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1. 发明授权

US06756030B1 Crystalline aluminosilicate zeolitic composition: UZM-8 有权
标题翻译：结晶硅铝酸盐沸石组合物：UZM-8
公开(公告)号：US06756030B1
公开(公告)日：2004-06-29
申请号：US10395466
申请日：2003-03-21
申请人： Lisa M. Rohde , Gregory J. Lewis , Mark A. Miller , Jaime G. Moscoso , Jana L. Gisselquist , R. Lyle Patton , Stephen T. Wilson , Deng Yang Jan
发明人： Lisa M. Rohde , Gregory J. Lewis , Mark A. Miller , Jaime G. Moscoso , Jana L. Gisselquist , R. Lyle Patton , Stephen T. Wilson , Deng Yang Jan
IPC分类号： C01B3948
CPC分类号： C10G45/62 , B01J29/70 , B01J29/74 , C01B39/06 , C01B39/065 , C01B39/48 , C10G45/10 , C10G45/12 , C10G45/64 , C10G47/14 , C10G47/20 , C10G49/06 , C10G49/08
摘要： Applicants have synthesized a family of microporous aluminosilicate zeolites and substituted versions thereof which are identified as UZM-8. These new compositions can be prepared using either only one or more organoammonium cations, such as diethyldimethylammonium or ethyltrimethylammonium cations and optionally an alkali and/or an alkaline earth cation as structure directing agents. The UZM-8 compositions are described by an empirical formula of Mmn+Rrp+Al1-xExSiyOz and have a unique x-ray diffraction pattern.
摘要翻译：申请人已经合成了一系列微孔硅铝酸盐沸石及其取代形式，其被鉴定为UZM-8。这些新的组合物可以使用仅一种或多种有机铵阳离子，如二乙基二甲基铵或乙基三甲基铵阳离子和任选的碱和/或碱土金属阳离子作为结构定向剂来制备。 UZM-8组合物由经验公式描述并具有独特的x射线衍射图。

2. 发明授权

US06713041B1 Crystalline aluminosilicate zeolitic composition: UZM-9 有权
标题翻译：结晶硅铝酸盐沸石组合物：UZM-9
公开(公告)号：US06713041B1
公开(公告)日：2004-03-30
申请号：US10074612
申请日：2002-02-12
申请人： Jaime G. Moscoso , Gregory J. Lewis , Jana L. Gisselquist , Mark A. Miller , Lisa M. Rohde
发明人： Jaime G. Moscoso , Gregory J. Lewis , Jana L. Gisselquist , Mark A. Miller , Lisa M. Rohde
IPC分类号： C01B3914
CPC分类号： C01B39/145 , B01J29/70 , B01J29/7003 , B01J2229/32 , C10G11/05 , C10G45/64 , C10G47/16 , Y10S423/24
摘要： Applicants have synthesized a new aluminosilicate zeolite identified as UZM-9. This new zeolite has the LTA topology and has an empirical formula of: Mmn+Rrp+Al1-xExSiyOz where M is an alkali or alkaline earth metal ion, R is at least two organic ions, at least one of which has an organic group with at least two carbon atoms and E can be gallium, iron, boron and mixtures thereof. The Si/Al ratio can range from greater than 3.5 to about 6.0.
摘要翻译：申请人合成了一种被认定为UZM-9的新型硅铝酸盐沸石。这种新沸石具有LTA拓扑结构，并且具有以下经验式：其中M是碱金属或碱土金属离子，R是至少两个有机离子，其中至少一个具有至少两个碳原子的有机基团，E 可以是镓，铁，硼及其混合物。 Si / Al比可以在大于3.5至约6.0的范围内。

3. 发明授权

US06613302B1 UZM-5, UZM-5P and UZM-6: crystalline aluminosilicate zeolites and processes using the same 有权
标题翻译： UZM-5，UZM-5P和UZM-6：结晶硅铝酸盐沸石及其使用方法
公开(公告)号：US06613302B1
公开(公告)日：2003-09-02
申请号：US09705860
申请日：2000-11-03
申请人： Jaime G. Moscoso , Gregory J. Lewis , Mark A. Miller , Deng-Yang Jan , R. Lyle Patton , Lisa M. Rohde
发明人： Jaime G. Moscoso , Gregory J. Lewis , Mark A. Miller , Deng-Yang Jan , R. Lyle Patton , Lisa M. Rohde
IPC分类号： C01B3948
CPC分类号： C07C5/2724 , B01J29/70 , B01J29/87 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , Y10S977/775 , Y10S977/776 , Y10S977/895 , Y10S977/896 , Y10S977/949 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A new family of crystalline alumino-silicate zeolites has been synthesized. These zeolites are represented by the empirical formula. Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl ammonium and E is a framework element such as gallium. They are also characterized by unique x-ray diffraction patterns and have catalytic properties for carrying out various hydrocarbon conversion processes.
摘要翻译：已经合成了一系列新型的结晶铝硅酸盐沸石。这些沸石由经验式表示，其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。它们的特征还在于独特的X射线衍射图，并且具有用于进行各种烃转化过程的催化性能。

4. 发明授权

US06500998B1 Aromatic alkylation process using UZM-5 and UZM-6 aluminosilicates 失效
标题翻译：使用UZM-5和UZM-6铝硅酸盐的芳香族烷基化方法
公开(公告)号：US06500998B1
公开(公告)日：2002-12-31
申请号：US10062691
申请日：2002-01-31
申请人： Deng-Yang Jan , Gregory J. Lewis , Jaime G. Moscoso , Mark A. Miller
发明人： Deng-Yang Jan , Gregory J. Lewis , Jaime G. Moscoso , Mark A. Miller
IPC分类号： C07C424
CPC分类号： C07C5/2724 , B01J29/04 , B01J29/70 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A process for transalkylating a polyalkylated aromatic compound with a non-alkylated aromatic compound using a new family of related crystalline aluminosilicate zeolites has been developed. These zeolites are represented by the empirical formula: Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl-ammonium and E is a framework element such as gallium.
摘要翻译：已经开发了使用新的相关结晶硅铝酸盐沸石系列将多烷基化芳族化合物与非烷基化芳族化合物烷基化的方法。这些沸石由经验式表示：其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。

5. 发明授权

US06890511B2 Crystalline aluminosilicate zeolitic composition: UZM-15 失效
标题翻译：结晶硅铝酸盐沸石组合物：UZM-15
公开(公告)号：US06890511B2
公开(公告)日：2005-05-10
申请号：US10395399
申请日：2003-03-21
申请人： Lisa M. Rohde , Gregory J. Lewis , Stephen T. Wilson , Deng-Yang Jan , R. Lyle Patton , Susan C. Koster , Jaime G. Moscoso , Mark A. Miller , Michael G. Gatter
发明人： Lisa M. Rohde , Gregory J. Lewis , Stephen T. Wilson , Deng-Yang Jan , R. Lyle Patton , Susan C. Koster , Jaime G. Moscoso , Mark A. Miller , Michael G. Gatter
IPC分类号： B01J29/70 , B01J29/87 , C01B39/02 , C01B39/08 , C01B39/48 , C07C7/13
CPC分类号： B01J29/87 , B01J29/70 , B01J2229/16 , B01J2229/32 , B01J2229/36 , B01J2229/37 , C01B39/026 , C01B39/082 , C01B39/48 , C01P2002/72 , C07C7/13
摘要： An aluminosilicate zeolite and substituted versions designated UZM-15 have been synthesized. These zeolites are prepared using an organoammonium cation as a template in which at least one organic group has at least 2 carbon atoms. An example of such a cation is diethyldimethylammonium cation. The template can optionally comprise other organoammonium cations, alkali metals and alkaline earth metals. These UZM-15 materials can be dealuminated by various processes to provide UZM-15HS compositions. Both the UZM-15 and UZM-15HS compositions are useful as catalysts or catalyst supports in various process such as the conversion of cyclic hydrocarbons to non-cyclic hydrocarbons and olefin oligomerization.
摘要翻译：已经合成了一种硅铝酸盐沸石，并且被认为是UZM-15的取代物。使用有机铵阳离子作为模板制备这些沸石，其中至少一个有机基团具有至少2个碳原子。这种阳离子的实例是二乙基二甲基铵阳离子。模板可任选地包含其它有机铵阳离子，碱金属和碱土金属。这些UZM-15材料可以通过各种工艺脱铝以提供UZM-15HS组合物。 UZM-15和UZM-15HS组合物可用作各种方法中的催化剂或催化剂载体，例如将环烃转化为非环烃和烯烃低聚。

6. 发明授权

US06419895B1 Crystalline aluminosilicate zeolitic composition: UZM-4 有权
标题翻译：结晶硅铝酸盐沸石组合物：UZM-4
公开(公告)号：US06419895B1
公开(公告)日：2002-07-16
申请号：US09705653
申请日：2000-11-03
申请人： Gregory J. Lewis , Jaime G. Moscoso , Mark A. Miller , Ben A. Wilson
发明人： Gregory J. Lewis , Jaime G. Moscoso , Mark A. Miller , Ben A. Wilson
IPC分类号： C01B3948
CPC分类号： C10G45/64 , B01J29/04 , B01J29/70 , C01B39/065 , C01B39/48 , C07C2/12 , C07C2/54 , C07C5/2708
摘要： Applicants have synthesized a new aluminosilicate zeolite identified as UZM-4. This new zeolite has the BPH morphology and is structurally related to zeolite Q. UZM-4 has en empirical formula of Mmn+Rrp+Al1−xExSiyOz where M is an alkali or alkaline earth metal ion, R can be a quaternary ammonium ion and E can be gallium, iron, boron, chromium, indium and mixtures thereof. The Si/Al ratio can range from 1.5 to about 4.0
摘要翻译：申请人合成了一种被认定为UZM-4的新型硅铝酸盐沸石。这种新沸石具有BPH形态，并且在结构上与沸石Q有关。UZM-4具有其中M是碱金属或碱土金属离子的经验式，R可以是季铵离子，E可以是镓，铁，硼，铬，铟及其混合物。 Si / Al比可以在1.5至约4.0的范围内

7. 发明授权

US06388157B1 Aromatic alkylation process using UZM-5 and UZM-6 aluminosilicates 失效
标题翻译：使用UZM-5和UZM-6铝硅酸盐的芳香族烷基化方法
公开(公告)号：US06388157B1
公开(公告)日：2002-05-14
申请号：US09706285
申请日：2000-11-03
申请人： Deng-Yang Jan , Gregory J. Lewis , Jaime G. Moscoso , Mark A. Miller
发明人： Deng-Yang Jan , Gregory J. Lewis , Jaime G. Moscoso , Mark A. Miller
IPC分类号： C07C268
CPC分类号： C07C5/2724 , B01J29/04 , B01J29/70 , C01B39/06 , C01B39/065 , C01B39/48 , C07C2/66 , C07C6/126 , C07C7/13 , C07C2529/70 , Y02P20/52 , C07C15/085 , C07C15/067 , C07C15/08
摘要： A process for alkylation of aromatic compounds using a new family of related crystalline aluminosilicate zeolites has been developed. These zeolites are represented by the empirical formula: Mmn+Rrp+Al(1−x)ExSiyOz where M is an alkali or alkaline earth metal such as lithium and strontium, R is a nitrogen containing organic cation such as tetramethyl-ammonium and E is a framework element such as gallium.
摘要翻译：已经开发了使用新的相关结晶硅铝酸盐沸石族烷基化芳族化合物的方法。这些沸石由经验式表示：其中M是碱金属或碱土金属如锂和锶，R是含氮有机阳离子如四甲基铵，E是骨架元素如镓。

8. 发明授权

US08349291B2 Calcined UZM-22 and UZM-22HS aluminosilicate zeolites 有权
标题翻译：煅烧的UZM-22和UZM-22HS铝硅酸盐沸石
公开(公告)号：US08349291B2
公开(公告)日：2013-01-08
申请号：US12821555
申请日：2010-06-23
申请人： Mark A. Miller , Jaime G. Moscoso , Gregory J. Lewis
发明人： Mark A. Miller , Jaime G. Moscoso , Gregory J. Lewis
IPC分类号： C01B39/46 , C01B39/48
CPC分类号： B01J29/70 , C01B39/06 , C01B39/48 , C10G29/205 , C10G45/64 , C10G49/08 , C10G50/00
摘要： Crystalline microporous zeolites designated calcined UZM-22 and UZM-22HS have been synthesized. The calcined UZM-22 is represented by the empirical formula: M1′mn+Al1-xExSiyOz and UZM-22HS has an empirical formula of: M1an+Al(1-x)ExSiy′Oz″ where M1 and M1′ are exchangeable cations such as lithium or strontium and E is a framework element such as gallium. Both zeolites are obtained from an as synthesized microporous crystalline composition having an empirical formula of: Mmn+RrAl1-xExSiyOz either by calcination for UZM-22 or by various treatments such as ammonium hexafluorosilicate treatment for UZM-22HS.M is an alkali, alkaline earth, or rare earth metal such as lithium and strontium, R is a singly charged organoammonium cation such as the choline cation and E is a framework element such as gallium.
摘要翻译：已经合成了称为煅烧UZM-22和UZM-22HS的结晶微孔沸石。煅烧的UZM-22由经验式表示：M1'mn + Al1-xExSiyOz，UZM-22HS具有经验式：M1an + Al（1-x）ExSiy'Oz“，其中M1和M1'是可交换阳离子作为锂或锶，E是诸如镓的骨架元素。两种沸石均由具有经验式：Mmn + RrAl1-xExSiyOz的合成微孔结晶组合物获得，其通过煅烧UZM-22或通过各种处理如六氟硅酸铵处理用于UZM-22HS。M是碱，碱土，或稀土金属如锂和锶，R是单电荷的有机铵阳离子，如胆碱阳离子，E是骨架元素如镓。

9. 发明授权

US07744850B2 UZM-22 aluminosilicate zeolite, method of preparation and processes using UZM-22 有权
标题翻译： UZM-22铝硅酸盐沸石，制备方法和使用UZM-22的方法
公开(公告)号：US07744850B2
公开(公告)日：2010-06-29
申请号：US11462056
申请日：2006-08-03
申请人： Mark A. Miller , Jaime G. Moscoso , Gregory J. Lewis
发明人： Mark A. Miller , Jaime G. Moscoso , Gregory J. Lewis
IPC分类号： C01B39/04
CPC分类号： B01J29/70 , C01B39/48 , C07C2/58 , C07C2/66 , C07C2529/70 , C10G29/205 , C10G45/64 , C10G50/00 , C07C9/16
摘要： A new family of crystalline aluminosilicate zeolites has been synthesized. These zeolites are represented by the empirical formula. Mmn+Rr+Al(1-x)ExSiyOz where M is an alkali, alkaline earth, or rare earth metal such as lithium and strontium, R is a singly charged organoammonium cation such as the choline cation and E is a framework element such as gallium. These zeolites are similar to ZSM-18 but are characterized by unique x-ray diffraction patterns and compositions and have catalytic properties for carrying out various hydrocarbon conversion processes.
摘要翻译：已经合成了一系列结晶硅铝酸盐沸石。这些沸石由经验公式表示。 Mmn + Rr + Al（1-x）ExSiyOz其中M是碱金属，碱土金属或稀土金属如锂和锶，R是单一带电的有机铵阳离子，如胆碱阳离子，E是骨架元素，镓。这些沸石类似于ZSM-18，但是其特征在于独特的x射线衍射图和组成，并具有用于进行各种烃转化方法的催化性能。

10. 发明授权

US07344694B2 UZM-12 and UZM-12HS: crystalline aluminosilicate zeolitic compositions and processes for preparing and using the compositions 有权
标题翻译： UZM-12和UZM-12HS：结晶硅铝酸盐沸石组合物和制备和使用组合物的方法
公开(公告)号：US07344694B2
公开(公告)日：2008-03-18
申请号：US10959453
申请日：2004-10-06
申请人： Mark A. Miller , Gregory J. Lewis , Jana L. Gisselquist , Jaime G. Moscoso , R. Lyle Patton
发明人： Mark A. Miller , Gregory J. Lewis , Jana L. Gisselquist , Jaime G. Moscoso , R. Lyle Patton
IPC分类号： C01B39/30
CPC分类号： C01B39/48 , B01J29/50 , C01B39/305
摘要： A series of crystalline alumino-silicate zeolites identified as UZM-12 have been synthesized. These UZM-12 compositions have the ERI topology, a Si/Al>5.5 and can be prepared as nanocrystallites having an average particle size of about 15 to about 50 nanometers and a spheroidal morphology. The UZM-12 composition can be treated to remove at least a fraction of the framework aluminum atoms thereby providing zeolites with a Si/Al>5.75 and identified as UZM-12HS. Both the UZM-12 and UZM-12HS can catalyze various hydrocarbon conversion processes.
摘要翻译：已经合成了一系列标准为UZM-12的结晶铝硅酸盐沸石。这些UZM-12组合物具有ERI拓扑结构，Si / Al> 5.5，并且可以制备为具有约15至约50纳米的平均粒度和球形形态的纳米晶体。可以处理UZM-12组合物以除去至少一部分骨架铝原子，从而提供具有Si / Al> 5.75的沸石并鉴定为UZM-12HS。 UZM-12和UZM-12HS都可以催化各种烃转化过程。

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