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1. 发明申请

US20070015028A1 PROTON CONDUCTOR AND METHOD FOR MANUFACTURING THE SAME, AND ELECTROCHEMICAL DEVICE 失效
标题翻译：原型导体及其制造方法以及电化学装置
公开(公告)号：US20070015028A1
公开(公告)日：2007-01-18
申请号：US11533674
申请日：2006-09-20
申请人： Yong Li , Koichiro Hinokuma
发明人： Yong Li , Koichiro Hinokuma
IPC分类号： H01M8/10 , C08J5/20
CPC分类号： H01B1/122 , B82Y30/00 , H01M6/181 , H01M8/1018 , H01M2300/0082 , Y02P70/56
摘要： A proton conductor, a method for manufacturing the same, and an electrochemical device using the proton conductor are provided. The proton conductor includes a carbon derivative which has a carbon material selected from the group consisting of a fullerene molecule, a cluster consisting essentially of carbon, a fiber-shaped carbon anPlease do not hesitate to contact us with any questions d a tube-regarding this matter shaped carbon, and mixtures thereof, and at least a proton dissociative group, the proton dissociative group being bonded to the carbon material via a cyclic structure of tricyclic or more. The method includes the steps of obtaining the carbon derivative, hydrolyzing the derivative with alkali hydroxide, subjecting the hydrolyzed product to ion exchange, and forming a group with proton-dissociating properties.
摘要翻译：提供质子导体，其制造方法和使用该质子导体的电化学装置。质子导体包括碳衍生物，其具有选自富勒烯分子，基本上由碳组成的簇的碳材料，纤维状碳。请勿随时与我们联系任何关于该事项的问题和至少一个质子解离基团，质子解离基团通过三环或更多的环状结构键合到碳材料上。该方法包括以下步骤：获得碳衍生物，用碱金属氢氧化物水解衍生物，使水解产物进行离子交换，并形成质子解离性质的基团。

2. 发明授权

US07578990B2 Proton conductor and method for manufacturing the same, and electrochemical device 失效
标题翻译：质子导体及其制造方法及电化学装置
公开(公告)号：US07578990B2
公开(公告)日：2009-08-25
申请号：US11533674
申请日：2006-09-20
申请人： Yong Ming Li , Koichiro Hinokuma
发明人： Yong Ming Li , Koichiro Hinokuma
IPC分类号： B01J19/08 , C01B31/02
CPC分类号： H01B1/122 , B82Y30/00 , H01M6/181 , H01M8/1018 , H01M2300/0082 , Y02P70/56
摘要： A proton conductor, a method for manufacturing the same, and an electrochemical device using the proton conductor are provided. The proton conductor includes a carbon derivative which has a carbon material selected from the group consisting of a fullerene molecule, a cluster consisting essentially of carbon, a fiber-shaped carbon anPlease do not hesitate to contact us with any questions d a tube-regarding this matter shaped carbon, and mixtures thereof, and at least a proton dissociative group, the proton dissociative group being bonded to the carbon material via a cyclic structure of tricyclic or more. The method includes the steps of obtaining the carbon derivative, hydrolyzing the derivative with alkali hydroxide, subjecting the hydrolyzed product to ion exchange, and forming a group with proton-dissociating properties.
摘要翻译：提供质子导体，其制造方法和使用该质子导体的电化学装置。质子导体包括碳衍生物，其具有选自富勒烯分子，基本上由碳组成的簇的碳材料，纤维状碳。请勿随时与我们联系任何关于该事项的问题和至少一个质子解离基团，质子解离基团通过三环或更多的环状结构键合到碳材料上。该方法包括以下步骤：获得碳衍生物，用碱金属氢氧化物水解衍生物，使水解产物进行离子交换，并形成质子解离性质的基团。

3. 发明授权

US07157183B2 Proton conductor, production method thereof, and electrochemical device using the same 有权
标题翻译：质子导体及其制造方法及使用其的电化学装置
公开(公告)号：US07157183B2
公开(公告)日：2007-01-02
申请号：US10171935
申请日：2002-06-14
申请人： Koichiro Hinokuma , Björn Pietzak , Constance Gertrud Rost , Masafumi Ata
发明人： Koichiro Hinokuma , Björn Pietzak , Constance Gertrud Rost , Masafumi Ata
IPC分类号： H01M6/04 , C01B31/00 , D01F9/12
CPC分类号： H01M6/18 , B82Y30/00 , B82Y40/00 , C01B32/15 , C01B32/152 , H01B1/04 , H01B1/122 , H01M4/8605 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M8/1048 , H01M10/0562 , H01M10/347 , H01M12/00 , H01M2300/0068 , H01M2300/0082 , H01M2300/0091 , Y02P70/56 , Y10S977/75 , Y10S977/752 , Y10S977/788 , Y10S977/842 , Y10S977/948
摘要： A proton conductor mainly contains a carbonaceous material derivative, such as, a fullerene derivative, a carbon cluster derivative, or a tubular carbonaceous material derivative in which groups capable of transferring protons, for example, —OH groups or —OSO3H groups are introduced to carbon atoms of the carbonaceous material derivative. The proton conductor is produced typically by compacting a powder of the carbonaceous material derivative. The proton conductor is usable, even in a dry state, in a wide temperature range including ordinary temperature. In particular, the proton conductor mainly containing the carbon cluster derivative is advantageous in increasing the strength and extending the selection range of raw materials. An electrochemical device, such as, a fuel cell, that employs the proton conductor is not limited by atmospheric conditions and can be of a small and simple construction. The proton conductor may contain a polymer in addition to the carbonaceous material derivative, which conductor can be formed, typically by extrusion molding, into a thin film having a large strength, a high gas permeation preventive ability, and a good proton conductivity.
摘要翻译：质子导体主要含有碳质材料衍生物，例如富勒烯衍生物，碳簇衍生物或管状碳质材料衍生物，其中能够转移质子的基团例如-OH基团或-OSO 3 H基团被引入碳质材料衍生物的碳原子。质子导体通常通过压实含碳材料衍生物的粉末来制备。质子导体即使在干燥状态下也可以在包括常温的宽温度范围内使用。特别地，主要含有碳簇衍生物的质子导体有利于提高强度并延长原料的选择范围。使用质子导体的诸如燃料电池的电化学装置不受大气条件限制，并且可以是小而简单的结构。质子导体除含碳材料衍生物之外还可以含有聚合物，该衍生物通常通过挤出成型形成具有大的强度，高透气性能和良好的质子传导性的薄膜。

4. 发明授权

US07128888B2 Proton conductor and method for manufacturing the same, and electrochemical device 有权
公开(公告)号：US07128888B2
公开(公告)日：2006-10-31
申请号：US10195235
申请日：2002-07-15
申请人： Yong Ming Li , Koichiro Hinokuma
发明人： Yong Ming Li , Koichiro Hinokuma
IPC分类号： B01J19/08 , C01B31/02
CPC分类号： H01B1/122 , B82Y30/00 , H01M6/181 , H01M8/1018 , H01M2300/0082 , Y02P70/56
摘要： A proton conductor, a method for manufacturing the same, and an electrochemical device using the proton conductor are provided. The proton conductor includes a carbon derivative which has a carbon material selected from the group consisting of a fullerene molecule, a cluster consisting essentially of carbon, a fiber-shaped carbon and a tube-shaped carbon, and mixtures thereof; and at least a proton dissociative group, the proton dissociative group being bonded to the carbon material via a cyclic structure of tricyclic or more. The method includes the steps of obtaining the carbon derivative, hydrolyzing the derivative with alkali hydroxide, subjecting the hydrolyzed product to ion exchange, and forming a group with proton-dissociating properties.

5. 发明授权

US09673481B2 Thin film solid state lithium ion secondary battery and method of manufacturing the same 有权
公开(公告)号：US09673481B2
公开(公告)日：2017-06-06
申请号：US13144625
申请日：2010-01-28
申请人： Yuichi Sabi , Katsunori Takahara , Hiroyuki Morioka , Tatsuya Furuya , Koichiro Hinokuma , Reina Ichikawa , Yui Senda , Momoe Adachi
发明人： Yuichi Sabi , Katsunori Takahara , Hiroyuki Morioka , Tatsuya Furuya , Koichiro Hinokuma , Reina Ichikawa , Yui Senda , Momoe Adachi
IPC分类号： H01M10/0525 , H01M2/02 , H01M4/131 , H01M4/136 , H01M6/40 , H01M10/0562 , H01M10/0585 , H01M10/05 , H01M10/054 , H01M10/12 , H01M4/1391 , H01M4/1397
CPC分类号： H01M10/0525 , H01M2/0212 , H01M4/131 , H01M4/136 , H01M4/1391 , H01M4/1397 , H01M6/40 , H01M10/05 , H01M10/054 , H01M10/0562 , H01M10/0585 , H01M10/126 , Y02P70/54 , Y10T29/49108 , Y10T29/49115
摘要： In one embodiment, a thin film solid state lithium ion secondary battery is able to be charged and discharged in the air and manufactured stably at a favorable yield. The thin film solid state lithium ion secondary battery has an electric insulating substrate formed from an organic resin, an inorganic insulating film provided on the substrate face, a cathode-side current collector film, a cathode active material film, a solid electrolyte film, an anode potential formation layer, and an anode-side current collector film. The cathode-side current collector film and/or the anode-side current collector film is formed on the inorganic insulating film face. The anode potential formation layer is a layer formed from the same material as that of the cathode active material film or a material different from that of the cathode active material film and is a layer provided for forming anode potential at the time of discharge.

6. 发明授权

US08007942B2 Ion-dissociative functional compound, method for production thereof, ionic conductor, and electrochemical device 失效
标题翻译：离子解离功能化合物，其制备方法，离子导体和电化学装置
公开(公告)号：US08007942B2
公开(公告)日：2011-08-30
申请号：US10567283
申请日：2004-08-04
申请人： Kazuaki Fukushima , Shuichi Takizawa , Koichiro Hinokuma , Atsushi Nishimoto , Kazuhiro Noda
发明人： Kazuaki Fukushima , Shuichi Takizawa , Koichiro Hinokuma , Atsushi Nishimoto , Kazuhiro Noda
IPC分类号： H01M6/18 , H01M8/10 , C07C313/00
CPC分类号： C07C309/24 , C07C311/48 , C07C2604/00 , C08J5/22 , C08J2327/12 , H01B1/122 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2300/0082 , Y02P70/56 , Y10S977/735
摘要： Disclosed herein are an ion-dissociative functional compound, a method for production thereof, an ionic conductor, and an electrochemical device, the ion-dissociative functional compound being thermally and chemically stable under the condition required of fuel cells and being suitable for use as a material such as protonic conductor in fuel cells.The proton-dissociative functional compound shown in FIG. 1A is composed of a fullerene C60 molecule and about 10 sulfonic acid groups —SO3H as proton-dissociative groups each attached to the fullerene through a difluoromethane group —CF2—. The proton-dissociative functional compound shown in FIG. 1B is composed of fullerene molecules three-dimensionally connected to each other through a linking group —CF2SO2NHSO2CF2—. It contains, as the proton-dissociative group, sulfoneimide groups —SO2NHSO2— and sulfoneamide groups —SO2H2 in addition to sulfonic acid groups. These compounds are prepared by introduction of difluoro(fluorosulfonyl)methyl groups into fullerene molecules, and ensuing imidization and hydrolysis.
摘要翻译：本文公开了离子解离官能化合物，其制备方法，离子导体和电化学装置，离子解离官能化合物在燃料电池所需的条件下是热和化学稳定的并且适合用作材料如燃料电池中的质子导体。图1所示的质子解离官能团化合物 1A由富勒烯C60分子和约10个磺酸基-SO 3 H组成，作为通过二氟甲烷基-CF2-连接到富勒烯的质子解离基团。图1所示的质子解离官能团化合物 1B由通过连接基团-CF 2 SO 2 NHSO 2 CF 2彼此三维连接的富勒烯分子组成。作为质子解离基团，除了磺酸基之外，还包含砜酰亚胺基团-SO 2 NH 2 2-和磺酰胺基团-SO 2 H 2。这些化合物是通过将二氟（氟磺酰基）甲基引入富勒烯分子中制备的，随后进行酰亚胺化和水解。

7. 发明申请

US20070092800A1 IONIC CONDUCTOR, PROCESS FOR PRODUCTION THEREOF, AND ELECTROCHEMICAL DEVICE 失效
标题翻译：离子导体，其制造方法和电化学装置
公开(公告)号：US20070092800A1
公开(公告)日：2007-04-26
申请号：US11561609
申请日：2006-11-20
申请人： Koichiro Hinokuma , Bjoern Pietzak , Constance Rost , Masafumi Ata , Yongming Li , Kazuaki Fukushima
发明人： Koichiro Hinokuma , Bjoern Pietzak , Constance Rost , Masafumi Ata , Yongming Li , Kazuaki Fukushima
IPC分类号： H01M10/40 , C08J5/20
CPC分类号： B82Y30/00 , H01B1/122 , H01M4/8605 , H01M6/18 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M8/1048 , H01M10/0562 , H01M10/347 , H01M12/00 , H01M2300/0068 , H01M2300/0082 , Y02P70/56
摘要： Disclosed herein are an ionic conductor including a proton conductor, a process for production thereof, and an electrochemical device (such as fuel cell) with said ionic conductor, said ionic conductor being superior in ionic conductivity, water resistance, and film forming properties. The ionic conductor is formed from a polymer in which carbon clusters having ion dissociating functional groups are bonded to each other through connecting groups. The polymer is less water-soluble and more chemically stable than a derivative composed solely of carbon clusters; therefore, it permits many ion dissociating functional group to be introduced thereinto. Moreover, if ion dissociating functional groups are introduced into also the connecting group, it is possible to prevent the concentration of ion dissociating functional groups from decreasing as the result of polymerization. The polymer can be easily synthesized by simple condensation, substitution, and hydrolysis. Therefore, the process is suitable for mass production in high yields.
摘要翻译：本文公开了包括质子导体，其制造方法和具有所述离子导体的电化学装置（例如燃料电池）的离子导体，所述离子导体的离子导电性，耐水性和成膜性优异。离子导体由具有离子解离官能团的碳簇通过连接基团彼此结合的聚合物形成。聚合物比仅由碳簇组成的衍生物更少的水溶性和化学稳定性; 因此，允许引入许多离子解离官能团。此外，如果将离子解离官能团引入连接基团，则可以防止离子解离官能团的浓度作为聚合的结果而降低。聚合物可以通过简单的缩合，取代和水解来容易地合成。因此，该方法适合大批量生产。

8. 发明授权

US06495290B1 Proton conductor, production method thereof, and electrochemical device using the same 有权
标题翻译：质子导体及其制造方法及使用其的电化学装置
公开(公告)号：US06495290B1
公开(公告)日：2002-12-17
申请号：US09619166
申请日：2000-07-19
申请人： Koichiro Hinokuma , Björn Pietzak , Constance Gertrud Rost , Masafumi Ata
发明人： Koichiro Hinokuma , Björn Pietzak , Constance Gertrud Rost , Masafumi Ata
IPC分类号： H01M458
CPC分类号： H01M6/18 , B82Y30/00 , B82Y40/00 , C01B32/15 , C01B32/152 , H01B1/04 , H01B1/122 , H01M4/8605 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M8/1048 , H01M10/0562 , H01M10/347 , H01M12/00 , H01M2300/0068 , H01M2300/0082 , H01M2300/0091 , Y02P70/56 , Y10S977/75 , Y10S977/752 , Y10S977/788 , Y10S977/842 , Y10S977/948
摘要： A proton conductor mainly contains a carbonaceous material derivative, such as, a fullerene derivative, a carbon cluster derivative, or a tubular carbonaceous material derivative in which groups capable of transferring protons, for example, —OH groups or —OSO3H groups are introduced to carbon atoms of the carbonaceous material derivative. The proton conductor is produced typically by compacting a powder of the carbonaceous material derivative. The proton conductor is usable, even in a dry state, in a wide temperature range including ordinary temperature. In particular, the proton conductor mainly containing the carbon cluster derivative is advantageous in increasing the strength and extending the selection range of raw materials. An electrochemical device, such as, a fuel cell, that employs the proton conductor is not limited by atmospheric conditions and can be of a small and simple construction. The proton conductor may contain a polymer in addition to the carbonaceous material derivative, which conductor can be formed, typically by extrusion molding, into a thin film having a large strength, a high gas permeation preventive ability, and a good proton conductivity.
摘要翻译：质子导体主要含有碳质材料衍生物，例如富勒烯衍生物，碳簇衍生物或管状碳质材料衍生物，其中可将质子转移的基团例如-OH基或-OSO 3 H基引入碳含碳材料衍生物的原子。质子导体通常通过压实含碳材料衍生物的粉末来制备。质子导体即使在干燥状态下也可以在包括常温的宽温度范围内使用。特别地，主要含有碳簇衍生物的质子导体有利于提高强度并延长原料的选择范围。使用质子导体的诸如燃料电池的电化学装置不受大气条件限制，并且可以是小而简单的结构。质子导体除含碳材料衍生物之外还可以含有聚合物，该衍生物通常通过挤出成型形成具有大的强度，高透气性能和良好的质子传导性的薄膜。

9. 发明授权

US06380710B1 Photovoltaic-charged secondary battery device 失效
标题翻译：光伏充电二次电池装置
公开(公告)号：US06380710B1
公开(公告)日：2002-04-30
申请号：US09609170
申请日：2000-06-30
申请人： Haruo Watanabe , Ritsuko Inoue , Koichiro Hinokuma , Tomikazu Watanabe , Hiroshi Miyazawa
发明人： Haruo Watanabe , Ritsuko Inoue , Koichiro Hinokuma , Tomikazu Watanabe , Hiroshi Miyazawa
IPC分类号： H01M1046
CPC分类号： H01M10/425 , H01L31/03921 , H01L31/046 , H01L31/048 , H01L31/056 , H01M2/105 , H01M10/465 , H01M2300/0014 , H02S30/20 , H02S40/38 , Y02E10/52
摘要： A photovoltaic-charged secondary battery device has a cylindrical core, a flexible photoelectric transducer sheet extractably rolled on the core, a chargeable/dischargeable storage battery, and a control circuit for controlling the charging and discharging operations of the storage battery. The photovoltaic-charged secondary battery device with the photoelectric transducer sheet fully rolled on the core generally exhibiting a substantially cylindrical form. The photovoltaic-charged secondary battery device further has a polymeric cover film formed on the light-receiving surface of the photoelectric transducer sheet. The polymeric cover film improves the durability of the photoelectric transducer sheet against repeated bending and sliding actions caused on the photoelectric transducer sheet. The photoelectric transducer sheet may be so arranged that, when the photoelectric transducer sheet is rolled on the core, the light-receiving surface faces outward of the roll. The photovoltaic-charged secondary battery device may have a cylindrical peripheral wall coaxial with the core and defining therebetween an annular space for accommodating the photoelectric transducer sheet rolled on the core. The photoelectric transducer sheet is retractable into and extractable from the annular space through a slit formed in the cylindrical peripheral wall member. The cylindrical peripheral wall member is rotatable relative to the core, so that the photoelectric transducer sheet can be retracted into the annular space and rolled on the core as the cylindrical peripheral wall member is rotated. The cylindrical peripheral wall member may have a plurality of projections formed on the inner surface thereof. The photovoltaic-charged secondary battery device may have a temperature-responsive mechanism operable to disconnect the storage battery from the electrical connection or to move the storage battery from a predetermined position.
摘要翻译：光伏充电二次电池装置具有圆筒形芯，可提取地卷绕在芯上的柔性光电传感器片，可充电/可放电的蓄电池，以及用于控制蓄电池的充电和放电操作的控制电路。具有光纤换能片的光伏充电二次电池装置通常呈现出基本圆柱形的形式。光电二次电池装置还具有在光电转换片的受光面上形成的聚合物覆盖膜。聚合物覆盖膜提高光电传感器片的耐久性，防止在光电传感器片上引起的反复弯曲和滑动。光电传感器片可以布置成使得当光电转换片在芯上滚动时，光接收表面面向卷的外侧。光伏充电的二次电池装置可以具有与芯部同轴的圆柱形周壁，并在其间限定用于容纳在芯上滚动的光电传感器片的环形空间。光电传感器片通过形成在圆筒形周壁构件中的狭缝可缩回到环形空间内并可从其中取出。圆筒形周壁构件可相对于芯部旋转，使得当圆筒形周壁构件旋转时，光电换能器片材可以缩回到环形空间中并在芯体上滚动。圆筒形周壁构件可以具有形成在其内表面上的多个突起。光伏充电的二次电池装置可以具有温度响应机构，其可操作以将蓄电池与电气连接断开或将蓄电池从预定位置移动。

10. 发明申请

US20110281167A1 THIN FILM SOLID STATE LITHIUM ION SECONDARY BATTERY AND METHOD OF MANUFACTURING THE SAME 审中-公开
标题翻译：薄膜固体锂离子二次电池及其制造方法
公开(公告)号：US20110281167A1
公开(公告)日：2011-11-17
申请号：US13146138
申请日：2010-01-28
申请人： Yuichi Sabi , Koichiro Hinokuma , Katsunori Takahara , Hiroyuki Morioka , Tatsuya Furuya
发明人： Yuichi Sabi , Koichiro Hinokuma , Katsunori Takahara , Hiroyuki Morioka , Tatsuya Furuya
IPC分类号： H01M10/052 , H01M10/058 , H01M4/131
CPC分类号： H01M2/0212 , H01M4/131 , H01M4/134 , H01M4/136 , H01M4/1391 , H01M4/1397 , H01M4/382 , H01M4/667 , H01M6/40 , H01M10/0525 , H01M10/0562 , H01M10/0585 , H01M2004/027
摘要： A high-performance and inexpensive thin film solid state lithium ion secondary battery that is able to be charged and discharged in the air and is able to be manufactured stably at a favorable yield, and a method of manufacturing the same are provided. The thin film solid state lithium ion secondary battery has an electric insulating substrate 10 formed from an organic resin, an inorganic insulating film provided on the substrate face, a cathode-side current collector film 30, a cathode active material film 40, a solid electrolyte film 50, an anode-side current collector protective film 68, and an anode-side current collector film 70. In the thin film solid state lithium ion secondary battery, the cathode-side current collector film and/or the anode-side current collector film is formed on the inorganic insulating film face. The anode-side current collector protective film is formed from a conductive oxide including at least any one of an oxide of Sn, In, and Zn, and holds the total amount of lithium associated with charge and discharge roughly constant. The thickness of the anode-side current collector protective film is 2 nm or more and 22 nm or less. The thickness of the inorganic insulating film is 5 nm or more and 500 nm or less. The inorganic insulating film contains at least any one of an oxide, a nitride, and a sulfide containing one of Si, Al, Cr, Zr, Ta, Ti, Mn, Mg, and Zn.
摘要翻译：提供能够在空气中充放电并且能够以良好的收率稳定地制造的高性能且廉价的薄膜固态锂离子二次电池及其制造方法。薄膜固态锂离子二次电池具有由有机树脂形成的电绝缘基板10，设置在基板面上的无机绝缘膜，阴极侧集电体膜30，正极活性物质膜40，固体电解质膜50，阳极侧集电体保护膜68和阳极侧集电体膜70.在薄膜固体锂离子二次电池中，阴极侧集电体膜和/或阳极侧集电体在无机绝缘膜面上形成膜。阳极侧集电体保护膜由包含Sn，In和Zn的氧化物中的至少任一种的导电氧化物形成，并且与充放电相关的总量保持大致恒定。阳极侧集电体保护膜的厚度为2nm以上且22nm以下。无机绝缘膜的厚度为5nm以上且500nm以下。无机绝缘膜含有包含Si，Al，Cr，Zr，Ta，Ti，Mn，Mg和Zn中的一种的氧化物，氮化物和硫化物中的至少一种。

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