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1. 发明授权

US06617299B1 Composition and method for bleaching a substrate 失效
标题翻译：用于漂白基材的组合物和方法
公开(公告)号：US06617299B1
公开(公告)日：2003-09-09
申请号：US09539756
申请日：2000-03-31
申请人： Riccardo Filippo Carina , Bernard Lucas Feringa , Ronald Hage , Catherine Hemmert , Jean Hypolites Koek , Rene Marcel LaCrois , Bernard Meunier , Michael Renz , Johannes Gerhardus Roelfes , Ebe Pieter Schudde , Rob Thijssen , Robin Stefan Twisker , Charon Zondervan
发明人： Riccardo Filippo Carina , Bernard Lucas Feringa , Ronald Hage , Catherine Hemmert , Jean Hypolites Koek , Rene Marcel LaCrois , Bernard Meunier , Michael Renz , Johannes Gerhardus Roelfes , Ebe Pieter Schudde , Rob Thijssen , Robin Stefan Twisker , Charon Zondervan
IPC分类号： C11D3395
CPC分类号： C07D401/14 , C07D213/38 , C07D213/55 , C11D3/3932 , D06L4/12 , D06L4/13 , D06L4/15
摘要： The invention relates to catalytically bleaching substrates, especially laundry fabrics, with atmospheric oxygen or air. A method of bleaching a substrate is provided that comprises applying to the substrate, in an aqueous medium, a specified ligand from a selected class which forms a complex with a transition metal, the complex catalysing bleaching of the substrate by atmospheric oxygen. Also provided is an aqueous bleaching composition substantially devoid of peroxygen bleach or a peroxy-based or -generating bleach system. Also provided is a method of treating a textile such as a laundry fabric whereby a complex catalyses bleaching of the textile by atmospheric oxygen after the treatment. The catalyst may be used in dry form, or in a liquor that is then dried, such as an aqueous spray-on fabric treatment fluid or a wash liquor for laundry cleaning, or a non-aqueous dry cleaning fluid or spray-on aerosol fluid. The method can confer cleaning benefits to the textile after the treatment. Also provided is a dry textile having a catalyst applied or deposited thereon, whereby bleaching by atmospheric oxygen is catalysed on the textile.
摘要翻译：本发明涉及用大气中的氧气或空气催化漂洗底物，特别是洗衣织物。提供了一种漂白底物的方法，其包括在水性介质中向所述底物施加与过渡金属形成络合物的所选类别的特定配体，所述复合物通过大气氧催化底物的漂白。还提供了基本上不含过氧漂白剂或过氧基或生成漂白体系的水性漂白组合物。还提供了一种处理织物如洗衣布的方法，由此复合物在处理后通过大气氧催化织物的漂白。催化剂可以以干式形式使用，也可以在随后干燥的液体中使用，例如水性喷涂织物处理流体或用于衣物清洗的洗涤液，或非水性干洗液或喷雾气溶胶流体。该方法可以在处理后赋予纺织品清洁效果。还提供了具有施加或沉积在其上的催化剂的干织物，由此通过大气氧气漂白在织物上被催化。

2. 发明授权

US06225275B1 Method for enhancing the activity of an enzyme 失效
标题翻译：提高酶活性的方法
公开(公告)号：US06225275B1
公开(公告)日：2001-05-01
申请号：US09093635
申请日：1998-06-04
申请人： Ronald Hage , Jiri Hora , Ton Swarthoff , Robin Stefan Twisker
发明人： Ronald Hage , Jiri Hora , Ton Swarthoff , Robin Stefan Twisker
IPC分类号： C11D328
CPC分类号： D21C5/005 , C11D3/0021 , C11D3/38654 , C12N9/00
摘要： A first aspect of the invention is a process for enhancing the activity of an oxidorecudtase by adding to the enzyme, certain specific compounds which are capable of enhancing the activity of said oxidoreductase enzyme. A second aspect of the invention is an enzymatic bleach composition comprising an oxidoreductase and enhancing compounds.
摘要翻译：本发明的第一方面是通过向酶中加入能够增强所述氧化还原酶的活性的某些特定化合物来增强氧化还原酶的活性的方法。本发明的第二方面是包含氧化还原酶和增强化合物的酶促漂白组合物。

3. 发明授权

US06169065A Method for the activity of an enzyme 失效
标题翻译：酶活性的方法
公开(公告)号：US06169065A
公开(公告)日：2001-01-02
申请号：US09140561
申请日：1998-08-27
申请人： Willem Antheunisse , Ronald Hage , Jiri Hora , Ton Swarthoff , Robin Stefan Twisker
发明人： Willem Antheunisse , Ronald Hage , Jiri Hora , Ton Swarthoff , Robin Stefan Twisker
IPC分类号： C11D3386
CPC分类号： C11D3/349 , C11D3/0021 , C11D3/28 , C11D3/3472 , C11D3/3481 , C11D3/38654
摘要： There is provided a process for enhancing the activity of an oxidoreductase, comprising adding to the enzyme, as an enhancer for the activity of said enzyme, a compound having the formula: wherein X represents (—O—) or (—S—) and R1, R2 and R3 may each independently represent hydrogen, hydroxy, halogen, nitroso, formyl, carboxyl, and esters and salts thereof, carbamoyl, sulfo, and esters and salts hereof, sulfamoyl, nitro, amino, phenyl, C1-C20 alkyl, C1-C8 alkoxy, carbonyl-C1-C6-alkoxy, aryl-C1-C6-alkyl, whereby: the carbamoyl, sulfamoyl and amino groups may be unsubstituted or substituted once or twice with hydroxy, C1-C6-alkyl, C1-C6-alkoxy, in which C1-C6-group may be saturated or unsaturated, branched or unbranched and may be substituted once or twice with halogen, nitroso, hydroxy, formyl, carboxy, and esters and salts thereof, carbamoyl, sulfo, and esters and salts hereof, sulfamoyl; and the phenyl group may be substituted with once or twice with halogen, nitroso, hydroxy, formyl, carboxy, and esters and salts thereof, carbamoyl, sulfo, and esters and salts hereof, sulfamoyl; and the C1-C20 alkyl, C1-C8 alkoxy, carbonyl-C1-C6-alkoxy, and aryl-C1-C6-alkyl groups may be saturated or unsaturated, branched or unbranched, and may be substituted with halogen, hydroxy, nitroso, formyl, carboxy, and esters and salts thereof, carbamoyl, sulfo, and esters and salts thereof, sulfamoyl, nitro, amino, phenyl, aminoalkyl, piperidino, piperazinyl, pyrrolidin-2-yl, C1-C6-alkyl, C1-C6-alkoxy; whereby two or more of the groups R1-R3 may be linked together by any group, and and A and B represent at least one six membered heterocyclic ring which may be optionally substituted with one or more of any of the radicals as defined for R1-R3.
摘要翻译：提供了一种增强氧化还原酶活性的方法，包括向所述酶中添加作为所述酶活性的增强剂，具有下式的化合物：其中X表示（-O-）或（-S-）和 R 1，R 2和R 3可各自独立地表示氢，羟基，卤素，亚硝基，甲酰基，羧基及其酯和盐，氨基甲酰基，磺基及其酯和盐，氨磺酰基，硝基，氨基，苯基，C 1 -C 20烷基， C 1 -C 8烷氧基，羰基-C 1 -C 6烷氧基，芳基-C 1 -C 6烷基，其中：氨基甲酰基，氨磺酰基和氨基可以是未被取代的或被羟基，C 1 -C 6烷基，C 1 -C 6 - 烷氧基，其中C 1 -C 6基可以是饱和或不饱和的，支链或非支链的，并且可以被卤素，亚硝基，羟基，甲酰基，羧基及其酯和盐，氨基甲酰基，磺基和酯取代一次或两次，以及盐，氨磺酰; 并且苯基可以被卤素，亚硝基，羟基，甲酰基，羧基及其酯和盐，氨基甲酰基，磺基以及它们的酯和盐取代一次或两次，氨磺酰基; C 1 -C 20烷基，C 1 -C 8烷氧基，羰基-C 1 -C 6烷氧基和芳基-C 1 -C 6烷基可以是饱和或不饱和的，支链或非支链的，并可被卤素，羟基，亚硝基，甲酰基，羧基及其酯和盐，氨基甲酰基，磺基及其酯和盐，氨磺酰，硝基，氨基，苯基，氨基烷基，哌啶子基，哌嗪基，吡咯烷-2-基，C 1 -C 6烷基，C 1 -C 6烷氧基其中两个或更多个基团R 1 -R 3可以通过任何基团连接在一起，并且A和B表示至少一个六元杂环，其可任选被一个或多个如R1- R3。

4. 发明授权

US06432900B1 Ligand and complex for catalytically bleaching a substrate 失效
标题翻译：用于催化漂白底物的配体和配合物
公开(公告)号：US06432900B1
公开(公告)日：2002-08-13
申请号：US09650148
申请日：2000-08-29
申请人： Adrianus Cornelis Appel , Ronald Hage , David Tetard , Robin Stefan Twisker
发明人： Adrianus Cornelis Appel , Ronald Hage , David Tetard , Robin Stefan Twisker
IPC分类号： C11D726
CPC分类号： C07D401/14 , C07D213/38 , C07D213/55 , C11D3/28 , C11D3/3932
摘要： The invention relates to ligands or complexes useful as catalysts for catalytically bleaching substrates with atmospheric oxygen, and as catalysts in the of treatment of textiles such as laundry fabrics whereby bleaching by atmospheric oxygen is catalysed after the treatment. The ligand is of the general formula: wherein R1, R2, and R3 independently represent a group selected from hydrogen, hydroxyl, halogen, —NH—C(NH)NH2, —R and —OR, wherein R=alkyl, alkenyl, cycloalkyl, heterocycloalkyl, aryl, heteroaryl or a carbonyl derivative group, R being optionally substituted by one or more functional groups, and provided that two of R1, R2 and R3 are coordinating groups and one of R1, R2 and R3 is a non-coordinating group; Q independently represents a group selected from C2-3-alkylene optionally substituted by H, benzyl or C1-8-alkyl; and Q1, Q2 and Q3 independently represent specified linking groups.
摘要翻译：本发明涉及可用作催化漂洗底物与大气氧的催化剂的配体或配合物，以及作为处理纺织品如洗涤织物的催化剂，由此在处理后催化大气中的漂白。配位体具有以下通式：其中R1，R2和R3独立地表示选自氢，羟基，卤素，-NH-C（NH）NH2，-R和-OR的基团，其中R =烷基，烯基，环烷基，杂环烷基，芳基，杂芳基或羰基衍生物基团，R任选被一个或多个官能团取代，并且条件是R 1，R 2和R 3中的两个为配位基团，R 1，R 2和R 3中的一个为非配位基团。 Q独立地表示选自任选被H，苄基或C 1-8 - 烷基取代的C 2-3 - 亚烷基的基团; 而Q1，Q2和Q3独立地表示指定的连接基团。

5. 发明授权

US06380146B1 Bleaching detergent compositions 失效
标题翻译：漂白洗涤剂组合物
公开(公告)号：US06380146B1
公开(公告)日：2002-04-30
申请号：US09596994
申请日：2000-06-20
申请人： Greta Johanna Breel , Daniel Convents , Willem Van Liemt , Ton Swarthoff , Robin Stefan Twisker
发明人： Greta Johanna Breel , Daniel Convents , Willem Van Liemt , Ton Swarthoff , Robin Stefan Twisker
IPC分类号： C11D742
CPC分类号： C11D3/30 , C11D3/26 , C11D3/349 , C11D3/38609 , C11D3/3942
摘要： There is provided a bleaching detergent composition comprising one or more surfactants, a phenol oxidizing enzyme and a compound which acts as enhancer for the phenol oxidizing enzyme, said composition having an Enhancer Index as herein defined of at least 12 and prefereably in the range of 15-50.
摘要翻译：提供了一种漂白洗涤剂组合物，其包含一种或多种表面活性剂，酚氧化酶和充当酚氧化酶的增强剂的化合物，所述组合物具有如本文所定义的至少12并且优选在15范围内的增强子指数 -50。

6. 发明授权

US06323014B1 Method and composition for enhancing the activity of an enzyme 失效
标题翻译：提高酶活性的方法和组合物
公开(公告)号：US06323014B1
公开(公告)日：2001-11-27
申请号：US09596998
申请日：2000-06-20
申请人： Greta Johanna Breel , Daniel Convents , Willem Van Liemt , Ton Swarthoff , Robin Stefan Twisker
发明人： Greta Johanna Breel , Daniel Convents , Willem Van Liemt , Ton Swarthoff , Robin Stefan Twisker
IPC分类号： C12N996
CPC分类号： C11D3/26 , C11D3/30 , C11D3/349 , C11D3/38609 , C11D3/3942
摘要： There is provided a process for enhancing the activity of a phenol oxidizing enzyme, comprising adding to the enzyme, as an enhancer for the activity of the enzyme, one or more compounds having the formula: wherein: A is an optionally substituted electron-withdrawing group, chosen from the group consisting of nitrile, carboxyl, and esters and salts thereof, amides, aldehydes, ketones, sulfoxides, sulfones, or sulphonates, and B is an optionally substituted electron-donating group, chosen from the group consisting of the oxide anion, sulfide anion, oxides, amines, imines, hydroxides, sulfides, ethers, carboxylic acids, and halogen substituents, and R1-R5 may each independently represent hydrogen, hydroxy, halogen, nitroso, formyl, carboxyl, and esters and salts thereof, carbamoyl, sulfo, and esters and salts hereof, sulfamoyl, nitro, amino, phenyl, C1-C20 alkyl, C1-C8 alkoxy, carbonyl-C1-C6-alkoxy, aryl-C1-C6-alkyl, and R2 and R5 together may form an alkylene group or an alkenylene group.
摘要翻译：提供了一种增强酚氧化酶的活性的方法，包括向酶中加入作为酶活性的增强剂，一种或多种具有下式的化合物：其中：A是任选取代的吸电子基团选自腈，羧基及其酯和盐，酰胺，醛，酮，亚砜，砜或磺酸盐，B是任选取代的给电子基团，其选自氧化物阴离子，硫化物阴离子，氧化物，胺，亚胺，氢氧化物，硫化物，醚，羧酸和卤素取代基，R 1 -R 5可各自独立地表示氢，羟基，卤素，亚硝基，甲酰基，羧基及其酯和盐，氨基甲酰基，，和其酯和盐，氨磺酰，硝基，氨基，苯基，C 1 -C 20烷基，C 1 -C 8烷氧基，羰基-C 1 -C 6 - 烷氧基，芳基-C 1 -C 6烷基和R 2和R 5一起可以形成亚烷基基团或亚烯基。

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