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1. 发明授权

US08753500B2 Process and system for blending synthetic and natural crude oils derived from offshore produced fluids 有权
标题翻译：用于混合源自海上生产流体的合成和天然原油的方法和系统
公开(公告)号：US08753500B2
公开(公告)日：2014-06-17
申请号：US12974337
申请日：2010-12-21
申请人： Charles Leonard Kibby , Dennis J. O'Rear , Robert James Saxton , Tapan K. Das , Kandaswamy Jothimurugesan
发明人： Charles Leonard Kibby , Dennis J. O'Rear , Robert James Saxton , Tapan K. Das , Kandaswamy Jothimurugesan
IPC分类号： C10B57/02
CPC分类号： C10G2/34 , C10G2/32 , C10G2/332 , C10G2/333 , C10G2/341 , C10G2/344 , C10G5/06 , C10G45/02 , C10G45/58 , C10G47/00 , C10G49/00 , C10G2300/1022 , C10G2300/1033 , C10G2300/302 , C10G2300/4062
摘要： A process and system are described for the processing of gas associated with crude oil production, i.e. associated gas. A separation complex is used to separate produced fluids produced from a hydrocarbon reservoir into crude oil, liquefied petroleum gas, water, and natural gas. At least a portion of the natural gas is converted into synthesis gas in a synthesis gas generator. A combination of a synthesis gas conversion catalysts and hydroconversion catalysts are used in a synthesis gas reactor to convert the synthesis gas into a liquid effluent stream containing liquefied petroleum gas and a synthetic crude oil. The liquefied petroleum gas and synthetic crude oil from the synthesis gas reactor is sent to the separation complex. Liquefied petroleum gas is separated both from the synthetic crude oil and a natural crude oil obtained from the produced fluids. The system and process permits synthetic crude oil to be blended with the natural crude oil producing a blended stabilized crude oil having 2 wt % or more of the synthetic crude oil and with a pour point of 60° C. or less. Use of a common facility for separation operations on the natural crude oil and synthetic crude oil thus reduces capital costs and allows converted associated gases to be shipped with the natural crude oil on a conventional crude oil tanker.
摘要翻译：描述了用于处理与原油生产相关的气体，即相关气体的方法和系统。分离复合物用于将由烃储层产生的产物分离成原油，液化石油气，水和天然气。至少一部分天然气在合成气发生器中被转化为合成气。在合成气反应器中使用合成气转化催化剂和加氢转化催化剂的组合，以将合成气转化为含有液化石油气和合成原油的液体流出物流。将来自合成气反应器的液化石油气和合成原油送至分离复合物。液化石油气与合成原油和从生产的流体获得的天然原油分离。该系统和方法允许合成原油与天然原油混合，产生具有2重量％或更多的合成原油并且倾点为60℃或更低的混合稳定的原油。在天然原油和合成原油上使用通用设施进行分离操作，从而降低资本成本，并允许转换的相关气体与常规原油油轮上的天然原油一起运输。

2. 发明申请

US20110240288A1 PROCESS AND SYSTEM FOR BLENDING SYNTHETIC AND NATURAL CRUDE OILS DERIVED FROM OFFSHORE PRODUCED FLUIDS 有权
标题翻译：从海洋生产的流体中混合合成和自然原油的方法和系统
公开(公告)号：US20110240288A1
公开(公告)日：2011-10-06
申请号：US12974337
申请日：2010-12-21
申请人： Charles Leonard Kibby , Dennis J. O'Rear , Robert James Saxton , Tapan K. Das , Kandaswamy Jothimurugesan
发明人： Charles Leonard Kibby , Dennis J. O'Rear , Robert James Saxton , Tapan K. Das , Kandaswamy Jothimurugesan
IPC分类号： E21B43/00
CPC分类号： C10G2/34 , C10G2/32 , C10G2/332 , C10G2/333 , C10G2/341 , C10G2/344 , C10G5/06 , C10G45/02 , C10G45/58 , C10G47/00 , C10G49/00 , C10G2300/1022 , C10G2300/1033 , C10G2300/302 , C10G2300/4062
摘要： A process and system are described for the processing of gas associated with crude oil production, i.e. associated gas. A separation complex is used to separate produced fluids produced from a hydrocarbon reservoir into crude oil, liquefied petroleum gas, water, and natural gas. At least a portion of the natural gas is converted into synthesis gas in a synthesis gas generator. A combination of a synthesis gas conversion catalysts and hydroconversion catalysts are used in a synthesis gas reactor to convert the synthesis gas into a liquid effluent stream containing liquefied petroleum gas and a synthetic crude oil. The liquefied petroleum gas and synthetic crude oil from the synthesis gas reactor is sent to the separation complex. Liquefied petroleum gas is separated both from the synthetic crude oil and a natural crude oil obtained from the produced fluids. The system and process permits synthetic crude oil to be blended with the natural crude oil producing a blended stabilized crude oil having 2 wt % or more of the synthetic crude oil and with a pour point of 60° C. or less. Use of a common facility for separation operations on the natural crude oil and synthetic crude oil thus reduces capital costs and allows converted associated gases to be shipped with the natural crude oil on a conventional crude oil tanker.
摘要翻译：描述了用于处理与原油生产相关的气体，即相关气体的方法和系统。分离复合物用于将由烃储层产生的产物分离成原油，液化石油气，水和天然气。至少一部分天然气在合成气发生器中被转化为合成气。在合成气反应器中使用合成气转化催化剂和加氢转化催化剂的组合，以将合成气转化为含有液化石油气和合成原油的液体流出物流。将来自合成气反应器的液化石油气和合成原油送至分离复合物。液化石油气与合成原油和从生产的流体获得的天然原油分离。该系统和方法允许合成原油与天然原油混合，产生具有2重量％或更多的合成原油并且倾点为60℃或更低的混合稳定的原油。在天然原油和合成原油上使用通用设施进行分离操作，从而降低资本成本，并允许转换的相关气体与常规原油油轮上的天然原油一起运输。

3. 发明授权

US09206091B2 Processes and systems for synthesis gas conversion using a hybrid fischer-tropsch catalyst in a compact heat exchange reactor 有权
标题翻译：在紧凑型热交换反应器中使用混合费 - 托催化剂进行合成气转化的方法和系统
公开(公告)号：US09206091B2
公开(公告)日：2015-12-08
申请号：US14219774
申请日：2014-03-19
申请人： Robert James Saxton, Jr. , Kandaswamy Jothimurugesan , Charles Leonard Kibby
发明人： Robert James Saxton, Jr. , Kandaswamy Jothimurugesan , Charles Leonard Kibby
IPC分类号： C07C27/00 , C07C1/04 , B01J19/00 , B01J35/00 , B01J8/00 , B01J23/75 , B01J23/89 , B01J29/00 , B01J35/02 , B01J35/10 , C10G2/00 , F28F3/00 , F28D9/00
CPC分类号： C07C1/0435 , B01J8/008 , B01J19/00 , B01J19/0093 , B01J23/75 , B01J23/8913 , B01J29/00 , B01J29/7669 , B01J35/0006 , B01J35/023 , B01J35/1019 , B01J2208/00026 , B01J2219/00049 , B01J2219/00761 , B01J2219/00783 , B01J2219/00822 , B01J2219/00826 , B01J2219/00835 , B01J2219/00873 , B01J2229/186 , C07C1/042 , C10G2/334 , F28D9/00 , F28D9/0062 , F28F3/00 , F28F3/025
摘要： Disclosed are a process and a system for synthesis gas conversion. The process includes contacting a synthesis gas feed of hydrogen and carbon monoxide having a H2/CO ratio from 0.5 to 3.0 with a hybrid catalyst of particles having a particle size from 50 to 500 μm and having at least one zeolite and a Fischer-Tropsch component wherein the ratio of zeolite to Fischer-Tropsch component is from 0.1:1 to 30:1 and the hybrid catalyst includes from 0.5 to 40 wt % Fischer-Tropsch component. The process is conducted in a compact heat exchange reactor having a set of reaction passages disposed between a synthesis gas feed header and a products header and a set of coolant passages disposed between a coolant inlet header and a coolant outlet header. The set of coolant passages conducts a coolant therethrough, and the set of reaction passages contains the hybrid catalyst therein and conducts synthesis gas and reaction products therethrough. The process is conducted at a temperature from 200 to 2800° C., a pressure from 5 to 40 atmospheres, a recycle ratio from 1 to 3, and a gaseous hourly space velocity less than 20,000 volumes of gas per volume of catalyst per hour. The effluent produced includes a hydrocarbon product containing at least 50 wt % C5+ hydrocarbons and less than 5 wt % C21+ hydrocarbons at a C5+ productivity from 0.05 to 2 gC5+/gcat/h.
摘要翻译：公开了合成气转化的方法和系统。该方法包括将H 2 / CO比为0.5至3.0的氢气和一氧化碳的合成气进料与粒度为50-500μm的颗粒的混合催化剂接触并具有至少一种沸石和费 - 托组分其中沸石与费 - 托组分的比例为0.1:1至30:1，并且所述混合催化剂包含0.5至40wt％的费 - 托组分。该过程在紧凑的热交换反应器中进行，其具有设置在合成气进料集管和产品集管之间的一组反应通道和设置在冷却剂入口集管和冷却剂出口集管之间的一组冷却剂通道。该组冷却剂通道使冷却剂通过其中，并且该组反应通道在其中包含混合催化剂，并通过其引导合成气和反应产物。该方法在200至2800℃的温度，5至40个大气压的压力，1至3的循环比和每小时体积的催化剂小于20,000体积的气体的气时空速下进行。产生的流出物包含含有至少50重量％的C 5+烃和少于5重量％的C 21+烃的烃产物，其C5 +生产率为0.05至2gC5 + / gcat / h。

4. 发明申请

US20140213670A1 HYBRID FISCHER-TROPSCH CATALYSTS AND PROCESSES FOR USE 有权
标题翻译：混合式螯合催化剂和使用方法
公开(公告)号：US20140213670A1
公开(公告)日：2014-07-31
申请号：US13750089
申请日：2013-01-25
申请人： Kandaswamy Jothimurugesan , Robert James Saxton
发明人： Kandaswamy Jothimurugesan , Robert James Saxton
IPC分类号： C07C1/04 , B01J29/76
CPC分类号： C07C1/0435 , B01J29/7661 , B01J37/0009 , B01J37/0203 , B01J2229/20 , B01J2229/42 , C07C9/00 , C10G2/332 , C10G2/333 , C10G2/334 , C10G2300/1022
摘要： Disclosed are hybrid Fischer-Tropsch catalysts containing cobalt and ZSM-48 zeolite. The hybrid Fischer-Tropsch catalysts can contain cobalt deposited on ZSM-48 extrudate supports. Alternatively, the Fischer-Tropsch catalysts can contain cobalt deposited on supports mixed with ZSM-48 particles. It has surprisingly been found that the use of hybrid Fischer-Tropsch catalysts containing ZSM-48 zeolite in synthesis gas conversion reactions results in improved C5+ productivity and catalyst activity, as well as a desirable product distribution including low formation of methane and C21+.
摘要翻译：公开了含有钴和ZSM-48沸石的混合费 - 托催化剂。混合费 - 托催化剂可以含有沉积在ZSM-48挤出物载体上的钴。或者，费 - 托催化剂可以含有沉积在与ZSM-48颗粒混合的载体上的钴。令人惊奇地发现，在合成气转化反应中使用含有ZSM-48沸石的混合费 - 托催化剂导致提高的C5 +生产率和催化剂活性，以及包括低甲烷和C21 +形成的理想产物分布。

5. 发明申请

US20130253079A1 HYBRID FISCHER-TROPSCH CATALYSTS AND PROCESSES FOR USE THEREOF 有权
标题翻译：混合型螯合催化剂及其使用方法
公开(公告)号：US20130253079A1
公开(公告)日：2013-09-26
申请号：US13603743
申请日：2012-09-05
申请人： Kandaswamy Jothimurugesan , Robert James Saxton
发明人： Kandaswamy Jothimurugesan , Robert James Saxton
IPC分类号： C10G2/00 , B01J29/80 , B01J29/76
CPC分类号： C10G2/334 , B01J23/8913 , B01J29/7669 , B01J29/80 , B01J35/006 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0009 , B01J37/0201 , B01J37/04 , C10G2/332
摘要： Disclosed are hybrid Fischer-Tropsch catalysts containing cobalt deposited on hybrid supports. The hybrid supports contain an acidic zeolite component and a silica-containing material. It has been found that the use of the hybrid Fischer-Tropsch catalysts in synthesis gas conversion reactions results in high C5+ productivity, high CO conversion rates and low olefin formation.
摘要翻译：公开了含有沉积在混合载体上的钴的混合费 - 托催化剂。杂化载体含有酸性沸石组分和含二氧化硅的材料。已经发现，在合成气转化反应中使用混合费 - 托催化剂导致高的C5 +生产率，高CO转化率和低烯烃形成。

6. 发明授权

US09023899B2 Hybrid fischer-tropsch catalysts and processes for use thereof 有权
标题翻译：混合费 - 托催化剂及其使用方法
公开(公告)号：US09023899B2
公开(公告)日：2015-05-05
申请号：US13603743
申请日：2012-09-05
申请人： Kandaswamy Jothimurugesan , Robert James Saxton
发明人： Kandaswamy Jothimurugesan , Robert James Saxton
IPC分类号： C07C27/00 , C10G2/00 , B01J29/76 , B01J29/80 , B01J23/89 , B01J37/00 , B01J37/02 , B01J37/04 , B01J35/00 , B01J35/10
CPC分类号： C10G2/334 , B01J23/8913 , B01J29/7669 , B01J29/80 , B01J35/006 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0009 , B01J37/0201 , B01J37/04 , C10G2/332
摘要： Disclosed are hybrid Fischer-Tropsch catalysts containing cobalt deposited on hybrid supports. The hybrid supports contain an acidic zeolite component and a silica-containing material. It has been found that the use of the hybrid Fischer-Tropsch catalysts in synthesis gas conversion reactions results in high C5+ productivity, high CO conversion rates and low olefin formation.
摘要翻译：公开了含有沉积在混合载体上的钴的混合费 - 托催化剂。杂化载体含有酸性沸石组分和含二氧化硅的材料。已经发现，在合成气转化反应中使用混合费 - 托催化剂导致高的C5 +生产率，高CO转化率和低烯烃形成。

7. 发明申请

US20140336286A1 Modified Fischer-Tropsch Monolith Catalysts and Methods For Preparation and Use Thereof 审中-公开
标题翻译：改性费托复合催化剂及其制备方法
公开(公告)号：US20140336286A1
公开(公告)日：2014-11-13
申请号：US14339866
申请日：2014-07-24
申请人： Charles Leonard Kibby , Robert James Saxton, JR. , Kandaswamy Jothimurugesan , Tapan Kumar Das , Howard Steven Lacheen , Michael Bartz , Alfred Hass
发明人： Charles Leonard Kibby , Robert James Saxton, JR. , Kandaswamy Jothimurugesan , Tapan Kumar Das , Howard Steven Lacheen , Michael Bartz , Alfred Hass
IPC分类号： B01J29/76 , B01J23/89 , C07C1/04
CPC分类号： B01J29/7669 , B01J23/8986 , B01J29/061 , B01J29/064 , B01J29/068 , B01J29/072 , B01J29/076 , B01J29/7469 , B01J29/7869 , B01J35/023 , B01J35/04 , B01J37/0036 , B01J37/0203 , B01J37/0225 , B01J37/0228 , B01J37/0244 , B01J37/0246 , B01J37/0248 , B01J2229/186 , B01J2229/42 , B01J2229/60 , C07C1/0435 , C07C2529/072 , C10G2/33 , Y10T428/31678
摘要： Disclosed are hybrid synthesis gas conversion catalysts containing at least one Fischer-Tropsch component and at least one acidic component deposited on a monolith catalyst support for use in synthesis gas conversion processes and methods for preparing the catalysts. Also disclosed are synthesis gas conversion processes in which the hybrid synthesis gas conversion catalysts are contacted with synthesis gas to produce a hydrocarbon product containing at least 50 wt % C5+ hydrocarbons. Also disclosed are synthesis gas conversion processes in which at least one layer of Fischer-Tropsch component deposited onto a monolith support is alternated with at least one layer of acidic component in a fixed bed reactor.
摘要翻译：公开了含有至少一种费 - 托组分和沉积在整体催化剂载体上的至少一种酸性组分的混合合成气转化催化剂，用于合成气转化方法和制备催化剂的方法。还公开了合成气转化方法，其中混合合成气转化催化剂与合成气体接触以产生含有至少50重量％的C 5+烃的烃产物。还公开了合成气转化方法，其中沉积在整料载体上的至少一层费 - 托成分与固定床反应器中的至少一层酸性组分交替。

8. 发明申请

US20130210942A1 MODIFIED FISCHER-TROPSCH MONOLITH CATALYSTS AND METHODS FOR PREPARATION AND USE THEREOF 审中-公开
标题翻译：改性FISCHER-TROPSCH单晶催化剂及其制备和使用方法
公开(公告)号：US20130210942A1
公开(公告)日：2013-08-15
申请号：US13396466
申请日：2012-02-14
申请人： Charles Leonard Kibby , Robert James Saxton, JR. , Kandaswamy Jothimurugesan , Tapan Kumar Das , Howard Steven Lacheen , Michael Bartz , Alfred Has
发明人： Charles Leonard Kibby , Robert James Saxton, JR. , Kandaswamy Jothimurugesan , Tapan Kumar Das , Howard Steven Lacheen , Michael Bartz , Alfred Has
IPC分类号： B01J35/02 , B01J23/75 , C07C1/04 , B01J37/02
CPC分类号： B01J29/7669 , B01J23/8986 , B01J29/061 , B01J29/064 , B01J29/068 , B01J29/072 , B01J29/076 , B01J29/7469 , B01J29/7869 , B01J35/023 , B01J35/04 , B01J37/0036 , B01J37/0203 , B01J37/0225 , B01J37/0228 , B01J37/0244 , B01J37/0246 , B01J37/0248 , B01J2229/186 , B01J2229/42 , B01J2229/60 , C07C1/0435 , C07C2529/072 , C10G2/33 , Y10T428/31678
摘要： Disclosed are hybrid synthesis gas conversion catalysts containing at least one Fischer-Tropsch component and at least one acidic component deposited on a monolith catalyst support for use in synthesis gas conversion processes and methods for preparing the catalysts. Also disclosed are synthesis gas conversion processes in which the hybrid synthesis gas conversion catalysts are contacted with synthesis gas to produce a hydrocarbon product containing at least 50 wt % C5+ hydrocarbons. Also disclosed are synthesis gas conversion processes in which at least one layer of Fischer-Tropsch component deposited onto a monolith support is alternated with at least one layer of acidic component in a fixed bed reactor.
摘要翻译：公开了含有至少一种费 - 托组分和沉积在整体催化剂载体上的至少一种酸性组分的混合合成气转化催化剂，用于合成气转化方法和制备催化剂的方法。还公开了合成气转化方法，其中混合合成气转化催化剂与合成气体接触以产生含有至少50重量％的C 5+烃的烃产物。还公开了合成气转化方法，其中沉积在整料载体上的至少一层费 - 托成分与固定床反应器中的至少一层酸性组分交替。

9. 发明申请

US20110306686A1 ZEOLITE SUPPORTED RUTHENIUM CATALYSTS FOR THE CONVERSION OF SYNTHESIS GAS TO HYDROCARBONS, AND METHOD FOR PREPARATION AND METHOD OF USE THEREOF 审中-公开
标题翻译：用于将合成气转化为烃类的ZEOLITE支持的钌催化剂及其制备方法及其使用方法
公开(公告)号：US20110306686A1
公开(公告)日：2011-12-15
申请号：US12797439
申请日：2010-06-09
申请人： Kandaswamy Jothimurugesan , Charles Leonard Kibby , Robert James Saxton
发明人： Kandaswamy Jothimurugesan , Charles Leonard Kibby , Robert James Saxton
IPC分类号： B01J29/068 , C07C1/12
CPC分类号： C10G2/333 , B01J29/068 , B01J29/076 , B01J29/44 , B01J29/46 , B01J29/7415 , B01J29/7815 , B01J35/002 , B01J35/1019 , B01J37/0009 , B01J37/12 , B01J37/18 , C10G2/334
摘要： A method for forming a catalyst for synthesis gas conversion and a synthesis gas conversion process impregnating a zeolite support wherein the catalyst contains ruthenium on a zeolite support, such as ZSM-5, ZSM-12, SSZ-32 or beta zeolite, and the product stream has less than 1 weight % C21+.
摘要翻译：形成合成气转化催化剂的方法和浸渍沸石载体的合成气转化方法，其中催化剂在沸石载体如ZSM-5，ZSM-12，SSZ-32或β沸石上含有钌，产物流具有小于1重量％的C21 +。

10. 发明申请

US20150105236A1 HYBRID FISCHER-TROPSCH CATALYSTS 有权
标题翻译：混合式螯合催化剂
公开(公告)号：US20150105236A1
公开(公告)日：2015-04-16
申请号：US14574741
申请日：2014-12-18
申请人： Kandaswamy Jothimurugesan , Robert James Saxton
发明人： Kandaswamy Jothimurugesan , Robert James Saxton
IPC分类号： B01J29/80 , B01J29/76
CPC分类号： B01J29/80 , B01J29/7669 , B01J35/006 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J37/0009 , B01J37/0201 , B01J37/04 , B01J2229/186 , C10G2/33 , C10G2/332 , C10G2/333 , C10G2/334
摘要： Disclosed are hybrid Fischer-Tropsch catalysts containing cobalt deposited on hybrid supports. The hybrid supports contain an acidic zeolite component and a silica-containing material. It has been found that the use of the hybrid Fischer-Tropsch catalysts in synthesis gas conversion reactions results in high C5+ productivity, high CO conversion rates and low olefin formation.
摘要翻译：公开了含有沉积在混合载体上的钴的混合费 - 托催化剂。杂化载体含有酸性沸石组分和含二氧化硅的材料。已经发现，在合成气转化反应中使用混合费 - 托催化剂导致高的C5 +生产率，高CO转化率和低烯烃形成。

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