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61. 发明授权

US5087600A Process for producing a catalyst for denitration by catalytic reduction using ammonia 失效
标题翻译：使用氨催化还原制备脱硝催化剂的方法
公开(公告)号：US5087600A
公开(公告)日：1992-02-11
申请号：US589452
申请日：1990-09-27
申请人： Yasuyoshi Kato , Kunihiko Konishi , Hiroshi Akama , Toshiaki Matsuda , Nobue Teshima
发明人： Yasuyoshi Kato , Kunihiko Konishi , Hiroshi Akama , Toshiaki Matsuda , Nobue Teshima
IPC分类号： B01D53/86 , B01J23/24
CPC分类号： B01J23/24 , B01D53/8628
摘要： A catalyst for denitration by catalytic reduction using ammonia capable of preventing catalyst deterioation due to vapors of heavy metal compounds contained in exhaust gases and having a high strength and a superior resistance to poisons and a process for producing the catalyst are provided, which catalyst comprises TiO.sub.2, oxide(s) of at least one of V, Cu, Fe and Mn and oxide(s) of at least one of Mo, W and Sn, the total of the mol number(s) of the oxide(s) of at least one of Mo, W and Sn falling within a range of 2.times.10.sup.-6 to 20.times.10.sup.-6 mol/m.sup.2 per the unit specific surface of the catalyst, and which process comprises having oxide(s) of at least one of Mo, W and Sn adsorbed and supported onto a composition comprising TiO.sub.2 prepared in advance and oxide(s) of at least one of V, Fe, Cu and Mn so as to give the above-specified total of the mol number(s) of oxide(s) of at least one of Mo, W and Sn.
摘要翻译：提供了一种使用氨进行催化还原的催化还原催化剂，其能够防止由于废气中含有的重金属化合物的蒸气而导致的催化剂降解，并且具有高强度和优异的抗毒性和催化剂的制备方法，该催化剂包含TiO 2 ，V，Cu，Fe和Mn中的至少一种的氧化物以及Mo，W和Sn中的至少一种的氧化物，以及氧化物的摩尔数（s）为 Mo，W和Sn中的至少一种相对于催化剂的单位比表面积为2×10 -6至20×10 -6 mol / m 2的范围，并且该方法包括具有至少一种Mo，W和 Sn吸附并负载在预先制备的TiO 2和V，Fe，Cu和Mn中的至少一种的氧化物的组合物上，以得到上述规定的氧化物摩尔数的总数，的Mo，W和Sn中的至少一种。

62. 发明授权

US5047378A Exhaust gas-purifying catalyst and process for purifying exhaust gases 失效
标题翻译：废气净化催化剂和废气净化工艺
公开(公告)号：US5047378A
公开(公告)日：1991-09-10
申请号：US422697
申请日：1989-10-17
申请人： Yasuyoshi Kato , Nobue Teshima , Kunihiko Konishi , Toshiaki Matsuda
发明人： Yasuyoshi Kato , Nobue Teshima , Kunihiko Konishi , Toshiaki Matsuda
IPC分类号： B01D53/94 , B01D53/86 , B01J29/072 , B01J29/18 , B01J29/24 , B01J37/04
CPC分类号： B01D53/865 , B01J29/072 , B01J37/04
摘要： An exhaust gas-purifying catalyst capable of carrying out the CO-oxidizing reaction and the reduction reaction of NO.sub.x with NH.sub.3 in the same reactor and with good efficiency, and a process for purifying exhaust gases using the catalyst are provided, which catalyst comprises Cu and/or Co supported by Zr oxide or Ti oxide mixed with a Cu-substituted type zeolite.

63. 发明授权

US4571329A Ammonia reduction-denitration process and apparatus therefor 失效
标题翻译：氨还原脱硝工艺及其设备
公开(公告)号：US4571329A
公开(公告)日：1986-02-18
申请号：US639933
申请日：1984-08-13
申请人： Yasuyoshi Kato , Kunihiko Konishi , Masao Ohta
发明人： Yasuyoshi Kato , Kunihiko Konishi , Masao Ohta
IPC分类号： B01D53/86 , B01J8/00 , C01B21/00
CPC分类号： B01D53/8625 , B01D53/8628 , Y02C20/10
摘要： An ammonia reduction-denitration process for exhaust gases containing NO.sub.x consisting mainly of NO.sub.2, and an apparatus therefor are provided, which process comprises treating the exhaust gases with ammonia using a catalyst which is active to both a reaction of (NO.sub.2 +NH.sub.3 .fwdarw.N.sub.2 +N.sub.2 O+H.sub.2 O) and a reaction of (N.sub.2 O+NH.sub.3 .fwdarw.N.sub.2 +H.sub.2 O) at an area velocity of 3 m/h or less and in a concentration ratio of NH.sub.3 /NO.sub.2 of 1.3 or more. According to this process, it is possible to reduce NO.sub.2 contained in the exhaust gases with ammonia at one stage without by-producing N.sub.2 O.
摘要翻译：提供了一种含有主要由NO 2组成的NOx的废气的氨还原脱硝方法及其装置，该方法包括使用对NO 2 + NH 3→N 2 + N 2 O + H 2 O）和（N 2 O + NH 3 - →N 2 + H 2 O）的反应，以3m / h以下的面积速度和NH 3 / NO 2的浓度比为1.3以上。根据该方法，可以在一个阶段用氨除去排气中的NO 2，而不产生N2O。

64. 发明授权

US09550146B2 NOx reduction catalyst for exhaust gas and method for producing same 有权
标题翻译：排气用NOx还原催化剂及其制造方法
公开(公告)号：US09550146B2
公开(公告)日：2017-01-24
申请号：US13821376
申请日：2011-09-05
申请人： Yasuyoshi Kato , Seiji Ikemoto
发明人： Yasuyoshi Kato , Seiji Ikemoto
IPC分类号： B01J29/06 , B01D53/56 , B01J29/40 , B01J29/18 , B01J29/08 , B01J29/48 , B01D53/86 , B01J23/28 , B01J35/00 , B01J37/00 , B01J37/02 , B01J37/28 , B01J29/26 , B01J27/199 , B01J21/06
CPC分类号： B01D53/565 , B01D53/8628 , B01D2251/2062 , B01D2255/20707 , B01D2255/20723 , B01D2255/20769 , B01D2255/20776 , B01D2255/50 , B01D2255/504 , B01D2255/70 , B01J21/063 , B01J23/002 , B01J23/28 , B01J23/30 , B01J27/199 , B01J29/084 , B01J29/088 , B01J29/18 , B01J29/185 , B01J29/26 , B01J29/40 , B01J29/405 , B01J29/48 , B01J35/0006 , B01J35/04 , B01J35/1014 , B01J35/1019 , B01J37/0009 , B01J37/0201 , B01J37/0225 , B01J37/08 , B01J37/088 , B01J37/28 , B01J2229/20 , B01J2229/42 , B01J2523/00 , B01J2523/31 , B01J2523/41 , B01J2523/47 , B01J2523/51 , B01J2523/55 , B01J2523/68 , B01J2523/69
摘要： To provide a catalyst having excellent performance and durability by improving a NOx reduction ratio at 350° C. or higher without deteriorating excellent durability of a Ti—V—Mo—P catalyst in view of problems of conventional art. A NOx reduction catalyst for exhaust gas, which is composed of a catalyst composition that comprises titanium (Ti), an oxide of phosphorous, molybdenum (Mo) and/or tungsten (W), oxide of vanadium (V), and high-silica zeolite that has an SiO2/Al2O3 ratio of not less than 20 is obtained by kneading in the presence of water, drying and calcining (1) titanium oxide, and phosphoric acid or an ammonium salt of phosphoric acid in an amount of more than 1% by weight and not more than 15% by weight relative to the titanium oxide in terms of H3PO4, (2) an oxo acid or oxo acid salt of molybdenum (Mo) and/or tungsten (W) and an oxo acid salt of vanadium (V) or vanadyl salt respectively in an amount of more than 0% by atom and not more than 8% by atom relative to the titanium oxide and (3) high-silica zeolite in an amount of more than 0% by weight and not more than 20% by weight relative to the titanium oxide.
摘要翻译：考虑到现有技术的问题，通过提高350℃以上的NOx还原率而不劣化Ti-V-Mo-P催化剂的优异耐久性，提供具有优异性能和耐久性的催化剂。用于排气的NOx还原催化剂由包含钛（Ti），磷的氧化物，钼（Mo）和/或钨（W），钒（V）的氧化物）和高二氧化硅通过在水的存在下捏合，干燥和煅烧（1）氧化钛，磷酸或磷酸铵盐的量大于1重量％，得到SiO 2 / Al 2 O 3比不小于20的沸石，（ⅱ）钼（Mo）和/或钨（W）和钒（W）的含氧酸盐的含氧酸或含氧酸盐（V）和钒的含氧酸盐（重量），并且不超过15重量％ V）或氧钒盐分别以相对于氧化钛大于0原子％且不超过8原子％的量，和（3）高于0重量％且不超过0重量％的高硅石沸石相对于氧化钛为20重量％以下。

65. 发明授权

US09067194B2 Method of regenerating used catalyst 有权
标题翻译：再生催化剂的方法
公开(公告)号：US09067194B2
公开(公告)日：2015-06-30
申请号：US12442997
申请日：2008-06-26
申请人： Yasuyoshi Kato
发明人： Yasuyoshi Kato
IPC分类号： B01J21/20 , B01J23/28 , B01J23/30 , B01D53/86 , B01J23/92 , B01J38/48 , B01J38/60
CPC分类号： B01J21/20 , B01D53/8628 , B01D2255/20707 , B01D2255/20723 , B01D2255/20769 , B01D2255/20776 , B01D2257/404 , B01J23/28 , B01J23/30 , B01J23/92 , B01J38/485 , B01J38/60
摘要： [Problem] Provided is a method for regenerating a catalyst, the method decreasing the SO2 oxidation rate, which has been increased by Fe and V compounds, of a spent denitration catalyst to an extremely low level, and improves the oxidation activity of the catalyst for metal mercury by the regeneration treatment.[Solving Means] A method for regenerating a catalyst, including steps of immersing a spent denitration catalyst composed mainly of titanium oxide in (a) a mixed aqueous solution containing phosphate ions and oxo-acid ions of one or more elements selected from vanadium (V), molybdenum (Mo), and tungsten (W), (b) a heteropoly acid compound aqueous solution containing phosphorus and one or more elements selected from V, M, and W, or (c) a mixed aqueous solution containing a phosphate compound and a vanadyl compound, and then drying the catalyst.
摘要翻译： [问题]提供一种催化剂再生方法，将废硝化催化剂的Fe 2 O化合物的SO 2氧化速率降低到极低水平的方法，提高了催化剂的氧化活性金属汞通过再生处理。 [解决方案]一种再生催化剂的方法，包括以下步骤：在（a）含有选自钒（V）的一种或多种元素的磷酸根离子和含氧酸离子的混合水溶液中浸渍主要由氧化钛组成的废硝化催化剂），钼（Mo）和钨（W），（b）含有磷和选自V，M和W中的一种或多种元素的杂多酸化合物水溶液，或（c）含有磷酸盐化合物和氧钒基化合物，然后干燥催化剂。

66. 发明申请

US20110268638A1 METHOD OF MERCURY REMOVAL FROM COMBUSTION EXHAUST GAS AND COMBUSTION EXHAUST GAS PURIFICATION APPARATUS 有权
标题翻译：从燃烧排放气体和燃烧中去除汞的方法排气净化装置
公开(公告)号：US20110268638A1
公开(公告)日：2011-11-03
申请号：US13142954
申请日：2010-12-13
申请人： Yasuyoshi Kato , Keiichiro Kai , Seiji Ikemoto
发明人： Yasuyoshi Kato , Keiichiro Kai , Seiji Ikemoto
IPC分类号： B01D53/64
CPC分类号： B01D53/75 , B01D53/501 , B01D53/64 , B01D53/8625 , B01D2251/2062 , B01D2251/2067 , B01D2255/20707 , B01D2255/20723 , B01D2255/20769 , B01D2255/2092 , B01D2255/30 , B01D2257/602 , B01D2258/0283 , B03C3/017 , Y02A50/2349
摘要： A method for removing mercury in a combustion exhaust gas includes injecting ammonia or urea as a reducing agent into a combustion exhaust gas containing nitrogen oxides, sulfur dioxide, metallic mercury, and hydrogen halides, and then introducing the combustion exhaust gas to a denitration apparatus filled with a denitration catalyst to cause a denitration reaction and oxidize the metallic mercury to produce mercury halide; and introducing the combustion exhaust gas through an air preheater and an electric dust collector to a wet desulfurization apparatus, thereby removing sulfur dioxides and the mercury halide, wherein the ammonia concentration of the combustion exhaust gas at an exit of the denitration apparatus is maintained at 5 ppm or higher, and the mercury halide is adsorbed or precipitated onto combustion ash and collected by the electric dust collector to discharge the mercury halide out of a system.
摘要翻译：一种除去燃烧废气中的汞的方法包括将氨或尿素作为还原剂注入到含有氮氧化物，二氧化硫，金属汞和卤化氢的燃烧废气中，然后将燃烧废气引入填充的脱硝装置用脱硝催化剂引起脱硝反应并氧化金属汞以产生卤化汞; 通过空气预热器和电除尘器将燃烧废气引入湿式脱硫装置，从而除去二氧化硫和卤化汞，其中脱硝装置出口处的燃烧废气的氨浓度保持在5 ppm或更高，并且卤化汞被吸附或沉淀到燃烧灰中并由电集尘器收集，以将汞卤化物排出系统。

67. 发明申请

US20110183839A1 CATALYST FOR CLEANING UP NITROGEN OXIDES AND A METHOD FOR PRODUCING SAME 有权
标题翻译：用于清除氮氧化物的催化剂及其生产方法
公开(公告)号：US20110183839A1
公开(公告)日：2011-07-28
申请号：US13056142
申请日：2009-07-29
申请人： Masatoshi Fujisawa , Yasuyoshi Kato
发明人： Masatoshi Fujisawa , Yasuyoshi Kato
IPC分类号： B01J27/055 , B01J37/02 , B01J37/08
CPC分类号： B01J27/055 , B01D53/8628 , B01D2251/208 , B01D2255/104 , B01D2255/2092 , B01J37/0205
摘要： Provided is a silver-supported alumina catalyst for reducing nitrogen oxides using ethanol, which has the drawbacks of the conventional silver-supported alumina catalysts improved, has high performance, is not likely to deteriorate over time, and has excellent initial performance and durability.A catalyst for purifying nitrogen oxides, which purifies nitrogen oxides in exhaust gas using an alcohol as a reducing agent, and contains alumina, aluminum sulfate and silver as main components.
摘要翻译：本发明提供一种使用乙醇还原氮氧化物的银负载氧化铝催化剂，其具有改进的常规银负载型氧化铝催化剂的缺点，具有高性能，不易随时间劣化，并且具有优异的初始性能和耐久性。一种用于净化氮氧化物的催化剂，其使用醇作为还原剂净化废气中的氮氧化物，并且包含氧化铝，硫酸铝和银作为主要成分。

68. 发明申请

US20050130836A1 Catalyst for removing nitrogen oxides, method for production thereof and method for removing nitrogen oxides 有权
标题翻译：用于除去氮氧化物的催化剂，其制造方法以及除去氮氧化物的方法
公开(公告)号：US20050130836A1
公开(公告)日：2005-06-16
申请号：US10506444
申请日：2003-02-28
申请人： Yasuyoshi Kato , Naomi Imada , Yoshinori Nagai
发明人： Yasuyoshi Kato , Naomi Imada , Yoshinori Nagai
IPC分类号： F01N3/08 , B01D53/86 , B01D53/94 , B01J21/06 , B01J23/10 , B01J23/30 , B01J37/02 , B01D53/56
CPC分类号： B01J23/30 , B01D53/8628 , B01D53/9418 , B01D2251/2062 , B01D2255/2065 , B01D2255/20707 , B01D2255/20776 , B01D2255/50 , B01J21/063 , B01J23/10 , B01J37/0215
摘要： Disclosed is a method for producing a catalyst for removing nitrogen oxides which comprises dispersing a hydrated titanium (Ti) oxide or dried material thereof, tungstic acid or a salt thereof, and cerium (Ce) dioxide in a dispersion medium to form a sol-like material, mixing the sol-like material with an aqueous medium to form a catalyst slurry or paste, supporting the catalyst slurry or paste on a catalyst carrier, and then calcinating the carrier; in which catalyst the Ce dioxide is prevented from being embedded in the Ti oxide to realize such a high degree of dispersion of the Ce dioxide on the surface of the Ti oxide as comparable with the case wherein cerium ions are dispersed in micro voids of a zeolite by ion exchange; and the catalyst is free from the occurrence of such phenomena as sintering of the Ti oxide, and deterioration of zeolite with steam when a zeolite is used as carrier.
摘要翻译：公开了一种用于除去氮氧化物的催化剂的方法，其包括在分散介质中分散水合钛（Ti）氧化物或其干燥物质，钨酸或其盐和铈（Ce）二氧化物以形成溶胶状材料，将溶胶状材料与水性介质混合以形成催化剂浆料或糊料，将催化剂浆料或糊料负载在催化剂载体上，然后煅烧载体; 在这种催化剂中，防止二氧化铈嵌入Ti氧化物中，以实现二氧化铈在Ti氧化物表面上的这种高度分散，与将铈离子分散在沸石微孔中的情况相当通过离子交换; 并且催化剂没有发生如氧化钛烧结这样的现象，并且当使用沸石作为载体时，催化剂不会发生沸石与蒸汽的劣化。

69. 发明授权

US6143687A Denitration catalyst, process for preparing the same, and exhaust gas purification method 失效
标题翻译：脱硝催化剂，其制备方法和废气净化方法
公开(公告)号：US6143687A
公开(公告)日：2000-11-07
申请号：US254376
申请日：1999-04-02
申请人： Naomi Imada , Yasuyoshi Kato
发明人： Naomi Imada , Yasuyoshi Kato
IPC分类号： B01D53/86 , B01J21/06 , B01J23/22 , B01J23/24 , B01J33/00 , B01J37/02 , B01J31/00 , B01J23/00 , C01B21/00
CPC分类号： B01J33/00 , B01D53/8628 , B01J37/0219 , B01J37/0244 , B01J21/063 , B01J23/22 , B01J23/24 , Y10S502/507
摘要： A denitration catalyst for use in the reduction of nitrogen oxides contained in an exhaust gas containing highly deliquescent salts as dust with ammonia, which bears thereon a porous coating of a water-repellent organic resin, a porous coating of a mixture of a water-repellent organic resin with inorganic oxide particles, or a porous coating of a mixture of a water-repellent organic resin with catalyst component particles. The denitration catalyst can be prepared, for example, by coating the surface of a denitration catalyst with an aqueous dispersion containing a water-repellent organic resin having a lower concentration, drying the coating, further coating the dried coating with an aqueous dispersion containing a water-repellent organic resin having a higher concentration, and then drying the coating to form a porous coating of a water-repellent organic resin. This denitration catalyst, even when used in the treatment of an exhaust gas containing ash containing highly deliquescent salts, enables the water-repellent porous coating formed on the surface to prevent the salts that have deliquesced from entering the catalyst. This can prevent the deterioration of the catalyst and enables a high catalytic activity to be maintained for a long period of time.
摘要翻译： PCT No.PCT / JP98 / 03083 Sec。一九九九年四月二日 102（e）1999年4月2日PCT PCT 1998年7月9日PCT公布。出版物WO99 / 02262 日期1999年1月21日用于还原包含在含有高度潮解性盐的废气中的氮氧化物的脱硝催化剂，其中所述废气含有氨，作为防尘有机树脂的多孔涂层，混合物的多孔涂层具有无机氧化物颗粒的防水有机树脂，或防水有机树脂与催化剂组分颗粒的混合物的多孔涂层。脱硝催化剂可以例如通过用含有较低浓度的拒水性有机树脂的水性分散体涂覆脱硝催化剂的表面来制备，干燥涂层，进一步用含有水的水分散体涂覆干燥的涂层 - 具有较高浓度的有机有机树脂，然后干燥该涂层以形成防水有机树脂的多孔涂层。该脱硝催化剂即使用于处理含有高度潮解盐的灰分的废气，也能够使表面上形成的防水多孔涂层防止已经潮解的盐进入催化剂。这可以防止催化剂的劣化，并且能够长期保持高的催化活性。

70. 发明授权

US5348987A NOx removal catalyst containing an inorganic fiber 失效
标题翻译：含有无机纤维的除氧催化剂
公开(公告)号：US5348987A
公开(公告)日：1994-09-20
申请号：US3446
申请日：1993-01-12
申请人： Yasuyoshi Kato , Kunihiko Konishi
发明人： Yasuyoshi Kato , Kunihiko Konishi
IPC分类号： B01D53/94 , B01J21/06 , B01J23/22 , B01J23/24 , B01J23/28 , B01J23/30 , B01J35/02 , B01J35/06 , B01J37/00 , B01J21/08
CPC分类号： B01J37/0009 , B01D53/9418 , B01J35/06 , B01J21/06 , B01J21/063 , B01J23/22 , B01J23/24
摘要： NOx removal catalyst can be obtained by kneading various kinds of inorganic fibers and water containing a surfactant to make a pulp-like substance, adding a catalytic component thereto and then further kneading the resultant mixture to prepare a catalyst paste. The thus obtained catalyst paste is shaped into a honeycomb-like, plate-like or column-like form according conventional various molding methods, and then dried and calcined for use. Instead of the above catalytic components; catalytic carriers such as titanium, zeolite, zirconia and the like may be shaped and calcined in the same manner and used for carrying a catalytic component. A particularly high performance and strength can be obtained with good result when a composition produced by calcining a molybdenum (Mo), vanadium (V) or tungsten (W) compound born on titanium oxide at 400.degree. to 700.degree. C. is used.
摘要翻译：可以通过将各种无机纤维和含有表面活性剂的水混合而制成脱脂催化剂，制成纸浆状物质，向其中加入催化剂成分，然后进一步捏合所得混合物，制备催化剂浆料。将如此得到的催化剂浆料按照常规的各种成型方法成形为蜂窝状，板状或柱状，然后干燥并煅烧使用。代替上述催化组分; 催化载体如钛，沸石，氧化锆等可以以相同的方式成型和煅烧并用于承载催化组分。当使用通过在400℃至700℃下煅烧出现在氧化钛上的钼（Mo），钒（V）或钨（W））化合物制备的组合物时，可以获得特别高的性能和强度。

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