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1. 发明申请

US20160251331A1 Metal-conjugated microporous polymers 有权
标题翻译：金属共轭微孔聚合物
公开(公告)号：US20160251331A1
公开(公告)日：2016-09-01
申请号：US14980238
申请日：2015-12-28
申请人： DALIAN INSTITUTE OF CHEMICAL PHYSICS, CHINESE ACADEMY OF SCIENCES
发明人： Weiqiao DENG , Yong XIE , Xiaohuan LIU
IPC分类号： C07D317/36 , B01J31/16
CPC分类号： C07D317/36 , B01J31/1691 , B01J31/2243 , B01J31/2295 , B01J2231/341 , B01J2531/0252 , B01J2531/16 , B01J2531/26 , B01J2531/31 , B01J2531/62 , B01J2531/845
摘要： A catalyst which can catalyze ring-addition reaction of CO2 and an alkylene oxide at 0˜180° C. under 0.1˜8.0 MPa to produce a corresponding cyclic carbonate, and the preparation thereof. The catalyst is a conjugated microporous macromolecule polymer complexed with cobalt, chromium, zinc, copper or aluminium, and by using the macromolecule catalyst complexed with different metals to catalyze the reaction of CO2 and alkylene oxide at normal temperature and normal pressure, a yield of the corresponding cyclic carbonate of 35%-90% can be obtained. The catalyst is easy to recover and the re-use of the catalyst has no influence on the yield; additionally, the yield can reach over 90% by controlling the reaction conditions.
摘要翻译：一种催化剂，其可以在0〜180℃，0.1〜8.0MPa下催化CO 2和环氧烷烃的加成反应，生成相应的环状碳酸酯及其制备。该催化剂是与钴，铬，锌，铜或铝络合的共轭微孔高分子聚合物，通过使用与不同金属配合的高分子催化剂催化常温常压下的CO 2和氧化烯的反应，可以获得35％-90％的相应的环状碳酸酯。催化剂易于回收，催化剂的再利用对产率无影响; 此外，通过控制反应条件，产率可以达到90％以上。

2. 发明申请

US20110015060A1 Catalyst for Desulfurization and Deodorization of Gasoline and Method for Preparation of the Same and Use Thereof 有权
标题翻译：汽油脱硫除臭催化剂及其制备方法及用途
公开(公告)号：US20110015060A1
公开(公告)日：2011-01-20
申请号：US12933313
申请日：2008-11-20
申请人： Can Li , Zongxuan Jiang , Yongna Zhang , Hongying Lv , Boyu Zhang
发明人： Can Li , Zongxuan Jiang , Yongna Zhang , Hongying Lv , Boyu Zhang
IPC分类号： B01J31/18
CPC分类号： B01J31/1805 , B01J27/188 , B01J31/0239 , B01J2231/62 , C10G25/003 , C10G27/12
摘要： A catalyst for the desulfurization and deodorization of gasoline, which is expressed by the formula: QlBmHn[AxMyOz](1+m+n)−, where: Q denotes a quaternary ammonium cation consisting of R1R2R3R4N+, in which R1, R2, R3, and R4 each denotes independently a C1 to C20 saturated alkyl group, respectively, provided that at least one of R1, R2, R3, and R4 denotes a C4 to C20 saturated alkyl group; B denotes a metal cation of Na+ or/and K+; H denotes a hydrogen atom; A denotes a central atom of B, P, As, Si or Al; M denotes a coordinated atom of W or Mo; O denotes an oxygen atom; 1≦l≦10, 0≦m≦3, 0≦n≦3, l+m+n≦14, x=1 or 2, 9≦y≦18, 34≦z≦62, and l, m, n, y and z all are integers. A method of the desulfurization and deodorization of gasoline by using the catalyst comprises the steps of: mixing the catalyst and an aqueous solution of hydrogen peroxide, and then adding the gasoline to react them with stirring under conditions of 25 to 90° C. and 0.1 to 1 MPa for 10 to 180 min. An odorless gasoline can be obtained through settlement or centrifugation, and the catalyst is recovered.
摘要翻译：一种用于汽油脱硫除臭的催化剂，其由下式表示：QlBmHn [AxMyOz]（1 + m + n） - ，其中：Q表示由R1R2R3R4N +组成的季铵阳离子，其中R1，R2，R3，并且R 4各自独立地表示C1〜C20饱和烷基，条件是R 1，R 2，R 3和R 4中的至少一个表示C 4至C 20饱和烷基; B表示Na +或/和K +的金属阳离子; H表示氢原子; A表示B，P，As，Si或Al的中心原子; M表示W或Mo的配位原子; O表示氧原子; 1＆nlE; l＆nlE; 10,0＆nlE; m＆nlE; 3,0＆nlE; n＆nlE; 3,1 + m + n＆nlE; 14，x = 1或2,9和nlE; y＆nlE; 18,34＆nlE; z＆nlE; 62和l，m，n ，y和z都是整数。通过使用催化剂对汽油进行脱硫除臭的方法包括以下步骤：将催化剂和过氧化氢水溶液混合，然后加入汽油使其在25〜90℃，0.1〜至1MPa 10至180分钟。可以通过沉降或离心获得无臭汽油，回收催化剂。

3. 发明申请

US20180244599A1 METHOD FOR PREPARING ACETIC ACID BY CARBONYLATION OF METHANOL 审中-公开
公开(公告)号：US20180244599A1
公开(公告)日：2018-08-30
申请号：US15758572
申请日：2015-12-08
申请人： Dalian Institute of Chemical Physics, Chinese Academy of Sciences
发明人： Youming NI , Wenliang ZHU , Lei SHI , Hongchao LIU , Yong LIU , Zhongmin LIU
IPC分类号： C07C51/12 , C07C53/08 , B01J29/18 , B01J29/65 , B01J29/24 , B01J29/67 , B01J31/26 , B01J31/02 , B01J37/30 , B01J37/08 , B01J37/00 , B01J37/02
CPC分类号： C07C51/12 , B01J29/00 , B01J29/18 , B01J29/24 , B01J29/65 , B01J29/67 , B01J31/0254 , B01J31/26 , B01J37/0072 , B01J37/0203 , B01J37/0207 , B01J37/08 , B01J37/30 , B01J2229/183 , C07C53/08 , C07C5/08
摘要： The present invention provides a method for preparing acetic acid by carbonylation of methanol, which comprises: passing a raw material containing methanol, carbon monoxide and water through a reaction region loaded with a catalyst containing an acidic molecular sieve with an adsorbed organic amine, and carrying out a reaction under the following conditions to prepare acetic acid. The method in the present invention offers high acetic acid selectivity and good catalyst stability. The catalyst in the present invention does not contain noble metals such as rhodium or iridium, and does not need additional agent containing iodine, and thus does not generate a strong corrosive hydroiodic acid and the like.

4. 发明授权

US08501657B2 Catalyst for desulfurization and deodorization of gasoline and method for preparation of the same and use thereof 有权
标题翻译：用于汽油脱硫除臭的催化剂及其制备方法及其应用
公开(公告)号：US08501657B2
公开(公告)日：2013-08-06
申请号：US12933313
申请日：2008-11-20
申请人： Can Li , Zongxuan Jiang , Yongna Zhang , Hongying Lv , Boyu Zhang
发明人： Can Li , Zongxuan Jiang , Yongna Zhang , Hongying Lv , Boyu Zhang
IPC分类号： B01J31/18 , C10L1/04 , C10G45/00 , C10G29/00 , C10G29/08
CPC分类号： B01J31/1805 , B01J27/188 , B01J31/0239 , B01J2231/62 , C10G25/003 , C10G27/12
摘要： A catalyst for the desulfurization and deodorization of gasoline, which is expressed by the formula: QlBmHn[AxMyOz](1+m+n)−, where: Q denotes a quaternary ammonium cation consisting of R1R2R3R4N+, in which R1, R2, R3, and R4 each denotes independently a C1 to C20 saturated alkyl group, respectively, provided that at least one of R1, R2, R3, and R4 denotes a C4 to C20 saturated alkyl group; B denotes a metal cation of Na+ or/and K+; H denotes a hydrogen atom; A denotes a central atom of B, P, As, Si or Al; M denotes a coordinated atom of W or Mo; O denotes an oxygen atom; 1≦l≦10, 0≦m≦3, 0≦n≦3, l+m+n≦14, x=1 or 2, 9≦y≦18, 34≦z≦62, and l, m, n, y and z all are integers. A method of the desulfurization and deodorization of gasoline by using the catalyst comprises the steps of: mixing the catalyst and an aqueous solution of hydrogen peroxide, and then adding the gasoline to react them with stirring under conditions of 25 to 90° C. and 0.1 to 1 MPa for 10 to 180 min. An odorless gasoline can be obtained through settlement or centrifugation, and the catalyst is recovered.
摘要翻译：一种用于汽油脱硫除臭的催化剂，其由下式表示：QlBmHn [AxMyOz]（1 + m + n） - ，其中：Q表示由R1R2R3R4N +组成的季铵阳离子，其中R1，R2，R3，并且R 4各自独立地表示C1〜C20饱和烷基，条件是R 1，R 2，R 3和R 4中的至少一个表示C 4至C 20饱和烷基; B表示Na +或/和K +的金属阳离子; H表示氢原子; A表示B，P，As，Si或Al的中心原子; M表示W或Mo的配位原子; O表示氧原子; 1 @ l @ 10，0 @ m @ 3，0 @ n @ 3，l + m + n @ 14，x = 1或2，9 @ y @ 18,34 @ z @ 62和l，m，n ，y和z都是整数。通过使用催化剂对汽油进行脱硫除臭的方法包括以下步骤：将催化剂和过氧化氢水溶液混合，然后加入汽油使其在25〜90℃，0.1〜至1MPa 10至180分钟。可以通过沉降或离心获得无臭汽油，回收催化剂。

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