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1. 发明授权

US5213779A Process for optimizing the removal of NO.sub.X and SO.sub.X from gases utilizing lanthanide compounds 失效
标题翻译：利用镧系元素化合物优化从气体中除去NO x和SO x的工艺
公开(公告)号：US5213779A
公开(公告)日：1993-05-25
申请号：US738893
申请日：1991-08-01
申请人： D. Alan R. Kay , William G. Wilson , Vinod Jalan
发明人： D. Alan R. Kay , William G. Wilson , Vinod Jalan
IPC分类号： C21C1/02 , C21C7/064
CPC分类号： C21C7/064 , C21C1/02
摘要： A process for optimizing the removal of nitrogen oxide (NO.sub.x) and sulfur oxide (SO.sub.X) from flue gases is provided in which the flue gases pass over a lanthanide-oxygen-sulfur catalyst. The catalyst has active sites provided on its surface which promote the dissociation of NO.sub.X and receive and entrap oxygen released during the dissociation of the NO.sub.X. While the flue gases pass over the catalyst, a reducing gas contacts the catalyst to reduce the oxygen on the active sites of the catalyst and permit the catalyst to continue to promote the dissociation of the NO.sub.x in the flue gas. If the flue gases contain SO.sub.X, they are then passed over a solid solution having a solvent of a first lanthanide oxide compound which crystallizes in the fluorite habit and a solute of at least one altervalent oxide of a second lanthanide. The SO.sub.X in the flue gases reacts with the solid solution to form a sulfated lanthanide oxide which is removed from the flue gases. The sulfated lanthanide oxide may then be dissociated by raising its temperature to regenerate the lanthanide oxide.
摘要翻译：提供了一种优化从烟道气中去除氮氧化物（NOx）和硫氧化物（SOX）的方法，其中烟道气通过镧系元素 - 氧 - 硫催化剂。该催化剂在其表面上提供了活性位点，其促进NO x的解离并且接收和截留在NOX解离过程中释放的氧。当烟气通过催化剂时，还原气体与催化剂接触以减少催化剂的活性位上的氧，并允许催化剂继续促进烟道气中的NOx的解离。如果烟道气含有SOX，则它们然后通过具有第一镧系氧化物化合物的溶剂的固溶体，其结晶为萤石习惯，并且含有至少一种第二镧系元素的交替氧化物的溶质。烟气中的SOX与固溶体反应形成从烟道气中除去的硫酸化镧系元素氧化物。然后硫酸化镧系元素氧化物可以通过升高其温度来解离以再生镧系元素氧化物。

2. 发明授权

US5326737A Cerium oxide solutions for the desulfurization of gases 失效
标题翻译：用于气体脱硫的氧化铈溶液
公开(公告)号：US5326737A
公开(公告)日：1994-07-05
申请号：US843312
申请日：1992-02-28
申请人： D. Alan R. Kay , William G. Wilson
发明人： D. Alan R. Kay , William G. Wilson
IPC分类号： C21C1/02 , C21C7/064 , B01J20/06 , B01J20/04 , B01J23/10 , C01F17/00
CPC分类号： C21C1/02 , C21C7/064
摘要： A solid solution for the desulfurization of sulfur containing gases is provided in which the solution contains oxides having oxygen ion vacancies provided therein. The solid solution has a solvent which has at least one lanthanide oxide which crystallizes in the fluorite habit. The solid solution has a solute which contains a second oxide having a valence which differs from the valence of the lanthanide oxide present in the solvent.
摘要翻译：提供了一种用于含硫气体脱硫的固溶体，其中溶液含有其中提供氧离子空位的氧化物。固溶体具有至少一种在萤石习惯中结晶的镧系元素氧化物的溶剂。固溶体具有含有与溶剂中存在的镧系元素氧化物的价态不同的第二氧化物的溶质。

3. 发明授权

US4714598A Methods of desulfurizing gases 失效
标题翻译：气体脱硫方法
公开(公告)号：US4714598A
公开(公告)日：1987-12-22
申请号：US846272
申请日：1986-03-31
申请人： D. Alan R. Kay , William G. Wilson
发明人： D. Alan R. Kay , William G. Wilson
IPC分类号： C21C1/02 , C21C7/064 , B01D53/36 , B01J8/00 , C01B17/00
CPC分类号： C21C7/064 , C21C1/02
摘要： A method for desulfurizing gases in which the sulfur is mainly in the form of hydrogen sulfide by reacting with one of the forms of cerium oxide with the formation of a cerium-oxygen-sulfur compound, which method can be conducted at temperatures as high as the lowest melting point of either the cerium oxides or cerium-oxygen-sulfur compounds formed by the reactions. The method also includes a definition of the temperature necessary for the regeneration of the cerium-oxygen-sulfur compounds back to cerium oxide which is capable of again reacting with the hydrogen sulfide of the gases being desulfurized whereby the emission of sulfur from the combustion of sulfur containing hydrocarbons is reduced to a level below that attainable with any other method when operated at the same high temperatures.
摘要翻译：通过与氧化铈中的一种与一种铈 - 氧 - 硫化合物反应，硫主要以硫化氢的形式硫化气体的方法，该方法可以在高达通过反应形成的氧化铈或铈 - 氧 - 硫化合物的最低熔点。该方法还包括将铈 - 氧 - 硫化合物再生成氧化铈所需的温度的定义，其能够再次与待脱硫气体的硫化氢反应，从而从硫的燃烧中排出硫当在相同的高温下操作时，含烃的碳氢化合物被降低至低于任何其他方法可达到的水平。

4. 发明授权

US4999174A Use of cerium oxide for removal of chlorine from fuel gases 失效
标题翻译：使用氧化铈从燃料气体中除去氯
公开(公告)号：US4999174A
公开(公告)日：1991-03-12
申请号：US542103
申请日：1990-06-22
申请人： William G. Wilson , D. Alan R. Kay
发明人： William G. Wilson , D. Alan R. Kay
IPC分类号： B01D53/68 , C01B3/56
CPC分类号： C01B3/56 , B01D53/68 , C01B2203/042 , C01B2203/0465 , C01B2203/0485
摘要： A process for the removal of chlorine from reducing gases is provided wherein the reducing gases are contacted with cerium oxide. The chlorided cerium oxide is regenerated in an oxidizing atmosphere to provide cerium oxide. This cerium oxide regenerated is again capable of reacting with chlorine in reducing gases.
摘要翻译：提供了一种从还原气体中除去氯的方法，其中还原气体与氧化铈接触。氯化氧化铈在氧化气氛中再生，得到氧化铈。再生的氧化铈再次能够与还原性气体中的氯反应。

5. 发明授权

US4885145A Method for providing oxygen ion vacancies in lanthanide oxides 失效
标题翻译：在镧系元素氧化物中提供氧离子空位的方法
公开(公告)号：US4885145A
公开(公告)日：1989-12-05
申请号：US100291
申请日：1987-09-23
申请人： D. Alan R. Kay , William G. Wilson
发明人： D. Alan R. Kay , William G. Wilson
IPC分类号： C21C1/02 , C21C7/064
CPC分类号： C21C7/064 , C21C1/02
摘要： A method for desulfurization of fuel gases resulting from the incomplete combustion of sulfur containing hydrocarbons whereby the gases are treated with lanthanide oxides containing large numbers of oxygen-ion vacancies providing ionic porosity which enhances the ability of the lanthanide oxides to react more rapidly and completely with the sulfur in the fuel gases whereby the sulfur in such gases is reduced to low levels suitable for fuels for firing into boilers of power plants generating electricity with steam turbine driven generators, gas turbines, fuel cells and precursors for liquid fuels such as methanol and the like.
摘要翻译：一种由含硫烃不完全燃烧产生的燃料气体脱硫的方法，由此气体用含有大量氧离子空位的镧系元素氧化物处理，提供离子孔隙率，这提高了镧系元素氧化物更快速和完全地反应的能力，燃料气体中的硫，其中这种气体中的硫被还原成适用于燃烧的燃料的低水平，用于燃烧发电的发电厂的锅炉，所述发电厂用蒸汽轮机驱动的发电机，燃气轮机，燃料电池和液体燃料如甲醇和喜欢。

6. 发明授权

US4224058A Methods of desulphurizing fluid materials 失效
标题翻译：脱硫流体材料的方法
公开(公告)号：US4224058A
公开(公告)日：1980-09-23
申请号：US31531
申请日：1979-04-19
申请人： William G. Wilson , D. Alan R. Kay
发明人： William G. Wilson , D. Alan R. Kay
IPC分类号： C21C1/02 , C21C7/064 , C21C7/02
CPC分类号： C21C7/064 , C21C1/02
摘要： A method for desulphurizing fluid materials such as molten iron, steel, stack gases, synthetic natural gases, boiler gases, coal gasification and liquification products and the like is provided in which one of the group rare earth oxides, rare earth fluocarbonates, rare earth oxyfluorides and mixtures thereof, including bastnasite concentrates are reacted at low oxygen potential, with the sulphur to be removed to form one of the group consisting of rare earth sulphides, rare earth oxysulphides and mixtures thereof. The low oxygen potential can be achieved by carrying out the reaction in the presence of vacuum, reducing gases, carbon, etc.
摘要翻译：提供一种稀土氧化物，稀土氟化碳，稀土氧氟化物中的一种，例如铁水，钢铁，烟气，合成天然气，锅炉气体，煤气化和液化产物等流体物质的脱硫方法及其混合物，包括硼砂矿浓缩物在低氧势下反应，待除去的硫形成由稀土硫化物，稀土氧硫化物及其混合物组成的组之一。低氧电位可以通过在真空存在下进行反应，还原气体，碳等来实现。

7. 发明授权

US4857280A Method for the regeneration of sulfided cerium oxide back to a form that is again capable of removing sulfur from fluid materials 失效
标题翻译：将硫化二氧化铈再生成再次能够从流体材料中除去硫的形式的方法
公开(公告)号：US4857280A
公开(公告)日：1989-08-15
申请号：US184400
申请日：1988-04-21
申请人： D. Alan R. Kay , William G. Wilson
发明人： D. Alan R. Kay , William G. Wilson
IPC分类号： C21C1/02 , C21C7/064
CPC分类号： C21C1/02 , C21C7/064
摘要： A method for the regeneration of sulfur containing cerium compounds formed by the desulfurization of fluid materials containing sulfur with cerium oxide back to its original form, CeO.sub.2, wherein the sulfur containing cerium compounds are removed from contact with the fluid material containing sulfur; the temperature of the sulfur containing cerium compounds is raised above the temperature at which cerium sulfate dissociates; and the sulfur containing cerium compounds whose temperature is above the temperature at which cerium sulfate dissociates is exposed to an oxidizing atmosphere.
摘要翻译：通过将硫与氧化铈的流体材料脱硫形成的含硫铈化合物的再生方法返回到其原始形式CeO 2，其中含硫的铈化合物与含有硫的流体材料接触脱除; 含硫铈化合物的温度升高到硫酸铈离解温度以上; 并且其温度高于硫酸铈解离温度的含硫铈化合物暴露于氧化气氛。

8. 发明授权

US4507149A Desulfurization of fluid materials 失效
标题翻译：流体材料脱硫
公开(公告)号：US4507149A
公开(公告)日：1985-03-26
申请号：US521751
申请日：1983-08-08
申请人： D. Alan R. Kay , William G. Wilson
发明人： D. Alan R. Kay , William G. Wilson
IPC分类号： C21C1/02 , C21C7/064 , C22C33/08
CPC分类号： C21C7/064 , C21C1/02
摘要： A method for desulfurizing fluid materials, comprising reacting sulfur to be removed with a rare earth compound, thereby forming rare earth sulfides, oxysulfides or mixtures thereof. The reaction is conducted under conditions of low oxygen potential. Rare earth sulfides and oxysulfides can be reacted with oxygen to restore a capacity for desulfurization.
摘要翻译：一种用于使流体材料脱硫的方法，包括使待除去的硫与稀土化合物反应，从而形成稀土硫化物，氧硫化物或其混合物。反应在低氧势的条件下进行。稀土硫化物和氧硫化物可以与氧气反应以恢复脱硫能力。

9. 发明授权

US4084960A Methods of desulphurizing iron and steel and gases, such as stack gases and the like 失效
标题翻译：钢铁和气体如烟道气等的脱硫方法
公开(公告)号：US4084960A
公开(公告)日：1978-04-18
申请号：US705525
申请日：1976-07-15
申请人： D. Alan R. Kay , William G. Wilson
发明人： D. Alan R. Kay , William G. Wilson
IPC分类号： C21C1/02 , C21C7/064 , C21C7/10 , C21C7/02
CPC分类号： C21C7/10 , C21C1/02 , C21C7/064
摘要： A method for desulphurizing iron, steel, stack gases and the like is provided in which rare earth oxides are reacted, in the presence of an agent, such as carbon, vacuum, reducing gases, etc. for reducing the oxygen level, with the sulphur to be removed to form one of the group consisting of rare earth sulphides, rare earth oxysulphides and mixtures thereof.
摘要翻译：提供了一种铁，钢，烟气等的脱硫方法，其中在诸如碳，真空，还原气体等的试剂存在下，稀土氧化物与硫降低，被除去以形成由稀土硫化物，稀土氧硫化物及其混合物组成的组之一。

10. 发明授权

US5051245A Ammonia for the desulfurization of sulfur containing gases 失效
标题翻译：用于含硫气体脱硫的氨
公开(公告)号：US5051245A
公开(公告)日：1991-09-24
申请号：US541394
申请日：1990-06-21
申请人： William G. Wilson , D. Alan R. Kay
发明人： William G. Wilson , D. Alan R. Kay
IPC分类号： B01D53/50 , C01C1/242
CPC分类号： B01D53/501 , C01C1/242
摘要： A process for the reduction of sulfur oxides from flue gases is provided in which ammonia is added to the flue gas to precipitate out (NH.sub.4).sub.2 SO.sub.4. The (NH.sub.4).sub.2 SO.sub.4 is collected and can be sold as a commercial product.
摘要翻译：提供了一种从烟道气中还原硫氧化物的方法，其中向烟道气中加入氨沉淀出（NH4）2SO4。收集（NH4）2SO4，可作为商品销售。

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