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1. 发明申请

US20140023789A1 COATING AGENTS HAVING HIGH SCRATCH RESISTANCE AND WEATHERING STABILITY 审中-公开
标题翻译：具有高耐蚀性和耐候性的涂料代理
公开(公告)号：US20140023789A1
公开(公告)日：2014-01-23
申请号：US14036367
申请日：2013-09-25
申请人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
发明人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
IPC分类号： C09D175/14
CPC分类号： C09D175/14 , C08G18/289 , C08G18/6254 , C08G18/778 , C08G18/809 , C09D175/04
摘要： Disclosed are coating compositions comprising (a) at least one hydroxyl-containing compound (A), (b) at least one compound (B) having isocyanate groups, and (c) at least one catalyst (D) for the crosslinking of silane groups, said catalyst (D) comprising phosphorus. It is an aspect of the disclosed coating compositions that (i) one or more constituents of the coating composition contain hydrolyzable silane groups and (ii) the coating composition can be finally cured to a coating which has statistically distributed regions of an Si—O—Si network.
摘要翻译：公开了包含（a）至少一种含羟基化合物（A），（b）至少一种具有异氰酸酯基团的化合物（B）和（c）至少一种用于硅烷基团交联的催化剂（D），所述催化剂（D）包含磷。所公开的涂料组合物的一个方面是（i）涂料组合物中的一种或多种组分含有可水解的硅烷基团，和（ii）涂料组合物可以最终固化成具有统计分布的Si-O- Si网络。

2. 发明申请

US20130196072A1 COATING AGENTS HAVING IMPROVED RUNOFF TENDENCY 有权
标题翻译：具有改进的流失趋势的涂料代理
公开(公告)号：US20130196072A1
公开(公告)日：2013-08-01
申请号：US13642630
申请日：2011-03-30
申请人： Matthijs Groenewolt , Manuela Niemeier
发明人： Matthijs Groenewolt , Manuela Niemeier
IPC分类号： C09D133/14
CPC分类号： C09D133/14 , B05D1/02 , B05D1/04 , B05D7/14 , B05D7/26 , C08G18/289 , C08G18/6254 , C08G18/792 , C08G18/809 , C09D175/04 , C09D175/12
摘要： Coating compositions comprising at least one hydroxyl-containing compound (A), at least one isocyanato-containing compound (B) and at least one urea-group-containing compound (H) different from (B), compound (H) comprising at least one structural unit selected from the group consisting of a structural unit (I) a structural unit (II) a structural unit (III) —NR′″—C(O)—N(X—SiR″x(OR′)3-x)n(X′—SiR″y(OR′)3-y)m, and combinations of two or more of the foregoing, compound (H) being obtained by reacting an isocyanato-containing compound (HG) with amino-containing compounds, wherein in compound (H) more than 90 mol % of the isocyanate groups originally present in (HG) have undergone reaction to form the structural units (I), (II), (III), or combinations thereof, where R′, R′″=hydrogen, alkyl, cycloalkyl, aryl or aralkyl; R, R″=alkyl, cycloalkyl, aryl or aralkyl; X, X′=linear and/or branched alkyl or cycloalkyl radical; x, y, n, m=0 to 2; and m+n=2.
摘要翻译：包含至少一种含羟基的化合物（A），至少一种含异氰酸酯基的化合物（B）和至少一种不同于（B）的含脲基化合物（H），化合物（H）选自结构单元（I），结构单元（II），结构单元（III）-NR“'-C（O）-N（X-SiR''x（OR'））的结构单元 3-x）n（X'-SiR''y（OR'）3-y）m，以及两种或多种上述化合物（H）的组合，其通过使含异氰酸酯基的化合物（HG）与原料存在于（HG）中的多于90摩尔％的异氰酸酯基的化合物（H）中的氨基化合物已经发生反应，形成结构单元（I），（II），（III）或其组合，其中R'，R“'=氢，烷基，环烷基，芳基或芳烷基; R，R“=烷基，环烷基，芳基或芳烷基; X，X'=直链和/或支链烷基或环烷基; x，y，n，m = 0〜2; m + n = 2。

3. 发明申请

US20100015344A1 COATING COMPOSITIONS WITH HIGH SCRATCH RESISTANCE AND WEATHERING STABILITY 审中-公开
标题翻译：具有高耐蚀性和耐候性的涂料组合物
公开(公告)号：US20100015344A1
公开(公告)日：2010-01-21
申请号：US12519466
申请日：2007-12-19
申请人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
发明人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
IPC分类号： B05D1/36 , C09D175/00
CPC分类号： C09D175/14 , C08G18/289 , C08G18/6254 , C08G18/778 , C08G18/809 , C09D175/04
摘要： Disclosed are coating compositions comprising (a) at least one hydroxyl-containing compound (A), (b) at least one compound (B) having free and/or blocked isocyanate groups, and (c) at least one catalyst (D) for the crosslinking of silane groups, where (i) one or more constituents of the coating composition contain hydrolyzable silane groups and (iii) the coating composition can be finally cured to a coating which has statistically distributed regions of an Si—O—Si network. The finally cured coating obtained from the coating composition has a post-crosslinking index (PCI) of less than 2, wherein (PCI) is defined as the ratio of the storage modulus E′(200) at 200° C. to the minimum of the storage modulus E′(min) at a temperature above the measured glass transition temperature Tg.
摘要翻译：公开了包含（a）至少一种含羟基的化合物（A），（b）至少一种具有游离和/或封闭的异氰酸酯基团的化合物（B）的涂料组合物，和（c）至少一种用于硅烷基团的交联，其中（i）涂料组合物中的一种或多种组分含有可水解的硅烷基团，和（iii）涂料组合物可最终固化成具有统计分布的Si-O-Si网络区域的涂层。从涂料组合物得到的最终固化涂层具有小于2的后交联指数（PCI），其中（PCI）定义为200℃下的储能模量E'（200）与最低在高于测量的玻璃化转变温度Tg的温度下的储能模量E'（min）。

4. 发明授权

US08658752B2 Use of partially silanized polyisocyanate-based compounds as crosslinking-agents in coating compositions, and coating compositions comprising the compounds 有权
标题翻译：在涂料组合物中使用部分硅烷化的多异氰酸酯基化合物作为交联剂，以及包含该化合物的涂料组合物
公开(公告)号：US08658752B2
公开(公告)日：2014-02-25
申请号：US13001170
申请日：2009-06-25
申请人： Matthijs Groenewolt , Simone Hesener , Wilfried Stübbe , Manuela Niemeier , Elke Westhoff
发明人： Matthijs Groenewolt , Simone Hesener , Wilfried Stübbe , Manuela Niemeier , Elke Westhoff
IPC分类号： C08G77/04
CPC分类号： C09D175/04 , C08G18/10 , C08G18/289 , C08G18/6229 , C08G18/6254 , C08G18/792 , Y10T428/31551 , C08G18/62
摘要： The invention relates to the use of partly silanized compounds based on polyisocyanate as crosslinking agents with heightened refractive index in curable coating compositions, more particularly in clearcoat materials for automotive finishing. The invention likewise relates to a coating composition which comprises these compounds as crosslinking agents, and to the use of the coating composition to produce a coating.
摘要翻译：本发明涉及在可固化涂料组合物中使用基于多异氰酸酯的部分硅烷化化合物作为具有较高折射率的交联剂，更具体地说，涉及用于汽车整理的透明涂料中。本发明同样涉及包含这些化合物作为交联剂的涂料组合物以及涂料组合物用于生产涂料的用途。

5. 发明申请

US20100028544A1 COATING COMPOSITIONS WITH HIGH SCRATCH RESISTANCE AND WEATHERING STABILITY 有权
标题翻译：具有高耐蚀性和耐候性的涂料组合物
公开(公告)号：US20100028544A1
公开(公告)日：2010-02-04
申请号：US12519449
申请日：2007-12-19
申请人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
发明人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
IPC分类号： B05D3/02 , C09D5/00 , B05D1/36
CPC分类号： C09D175/14 , C08G18/289 , C08G18/6254 , C08G18/778 , C08G18/809 , C09D175/04
摘要： Disclosed are coating compositions comprising at least one hydroxyl-containing compound (A) and at least one isocyanato-containing compound (B), wherein one or more of the constituents of the coating composition comprise between 2.5 and 97.5 mol %, based on the entirety of structural units (I) and (II), of at least one structural unit of the formula (I) —N(X—SiR″x(OR′)3-x)n(X′—SiR″y(OR′)3-y)m (I) and between 2.5 and 97.5 mol %, based on the entirety of structural units (I) and (II), of at least one structural unit of the formula (II) —Z—(X—SiR″x(OR′)3-x) (II).
摘要翻译：公开了包含至少一种含羟基的化合物（A）和至少一种含异氰酸酯基的化合物（B）的涂料组合物，其中所述涂料组合物的一种或多种组分包含2.5至97.5mol％的结构单元（I）和（II）的至少一种结构单元的式（I）-N（X-SiR''x（OR'）3-x）n（X'-SiR''y OR'）3-y）m（I），并且基于整个结构单元（I）和（II），2.5至97.5mol％的至少一种式（II）-Z-（ X-SiR''x（OR'）3-x）（II）。

6. 发明授权

US09777190B2 Aqueous polyurethane coating material and coatings produced therefrom and having high scratch resistance and good chemicals resistance 有权
公开(公告)号：US09777190B2
公开(公告)日：2017-10-03
申请号：US13980779
申请日：2012-01-04
申请人： Matthijs Groenewolt , Manuela Niemeier , Wilfried Stübbe , Alexandra Steffens , Britta Schnieders
发明人： Matthijs Groenewolt , Manuela Niemeier , Wilfried Stübbe , Alexandra Steffens , Britta Schnieders
IPC分类号： B05D3/02 , C09D175/04 , C08G18/08 , C08G18/18 , C08G18/28 , C08G18/62 , C08G18/77 , C08G18/79 , C08G18/80 , B05D1/36 , B05D1/38
CPC分类号： C09D175/04 , B05D1/36 , B05D1/38 , C08G18/0823 , C08G18/0866 , C08G18/1883 , C08G18/289 , C08G18/622 , C08G18/778 , C08G18/792 , C08G18/809
摘要： Disclosed are aqueous coating compositions comprising at least one hydroxyl-containing compound (A), at least one compound (B) having isocyanate groups and also having hydrolyzable silane groups, and at least one catalyst (C)wherein the compound (B) has 10 mol % to less than 90 mol % of at least one structural unit (I) —N(X—SiR″x(OR′)3-x)n(X′—SiR″y(OR′)3-y)m (I) Where R′=hydrogen, alkyl or cycloalkyl, X, X′=linear and/or branched alkylene or cycloalkylene radical having 1 to 20 carbon atoms, R″=alkyl, cycloalkyl, aryl or aralkyl, n=0 to 2, m=0 to 2, m+n=2, and x, y=0 to 2, and more than 10 to 90 mol % of at least one structural unit (II) —Z—(X—SiR″x(OR′)3-x) (II), where Z=—NH—, —NR—, —O— or —S—, where R=alkyl, cycloalkyl, aryl or aralkyl, and x, X, R′ and R″ have the definition indicated for formula (I).

7. 发明申请

US20110269897A1 USE OF PARTIALLY SILANIZED POLYISOCYANATE-BASED COMPOUNDS AS CROSSLINKING-AGENTS IN COATING COMPOSITIONS, AND COATING COMPOSITIONS COMPRISING THE COMPOUNDS 有权
标题翻译：使用部分硅烷基聚异氰酸酯化合物作为涂料组合物中的交联剂，以及包含该化合物的涂料组合物
公开(公告)号：US20110269897A1
公开(公告)日：2011-11-03
申请号：US13001170
申请日：2009-06-25
申请人： Matthijs Groenewolt , Simone Hesener , Wilfried Stubbe , Manuela Niemeier , Elke Westhoff
发明人： Matthijs Groenewolt , Simone Hesener , Wilfried Stubbe , Manuela Niemeier , Elke Westhoff
IPC分类号： C09D133/10 , C07F7/10
CPC分类号： C09D175/04 , C08G18/10 , C08G18/289 , C08G18/6229 , C08G18/6254 , C08G18/792 , Y10T428/31551 , C08G18/62
摘要： The invention relates to the use of partly silanized compounds based on polyisocyanate as crosslinking agents with heightened refractive index in curable coating compositions, more particularly in clearcoat materials for automotive finishing. The invention likewise relates to a coating composition which comprises these compounds as crosslinking agents, and to the use of the coating composition to produce a coating.
摘要翻译：本发明涉及在可固化涂料组合物中使用基于多异氰酸酯的部分硅烷化化合物作为具有较高折射率的交联剂，更具体地说，涉及用于汽车整理的透明涂料中。本发明同样涉及包含这些化合物作为交联剂的涂料组合物以及涂料组合物用于生产涂料的用途。

8. 发明申请

US20100143596A1 COATING AGENTS HAVING HIGH SCRATCH RESISTANCE AND WEATHERING STABILITY 有权
标题翻译：具有高耐蚀性和耐候性的涂料代理
公开(公告)号：US20100143596A1
公开(公告)日：2010-06-10
申请号：US12519458
申请日：2007-12-19
申请人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
发明人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
IPC分类号： B05D1/38 , B05D1/36 , B05D3/02 , C08L83/06
CPC分类号： C09D175/14 , C08G18/289 , C08G18/6254 , C08G18/778 , C08G18/809 , C09D175/04
摘要： Disclosed are coating compositions comprising (a) at least one hydroxyl-containing compound (A), (b) at least one compound (B) having isocyanate groups, and (c) at least one catalyst (D) for the crosslinking of silane groups, said catalyst (D) comprising phosphorus. It is an aspect of the disclosed coating compositions that (i) one or more constituents of the coating composition contain hydrolyzable silane groups and (ii) the coating composition can be finally cured to a coating which has statistically distributed regions of an Si—O—Si network.
摘要翻译：公开了包含（a）至少一种含羟基化合物（A），（b）至少一种具有异氰酸酯基团的化合物（B）和（c）至少一种用于硅烷基团交联的催化剂（D），所述催化剂（D）包含磷。所公开的涂料组合物的一个方面是（i）涂料组合物中的一种或多种组分含有可水解的硅烷基团，和（ii）涂料组合物可以最终固化成具有统计分布的Si-O- Si网络。

9. 发明授权

US09404011B2 Coating agents having improved runoff tendency 有权
标题翻译：涂层剂具有改善的径流倾向
公开(公告)号：US09404011B2
公开(公告)日：2016-08-02
申请号：US13642630
申请日：2011-03-30
申请人： Matthijs Groenewolt , Manuela Niemeier
发明人： Matthijs Groenewolt , Manuela Niemeier
IPC分类号： B05D1/02 , B05D1/04 , B05D7/14 , B05D7/26 , C08G18/28 , C08G18/62 , C08G18/79 , C08G18/80 , C09D133/14 , C09D175/04 , C09D175/12
CPC分类号： C09D133/14 , B05D1/02 , B05D1/04 , B05D7/14 , B05D7/26 , C08G18/289 , C08G18/6254 , C08G18/792 , C08G18/809 , C09D175/04 , C09D175/12
摘要： Coating compositions comprising at least one hydroxyl-containing compound (A), at least one isocyanato-containing compound (B) and at least one urea-group-containing compound (H) different from (B), compound (H) comprising at least one structural unit selected from the group consisting of a structural unit (I) a structural unit (II) a structural unit (III) —NR′″—C(O)—N(X—SiR″x(OR′)3-x)n(X′—SiR″y(OR′)3-y)m, and combinations of two or more of the foregoing, compound (H) being obtained by reacting an isocyanato-containing compound (HG) with amino-containing compounds, wherein in compound (H) more than 90 mol % of the isocyanate groups originally present in (HG) have undergone reaction to form the structural units (I), (II), (III), or combinations thereof, where R′, R′″=hydrogen, alkyl, cycloalkyl, aryl or aralkyl; R, R″=alkyl, cycloalkyl, aryl or aralkyl; X, X′=linear and/or branched alkyl or cycloalkyl radical; x, y, n, m=0 to 2; and m+n=2.
摘要翻译：包含至少一种含羟基的化合物（A），至少一种含异氰酸酯基的化合物（B）和至少一种不同于（B）的含脲基化合物（H），化合物（H）选自结构单元（I），结构单元（II），结构单元（III）-NR'-C（O）-N（X-SiR“x（OR'）3 - ）的结构单元 x）n（X'-SiR“y（OR'）3-y）m和上述两种或更多种的组合，化合物（H）是通过含异氰酸酯基的化合物（HG）与含氨基的化合物化合物，其中在（HG）中原子存在的大于90摩尔％的异氰酸酯基团的化合物（H）中已经发生反应以形成结构单元（I），（II），（III）或其组合，其中R' R'“=氢，烷基，环烷基，芳基或芳烷基; R，R“=烷基，环烷基，芳基或芳烷基; X，X'=直链和/或支链烷基或环烷基; x，y，n，m = 0〜2; m + n = 2。

10. 发明授权

US09353287B2 Coating agents having high scratch resistance and weathering stability 有权
标题翻译：具有高耐刮擦性和耐候稳定性的涂层剂
公开(公告)号：US09353287B2
公开(公告)日：2016-05-31
申请号：US12519449
申请日：2007-12-19
申请人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
发明人： Matthijs Groenewolt , Andreas Poppe , Gunter Klein , Manuela Niemeier , Elke Westhoff , Wilfried Stubbe , Simone Hesener
IPC分类号： D06M15/643 , C09D175/14 , C08G18/28 , C08G18/62 , C08G18/77 , C08G18/80 , C09D175/04
CPC分类号： C09D175/14 , C08G18/289 , C08G18/6254 , C08G18/778 , C08G18/809 , C09D175/04
摘要： Disclosed are coating compositions comprising at least one hydroxyl-containing compound (A) and at least one isocyanato-containing compound (B), wherein one or more of the constituents of the coating composition comprise between 2.5 and 97.5 mol %, based on the entirety of structural units (I) and (II), of at least one structural unit of the formula (I) —N(X—SiR″x(OR′)3-x)n(X′—SiR″y(OR′)3-y)m (I) and between 2.5 and 97.5 mol %, based on the entirety of structural units (I) and (II), of at least one structural unit of the formula (II) —Z—(X—SiR″x(OR′)3-x) (II).
摘要翻译：公开了包含至少一种含羟基的化合物（A）和至少一种含异氰酸酯基的化合物（B）的涂料组合物，其中涂料组合物的一种或多种组分包含2.5至97.5mol％结构单元（I）和（II）的至少一种结构单元的式（I）-N（X-SiR“x（OR'）3-x）n（X'-SiR”y（OR' ）（I）和（II）的至少一种结构单元，基于整个结构单元（I）和（II），2.5至97.5摩尔％ SiR“x（OR'）3-x）（II）。

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