shibata , Junji Morita
IPC分类号： H01M8/04 , H01M8/10
CPC分类号： H01M8/04223 , H01M4/8875 , H01M8/026 , H01M8/0267 , H01M8/0271 , H01M8/04029 , H01M8/04089 , H01M8/04328 , H01M8/04335 , H01M8/04388 , H01M8/04395 , H01M8/04559 , H01M8/04753 , H01M8/0668 , H01M8/2405 , H01M8/241 , H01M8/2457 , H01M8/2483 , H01M2008/1095
摘要： In a fuel cell system, during the state where the fuel cell system is not generating an electric power, a fuel gas passage and an oxidizing gas passage are closed, and an inert gas supply device (54, 58) supplies an inert gas to an anode space (111) which is substantially isolated from outside, the anode space including the closed fuel gas passage and a space connected to the closed fuel gas passage, while an air supply device (67, 70) supplies air to a cathode space (112) which is substantially isolated from outside, the cathode space including the closed oxidizing gas passage and a space connected to the closed oxidizing gas passage. With this, the fuel cell system is capable of achieving high energy efficiency and of surely preventing degradation of electrodes during the state where the fuel cell system is not generating the electric power, irrespective of repeated start-up and stop.
摘要翻译：在燃料电池系统中，在燃料电池系统不产生电力的状态下，关闭燃料气体通路和氧化气体通路，惰性气体供给装置（54,58）向惰性气体供给装置阳极空间（111），其与外部基本上隔离，所述阳极空间包括封闭的燃料气体通道和连接到封闭的燃料气体通道的空间，而空气供应装置（67,70）将空气供应到阴极空间），其包括封闭的氧化气体通道的阴极空间和与封闭的氧化气体通道连接的空间。由此，无论重复启动停止，燃料电池系统能够实现高能量效率，并且可靠地防止燃料电池系统不产生电力的状态下的电极劣化。

27. 发明申请

US20070099040A1 Fuel cell system, method of starting fuel cell system 有权
标题翻译：燃料电池系统，燃料电池系统启动方法
公开(公告)号：US20070099040A1
公开(公告)日：2007-05-03
申请号：US10561386
申请日：2004-08-24
申请人： Junji Morita , Makoto Uchida , Yasushi Sugawara , Takayuki Urata , Shinya Kosako , Takahiro Umeda , Soichi Shibata , Yoichiro Tsuji , Masataka Ozeki , Akinari Nakamura , Yoshikazu Tanaka
发明人： Junji Morita , Makoto Uchida , Yasushi Sugawara , Takayuki Urata , Shinya Kosako , Takahiro Umeda , Soichi Shibata , Yoichiro Tsuji , Masataka Ozeki , Akinari Nakamura , Yoshikazu Tanaka
IPC分类号： H01M8/04
CPC分类号： H01M8/0606 , H01M8/04231 , H01M8/04365 , H01M8/04388 , H01M8/04395 , H01M8/04425 , H01M8/04559 , H01M8/04649 , H01M8/04746 , H01M8/04776 , H01M8/04955 , H01M2008/1095
摘要： Problems of acceleration of drying of electrolyte membrane and local reaction, etc. can be properly coped with to attain the stabilization of performance of fuel cell. There are provided a fuel cell 121 which generates electric power from a fuel gas and an oxidizing agent gas, a fuel gas feed pipe 161 and a first switch valve 129 as fuel gas supplying unit which supplies the said fuel gas into the said fuel cell on the anode side thereof, an oxidizing gas supplying pipe 162 and a second cut-off valve 131 as oxidizing agent gas supplying unit which supplies the said oxidizing agent into the said fuel cell on the cathode side thereof, a raw material gas supplying pipe 151 and a third switch valve 143 as raw material gas supplying unit which supplies raw material of the said fuel gas into the fuel cell and a control portion 127 which controls the supply of the said fuel gas, the supply of the said oxidizing agent and the supply of the said raw material and the control portion 127 controls during the starting of electricity generation of the fuel cell 121 such that the said raw material gas supplying unit purges the fuel cell 121 at least on the cathode side thereof with the said raw material gas before the oxidizing agent gas supplying unit and the fuel gas supplying unit supply the fuel gas and the said oxidizing agent gas into the fuel cell 121, respectively.
摘要翻译：可以适当应对电解质膜干燥加速和局部反应等问题，以达到燃料电池性能的稳定。设置有从燃料气体和氧化剂气体产生电力的燃料电池121，作为燃料气体供给单元的燃料气体供给管161和第一切换阀129，将燃料气体供给到所述燃料电池中其阳极侧，氧化剂气体供给管162和作为氧化剂气体供给单元的第二截止阀131，其将所述氧化剂供给到阴极侧的所述燃料电池中，原料气体供给管151和作为将燃料气体的原料供给燃料电池的原料气体供给部的第三切换阀143以及控制部127，控制部127控制所述燃料气体的供给，所述氧化剂的供给和供给所述原料和控制部127在燃料电池121的发电开始期间进行控制，使得所述原料气体供给单元至少在阴极上清除燃料电池121 在氧化剂气体供给单元和燃料气体供给单元之间分别将燃料气体和所述氧化剂气体供应到燃料电池121中的同时与所述原料气体一起。

28. 发明申请

US20070003805A1 Fuel cell system and method for stopping operation of fuel cell system 失效
标题翻译：燃料电池系统及燃料电池系统停机运行方法
公开(公告)号：US20070003805A1
公开(公告)日：2007-01-04
申请号：US10556466
申请日：2004-08-24
申请人： Yasushi Sugawara , Junji Morita , Makoto Uchida , Takayuki Urata , Shinya Kosako , Takahiro Umeda , Soichi Shibata , Masataka Ozeki , Akinari Nakamura , Yoshikazu Tanaka , Yoichiro Tsuji
发明人： Yasushi Sugawara , Junji Morita , Makoto Uchida , Takayuki Urata , Shinya Kosako , Takahiro Umeda , Soichi Shibata , Masataka Ozeki , Akinari Nakamura , Yoshikazu Tanaka , Yoichiro Tsuji
IPC分类号： H01M8/04
CPC分类号： H01M8/04231 , H01M8/04089 , H01M8/04201 , H01M8/04365 , H01M8/04388 , H01M8/04395 , H01M8/04559 , H01M8/04619 , H01M8/04753 , H01M8/04955 , H01M8/0606 , H01M8/0662 , H01M2008/1095
摘要： The deterioration of the catalyst can occur during prolonged storage, occasionally causing the deterioration of the durability of the fuel cell. There are provided a stack 38 which generates electric power from a fuel gas and an oxidizing agent, a fuel gas pipe 37 and an on-off valve 49 as fuel gas supplying unit of supplying the fuel gas into the fuel cell on the anode side thereof, an oxidizing agent supplying unit an oxidizing agent gas pipe 40a and an on-off valve 57 as oxidizing agent gas supplying unit of supplying the oxidizing agent into the fuel cell on the cathode side thereof, a raw material gas pipe 33, a bypass pipe 55 and dispensing valves 56, 60 as raw material gas supplying unit of supplying the raw material of the fuel gas into the fuel cell and a control portion 44 of controlling the supply of the fuel gas, the supply of the oxidizing agent and the supply of the raw material, wherein after the switching-off of the output of electric power of the fuel cell, the fuel gas supplying unit suspends the supply of the fuel gas into the fuel cell on the anode side thereof, the oxidizing agent gas supplying unit suspends the supply of the oxidizing agent into the fuel cell on the cathode side thereof and the raw material gas supplying unit supplies the raw material into the fuel cell from the inlet side of the cathode to purge the fuel cell on the cathode side thereof.
摘要翻译：催化剂的劣化可以在长时间储存期间发生，有时会导致燃料电池的耐久性恶化。设置有从燃料气体和氧化剂产生电力的堆叠件38，作为将燃料气体供给到其阳极侧的燃料电池的燃料气体供给单元的燃料气体管37和开关阀49 氧化剂供给部，氧化剂气体配管40a和开闭阀57，作为将氧化剂供给到阴极侧的燃料电池的氧化剂气体供给部，原料气体管33，旁路作为将燃料气体的原料供给到燃料电池的原料气体供给部的管55和分配阀56,60以及控制燃料气体的供给，氧化剂的供给和供给的控制部44 所述燃料气体供给部在所述燃料电池的电力输出切断后，将所述燃料气体的供给暂停在所述燃料电池的阳极侧，所述氧化剂气体供给部怀疑将氧化剂供给到阴极侧的燃料电池中，原料气体供给单元从阴极的入口侧将原料供给燃料电池，以在其阴极侧吹扫燃料电池。

29. 发明授权

US07150934B2 Electrolyte film electrode union, fuel cell containing the same and process for producing them 失效
标题翻译：电解质膜电极联合体，含有它们的燃料电池及其制造方法
公开(公告)号：US07150934B2
公开(公告)日：2006-12-19
申请号：US10508971
申请日：2003-03-25
申请人： Akihiko Yoshida , Yoshihiro Hori , Makoto Uchida , Eiichi Yasumoto , Yasuo Takebe , Osamu Sakai , Shinya Kosako , Takeshi Yonamine , Masaki Yamauchi , Yasushi Sugawara , Junji Morita
发明人： Akihiko Yoshida , Yoshihiro Hori , Makoto Uchida , Eiichi Yasumoto , Yasuo Takebe , Osamu Sakai , Shinya Kosako , Takeshi Yonamine , Masaki Yamauchi , Yasushi Sugawara , Junji Morita
IPC分类号： H01M4/00
CPC分类号： H01M8/0234 , D03D15/00 , D03D15/0083 , D10B2101/12 , D10B2201/24 , D10B2321/10 , D10B2401/063 , D10B2401/16 , H01M4/8605 , H01M4/92 , H01M4/96 , H01M8/0247 , H01M8/1004 , Y02P70/56
摘要： By using a gas diffusion layer for a fuel cell comprising a fabric comprising a warp thread and a weft thread which are made of carbon fiber, wherein the distance X between adjacent intersections where the warp and weft threads cross each other and the thickness Y of the fabric satisfy the equation: 1.4≦X/Y≦3.5, the present invention reduces the surface asperities of the substrate and prevents a micro short-circuit resulting from the piercing of the polymer electrolyte membrane of the fuel cell by the carbon fibers of the fabric so as to improve the characteristics of the fuel cell.In order to further prevent the piercing of the polymer electrolyte membrane by the carbon fibers of the gas diffusion layer substrate, the rough surface of the carbon fabric is smoothed by: (1) applying a clamping pressure of 1 to 20 kgf/cm2 to the contact area between each electrode and each conductive separator plate of the fuel cell; or (2) heating the gas diffusion layer surface before the gas diffusion layer is disposed onto the polymer electrolyte membrane.
摘要翻译：通过使用包括由碳纤维制成的包括经线和纬纱的织物的燃料电池用气体扩散层，其中，经线和纬线彼此交叉的相邻交点之间的距离X和织物满足以下等式：1.4 <= X / Y <= 3.5，本发明减小了基板的表面粗糙度，并且防止了燃料电池的聚合物电解质膜被碳纤维刺穿导致的微短路织物，以改善燃料电池的特性。为了进一步防止高分子电解质膜被气体扩散层基材的碳纤维刺穿，碳纤维织物的粗糙表面通过以下方式进行平滑化：（1）施加1〜20kgf / cm·SUP > 2 到燃料电池的每个电极和每个导电隔板之间的接触面积; 或者（2）在将气体扩散层配置在高分子电解质膜上之前加热气体扩散层表面。

30. 发明申请

US20060229194A1 METHOD FOR MANUFACTURING POLYMER ELECTROLYTE FUEL CELL 有权
标题翻译：制造聚合物电解质燃料电池的方法
公开(公告)号：US20060229194A1
公开(公告)日：2006-10-12
申请号：US11425191
申请日：2006-06-20
申请人： Makoto Uchida , Yasushi Sugawara , Eiichi Yasumoto , Akihiko Yoshida , Junji Morita , Masao Yamamoto , Shinya Kosako , Osamu Sakai , Yoshihiro Hori
发明人： Makoto Uchida , Yasushi Sugawara , Eiichi Yasumoto , Akihiko Yoshida , Junji Morita , Masao Yamamoto , Shinya Kosako , Osamu Sakai , Yoshihiro Hori
IPC分类号： H01M4/88 , B05D5/12
CPC分类号： H01M4/8605 , H01M4/8807 , H01M4/8828 , H01M4/921 , H01M4/926 , H01M8/0234 , Y02P70/56 , Y10T29/49115
摘要： The present invention provides a polymer electrolyte fuel cell having an increased reaction area by forming a gas channel, a proton channel and an electron channel very close to each other inside a catalyst layer. This polymer electrolyte fuel cell includes a hydrogen ion conductive polymer electrolyte membrane; and a pair of electrodes having catalyst layers sandwiching the hydrogen ion conductive polymer electrolyte membrane between them and gas diffusion layers in contact with the catalyst layers, in which the catalyst layer of at least one of the electrodes comprises carbon particles supporting a noble metal catalyst, and the carbon particles include at least two kinds of carbon particles adsorbing a hydrogen ion conductive polymer electrolyte in mutually different dispersed states.
摘要翻译：本发明通过在催化剂层内形成非常接近的气体通道，质子通道和电子通道，提供了具有增加的反应面积的聚合物电解质燃料电池。该聚合物电解质燃料电池包括氢离子导电聚合物电解质膜; 以及一对电极，其具有夹在其间的氢离子导电性高分子电解质膜和与催化剂层接触的气体扩散层的催化剂层，其中至少一个电极的催化剂层包含负载贵金属催化剂的碳粒子，并且所述碳粒子包含以相互不同的分散状态吸附氢离子导电性高分子电解质的至少2种碳粒子。

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