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11. 发明授权

US07312284B2 Process for producing polar olefin copolymer and polar olefin copolymer obtained thereby 有权
标题翻译：制备极性烯烃共聚物和极性烯烃共聚物的方法
公开(公告)号：US07312284B2
公开(公告)日：2007-12-25
申请号：US11253963
申请日：2005-10-20
申请人： Yoshihisa Inoue , Shigekazu Matsui , Yasuhiko Suzuki , Yasunori Yoshida , Yukihiro Takagi , Terunori Fujita , Tomoaki Matsugi , Takashi Nakano
发明人： Yoshihisa Inoue , Shigekazu Matsui , Yasuhiko Suzuki , Yasunori Yoshida , Yukihiro Takagi , Terunori Fujita , Tomoaki Matsugi , Takashi Nakano
IPC分类号： C08F4/44 , C08F4/602 , C08F4/605 , C08F220/00
CPC分类号： C08F210/02 , C08F4/619 , C08F4/639 , C08F4/659 , C08F10/00 , C08F4/54 , C08F4/64048 , C08F220/06 , C08F2500/20 , C08F2500/17 , C08F220/12 , C08F220/04 , C08F232/00 , C08F222/06 , C08F4/6812 , C08F4/6912 , C08F4/7022 , C08F4/64044 , C08F4/68112 , C08F4/69112 , C08F4/69474 , C08F4/68474 , C08F4/64189 , C08F4/64051 , C08F4/68129 , C08F4/69129 , C08F4/68293 , C08F4/64186 , C08F4/68465 , C08F4/69465 , C08F4/69103 , C08F4/68103
摘要： A process for producing a polar olefin copolymer comprises copolymerizing a non-polar olefin and a polar olefin in the presence of a transition metal compound selected from Groups 4, 5, 6 and 11 of the periodic table, which is represented by the following formula (IV): wherein M′ is a transition metal atom selected from Groups 4, 5, 6 and 11 of the periodic table, m is an integer of 1 to 6, A is —O—, —Si—, —Se—, —N(R6)—, n is a number satisfying a valence of M′, R1 to R4 and R6 are each a hydrogen atom, a halogen atom, a hydrocarbon group and the like, and X is a halogen atom, an oxygen atom, a hydrocarbon group and the like, and at least one compound (B) selected from the group consisting of an organometallic compound (B-1), an organoaluminum oxy-compound (B-2) and an ionic ionizing compound (B-3). Therefore, the process is capable of obtaining a polar olefin copolymer having excellent properties under mild polymerization conditions.
摘要翻译：一种制备极性烯烃共聚物的方法，包括在选自元素周期表第4,5,6和11族的过渡金属化合物存在下使非极性烯烃和极性烯烃共聚合，其由下式（ IV）：其中M'是选自元素周期表第4,5,6和11族的过渡金属原子，m是1至6的整数，A是-O - ， - Si-，-Se-， - N（R 6） - ，n是满足M'，R 1至R 4和R 6的价数的数各自为氢原子，卤素原子，烃基等，X为卤素原子，氧原子，烃基等，以及至少一种选自以下的化合物（B）：由有机金属化合物（B-1），有机铝氧化合物（B-2）和离子电离化合物（B-3）组成的组。因此，该方法能够获得在温和聚合条件下具有优异性能的极性烯烃共聚物。

12. 发明申请

US20030004290A1 Olefin polymerization catalyst and process for olefin polymerization using the olefin polymerization catalyst 有权
标题翻译：烯烃聚合催化剂和使用烯烃聚合催化剂的烯烃聚合方法
公开(公告)号：US20030004290A1
公开(公告)日：2003-01-02
申请号：US10127720
申请日：2002-04-23
申请人： Mitsui Chemicals, Inc.
发明人： Naoto Matsukawa , Kazutaka Tsuru , Masatoshi Nitabaru , Junji Saito , Tetsuhiro Matsumoto
IPC分类号： C08F004/06 , B01J031/00
CPC分类号： C08F10/02 , C08F110/02 , C08F4/659 , C08F4/64048 , C08F2500/17 , C08F4/64051 , C08F4/64044 , C08F4/64041
摘要： An olefin polymerization catalyst having a high polymerization activity at high temperatures and a process for olefin polymerization using the catalyst are disclosed. The olefin polymerization catalyst comprises a transition metal compound which is represented by the following formula (I) and in which the net charge parameter of the central metal is not more than 2.00. 1 wherein M is a transition metal atom of Group 4 to Group 5 of the periodic table, m is an integer of 1 to 5, Q is nullNnullor nullC(R2)null, A is null0null, nullSnull, nullSenull or nullN(R5)null, R1 is an aliphatic hydrocarbon group or an alicyclic hydrocarbon group, R2 to R5 are each a hydrogen atom, a hydrocarbon group, an oxygen-containing group or the like, n is a number satisfying a valence of M, and X is a hydrogen atom, a halogen atom, a hydrocarbon group or the like.
摘要翻译：公开了一种在高温下具有高聚合活性的烯烃聚合催化剂和使用该催化剂的烯烃聚合方法。烯烃聚合催化剂包含由下式（I）表示的过渡金属化合物，其中中心金属的净电荷参数不大于2.00。其中M是周期表第4族至第5族的过渡金属原子，m是1至5的整数，Q是-N =或-C（R 2）=，A是-O - ， - S-， -Se-或-N（R5） - ，R1是脂族烃基或脂环族烃基，R2〜R5各自为氢原子，烃基，含氧基等，n为满足 M的化合价，X为氢原子，卤原子，烃基等。

13. 发明申请

WO99054364A1 CATALYST FOR OLEFIN POLYMERIZATION AND METHOD OF POLYMERIZING OLEFIN 审中-公开
标题翻译：用于烯烃聚合的催化剂和聚烯烃的方法
公开(公告)号：WO99054364A1
公开(公告)日：1999-10-28
申请号：PCT/JP1999/002018
申请日：1999-04-15
IPC分类号： F24F1/00 , C08F4/16 , C08F4/26 , C08F4/44 , C08F4/642 , C08F4/70 , C08F10/00 , C08F110/02
CPC分类号： C08F10/00 , C08F110/02 , C08F4/659 , C08F2500/17 , C08F4/64051 , C08F4/64044 , C08F4/64048 , C08F4/6411 , C08F4/6412 , C08F4/7008 , C08F4/7054 , C08F4/64113 , C08F4/64148 , C08F4/64151 , C08F4/64141
摘要： A catalyst for olefin polymerization which comprises a novel transition metal compound and has excellent activity in olefin polymerization; and a method of polymerizing an olefin using this catalyst. The catalyst comprises a transition metal compound (A-1) represented by formula (I) or a transition metal compound (A-2) represented by formula (II) and optionally further contains at least one compound (B) selected from the group consisting of organometallic compounds (B-1), organoaluminumoxy compounds (B-2), and compounds (B-3) which react with the transition metal compound (A-1) or (A-2) to form an ion pair. (In the formulae, M represents a transition metal in Groups 3 to 11 of the Periodic Table; m is an integer of 1 to 3 in formula (I) and is an integer of 1 to 6 in formula (II); Q represents -N= or -C(R )=; A represents -O-, -S-, -Se-, or -N(R )-; R to R each represents hydrogen, a hydrocarbon group, etc., provided that two or more of R to R may be bonded to each other to form a ring; n is a number equal to the valence of M; and X represents halogeno, a hydrocarbon group, etc.).
摘要翻译：一种用于烯烃聚合的催化剂，其包含新型过渡金属化合物，并且在烯烃聚合中具有优异的活性; 以及使用该催化剂聚合烯烃的方法。催化剂包含式（I）表示的过渡金属化合物（A-1）或由式（II）表示的过渡金属化合物（A-2），并任选地还含有至少一种选自以下的化合物（B）：的有机金属化合物（B-1），有机铝氧化合物（B-2）和与过渡金属化合物（A-1）或（A-2）反应形成离子对的化合物（B-3）。（式中，M表示周期表第3〜11族中的过渡金属，m为式（I）中的1〜3的整数，式（II）中的1〜6的整数，Q表示 - N =或-C（R 2）=; A表示-O - ， - S-，-Se-或-N（R 6） - ; R 1至R 6各自表示氢，烃基等，条件是R 1至R 6中的两个或多个可以彼此键合形成环; n等于M的化合价; X表示卤代，烃基等）。

14. 发明授权

EP2050769B1 Olefin polymerization catalyst and process for olefin polymerization 有权
标题翻译：用于烯烃聚合的烯烃聚合催化剂和工艺
公开(公告)号：EP2050769B1
公开(公告)日：2013-05-22
申请号：EP09000431.8
申请日：1999-04-15
申请人： Mitsui Chemicals, Inc.
发明人： Matsui, Shigekazu , Nitabaru, Masatoshi , Tsuru, Kazutaka , Fujita, Terunori , Suzuki, Yasuhiko , Takagi, Yukihiro , Tanaka, Hidetsugu
IPC分类号： C08F4/80 , C08F4/70 , C08F10/02 , C08F4/64
CPC分类号： C08F10/00 , C08F110/02 , C08F4/659 , C08F2500/17 , C08F4/64051 , C08F4/64044 , C08F4/64048 , C08F4/6411 , C08F4/6412 , C08F4/7008 , C08F4/7054 , C08F4/64113 , C08F4/64148 , C08F4/64151 , C08F4/64141

15. 发明公开

EP1170308A3 Process for producing a copolymer of a non-polar olefin and a polar olefin and the copolymer obtained thereby 有权
标题翻译：如此制备一种制备非极性烯烃的共聚物和极性烯烃和所述共聚物的方法
公开(公告)号：EP1170308A3
公开(公告)日：2002-07-31
申请号：EP01115672.6
申请日：2001-07-04
申请人： MITSUI CHEMICALS, INC.
发明人： Inoue, Yoshihisa , Matsui, Shigekazu , Suzuki, Yasuhiko , Yoshida, Yasunori , Takagi, Yukihiro , Fujita, Terunori , Matsugi, Tomoaki , Nakano, Takashi
IPC分类号： C08F210/02 , C08F210/16 , C08F4/622 , C08F4/54
CPC分类号： C08F210/02 , C08F4/619 , C08F4/639 , C08F4/659 , C08F10/00 , C08F4/54 , C08F4/64048 , C08F220/06 , C08F2500/20 , C08F2500/17 , C08F220/12 , C08F220/04 , C08F232/00 , C08F222/06 , C08F4/6812 , C08F4/6912 , C08F4/7022 , C08F4/64044 , C08F4/68112 , C08F4/69112 , C08F4/69474 , C08F4/68474 , C08F4/64189 , C08F4/64051 , C08F4/68129 , C08F4/69129 , C08F4/68293 , C08F4/64186 , C08F4/68465 , C08F4/69465 , C08F4/69103 , C08F4/68103
摘要： A process for producing a polar olefin copolymer comprises copolymerizing a non-polar olefin and a polar olefin in the presence of a transition metal compound selected from Groups 4, 5, 6 and 11 of the periodic table, which is represented by the following formula (IV): wherein M' is a transition metal atom selected from Groups 4, 5, 6 and 11 of the periodic table, m is an integer of 1 to 6, A is -O-, -Si-, -Se-, -N(R 6 )-, n is a number satisfying a valence of M', R 1 to R 4 and R 6 are each a hydrogen atom, a halogen atom, a hydrocarbon group and the like, and X is a halogen atom, an oxygen atom, a hydrocarbon group and the like, and at least one compound (B) selected from the group consisting of an organometallic compound (B-1), an organoaluminum oxy-compound (B-2) and an ionic ionizing compound (B-3). Therefore, the process is capable of obtaining a polar olefin copolymer having excellent properties under mild polymerization conditions.
摘要翻译：一种用于制造极性烯烃共聚物的方法包括共聚合的非极性烯烃和选自4，5，6和周期表的第11族的过渡金属化合物的存在下，极性烯烃，所有这是由下述式（ IV）： worin m“为选自4，5，6和周期表的第11中的过渡金属原子，m是1至6的整数，A为-O-，-Si-，硒 - ， - N（R <6>） - ，n是一个满足M化合价”，R <1>至R的数<4>和R <6>各自为氢原子，卤原子，烃基和类似物，和X是卤原子与氧原子，烃基等，和至少一种化合物选自以下的有机金属化合物中选择的（B）（B-1）至有机铝氧化合物（B-2）和电离化离子化合物（B-3）。因此，该方法能够获得具有温和的聚合条件下优异特性的极性烯烃共聚物。

16. 发明授权

US06962890B2 Olefin polymerization catalyst and process for olefin polymerization using the olefin polymerization catalyst 有权
标题翻译：烯烃聚合催化剂和使用烯烃聚合催化剂的烯烃聚合方法
公开(公告)号：US06962890B2
公开(公告)日：2005-11-08
申请号：US10127720
申请日：2002-04-23
申请人： Naoto Matsukawa , Kazutaka Tsuru , Masatoshi Nitabaru , Junji Saito , Tetsuhiro Matsumoto
发明人： Naoto Matsukawa , Kazutaka Tsuru , Masatoshi Nitabaru , Junji Saito , Tetsuhiro Matsumoto
IPC分类号： C08F4/42 , C08F4/642 , C08F10/02 , C08F110/02 , B01J31/38 , C08F4/72
CPC分类号： C08F10/02 , C08F110/02 , C08F4/659 , C08F4/64048 , C08F2500/17 , C08F4/64051 , C08F4/64044 , C08F4/64041
摘要： An olefin polymerization catalyst having a high polymerization activity at high temperatures and a process for olefin polymerization using the catalyst are disclosed. The olefin polymerization catalyst comprises a transition metal compound which is represented by the following formula (I) and in which the net charge parameter of the central metal is not more than 2.00: wherein M is a transition metal atom of Group 4 to Group 5 of the periodic table, m is an integer of 1 to 5, Q is —N═ or —C(R2)═, A is —O—, —S—, —Se— or —N(R5)—, R1 is an aliphatic hydrocarbon group or an alicyclic hydrocarbon group, R2 to R5 are each a hydrogen atom, a hydrocarbon group, an oxygen-containing group or the like, n is a number satisfying a valence of M, and X is a hydrogen atom, a halogen atom, a hydrocarbon group or the like.
摘要翻译：公开了一种在高温下具有高聚合活性的烯烃聚合催化剂和使用该催化剂的烯烃聚合方法。烯烃聚合催化剂包括由下式（I）表示的过渡金属化合物，其中中心金属的净电荷参数不大于2.00：其中M是第4族至第5族的过渡金属原子元素周期表，m为1至5的整数，Q为-N-或-C（R 2） - ，A为-O - ， - S - ， - S - 或-N （R 5） - ，R 1是脂族烃基或脂环族烃基，R 2至R 5， SUP>各自为氢原子，烃基，含氧基等，n为满足M价的数，X为氢原子，卤素原子，烃基等。

17. 发明授权

US06593266B1 Olefin polymerization catalyst and polymerization process 有权
标题翻译：烯烃聚合催化剂和聚合方法
公开(公告)号：US06593266B1
公开(公告)日：2003-07-15
申请号：US09291950
申请日：1999-04-15
申请人： Shigekazu Matsui , Kazutaka Tsuru , Masatoshi Nitabaru , Terunori Fujita , Makoto Mitani , Yukihiro Takagi , Takashi Nakano
发明人： Shigekazu Matsui , Kazutaka Tsuru , Masatoshi Nitabaru , Terunori Fujita , Makoto Mitani , Yukihiro Takagi , Takashi Nakano
IPC分类号： B01J3100
CPC分类号： C08F10/00 , C08F110/02 , C08F4/64048 , C08F2500/17 , C08F4/64044 , C08F4/64051 , C08F4/64075
摘要： An olefin polymerization catalyst having an excellent polymerization activity and an olefin polymerization process using the catalyst are disclosed. The olefin polymerization catalyst comprises (A) a transition metal compound represented by, for example, the following formula (I) and optionally (B) at least one compound selected from an organometallic compound, an organoaluminum oxy-compound and a compound which reacts with the transition metal compound (A) to from an ion pair; wherein M is a transition metal atom of Group 3 to Group 11 of the periodic table; m is an integer of 1 to 6; A is —O—, —S—, —Se— or —N(R5)—; D is —C(R7)(R8)—, —Si(R9)(R10)— or the like; Z is —R13 and —R14, ═C(R15)R16, ═NR17 or the like; R1 to R17 are each H, a hydrocarbon group or the like; n is a number satisfying a valence of M; and X is halogen, a hydrocarbon group or the like.
摘要翻译：公开了具有优异聚合活性的烯烃聚合催化剂和使用该催化剂的烯烃聚合方法。烯烃聚合催化剂包含（A）由下式（I）表示的过渡金属化合物和任选的（B）至少一种选自有机金属化合物，有机铝氧化合物和与过渡金属化合物（A）离子对;其中M是周期表第3族至第11族的过渡金属原子; m为1〜6的整数。 A是-O - ， - S - ， - Se-或-N（R 5） - ; D是-C（R7）（R8） - ，-Si（R9）（R10） - 等; Z是-R13和-R14，= C（R15）R16，= NR17等; R 1〜R 17分别为H，烃基等; n是满足M价的数; X为卤素，烃基等。

18. 发明申请

US20020099155A1 Process for producing polar olefin copolymer and polar olefin copolymer obtained thereby 有权
标题翻译：制备极性烯烃共聚物和极性烯烃共聚物的方法
公开(公告)号：US20020099155A1
公开(公告)日：2002-07-25
申请号：US09897111
申请日：2001-07-03
发明人： Yoshihisa Inoue , Shigekazu Matsui , Yasuhiko Suzuki , Yasunori Yoshida , Yukihiro Takagi , Terunori Fujita , Tomoaki Matsugi , Takashi Nakano
IPC分类号： C08F004/06
CPC分类号： C08F210/02 , C08F4/619 , C08F4/639 , C08F4/659 , C08F10/00 , C08F4/54 , C08F4/64048 , C08F220/06 , C08F2500/20 , C08F2500/17 , C08F220/12 , C08F220/04 , C08F232/00 , C08F222/06 , C08F4/6812 , C08F4/6912 , C08F4/7022 , C08F4/64044 , C08F4/68112 , C08F4/69112 , C08F4/69474 , C08F4/68474 , C08F4/64189 , C08F4/64051 , C08F4/68129 , C08F4/69129 , C08F4/68293 , C08F4/64186 , C08F4/68465 , C08F4/69465 , C08F4/69103 , C08F4/68103
摘要： A process for producing a polar olefin copolymer comprises copolymerizing a non-polar olefin and a polar olefin in the presence of a transition metal compound selected from Groups 4, 5, 6 and 11 of the periodic table, which is represented by the following formula (IV): 1 wherein Mnull is a transition metal atom selected from Groups 4, 5, 6 and 11 of the periodic table, m is an integer of 1 to 6, A is nullOnull, nullSinull, nullSenull, nullN(R6)null, n is a number satisfying a valence of Mnull, R1 to R4 and R6 are each a hydrogen atom, a halogen atom, a hydrocarbon group and the like, and X is a halogen atom, an oxygen atom, a hydrocarbon group and the like, and at least one compound (B) selected from the group consisting of an organometallic compound (B-1), an organoaluminum oxy-compound (B-2) and an ionic ionizing compound (B-3). Therefore, the process is capable of obtaining a polar olefin copolymer having excellent properties under mild polymerization conditions.
摘要翻译：一种制备极性烯烃共聚物的方法，包括在选自元素周期表第4,5,6和11族的过渡金属化合物存在下使非极性烯烃和极性烯烃共聚合，其由下式（ IV）：其中M'是选自元素周期表第4,5,6和11族的过渡金属原子，m是1至6的整数，A是-O - ， - Si-，-Se-， - N（R6） - ，n为满足M'的化合价的数，R 1〜R 4，R 6为氢原子，卤素原子，烃基等，X为卤素原子，氧原子，烃基等，以及选自有机金属化合物（B-1），有机铝氧化合物（B-2）和离子电离化合物（B-3）中的至少一种化合物（B）。因此，该方法能够获得在温和聚合条件下具有优异性能的极性烯烃共聚物。

19. 发明授权

US06399724B1 Catalyst for olefin polymerization and method of polymerizing olefin 有权
标题翻译：用于烯烃聚合的催化剂和烯烃聚合方法
公开(公告)号：US06399724B1
公开(公告)日：2002-06-04
申请号：US09424971
申请日：1999-12-03
申请人： Shigekazu Matsui , Masatoshi Nitabaru , Kazutaka Tsuru , Terunori Fujita , Yasuhiko Suzuki , Yukihiro Takagi , Hidetsugu Tanaka
发明人： Shigekazu Matsui , Masatoshi Nitabaru , Kazutaka Tsuru , Terunori Fujita , Yasuhiko Suzuki , Yukihiro Takagi , Hidetsugu Tanaka
IPC分类号： C08F444
CPC分类号： C08F10/00 , C08F110/02 , C08F4/659 , C08F2500/17 , C08F4/64051 , C08F4/64044 , C08F4/64048 , C08F4/6411 , C08F4/6412 , C08F4/7008 , C08F4/7054 , C08F4/64113 , C08F4/64148 , C08F4/64151 , C08F4/64141
摘要： The present invention is intended to provide an olefin polymerization catalyst comprising a novel transition metal compound and having an excellent olefin polymerization activity and to provide a process for olefin polymerization.
摘要翻译：本发明旨在提供一种包含新型过渡金属化合物并具有优异的烯烃聚合活性并提供烯烃聚合方法的烯烃聚合催化剂。

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