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1. 发明授权

US08568665B2 Catalyst structure and hydrogenation/dehydrogenation reaction module using the same catalyst structure 有权
标题翻译：催化剂结构和氢化/脱氢反应模块采用相同的催化剂结构
公开(公告)号：US08568665B2
公开(公告)日：2013-10-29
申请号：US13123913
申请日：2010-12-28
申请人： Takayuki Seo , Tsuneo Akiura , Masaru Ichikawa
发明人： Takayuki Seo , Tsuneo Akiura , Masaru Ichikawa
IPC分类号： B01J8/02 , B01J35/02 , B01J19/00 , B01J8/00 , B01J23/00 , B01J23/02
CPC分类号： B01J10/007 , B01J19/2415 , B01J19/2425 , B01J21/04 , B01J21/063 , B01J23/42 , B01J23/6522 , B01J23/6527 , B01J23/72 , B01J23/74 , B01J23/745 , B01J23/755 , B01J35/0013 , B01J35/023 , B01J35/026 , B01J35/06 , B01J37/0203 , B01J37/0207 , B01J37/0211 , B01J37/0225 , B01J2219/00132 , B01J2219/00139 , B01J2219/00159 , C01B3/0015 , C01B3/24 , C01B2203/0266 , C01B2203/1252 , Y02E60/328
摘要： A catalyst structure 1 used for hydrogenation reaction or dehydrogenation reaction is characterized by the inclusion of a first coiled catalytic wire body 4 formed by coiling a catalytic wire in which a catalytic material is supported on the surface of a metallic core material, and a second catalytic member 5 disposed on the inner surface side and/or outer surface side of the coiled catalytic wire body 4.
摘要翻译：用于氢化反应或脱氢反应的催化剂结构1的特征在于，包括通过将催化材料卷绕在金属芯材表面上的催化丝线形成的第一卷绕催化丝体4和第二催化剂设置在线圈状催化线体4的内表面侧和/或外表面侧的构件5。

2. 发明授权

US09180438B2 Wire catalyst for hydrogenation/dehydrogenation reaction and manufacturing method therefor 有权
标题翻译：用于氢化/脱氢反应的丝催化剂及其制备方法
公开(公告)号：US09180438B2
公开(公告)日：2015-11-10
申请号：US14202978
申请日：2014-03-10
申请人： NIPPON SEISEN CO., LTD. , Masaru Ichikawa
发明人： Masaru Ichikawa , Yoshinori Tanimoto , Tsuneo Akiura
IPC分类号： B01J37/12 , B01J35/10 , B01J23/89 , B01J21/04 , B01J21/06 , B01J23/42 , B01J23/652 , B01J23/656 , B01J23/755 , B01J23/86 , B01J35/00 , B01J35/02 , B01J35/06 , B01J37/02 , B01J37/34
CPC分类号： B01J23/8993 , B01J21/04 , B01J21/063 , B01J21/066 , B01J23/42 , B01J23/6525 , B01J23/6527 , B01J23/6567 , B01J23/755 , B01J23/866 , B01J23/892 , B01J35/0006 , B01J35/026 , B01J35/06 , B01J37/0215 , B01J37/0225 , B01J37/342 , Y10T29/49986
摘要： A wire catalyst for hydrogenation reaction and/or dehydrogenation reaction comprises a metallic core and an oxide surface layer covering at least part of the surface thereof. The metallic core is electrically conductive so that the metallic core itself can generate heat by directly passing an electric current therethrough or electromagnetic induction. The oxide surface layer is made of an oxide of a metallic element constituting the metallic core. The oxide surface layer is provided with a porous structure having pores opening at the surface of the oxide surface layer. The catalytic material is supported in the pores of the oxide surface layer. When a shaped wire catalyst is manufactured, the shaping into a specific shape is made before the oxide surface layer having the porous structure is formed and the catalytic material is supported thereon.
摘要翻译：用于氢化反应和/或脱氢反应的线催化剂包括覆盖其表面的至少一部分的金属芯和氧化物表面层。金属芯是导电的，使得金属芯本身可以通过直接通过电流或电磁感应来产生热量。氧化物表面层由构成金属芯的金属元素的氧化物构成。氧化物表面层设置有在氧化物表面层的表面开口的多孔结构。催化材料负载在氧化物表面层的孔中。当制造成形网状催化剂时，在形成具有多孔结构的氧化物表面层之前进行成形为特定形状，并且催化材料被支撑在其上。

3. 发明申请

US20140194273A1 WIRE CATALYST FOR HYDROGENATION/DEHYDROGENATION REACTION AND MANUFACTURING METHOD THEREFOR 审中-公开
标题翻译：用于氢化/脱氢反应的线路催化剂及其制造方法
公开(公告)号：US20140194273A1
公开(公告)日：2014-07-10
申请号：US14202978
申请日：2014-03-10
申请人： Masaru ICHIKAWA , NIPPON SEISEN CO., LTD.
发明人： Masaru ICHIKAWA , Yoshinori TANIMOTO , Tsuneo AKIURA
IPC分类号： B01J23/89
CPC分类号： B01J23/8993 , B01J21/04 , B01J21/063 , B01J21/066 , B01J23/42 , B01J23/6525 , B01J23/6527 , B01J23/6567 , B01J23/755 , B01J23/866 , B01J23/892 , B01J35/0006 , B01J35/026 , B01J35/06 , B01J37/0215 , B01J37/0225 , B01J37/342 , Y10T29/49986
摘要： A wire catalyst for hydrogenation reaction and/or dehydrogenation reaction comprises a metallic core and an oxide surface layer covering at least part of the surface thereof. The metallic core is electrically conductive so that the metallic core itself can generate heat by directly passing an electric current therethrough or electromagnetic induction. The oxide surface layer is made of an oxide of a metallic element constituting the metallic core. The oxide surface layer is provided with a porous structure having pores opening at the surface of the oxide surface layer. The catalytic material is supported in the pores of the oxide surface layer. When a shaped wire catalyst is manufactured, the shaping into a specific shape is made before the oxide surface layer having the porous structure is formed and the catalytic material is supported thereon.
摘要翻译：用于氢化反应和/或脱氢反应的线催化剂包括覆盖其表面的至少一部分的金属芯和氧化物表面层。金属芯是导电的，使得金属芯本身可以通过直接通过电流或电磁感应来产生热量。氧化物表面层由构成金属芯的金属元素的氧化物构成。氧化物表面层设置有在氧化物表面层的表面开口的多孔结构。催化材料负载在氧化物表面层的孔中。当制造成形网状催化剂时，在形成具有多孔结构的氧化物表面层之前进行成形为特定形状，并且催化材料被支撑在其上。

4. 发明授权

US08709967B2 Wire catalyst for hydrogenation/dehydrogenation reaction and manufacturing method therefor 有权
标题翻译：用于氢化/脱氢反应的丝催化剂及其制备方法
公开(公告)号：US08709967B2
公开(公告)日：2014-04-29
申请号：US13095522
申请日：2011-04-27
申请人： Masaru Ichikawa , Yoshinori Tanimoto , Tsuneo Akiura
发明人： Masaru Ichikawa , Yoshinori Tanimoto , Tsuneo Akiura
IPC分类号： B01J21/04
CPC分类号： B01J23/8993 , B01J21/04 , B01J21/063 , B01J21/066 , B01J23/42 , B01J23/6525 , B01J23/6527 , B01J23/6567 , B01J23/755 , B01J23/866 , B01J23/892 , B01J35/0006 , B01J35/026 , B01J35/06 , B01J37/0215 , B01J37/0225 , B01J37/342 , Y10T29/49986
摘要： A wire catalyst for hydrogenation reaction and/or dehydrogenation reaction comprises a metallic core and an oxide surface layer covering at least part of the surface thereof. The metallic core is electrically conductive so that the metallic core itself can generate heat by directly passing an electric current therethrough or electromagnetic induction. The oxide surface layer is made of an oxide of a metallic element constituting the metallic core. The oxide surface layer is provided with a porous structure having pores opening at the surface of the oxide surface layer. The catalytic material is supported in the pores of the oxide surface layer. When a shaped wire catalyst is manufactured, the shaping into a specific shape is made before the oxide surface layer having the porous structure is formed and the catalytic material is supported thereon.
摘要翻译：用于氢化反应和/或脱氢反应的线催化剂包括覆盖其表面的至少一部分的金属芯和氧化物表面层。金属芯是导电的，使得金属芯本身可以通过直接通过电流或电磁感应来产生热量。氧化物表面层由构成金属芯的金属元素的氧化物构成。氧化物表面层设置有在氧化物表面层的表面开口的多孔结构。催化材料负载在氧化物表面层的孔中。当制造成形网状催化剂时，在形成具有多孔结构的氧化物表面层之前进行成形为特定形状，并且催化材料被支撑在其上。

5. 发明申请

US20080312483A1 Process for Producing Aromatic Hydrocarbon and Hydrogen 有权
标题翻译：生产芳香烃和氢的方法
公开(公告)号：US20080312483A1
公开(公告)日：2008-12-18
申请号：US11658399
申请日：2005-07-28
申请人： Masaru Ichikawa , Ryoichi Kojima , Yuji Ogawa , Masamichi Kuramoto
发明人： Masaru Ichikawa , Ryoichi Kojima , Yuji Ogawa , Masamichi Kuramoto
IPC分类号： C07C5/367
CPC分类号： B01J37/0009 , B01J29/48 , B01J29/90 , B01J37/0018 , B01J38/10 , B01J2229/18 , B01J2229/42 , C01B3/26 , C01B2203/0277 , C01B2203/1041 , C01B2203/1047 , C01B2203/1082 , C01B2203/1241 , C07C2/84 , Y02P20/584 , Y02P20/588 , Y10S585/943
摘要： A process for producing aromatic hydrocarbons and hydrogen, in which a lower hydrocarbons-containing feedstock gas is reformed by being supplied to and being brought into contact with a catalyst under high temperature conditions thereby forming aromatic hydrocarbons and hydrogen. The method includes the steps of (a) supplying a hydrogen gas together with the feedstock gas during a supply of the feedstock gas; and (b) suspending the supply of the feedstock gas for a certain period of time while keeping a condition of a supply of the hydrogen gas. The catalyst is exemplified by a metallo-silicate carrying molybdenum and a metallo-silicate carrying molybdenum and rhodium. An amount of the hydrogen gas supplied together with the feedstock gas is set to be preferably larger than 2% and smaller than 10%, more preferably within a range of from 4 to 8%, much more preferably 8%. As a pretreatment for a reforming reaction by which aromatic hydrocarbons and hydrogen are formed, the catalyst is increased in temperature and kept at the temperature for a certain period of time while a gas containing methane and hydrogen is supplied thereto.
摘要翻译：一种生产芳烃和氢的方法，其中含低级烃的原料气体通过在高温条件下被供给并与催化剂接触而重整，从而形成芳族烃和氢。该方法包括以下步骤：（a）在原料气体的供给期间，与原料气体一起供应氢气; 和（b）在保持氢气供应状态的同时暂停供应原料气一段时间。催化剂的例子是载有钼的金属硅酸盐和携带钼和铑的金属硅酸盐。与原料气体一起供给的氢气的量优选设定为2％以上且小于10％，更优选在4〜8％的范围内，进一步优选为8％以下。作为形成芳烃和氢的重整反应的预处理，催化剂的温度升高并在该温度下保持一段时间，同时向其中供给含有甲烷和氢气的气体。

6. 发明申请

US20120164034A1 CATALYST STRUCTURE AND HYDROGENATION/DEHYDROGENATION REACTION MODULE USING THE SAME CATALYST STRUCTURE 有权
标题翻译：使用相同催化剂结构的催化剂结构和加氢/脱氢反应模块
公开(公告)号：US20120164034A1
公开(公告)日：2012-06-28
申请号：US13123913
申请日：2010-12-28
申请人： Takayuki Seo , Tsuneo Akiura , Masaru Ichikawa
发明人： Takayuki Seo , Tsuneo Akiura , Masaru Ichikawa
IPC分类号： B01J19/00 , B01J27/053 , B01J23/755 , B01J35/02
CPC分类号： B01J10/007 , B01J19/2415 , B01J19/2425 , B01J21/04 , B01J21/063 , B01J23/42 , B01J23/6522 , B01J23/6527 , B01J23/72 , B01J23/74 , B01J23/745 , B01J23/755 , B01J35/0013 , B01J35/023 , B01J35/026 , B01J35/06 , B01J37/0203 , B01J37/0207 , B01J37/0211 , B01J37/0225 , B01J2219/00132 , B01J2219/00139 , B01J2219/00159 , C01B3/0015 , C01B3/24 , C01B2203/0266 , C01B2203/1252 , Y02E60/328
摘要： A catalyst structure 1 used for hydrogenation reaction or dehydrogenation reaction is characterized by the inclusion of a first coiled catalytic wire body 4 formed by coiling a catalytic wire in which a catalytic material is supported on the surface of a metallic core material, and a second catalytic member 5 disposed on the inner surface side and/or outer surface side of the coiled catalytic wire body 4.
摘要翻译：用于氢化反应或脱氢反应的催化剂结构1的特征在于，包括通过将催化材料卷绕在金属芯材表面上的催化丝线形成的第一卷绕催化丝体4和第二催化剂设置在线圈状催化线体4的内表面侧和/或外表面侧的构件5。

7. 发明申请

US20090240093A1 PROCESS FOR PRODUCTION OF AROMATIC COMPOUND 有权
标题翻译：芳香化合物生产工艺
公开(公告)号：US20090240093A1
公开(公告)日：2009-09-24
申请号：US12067148
申请日：2006-09-29
申请人： Masaru Ichikawa , Ryoichi Kojima , Yuji Ogawa , Masamichi Kuramoto
发明人： Masaru Ichikawa , Ryoichi Kojima , Yuji Ogawa , Masamichi Kuramoto
IPC分类号： C07C2/00
CPC分类号： C07C2/76 , C07C15/02
摘要： An aromatic compound, particularly benzene, is stably produced in the presence of a catalyst from a lower hydrocarbon having 2 or more carbon atoms, particularly from an ethane-containing gas composition such as ethane gas and natural gas. Disclosed is a process for producing an aromatic compound by reacting ethane or an ethane-containing raw gas in the presence of a catalyst. The catalyst may comprise molybdenum carried on metallosilicate such as H-type ZSM-5H or H-type MCM-22. In the reaction, the temperature is from 550 to 750° C., preferably not lower than 600° C. and not higher than 680° C. Additionally, the raw gas further contains methane and hydrogen is added thereto, thereby improving the production efficiency and stability.
摘要翻译：在具有2个或更多个碳原子的低级烃的催化剂的存在下，特别是从含乙烷的气体组合物如乙烷气体和天然气中稳定地制备芳族化合物，特别是苯。公开了一种在催化剂存在下使乙烷或含乙烷的原料气体反应生成芳族化合物的方法。催化剂可以包括载在金属硅酸盐上的钼，例如H型ZSM-5H或H型MCM-22。在该反应中，温度为550〜750℃，优选为600℃以上且不高于680℃。此外，原料气体还含有甲烷，向其中添加氢，从而提高生产效率和稳定性。

8. 发明申请

US20090076316A1 PROCESS FOR PRODUCTION OF AROMATIC HYDROCARBON 审中-公开
标题翻译：生产芳香烃的方法
公开(公告)号：US20090076316A1
公开(公告)日：2009-03-19
申请号：US11816068
申请日：2006-02-08
申请人： Masaru Ichikawa , Ryoichi Kojima , Satoshi Kikuchi
发明人： Masaru Ichikawa , Ryoichi Kojima , Satoshi Kikuchi
IPC分类号： C07C2/52
CPC分类号： B01J29/076 , B01J29/48 , B01J29/7815 , B01J29/7876 , B01J2229/12 , B01J2229/18 , B01J2229/32 , C07C2/84 , C07C2529/48 , C07C2529/78 , C07C15/02
摘要： A process for producing an aromatic hydrocarbon, comprises heating the hydrocarbon in the presence of a catalyst carrying a molybdenum compound or a rhenium compound on a metallosilicate carrier modified with a silicon compound, a sodium compound or a calcium compound. The silicon compound is a silane compound having a basic group selected from amino, alkylamino and pyridyl groups and an organic group of a size equal to or greater than the pore size of the metallosilicate and selected from trialkoxy and triphenyl groups and the sodium compound or the calcium compound is a compound having an organic group of a size equal to or greater than the pore size of the metallosilicate and selected from crown ether, hexafluoropentanedione and acetylacetonate. The silane compound, the sodium compound or the calcium compound is modified so as to make an oxide thereof by impregnating the metallosilicate carrier with it and subsequently heat-treating it in an oxygen-containing atmosphere.
摘要翻译：一种制备芳族烃的方法，包括在载有钼化合物或铼化合物的催化剂存在下，在用硅化合物，钠化合物或钙化合物改性的金属硅酸盐载体上加热烃。硅化合物是具有选自氨基，烷基氨基和吡啶基的碱性基团的硅烷化合物和等于或大于金属硅酸盐孔径的有机基团，选自三烷氧基和三苯基，并且钠化合物或钙化合物是具有等于或大于金属硅酸盐孔径的有机基团并选自冠醚，六氟戊二酮和乙酰丙酮化物的化合物。对硅烷化合物，钠化合物或钙化合物进行改性以通过用其浸渍金属硅酸盐载体并随后在含氧气氛中进行热处理来制备其氧化物。

9. 发明授权

US08057559B2 Hydrogen generator and hydrogenation apparatus 有权
标题翻译：氢发生器和加氢装置
公开(公告)号：US08057559B2
公开(公告)日：2011-11-15
申请号：US12281869
申请日：2007-01-09
申请人： Masaru Ichikawa , Katsumori Tanabe , Masashi Sakuramoto , Satoru Kikuchi , Yukimitsu Mita
发明人： Masaru Ichikawa , Katsumori Tanabe , Masashi Sakuramoto , Satoru Kikuchi , Yukimitsu Mita
IPC分类号： B01J7/00 , B01J19/00
CPC分类号： F17C11/005 , B01J8/0411 , B01J8/0496 , B01J12/007 , B01J15/005 , B01J21/04 , B01J23/42 , B01J35/04 , B01J37/348 , B01J2208/00123 , B01J2208/00309 , B01J2208/00504 , B01J2208/0053 , B01J2219/00078 , B01J2219/00117 , B01J2219/00157 , B01J2219/00159 , B01J2219/00768 , C01B3/26 , C01B2203/0277 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/1023 , C01B2203/1035 , Y02E60/321 , Y02E60/324 , Y02P20/128
摘要： The efficiency of dehydrogenation and that of hydrogenation are improved. A hydrogen generator for generating hydrogen by dehydrogenation of organic hydrides in the presence of a catalyst is characterized by comprising a reactor vessel (10) of a multi-tubular structure having a region (12) for supplying fuel to generate heat necessary for dehydrogenation, the region containing a combustion catalyst for combusting fuel, and a region (11) containing a dehydrogenation catalyst necessary for dehydrogenation, the regions being arranged radially side by side with a wall separating them. A hydrogenation apparatus which synthesizes organic hydrides by way of hydrogenation of unsaturated hydrocarbons in the presence of a catalyst is characterized by comprising a reactor vessel (10) of a multi-tubular structure having a region (12) for removing the heat generated by hydrogenation and a region (11) containing a hydrogenation catalyst necessary for hydrogenation, the regions being arranged radially side by side with a wall separating them.
摘要翻译：脱氢效率和氢化效率提高。一种用于在催化剂存在下通过有机氢化物脱氢产生氢的氢发生器的特征在于包括具有用于供应燃料以产生脱氢所需热量的区域（12）的多管状结构的反应器容器（10），含有用于燃烧燃料的燃烧催化剂的区域和含有脱氢所需的脱氢催化剂的区域（11），所述区域与其分离的壁径向并排配置。通过在催化剂存在下通过氢化不饱和烃合成有机氢化物的氢化装置的特征在于包括具有用于除去由氢化产生的热量的区域（12）的多管状结构的反应器容器（10）含有氢化催化剂所需的氢化催化剂的区域（11），所述区域与其分离的壁径向并排配置。

10. 发明申请

US20110036310A1 HYDROGEN SUPPLY UNIT FOR INTERNAL COMBUSTION ENGINE AND METHOD OF OPERATING INTERNAL COMBUSTION ENGINE 审中-公开
标题翻译：用于内燃机的氢气供应单元和内燃机的运行方法
公开(公告)号：US20110036310A1
公开(公告)日：2011-02-17
申请号：US12867678
申请日：2008-07-04
申请人： Masaru Ichikawa , Akira Koikeda , Kunio Komori , Satoru Kikuchi , Takeshiro Ito
发明人： Masaru Ichikawa , Akira Koikeda , Kunio Komori , Satoru Kikuchi , Takeshiro Ito
IPC分类号： F02B43/08
CPC分类号： F01N5/02 , F01N3/103 , F01N3/2053 , F01N3/206 , F01N3/30 , F01N3/36 , F01N13/009 , F01N2610/04 , F02D19/0644 , F02D19/0671 , F02D19/0684 , F02D19/0692 , F02M25/12 , F02M27/02 , Y02T10/121 , Y02T10/16 , Y02T10/36
摘要： An efficient internal combustion engine jointly using hydrogen obtained by dehydrogenation of a hydrogen supply mass. There is disclosed a hydrogen supply unit for internal combustion engine comprising hydrogen separating means, storage means for storage of separated hydrogen, means for storage of dehydrogenation products and means for addition supply of produced hydrogen to a fuel source. The hydrogen separating means for separating produced hydrogen from dehydrogenation products, includes a dehydrogenation reactor for production of hydrogen from a hydrogen supply mass using at least either the hydrogen supply mass or a hydrocarbon fuel as the fuel source, which dehydrogenation reactor on its one face is provided with a hydrogen production section bearing a dehydrogenation catalyst and on its other face is provided with an oxidation reaction section allowing passage of an exhaust from the internal combustion engine and bearing an oxidation catalyst for oxidizing any dehydrogenation products from the hydrogen supply mass to thereby bring about heat generation.
摘要翻译：联合使用通过氢供给物质脱氢获得的氢的有效内燃机。公开了一种用于内燃机的氢气供应单元，其包括氢气分离装置，用于储存分离的氢的储存装置，用于储存脱氢产物的装置和用于向燃料源添加产生的氢气的装置。用于从脱氢产物中分离生成的氢的氢分离装置包括使用至少氢供体或烃燃料作为燃料源从氢供应质量产生氢的脱氢反应器，其一面为脱氢反应器设置有带有脱氢催化剂的氢气生产部分，并且在另一个表面上设置有氧化反应部分，其允许来自内燃机的排气通过，并具有用于氧化来自氢气供应物质的任何脱氢产物的氧化催化剂，从而带来关于发热。

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