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1. 发明申请

US20070249880A1 Production of aromatics from methane 有权
标题翻译：从甲烷生产芳烃
公开(公告)号：US20070249880A1
公开(公告)日：2007-10-25
申请号：US11787958
申请日：2007-04-18
申请人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
发明人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
IPC分类号： C07C2/52 , C07C6/00
CPC分类号： C07C2/76 , C07C2529/48 , C10G45/44 , Y02P20/142 , Y02P20/52 , Y10S585/943 , C07C15/04 , C07C15/02
摘要： In a process for converting methane to aromatic hydrocarbons, a feed containing methane is supplied to one or more reaction zone(s) containing catalytic material operating under reaction conditions effective to convert at least a portion of the methane to aromatic hydrocarbons; the reaction zone(s) being operated with an inverse temperature profile.
摘要翻译：在将甲烷转化为芳族烃的方法中，含有甲烷的进料被供应到一个或多个反应区，该反应区含有在有效将甲烷的至少一部分转化为芳烃的反应条件下运行的催化材料; 反应区域以反向温度曲线运行。

2. 发明授权

US07795490B2 Production of aromatics from methane 有权
标题翻译：从甲烷生产芳烃
公开(公告)号：US07795490B2
公开(公告)日：2010-09-14
申请号：US11787958
申请日：2007-04-18
申请人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
发明人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
IPC分类号： C07C2/78
CPC分类号： C07C2/76 , C07C2529/48 , C10G45/44 , Y02P20/142 , Y02P20/52 , Y10S585/943 , C07C15/04 , C07C15/02
摘要： In a process for converting methane to aromatic hydrocarbons, a feed containing methane is supplied to one or more reaction zone(s) containing catalytic material operating under reaction conditions effective to convert at least a portion of the methane to aromatic hydrocarbons; the reaction zone(s) being operated with an inverse temperature profile.
摘要翻译：在将甲烷转化为芳族烃的方法中，含有甲烷的进料被供应到一个或多个反应区，该反应区含有在有效将甲烷的至少一部分转化为芳烃的反应条件下运行的催化材料; 反应区域以反向温度曲线运行。

3. 发明授权

US07968759B2 Production of aromatics from methane 失效
标题翻译：从甲烷生产芳烃
公开(公告)号：US07968759B2
公开(公告)日：2011-06-28
申请号：US12851244
申请日：2010-08-05
申请人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
发明人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
IPC分类号： C07C2/78
CPC分类号： C07C2/76 , C07C2529/48 , C10G45/44 , Y02P20/142 , Y02P20/52 , Y10S585/943 , C07C15/04 , C07C15/02
摘要： In a process for converting methane to aromatic hydrocarbons, a feed containing methane is supplied to one or more reaction zone(s) containing catalytic material operating under reaction conditions effective to convert at least a portion of the methane to aromatic hydrocarbons; the reaction zone(s) being operated with an inverse temperature profile.
摘要翻译：在将甲烷转化为芳族烃的方法中，含有甲烷的进料被供应到一个或多个反应区，该反应区含有在有效将甲烷的至少一部分转化为芳烃的反应条件下运行的催化材料; 反应区域以反向温度曲线运行。

4. 发明申请

US20100305374A1 Production Of Aromatics From Methane 失效
标题翻译：从甲烷生产芳烃
公开(公告)号：US20100305374A1
公开(公告)日：2010-12-02
申请号：US12851244
申请日：2010-08-05
申请人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
发明人： Larry L. Iaccino , Elizabeth L. Stavens , Neeraj Sangar , Jeremy J. Patt
IPC分类号： C07C5/02 , C07C2/00
CPC分类号： C07C2/76 , C07C2529/48 , C10G45/44 , Y02P20/142 , Y02P20/52 , Y10S585/943 , C07C15/04 , C07C15/02
摘要： In a process for converting methane to aromatic hydrocarbons, a feed containing methane is supplied to one or more reaction zone(s) containing catalytic material operating under reaction conditions effective to convert at least a portion of the methane to aromatic hydrocarbons; the reaction zone(s) being operated with an inverse temperature profile.
摘要翻译：在将甲烷转化为芳族烃的方法中，含有甲烷的进料被供应到一个或多个反应区，该反应区含有在有效将甲烷的至少一部分转化为芳烃的反应条件下运行的催化材料; 反应区域以反向温度曲线运行。

5. 发明授权

US07589246B2 Production of aromatics from methane 有权
标题翻译：从甲烷生产芳烃
公开(公告)号：US07589246B2
公开(公告)日：2009-09-15
申请号：US12041275
申请日：2008-03-03
申请人： Larry L. Iaccino , Teng Xu , J. Scott Buchanan , Neeraj Sangar , Jeremy J. Patt , Mark A. Nierode , Kenneth R. Clem , Mobae Afeworki
发明人： Larry L. Iaccino , Teng Xu , J. Scott Buchanan , Neeraj Sangar , Jeremy J. Patt , Mark A. Nierode , Kenneth R. Clem , Mobae Afeworki
IPC分类号： C07C2/42 , C07C2/46
CPC分类号： B01J38/10 , B01J23/92 , B01J29/405 , B01J29/48 , B01J29/90 , B01J37/0036 , C07C2/78 , C07C2529/48 , Y02P20/142 , Y02P20/584 , Y02P20/588 , Y10S585/943 , C07C15/02
摘要： In a process for converting methane to aromatic hydrocarbons, a feed containing methane and a particulate catalytic material are supplied to a reaction zone operating under reaction conditions effective to convert at least a portion of the methane to aromatic hydrocarbons and to deposit carbonaceous material on the particulate catalytic material causing catalyst deactivation. At least a portion of the deactivated particulate catalytic material is removed from the reaction zone and is heated to a temperature of about 700° C. to about 1200° C. by direct and/or indirect contact with combustion gases produced by combustion of a supplemental fuel. The heated particulate catalytic material is then regenerated with a hydrogen-containing gas under conditions effective to convert at least a portion of the carbonaceous material thereon to methane and the regenerated catalytic particulate material is recycled back to the reaction zone.
摘要翻译：在将甲烷转化为芳族烃的方法中，将含有甲烷和颗粒催化材料的进料供应到在有效将甲烷的至少一部分转化为芳族烃的反应条件下运行的反应区，并将含碳材料沉积在颗粒上催化材料引起催化剂失活。将至少一部分失活的颗粒催化材料从反应区中除去，并通过与补充物的燃烧产生的燃烧气体的直接和/或间接接触将其加热至约700℃至约1200℃的温度汽油。然后在有效将其上的至少一部分碳质材料转化为甲烷的条件下，用含氢气体再生加热的颗粒催化材料，再生的催化颗粒材料再循环回到反应区。

6. 发明申请

US20080249342A1 Production of Aromatics from Methane 有权
标题翻译：从甲烷生产芳烃
公开(公告)号：US20080249342A1
公开(公告)日：2008-10-09
申请号：US12041275
申请日：2008-03-03
申请人： Larry L. Iaccino , Teng Xu , J. Scott Buchanan , Neeraj Sangar , Jeremy J. Patt , Mark A. Nierode , Kenneth R. Clem , Mobae Afeworki
发明人： Larry L. Iaccino , Teng Xu , J. Scott Buchanan , Neeraj Sangar , Jeremy J. Patt , Mark A. Nierode , Kenneth R. Clem , Mobae Afeworki
IPC分类号： C07C2/00
CPC分类号： B01J38/10 , B01J23/92 , B01J29/405 , B01J29/48 , B01J29/90 , B01J37/0036 , C07C2/78 , C07C2529/48 , Y02P20/142 , Y02P20/584 , Y02P20/588 , Y10S585/943 , C07C15/02
摘要： In a process for converting methane to aromatic hydrocarbons, a feed containing methane and a particulate catalytic material are supplied to a reaction zone operating under reaction conditions effective to convert at least a portion of the methane to aromatic hydrocarbons and to deposit carbonaceous material on the particulate catalytic material causing catalyst deactivation. At least a portion of the deactivated particulate catalytic material is removed from the reaction zone and is heated to a temperature of about 700° C. to about 1200° C. by direct and/or indirect contact with combustion gases produced by combustion of a supplemental fuel. The heated particulate catalytic material is then regenerated with a hydrogen-containing gas under conditions effective to convert at least a portion of the carbonaceous material thereon to methane and the regenerated catalytic particulate material is recycled back to the reaction zone.
摘要翻译：在将甲烷转化为芳香族烃的方法中，将含有甲烷和颗粒状催化材料的原料供给到在有效将甲烷的至少一部分转化为芳族烃并将含碳材料沉积在颗粒物上的反应条件下运行的反应区催化材料引起催化剂失活。将至少一部分失活的颗粒催化材料从反应区中除去，并通过与补充物的燃烧产生的燃烧气体的直接和/或间接接触将其加热至约700℃至约1200℃的温度汽油。然后在有效将其上的至少一部分碳质材料转化为甲烷的条件下，用含氢气体再生加热的颗粒催化材料，再生的催化颗粒材料再循环回到反应区。

7. 发明申请

US20090030253A1 Production of Aromatics from Aliphatics 有权
标题翻译：从芳烃生产芳烃
公开(公告)号：US20090030253A1
公开(公告)日：2009-01-29
申请号：US12166153
申请日：2008-07-01
申请人： Teng Xu , Kenneth R. Clem , Jeremy J. Patt , J. Scott Buchanan , Larry L. Iaccino
发明人： Teng Xu , Kenneth R. Clem , Jeremy J. Patt , J. Scott Buchanan , Larry L. Iaccino
IPC分类号： C07C2/00
CPC分类号： C07C2/76 , C07C15/02
摘要： In a process for converting a low carbon number aliphatic hydrocarbon to higher hydrocarbons including aromatic hydrocarbons, a feed containing the aliphatic hydrocarbon is contacted with a dehydrocyclization catalyst under conditions effective to convert the aliphatic hydrocarbon to aromatic hydrocarbons and produce an effluent stream comprising aromatic hydrocarbons and hydrogen. The dehydrocyclization catalyst comprises a metal or metal compound and a molecular sieve wherein the ratio of the amount of any Bronsted acid sites in the catalyst to the amount of said metal in the catalyst is less than 0.4 mol/mol of said metal.
摘要翻译：在将低碳数脂肪族烃转化成包括芳烃的高级烃的方法中，将含有脂族烃的进料与脱氢环化催化剂在有效将脂肪烃转化为芳族烃并产生包含芳族烃的流出物流的条件下接触，氢。脱氢环化催化剂包括金属或金属化合物和分子筛，其中催化剂中任何布朗斯台德酸位点的量与催化剂中所述金属的量的比例小于所述金属的0.4mol / mol。

8. 发明申请

US20100240935A1 Use of Isotopic Analysis for Determination of Aromatic Hydrocarbons Produced From Methane 审中-公开
标题翻译：使用同位素分析测定甲烷产生的芳香烃
公开(公告)号：US20100240935A1
公开(公告)日：2010-09-23
申请号：US12790204
申请日：2010-05-28
申请人： Larry L. Iaccino , Jeremy J. Patt
发明人： Larry L. Iaccino , Jeremy J. Patt
IPC分类号： C07C15/04
CPC分类号： C07C2/66 , C07C2/76 , Y10S585/941 , C07C15/08 , C07C15/04
摘要： Benzene and xylene are described having a unique distribution of deuterium and 13C such that δ(deuterium) for each of the benzene and xylene is less than −250 and δ(13C) for the benzene is greater than −36 and for xylene is less than −24, wherein δ(deuterium)=(R′sample/R′standard−1)×1000 where R′sample is the ratio of deuterium to hydrogen in the benzene/xylene; and R′standard is the ratio of the natural abundance of deuterium to the natural abundance of hydrogen; and wherein δ(13C)=(R″sample/R″standard−1)×1000 where R″sample is the ratio of 13C to 12C in the benzene/xylene; and R″standard is the ratio of the natural abundance of 13C to the natural abundance of 12C.
摘要翻译：描述苯和二甲苯具有氘和13C的独特分布，使得苯和二甲苯中的每一个的δ（氘）小于-250，苯的δ（13℃）大于-36，并且对于二甲苯小于 -24，其中δ（氘）=（R'sample / R'standard-1）×1000其中R'示例是苯/二甲苯中氘与氢的比例; R'standard是氘的天然丰度与氢的天然丰度之比; 其中δ（13C）=（R“样品/ R”标准-1）×1000其中R“样品是苯/二甲苯中13C至12C的比例; 而R“标准是13C的天然丰度与12C的天然丰度之比。

9. 发明授权

US07982080B2 Production of aromatics from aliphatics 有权
标题翻译：从脂肪生产芳烃
公开(公告)号：US07982080B2
公开(公告)日：2011-07-19
申请号：US12166153
申请日：2008-07-01
申请人： Teng Xu , Kenneth R. Clem , Jeremy J. Patt , J. Scott Buchanan , Larry L. Iaccino
发明人： Teng Xu , Kenneth R. Clem , Jeremy J. Patt , J. Scott Buchanan , Larry L. Iaccino
IPC分类号： C07C2/46
CPC分类号： C07C2/76 , C07C15/02
摘要： In a process for converting a low carbon number aliphatic hydrocarbon to higher hydrocarbons including aromatic hydrocarbons, a feed containing the aliphatic hydrocarbon is contacted with a dehydrocyclization catalyst under conditions effective to convert the aliphatic hydrocarbon to aromatic hydrocarbons and produce an effluent stream comprising aromatic hydrocarbons and hydrogen. The dehydrocyclization catalyst comprises a metal or metal compound and a molecular sieve wherein the ratio of the amount of any Bronsted acid sites in the catalyst to the amount of said metal in the catalyst is less than 0.4 mol/mol of said metal.
摘要翻译：在将低碳数脂肪族烃转化成包括芳烃的高级烃的方法中，将含有脂族烃的进料与脱氢环化催化剂在有效将脂肪烃转化为芳族烃并产生包含芳族烃的流出物流的条件下接触，氢。脱氢环化催化剂包括金属或金属化合物和分子筛，其中催化剂中任何布朗斯台德酸位点的量与催化剂中所述金属的量的比例小于所述金属的0.4mol / mol。

10. 发明申请

US20070282145A1 Use of isotopic analysis for determination of aromatic hydrocarbons produced from methane 有权
标题翻译：使用同位素分析测定甲烷产生的芳烃
公开(公告)号：US20070282145A1
公开(公告)日：2007-12-06
申请号：US11805868
申请日：2007-05-24
申请人： Larry L. Iaccino , Jeremy J. Patt
发明人： Larry L. Iaccino , Jeremy J. Patt
IPC分类号： C07C13/00 , C07C15/00
CPC分类号： C07C2/66 , C07C2/76 , Y10S585/941 , C07C15/08 , C07C15/04
摘要： Benzene and xylene are described having a unique distribution of deuterium and 13C such that δ(deuterium) for each of the benzene and xylene is less than −250 and δ(13C) for the benzene is greater than −36 and for xylene is less than −24, wherein δ(deuterium)=(R′sample/R′standard−1)×1000 where R′sample is the ratio of deuterium to hydrogen in the benzene/xylene; and R′standard is the ratio of the natural abundance of deuterium to the natural abundance of hydrogen; and wherein δ(13C)=(R″sample/R″standard−1)×1000 where R″sample is the ratio of 13C to 12C in the benzene/xylene; and R″standard is the ratio of the natural abundance of 13C to the natural abundance of 12C.
摘要翻译：描述苯和二甲苯具有独特的氘和13 C的分布，使得苯和二甲苯中的每一个的δ（氘）小于-250，并且δ（< C）对于苯大于-36，二甲苯小于-24，其中<？在线公式描述=“在线公式”end =“lead”→delta（氘）=（R' 标准 -1）x1000 <？in-line-formula description =“In-line Formulas”end =“tail”？>其中R'_{样品是苯/二甲苯中氘与氢的比例; 和R'标准是氘的天然丰度与氢的天然丰度之比; 并且其中<？in-line-formula description =“In-line Formulas”end =“lead”？> delta（13 C）=（R“'样品/ 标准 -1）x1000 <？in-line-formula description =“In-line Formulas”end =“tail”？>其中R“' 苯/二甲苯中的13 C与12 C的比例; 而“标准”是“自然丰度”的天然丰度与12 C“天然丰度之比”。}

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