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11. 发明申请

US20040225082A1 Modified polyphenylene ether resin 失效
标题翻译：改性聚苯醚树脂
公开(公告)号：US20040225082A1
公开(公告)日：2004-11-11
申请号：US10858180
申请日：2004-06-01
发明人： Mutsumi Maeda , Hiroaki Adachi
IPC分类号： C08G065/38
CPC分类号： C08G65/485
摘要： A modified polyphenylene ether resin is provided which is a product of the reaction of 100 parts by weight of (A) a polyphenylene ether having a main chain structure of the following formula (1): 1 (wherein R1 and R4 each independently represents hydrogen, a primary or secondary lower alkyl, a phenyl, an aminoalkyl or a hydrocarbonoxy, and R2 and R3 each independently represents hydrogen, a primary or secondary lower alkyl or a phenyl), with 0.01 to 10.0 parts by weight of (B) a modifier selected from conjugated non-aromatic diene compounds, dienophilic compounds having one dienophile group and precursors of the diene or dienophilic compounds, wherein the number of rearrangement structures each represented by the following formula (2): 2 (wherein R1, R2, R3, and R4 have the same meanings as defined above in the formula (1)) is less than 0.01 per 100 phenylene ether units of the formula (1).
摘要翻译：提供了改性聚苯醚树脂，它是100重量份的（A）具有下式（1）的主链结构的聚苯醚的反应的产物：其中R 1和R 4各自独立地表示氢，伯或仲低级烷基，苯基，氨基烷基或烃氧基，并且R 2和R 3各自独立地表示氢，伯或仲低级烷基或苯基），和0.01至10.0重量份的（B）选自共轭非芳族二烯化合物，具有一个亲双烯基的二亲性化合物和二烯或二亲烯化合物的前体，其中各自由下式（2）表示的重排结构的数目：（其中R1，R2，R3和R4具有与式（1）中定义相同的含义）每100个式（1）的亚苯基醚单元小于0.01。

12. 发明申请

US20040147710A1 Fluorinated aromatic polymer and use thereof 失效
标题翻译：氟化芳族聚合物及其用途
公开(公告)号：US20040147710A1
公开(公告)日：2004-07-29
申请号：US10754601
申请日：2004-01-12
申请人： ASAHI GLASS COMPANY LIMITED
发明人： Shunsuke Yokotsuka , Fusaaki Takeo
IPC分类号： C08G065/38
CPC分类号： H01L21/7682 , C08G61/10 , H01L21/0212 , H01L21/02282 , H01L21/3127 , H01L23/49894 , H01L23/5329 , H01L2221/1047 , H01L2924/0002 , H05K1/034 , H05K3/4676 , H01L2924/00
摘要： To provide a fluorinated aromatic polymer having excellent heat resistance and a low relative permittivity; and an insulating film for electronic devices and an insulating film for multilayered wiring boards, which are made of the polymer. A fluorinated aromatic polymer which contains two or more crosslinkable functional groups (A) per molecule and has a number average molecular weight of from 1null103 to 5null105 and an ether linkage and which is produced by e.g. a method in which a branched fluorinated aromatic compound (B) represented by the formula 1 and a compound (Y1) having a crosslinkable functional group (A) and a phenolic hydroxyl group, are subjected to a condensation reaction in the presence of a HF-removing agent: 1
摘要翻译：提供具有优异的耐热性和低相对介电常数的氟化芳族聚合物; 以及由聚合物制成的用于电子器件的绝缘膜和用于多层布线板的绝缘膜。每分子含有两个或更多个可交联官能团（A）并具有1×10 3至5×10 5的数均分子量和醚键的氟化芳族聚合物，将由式1表示的支链氟化芳族化合物（B）和具有交联性官能团（A）的化合物（Y1）和酚羟基的方法在HF- 去除剂：

13. 发明申请

US20040054121A1 METHOD AND APPARATUS FOR PREPARING A POLY(ARYLENE ETHER) 失效
标题翻译：制备聚（亚乙基醚）的方法和装置
公开(公告)号：US20040054121A1
公开(公告)日：2004-03-18
申请号：US10065062
申请日：2002-09-13
发明人： Rudy Francois Alain Jos Peemans , Wiebe Knol , Peter Groefsema
IPC分类号： C08G065/38 , B01J019/00
CPC分类号： C08G65/46
摘要： A method of precipitating a poly(arylene ether) includes preparing a poly(arylene ether) solution comprising a poly(arylene ether) and a solvent, combining the poly (arylene ether) solution with an antisolvent to form a poly(arylene ether) dispersion comprising a poly(arylene ether) solid, separating the poly(arylene ether) solid from the poly(arylene ether) dispersion to form an isolated poly(arylene ether) solid, determining a particle size distribution of the poly(arylene ether) solid prior to separating the poly(arylene ether) solid from the poly(arylene ether) dispersion, and adjusting a precipitation parameter in response to the particle size distribution. Although the measured particle size distribution is very different from the particle size distribution of the solid poly(arylene ether) ultimately isolated, it is useful for controlling the process. The method may be automated to rapidly adjust precipitation conditions in response to the particle size distribution measurements. An apparatus for carrying out the method is also described.
摘要翻译：沉淀聚（亚芳基醚）的方法包括制备包含聚（亚芳基醚）和溶剂的聚（亚芳基醚）溶液，将聚（亚芳基醚）溶液与抗溶剂结合以形成聚（亚芳基醚）分散体包括聚（亚芳基醚）固体，从聚（亚芳基醚）分散体中分离聚（亚芳基醚）固体以形成分离的聚（亚芳基醚）固体，以前测定聚（亚芳基醚）固体的粒度分布从聚（亚芳基醚）分散体中分离聚（亚芳基醚）固体，并根据粒度分布调节沉淀参数。虽然测量的粒度分布与最终分离的固体聚（亚芳基醚）的粒度分布非常不同，但是对于控制该方法是有用的。该方法可以自动化以响应于粒度分布测量快速调节沉淀条件。还描述了用于执行该方法的装置。

14. 发明申请

US20030088050A1 Substituted poly(arylenevinylenes), process for their preparation, and their use in electroluminescent elements 有权
标题翻译：取代的聚（亚芳基亚乙烯基），其制备方法及其在电致发光元件中的应用
公开(公告)号：US20030088050A1
公开(公告)日：2003-05-08
申请号：US10185061
申请日：2002-06-28
发明人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Hermann Schenk , Nu Yu
IPC分类号： C08G065/38
CPC分类号： H01L51/0038 , C08G61/02 , C09K11/06 , H01B1/128 , H01L51/5012 , H05B33/14 , Y10S428/917
摘要： Poly(arylenevinylenes) comprising at least 20% of recurring units of the formula (I), 1 where the symbols and indices have the following meanings: Aryl: is an aryl group having 4 to 14 carbon atoms; Rnull: is a substituent which is either in the labeled phenylene position 5 or 6 and is CN, F, Cl, N(R1R2) or a straight-chain, branched or cyclic alkyl, alkoxy or thioalkoxy group having 1 to 20 carbon atoms, in which, in addition, one or more H atoms may be replaced by F; Rnull: are identical or different and are CN, F, Cl or a straight-chain, branched or cyclic alkyl or alkoxy group having 1 to 20 carbon atoms, where one or more non-adjacent CH2 groups may be replaced by nullOnull, nullSnull, nullCOnull, nullCOOnull, nullOnullCOnull, nullNR1null, null(NR2R3)null-Anull or nullCONR4null, and where one or more H atoms may be replaced by F, or an aryl group having 4 to 14 carbon atoms, which may be substituted by one or more non-aromatic radicals Rnull; R1, R2, R3, R4 are identical or different and are H or an aliphatic or aromatic hydrocarbon radical having 1 to 20 carbon atoms; Anull: is a singly charged anion or an equivalent thereof; and n: is 0, 1, 2, 3, 4 or 5. are suitable as electroluminescent materials.
摘要翻译：包含至少20％式（I）的重复单元的聚（亚芳基亚乙烯基），其中符号和指数具有以下含义：芳基：具有4至14个碳原子的芳基; R'：是在标记的亚苯基位置5或6中的取代基，是CN，F，Cl，N（R 1 R 2）或具有1至20个碳原子的直链，支链或环烷基，烷氧基或硫代烷氧基，其中另外一个或多个H原子可被F取代; R“相同或不同，为CN，F，Cl或具有1至20个碳原子的直链，支链或环状烷基或烷氧基，其中一个或多个不相邻的CH 2基团可被-O - ， - S - ， - CO - ， - COO - ， - O-CO-， - NR1 - ， - （NR2R3）+ - 或 - CONR4-，并且其中一个或多个H原子可被F取代，或具有4至14个碳原子的芳基，其可以被一个或多个非芳族基团R'取代; R1，R2，R3，R4相同或不同，为H或碳原子数1〜20的脂肪族或芳香族烃基; A-：是单电荷的阴离子或其等同物; 并且n：为0,1,2,3,4或5.适合作为电致发光材料。

15. 发明申请

US20030045757A1 Modified polyphenylene ether 审中-公开
标题翻译：改性聚苯醚
公开(公告)号：US20030045757A1
公开(公告)日：2003-03-06
申请号：US10182648
申请日：2002-07-31
发明人： Yoshiyuki Ishii , Kumi Sorita
IPC分类号： C08G063/00 , C08G065/38 , C07C043/263
CPC分类号： C08L71/126 , C08G65/485 , H05K3/4626 , C08L2666/14 , C08L63/00
摘要： Disclosed is a modified polyphenylene ether having a number average molecular weight of not smaller than 4,000, which is obtained by reacting a precursory modified polyphenylene ether with a phenolic compound in the presence of a radical generator, wherein the precursory modified polyphenylene ether comprises a plurality of polyphenylene ether chains each having a terminal phenolic hydroxyl group, wherein the plurality of polyphenylene ether chains collectively have at least one terminal phenolic hydroxyl group modified and wherein not all of the terminal phenolic hydroxyl groups of the plurality of polyphenylene ether chains are modified. Also disclosed is a method for producing the modified polyphenylene ether.
摘要翻译：公开了一种数均分子量不小于4000的改性聚苯醚，其通过在自由基发生剂存在下使前体改性的聚苯醚与酚类化合物反应获得，其中前体改性聚苯醚包括多个每个具有末端酚羟基的聚苯醚链，其中多个聚苯醚链共同具有至少一个修饰的末端酚羟基，并且其中并不全部多个聚苯醚链的末端酚羟基被改性。还公开了改性聚苯醚的制造方法。

16. 发明申请

US20010053842A1 2,7-aryl-9-substituted fluorenes and 9-substituted fluorene oligomers and polymers 失效
标题翻译： 2,7-芳基-9-取代的芴和9-取代的芴低聚物和聚合物
公开(公告)号：US20010053842A1
公开(公告)日：2001-12-20
申请号：US09755507
申请日：2001-01-05
发明人： Edmund P. Woo , William R. Shiang , Michael Inbasekaran , Gordon R. Roof
IPC分类号： C08G061/00 , C08G061/02 , C08G065/26 , C08G065/02 , C08G065/38 , C08G059/24
CPC分类号： H01L51/0052 , C07C17/2637 , C07C17/266 , C07C25/22 , C07C25/24 , C07C211/48 , C07C2603/18 , C08G61/00 , C08G61/02 , C08G61/10 , C09K11/06 , H01L21/28035 , H01L21/28167 , H01L22/20 , H01L29/42364 , H01L29/42376 , H01L29/66575 , H01L51/0039 , H01L51/0043 , H01L51/0058 , H01L51/0094 , H01L51/42 , H01L51/5012 , Y10S428/917 , Y10T428/3154
摘要： The invention relates to 2,7-substituted-9-substituted fluorenes and 9-substituted fluorene oligomers and polymers. The fluorenes, oligomers and polymers are substituted at the 9-position with two hydrocarbyl moieties which may optionally contain one or more of sulfur, nitrogen, oxygen, phosphorous or silicon heteroatoms; a C5-20 ring structure formed with the 9-carbon on the fluorene ring or a C4-20 ring structure formed with the 9-carbon containing one or more heteroatoms of sulfur, nitrogen or oxygen; or a hydrocarbylidene moiety. In one embodiment, the fluorenes are substituted at the 2- and 7-positions with aryl moieties which may further be substituted with moieties which are capable of crosslinking or chain extension or a trialkylsiloxy moiety. The fluorene polymers and oligomers may be substituted at the 2- and 7null-positions. The monomer units of the fluorene oligomers and polymers are bound to one another at the 2- and 7null-positions. The 2,7null-aryl-9-substituted fluorene oligomers and polymers may be further reacted with one another to form higher molecular weight polymers by causing the optional moieties on the terminal 2,7null-aryl moieties, which are capable of crosslinking or chain extension, to undergo chain extension or crosslinking. Also disclosed are processes for preparing the disclosed compounds.
摘要翻译：本发明涉及2,7-取代的9-取代的芴和9-取代的芴低聚物和聚合物。芴，低聚物和聚合物在9位被两个烃基部分取代，该烃基部分可任选地含有一个或多个硫，氮，氧，磷或硅杂原子; 由芴环上的9-碳形成的C5-20环结构或由含有一个或多个硫，氮或氧杂原子的9-碳形成的C 4-20环结构; 或亚烃基部分。在一个实施方案中，芴在2-和7-位被芳基部分取代，芳基部分可进一步被能够交联或延伸的部分或三烷基甲硅烷氧基部分取代。芴聚合物和低聚物可以在2-和7-位取代。芴低聚物和聚合物的单体单元在2和7'位置彼此结合。 2,7'-芳基-9-取代的芴低聚物和聚合物可以进一步彼此反应以通过在端基2,7'-芳基部分上引入任选的部分来形成较高分子量的聚合物，其能够交联或链延伸，进行链延长或交联。还公开了制备所公开的化合物的方法。

17. 发明申请

US20040236060A1 2, 6-dimethyphenol composition 有权
标题翻译： 2,6-二甲苯酚组成
公开(公告)号：US20040236060A1
公开(公告)日：2004-11-25
申请号：US10485963
申请日：2004-02-06
发明人： Akira Mitsui , Osamu Shoji , Hitoshi Ota
IPC分类号： C08G065/38
CPC分类号： C09K21/14 , C07C37/84 , C07C39/07 , C08G65/44 , C09K3/10 , C09K2200/0657
摘要： A 2,6-dimethylphenol composition having an m-cresol content of from 15 to 700 ppm on a weight basis has effects of drastically improving polymerization activity and particularly, improving the color tone of polyphenylene ethers. Therefore, the composition makes it possible to provide a preparation process having improved productivity, and at the same time, provide polyphenylene ethers having good quality.
摘要翻译：基于重量，间甲酚含量为15〜700ppm的2,6-二甲基苯酚组合物具有显着改善聚合活性的作用，特别是提高聚苯醚的色调。因此，组合物可以提供具有提高的生产率的制备方法，同时提供质量好的聚苯醚。

18. 发明申请

US20040186262A1 Ion conductive membrane made from a block copolymer and methods of making a block copolymer 有权
标题翻译：由嵌段共聚物制成的离子导电膜和制备嵌段共聚物的方法
公开(公告)号：US20040186262A1
公开(公告)日：2004-09-23
申请号：US10768507
申请日：2004-01-30
发明人： Gerhard Maier , Gunther G. Scherer , Chong-Kyu Shin
IPC分类号： C08G065/38
CPC分类号： C08G75/23 , B01D67/0009 , B01D67/0093 , B01D69/00 , B01D69/02 , B01D71/80 , B01D71/82 , B01D2325/24 , B01D2325/26 , B01D2325/36 , B01D2325/38 , B01D2325/42 , C08G65/48 , C08G2650/40 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/1032 , H01M8/1037 , H01M8/1039 , H01M2300/0082 , Y02P70/56
摘要： A block copolymer for use as a solid polymer electrolyte, said block copolymer having at least first and second segments, the first segments being hydrophilic segments provided with acidic substituents for proton transport and the second segments being hydrophobic segments having substantially no acidic substituents and serving for the mechanical integrity of the solid polymer electrolyte. Also described and claimed are an ion-conductive membrane made from block copolymers of the aforementioned kind as well as methods of preparing such block copolymers and membranes based thereon. The membranes have improved proton conductivity and improved mechanical properties in the presence of water making them particularly suitable for use in fuel cells.
摘要翻译：一种用作固体聚合物电解质的嵌段共聚物，所述嵌段共聚物至少具有第一和第二链段，第一链段是提供质子转运的酸性取代基的亲水链段，第二链段是基本上不含酸性取代基的疏水链段，固体聚合物电解质的机械完整性。还描述和要求保护的是由上述类型的嵌段共聚物制成的离子传导膜以及基于其制备这种嵌段共聚物和膜的方法。膜在水的存在下具有改善的质子传导性和改善的机械性能，使得它们特别适用于燃料电池。

19. 发明申请

US20040181028A1 Oligomeric hydroxy arylether phthalonitiles and synthesis thereof 有权
标题翻译：低聚羟基芳基醚酞腈及其合成
公开(公告)号：US20040181028A1
公开(公告)日：2004-09-16
申请号：US10808265
申请日：2004-03-17
发明人： Teddy M. Keller , Dawn D. Dominguez
IPC分类号： C08G065/38
CPC分类号： G02F1/133615 , C08G65/40 , C08G65/48 , C08G2650/04 , C08G2650/20 , C08L2312/00
摘要： An aromatic ether oligomer or polyaromatic ether comprising the formula: 1 wherein Ar is an independently selected divalent aromatic radical; formed by reacting a dihydroxyaromatic with a dihaloaromatic; and wherein the reaction is performed in the presence of a copper compound and cesium carbonate. The polyaromatic ether is formed when neither the dihydroxyaromatic nor the dihaloaromatic is present in an excess amount. The aromatic ether oligomer is formed by using an excess of either dihydroxyaromatic or dihaloaromatic. A phthalonitrile monomer comprising the formula: 2 formed by reacting a 3- or 4-nitrophthalonitrile with a hydroxy-terminated aromatic ether oligomer. A thermoset formed by curing the phthalonitrile monomer. Processes for forming all the above.
摘要翻译：芳族醚低聚物或聚芳醚，其包含下式：其中Ar是独立选择的二价芳族基团; 通过二羟基芳族化合物与二卤代芳族化合物反应形成; 并且其中所述反应在铜化合物和碳酸铯存在下进行。当二羟基芳族化合物和二卤代芳族化合物都不存在时，形成多芳香族醚。芳族醚低聚物通过使用过量的二羟基芳族化合物或二卤代芳族化合物形成。包含下式的邻苯二甲腈单体：通过使3-或4-硝基邻苯二腈与羟基封端的芳族醚低聚物反应形成。通过固化邻苯二甲腈单体形成的热固性材料。用于形成上述所有方法。

20. 发明申请

US20030176623A1 Poly-o-hydroxyamides, polybenzoxazoles, processes for producing poly-o-hydroxyamides, processes for producing polybenzoxazoles, dielectrics including a polybenzoxazole, electronic components including the dielectrics, and processes for manufacturing the electronic components 失效
标题翻译：聚邻羟基酰胺，聚苯并恶唑，聚邻羟基酰胺的制造方法，聚苯并恶唑的制造方法，包括聚苯并恶唑的电介质，包含电介质的电子部件，以及电子部件的制造方法
公开(公告)号：US20030176623A1
公开(公告)日：2003-09-18
申请号：US10261034
申请日：2002-09-30
发明人： Klaus Lowack , Anna Maltenberger , Recai Sezi , Andreas Walter
IPC分类号： C08G065/38 , C08G069/26
CPC分类号： H01L21/02118 , C08G73/00 , C08G73/10 , H01B3/305 , H01L21/02282 , H01L21/312 , H01L23/5329 , H01L2924/0002 , H01L2924/3011 , H01L2924/00
摘要： Poly-o-hydroxyamides are cyclicized to obtain polybenzoxazoles. The poly-o-hydroxyamides provide effective filling of trenches. In particular, the poly-o-hydroxyamides can fill trenches having a width of less than 100 nm and an aspect ratio of more than 4. Further, the polybenzoxazoles of the invention are very suitable for the damascene process. A dielectric can be made from the polybenzoxazole. In turn, semiconductor devices can include the dieletric. Processes for making the poly-o-hydroxyamides, polybenzoxazoles, and semiconductor devices are included.
摘要翻译：环氧化聚邻羟基酰胺得到聚苯并恶唑。聚邻羟基酰胺提供有效填充沟槽。特别地，聚邻羟基酰胺可以填充宽度小于100nm，纵横比大于4的沟槽。此外，本发明的聚苯并恶唑非常适用于镶嵌工艺。电介质可以由聚苯并恶唑制成。反过来，半导体器件可以包括消毒的。包括制备聚邻羟基酰胺，聚苯并恶唑和半导体器件的方法。

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