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1. 发明授权

US09364816B2 Concentrated solutions comprising group VI metal, group VII metal, and phosphorus 有权
标题翻译：含有VI族金属，VII族金属和磷的浓缩溶液
公开(公告)号：US09364816B2
公开(公告)日：2016-06-14
申请号：US13394971
申请日：2010-08-24
申请人： Sona Eijsbouts-Spickova , Marcel Adriaan Jansen
发明人： Sona Eijsbouts-Spickova , Marcel Adriaan Jansen
IPC分类号： B01J27/19 , B01J27/185 , B01J37/02 , B01J23/888 , B01J23/88 , B01J37/08 , C10G49/04 , C10G45/04 , C10G45/08 , B01J27/14 , B01J27/188 , B01J37/00 , B01J37/03
CPC分类号： B01J23/888 , B01J23/88 , B01J27/1853 , B01J27/19 , B01J37/0203 , B01J37/0213 , B01J37/0236 , B01J37/08 , C10G45/04 , C10G45/08 , C10G49/04
摘要： This invention provides processes for forming solution compositions, which processes comprises bringing together, in an aqueous medium, i) at least one phosphorus compound; ii) at least one Group VI metal compound; and iii) at least one Group VIII metal compound, such that a solution having a Group VI metal concentration of more than about 5.6 mol/L is formed. Also provided are compositions formed by such processes, processes for forming catalyst compositions from these compositions, and catalyst compositions formed by these processes.
摘要翻译：本发明提供了形成溶液组合物的方法，该方法包括在水性介质中使i）至少一种磷化合物; ii）至少一种VI族金属化合物; 和iii）至少一种VIII族金属化合物，使得形成具有大于约5.6mol / L的VI族金属浓度的溶液。还提供了通过这些方法形成的组合物，由这些组合物形成催化剂组合物的方法，以及由这些方法形成的催化剂组合物。

2. 发明申请

US20130225887A1 Hydrodeoxygenation Of Pyrolysis Oil In Presence Of Admixed Alcohol 有权
标题翻译：溶解油在混合醇存在下的加氢脱氧作用
公开(公告)号：US20130225887A1
公开(公告)日：2013-08-29
申请号：US13883089
申请日：2011-08-30
申请人： Emanuel Hermanus Van Broekhoven , Ralph Klomp , Ruben Theodoor Fronk , Leendert Arie Gerritsen , Frans Lodewijk Plantenga , Edgar Evert Steenminkel
发明人： Emanuel Hermanus Van Broekhoven , Ralph Klomp , Ruben Theodoor Fronk , Leendert Arie Gerritsen , Frans Lodewijk Plantenga , Edgar Evert Steenminkel
IPC分类号： C07C1/22
CPC分类号： C07C1/22 , B01J23/85 , B01J23/883 , B01J37/20 , C10G3/46 , C10G3/50 , C10G2300/4006 , C10G2300/4081 , C10G2300/42 , Y02P30/20
摘要： The present invention relates to the hydrodeoxygenation of pyrolysis oils in the presence of an alcohol.
摘要翻译：本发明涉及在醇存在下热解油的加氢脱氧。

3. 发明申请

US20110303585A1 PROCESS FOR AROMATIC HYDROGENATION AND CETANE VALUE INCREASE OF MIDDLE-DISTILLATE FEEDSTOCKS 审中-公开
标题翻译：芳烃加氢方法和中等离子交换剂的增值价格
公开(公告)号：US20110303585A1
公开(公告)日：2011-12-15
申请号：US13139451
申请日：2009-12-11
申请人： Jean-Pierre Dath , Sander Van Donk , Giacomo Grasso , Frans Plantenga , Jan Nieman
发明人： Jean-Pierre Dath , Sander Van Donk , Giacomo Grasso , Frans Plantenga , Jan Nieman
IPC分类号： C10G45/50 , C10G45/52 , C10G45/46
CPC分类号： C10G45/52 , B01J23/44 , B01J23/63 , B01J23/652 , B01J23/89 , B01J35/0066 , B01J35/1019 , B01J35/1042 , C10G45/04 , C10G45/08 , C10G65/08
摘要： The instant invention pertains to a process for treating a feed, for example a Light Cycle Oil (LCO), having a high content of S and/or N impurities and/or a high content of aromatics, comprising the following steps, in particular in such an order a step of desulphurisation (HDS) and denitrification (HDN) of a feed, in particular LCO, is passed in presence of hydrogen over a catalyst, containing metals of the group VI B and VIII, leading to an effluent, optionally a step of stripping of the effluent, at least a subsequent step for dearomatization (HDA) in which at least a portion of the effluent, optionally stripped, is passed in presence of hydrogen over a catalyst comprising a combination of platinum and palladium supported on a carrier comprising silica-alumina dispersed in an alumina binder wherein the amount of alumina binder is 5-50 wt. % based on the total weight of the silica-alumina and alumina binder present in the carrier and wherein the silica-alumina comprises 5-50 wt. % of alumina based on the weight of the silica-alumina, and recovering the final load obtained, the use of a specific catalyst and a process for preparing diesel comprising the step of mixing the final effluent obtained by a process of the invention.
摘要翻译：本发明涉及用于处理具有高含量的S和/或N杂质和/或高含量芳族化合物的进料例如轻循环油（LCO）的方法，其包括以下步骤，特别是在进料的脱硫（HDS）和脱氮（HDN），特别是LCO的步骤在氢气存在下通过含有VIB和VIII族的金属的催化剂，导致流出物，任选地至少后续的脱气步骤（HDA），其中至少一部分流出物（任选地被汽提）在氢气存在下通过催化剂，所述催化剂包含负载在载体上的铂和钯的组合包括分散在氧化铝粘合剂中的二氧化硅 - 氧化铝，其中氧化铝粘合剂的量为5-50wt。基于存在于载体中的二氧化硅 - 氧化铝和氧化铝粘合剂的总重量，其中二氧化硅 - 氧化铝包含5-50wt。基于二氧化硅 - 氧化铝的重量的氧化铝的百分比，并且回收所获得的最终载荷，使用特定催化剂和制备柴油的方法，包括混合通过本发明的方法获得的最终流出物的步骤。

4. 发明申请

US20210162378A1 NICKEL CONTAINING MIXED METAL-OXIDE/CARBON BULK HYDROPROCESSING CATALYSTS AND THEIR APPLICATION 有权
公开(公告)号：US20210162378A1
公开(公告)日：2021-06-03
申请号：US17176252
申请日：2021-02-16
申请人： ALBEMARLE EUROPE SPRL
发明人： JACOB ARIE BERGWERFF , WILHELMUS CLEMENS JOZEF VEERMAN , RONALD JAN HUIBERTS , SONA EIJSBOUTS-SPICKOVA
IPC分类号： B01J27/051 , B01J35/10 , B01J35/00 , B01J37/08 , C10G45/08 , B01J31/02 , B01J31/22 , B01J37/04 , B01J37/00 , B01J23/888 , B01J31/04 , B01J23/883 , B01J37/20 , B01J35/02 , B01J31/34 , B01J37/02
摘要： The current invention relates a process for making and using a bulk catalyst precursor (i.e. no support material is added as such) comprising Ni and Mo and/or W and an organic component, wherein the molar ratio of C:(Mo+W) ranges from 1.5 to 10. The bulk catalyst precursor is prepared from a mixture of metal-precursors with an organic agent. The organic agent is partly decomposed to form a mixed metal-oxide/C phase which is in effect the bulk catalyst precursor. This bulk catalyst precursor (i) is effectively insoluble in water (ii) does not have any appreciable pore volume or surface area and (iii) does not contain a (nano)crystalline metal-oxide phase as characterized by XRD.

5. 发明申请

US20110313227A1 ALKYLATION CATALYST AND RELATED PROCESS 审中-公开
标题翻译：烷基化催化剂及相关工艺
公开(公告)号：US20110313227A1
公开(公告)日：2011-12-22
申请号：US13148447
申请日：2010-02-09
申请人： Emanuel Hermanus van Broekhoven , Kar-Ming Au-Yeung
发明人： Emanuel Hermanus van Broekhoven , Kar-Ming Au-Yeung
IPC分类号： C07C2/58 , B01J29/04 , B01J29/08 , B01J29/00
CPC分类号： B01J29/068 , B01J23/42 , B01J29/087 , B01J29/088 , B01J29/123 , B01J29/126 , B01J29/22 , B01J29/7415 , B01J29/7476 , B01J29/90 , B01J35/1038 , B01J35/1042 , B01J35/1061 , B01J35/1066 , B01J37/0009 , B01J37/0201 , B01J2229/16 , B01J2229/20 , B01J2229/36 , B01J2229/42 , C07C2/58 , C07C2529/08 , Y02P20/584 , C07C9/16
摘要： A solid alkylation catalyst having a hydrogenation metal and a solid acid in the form of a rare earth exchanged molecular sieve, wherein the catalyst is at least characterized by a porosity of less than 0.20 ml/g in pores below 100 nm in diameter, and a total porosity of greater than 0.30 ml/g. A process for alkylation using the catalyst is also described.
摘要翻译：一种具有氢化金属和稀土交换分子筛形式的固体酸的固体烷基化催化剂，其中该催化剂的特征至少在于直径小于100nm的孔中孔隙率小于0.20ml / g，和总孔隙率大于0.30ml / g。还描述了使用催化剂的烷基化方法。

6. 发明授权

US10953389B2 Nickel containing mixed metal-oxide/carbon bulk hydroprocessing catalysts and their applications 有权
公开(公告)号：US10953389B2
公开(公告)日：2021-03-23
申请号：US16074628
申请日：2017-02-01
申请人： ALBEMARLE EUROPE SPRL
发明人： Jacob Arie Bergwerff , Wilhelmus Clemens Jozef Veerman , Ronald Jan Huiberts , So{hacek over (n)}a Eijsbouts-Spi{hacek over (c)}ková
IPC分类号： B01J23/888 , B01J27/051 , B01J37/20 , B01J37/00 , C10G45/08 , B01J23/883 , B01J31/22 , B01J35/00 , B01J35/10 , B01J35/02 , B01J37/08 , B01J31/02 , B01J31/04 , B01J31/34 , B01J37/04 , B01J37/02
摘要： The current invention relates a bulk catalyst precursor (i.e. no support material is added as such) comprising Ni and Mo and/or W and an organic component, wherein the molar ratio of C:(Mo+W) ranges from 1.5 to 10. The bulk catalyst precursor is prepared from a mixture of metal-precursors with an organic agent. The organic agent is partly decomposed to form a mixed metal-oxide/C phase which is in effect the bulk catalyst precursor. This bulk catalyst precursor (i) is effectively insoluble in water (ii) does not have any appreciable pore volume or surface area and (iii) does not contain a (nano)crystalline metal-oxide phase as characterized by XRD. A bulk catalyst is made from the bulk catalyst precursor.

7. 发明授权

US09701594B2 Hydrodeoxygenation of pyrolysis oil in presence of admixed alcohol 有权
公开(公告)号：US09701594B2
公开(公告)日：2017-07-11
申请号：US13883089
申请日：2011-08-30
申请人： Emanuel Hermanus Van Broekhoven , Ralph Klomp , Ruben Theodoor Pronk , Leendert Arie Gerritsen , Frans Lodewijk Plantenga , Edgar Evert Steenwinkel
发明人： Emanuel Hermanus Van Broekhoven , Ralph Klomp , Ruben Theodoor Pronk , Leendert Arie Gerritsen , Frans Lodewijk Plantenga , Edgar Evert Steenwinkel
IPC分类号： C07C1/22 , C10G3/00 , B01J37/20 , B01J23/85 , B01J23/883
CPC分类号： C07C1/22 , B01J23/85 , B01J23/883 , B01J37/20 , C10G3/46 , C10G3/50 , C10G2300/4006 , C10G2300/4081 , C10G2300/42 , Y02P30/20
摘要： The present invention relates to the hydrodeoxygenation of pyrolysis oils in the presence of an alcohol.

8. 发明授权

US09492818B2 SAPO molecular sieve catalysts and their preparation and uses 有权
标题翻译： SAPO分子筛催化剂及其制备及应用
公开(公告)号：US09492818B2
公开(公告)日：2016-11-15
申请号：US12813244
申请日：2010-06-10
申请人： Martijn J. M. Mies , Mark H. Harte , Edgar Evert Steenwinkel , Emanuel Hermanus van Broekhoven
发明人： Martijn J. M. Mies , Mark H. Harte , Edgar Evert Steenwinkel , Emanuel Hermanus van Broekhoven
IPC分类号： B01J29/068 , B01J29/85 , B01J29/00 , B01J37/10 , C01B39/54 , C07C5/27 , C10G45/64
CPC分类号： B01J29/85 , B01J29/005 , B01J37/10 , B01J2229/18 , C01B39/54 , C07C5/2775 , C07C2529/85 , C10G45/64 , C07C9/22
摘要： Novel silicoaluminophosphate molecular sieve compositions comprising SAPO-11 and SAPO-41 with at least about 5 wt % of in situ-produced amorphous portion. Such compositions can be uncalcined or calcined and novel processes for their preparation are described. These compositions, when loaded or impregnated with a catalytically active species such as a Group VIII noble metal are novel, and are excellent hydroisomerization catalysts.
摘要翻译：新型硅铝磷酸盐分子筛组合物，其包含SAPO-11和SAPO-41，其具有至少约5重量％的原位产生的无定形部分。这些组合物可以是未煅烧的或煅烧的，并且描述了它们制备的新方法。当用催化活性物质如VIII族贵金属负载或浸渍时，这些组合物是新颖的，并且是优异的加氢异构化催化剂。

9. 发明申请

US20120145600A1 Solutions and Catalysts Comprising Group VI Metal, Group VIII Metal, Phosphorus and An Additive 有权
标题翻译：包括VI族金属，VIII族金属，磷和添加剂的溶液和催化剂
公开(公告)号：US20120145600A1
公开(公告)日：2012-06-14
申请号：US13391336
申请日：2010-08-24
申请人： Sona Eijsbouts-Spickova , Marcel Adriaan Jansen
发明人： Sona Eijsbouts-Spickova , Marcel Adriaan Jansen
IPC分类号： C10G45/04 , B01J31/02 , B01J31/06 , B01J27/19 , B01J27/188 , B01J37/02 , B01J37/08 , C10G45/00 , B01J31/04
CPC分类号： B01J27/19 , B01J21/04 , B01J23/88 , B01J23/888 , B01J27/1853 , B01J37/0203 , B01J37/0213 , B01J37/0236 , B01J37/08 , C10G45/00 , C10G45/08 , C10G49/04
摘要： This invention provides a process for forming a solution composition, which process comprises forming a primary solution by bringing together, in an aqueous medium, i) at least one phosphorus compound, ii) at least one Group VI metal compound, iii) at least one Group VIII metal compound, and iv) an additive which is a) tetraethylene glycol, b) polyethylene glycol having an average molecular weight in the range of about 200 to about 400, c) a mixture of tetraethylene glycol and polyethylene glycol having an average molecular weight in the range of about 200 to about 400, or d) a mixture of (1) tetraethylene glycol and/or polyethylene glycol having an average molecular weight in the range of about 200 to about 400 and (2) one or more of monoethylene glycol, diethylene glycol, and triethylene glycol. The molar ratio of additive to the total moles of Group VI metal and Group VIII metal is above 0.30:1, and the atomic ratio of phosphorus to Group VI metal is at least about 0.33:1. Optionally, the primary solution is heated at a temperature above about 40° C. to form a heated solution. The heated solution is optionally cooled to form a cooled solution. Also provided are compositions formed by such processes, processes for forming catalyst compositions from these compositions, and catalyst compositions formed by these processes.
摘要翻译：本发明提供一种形成溶液组合物的方法，该方法包括通过在水性介质中混合形成初级溶液，i）至少一种磷化合物，ii）至少一种VI族金属化合物，iii）至少一种 VIII族金属化合物，和iv）a）四乙二醇，b）平均分子量在约200至约400范围内的聚乙二醇的添加剂，c）四甘醇和聚乙二醇的混合物，其平均分子量重量在约200至约400的范围内，或d）平均分子量在约200至约400范围内的（1）四甘醇和/或聚乙二醇的混合物，和（2）一种或多种单乙烯乙二醇，二甘醇和三甘醇。 VI族金属和VIII族金属的添加剂与总摩尔数的摩尔比大于0.30:1，磷与Ⅵ族金属的原子比为至少约0.33:1。任选地，将主溶液在高于约40℃的温度下加热以形成加热溶液。加热的溶液任选地冷却以形成冷却的溶液。还提供了通过这些方法形成的组合物，由这些组合物形成催化剂组合物的方法，以及由这些方法形成的催化剂组合物。

10. 发明申请

US20110319505A1 BULK SULFIDIC MIXED METAL CATALYST AND METHODS FOR ITS MANUFACTURE AND USE IN CONVERTING SYNGAS TO ALCOHOL 有权
标题翻译：大容量硫化金属催化剂及其制造方法及其在酒精转化中的应用
公开(公告)号：US20110319505A1
公开(公告)日：2011-12-29
申请号：US13203845
申请日：2010-03-05
申请人： Stephan Janbroers , Bob Gerardus Oogjen , Frans Lodewijk Plantenga , Harmannus Willem Homan Free , Sona Eijsbouts-Spickova , Edgar Evert Steenwinkel , Edwin Nuberg
发明人： Stephan Janbroers , Bob Gerardus Oogjen , Frans Lodewijk Plantenga , Harmannus Willem Homan Free , Sona Eijsbouts-Spickova , Edgar Evert Steenwinkel , Edwin Nuberg
IPC分类号： C07C27/00 , B01J27/051
CPC分类号： B01J27/0515 , B01J23/8872 , B01J37/0009 , B01J37/20 , C07C29/1518 , Y02P20/52 , C07C31/08 , C07C31/04
摘要： A process for sulfiding a cobalt-molybdenum bulk catalyst precursor to form a bulk sulfided alcohol synthesis catalyst. The process steps include contacting an oxidic bulk cobalt-molybdenum catalyst precursor with an amount of a sulfur-containing compound which is in the range of about 1 to about 10 moles of sulfur per mole of metals, at one or more temperatures at or in excess of about 300° C. in a medium which is substantially devoid of added hydrogen, so as to form a sulfided bulk cobalt-molybdenum catalyst product. Also described are processes for forming the catalyst precursor, processes for producing an alcohol using the catalyst product and the catalyst product itself.
摘要翻译：硫化钴 - 钼体积催化剂前体以形成本体硫化醇合成催化剂的方法。所述方法步骤包括使氧化体钴钴钼催化剂前体与一定量的含硫化合物接触，所述含硫化合物的量在约或约10摩尔硫/每摩尔金属的一个或多个温度下或过量在基本上不加入氢气的介质中约300℃，以便形成硫化体积的钴 - 钼催化剂产物。还描述了形成催化剂前体的方法，使用催化剂产物和催化剂产物本身生产醇的方法。

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