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31. 发明申请

US20070082968A1 Fluorine-containing photocurable polymer composition 有权
标题翻译：含氟光固化聚合物组合物
公开(公告)号：US20070082968A1
公开(公告)日：2007-04-12
申请号：US11528691
申请日：2006-09-28
申请人： Hisanobu Minamisawa , Mikio Yamahiro , Akira Meguro
发明人： Hisanobu Minamisawa , Mikio Yamahiro , Akira Meguro
IPC分类号： C08J3/28
CPC分类号： C08F220/32 , C08F220/22 , C08L33/16 , C09D133/02 , Y10T428/1045 , Y10T428/105 , Y10T428/1055 , Y10T428/1059 , Y10T428/1068 , Y10T428/1082 , Y10T428/31504 , Y10T428/3154 , Y10T428/31663 , C08L2666/04
摘要： The invention provides a photocurable polymer composition having a fluorine-containing polymer and a fluorine-free polymer, and preferably further having a polymerizable double bond-containing compound and a photopolymerization initiator. The fluorine-containing polymer preferably includes a fluorosilsesquioxane skeleton.
摘要翻译：本发明提供具有含氟聚合物和无氟聚合物的光固化性聚合物组合物，优选进一步具有可聚合双键的化合物和光聚合引发剂。含氟聚合物优选包含氟倍半硅氧烷骨架。

32. 发明申请

US20060287454A1 Silicon compounds 有权
标题翻译：硅化合物
公开(公告)号：US20060287454A1
公开(公告)日：2006-12-21
申请号：US10548365
申请日：2004-03-05
申请人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Yasuhiro Yamamoto , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
发明人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Yasuhiro Yamamoto , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
IPC分类号： C08F230/08 , C07F7/04
CPC分类号： C08G77/04 , C07F7/21 , C08F10/00 , C08F30/08 , C08F2500/03
摘要： The present invention provides a silicon compound represented by Formula (1) and a polymer obtained by using the same, and this makes it possible not only to obtain an organic-inorganic composite material having a distinct structure but also to control the structure of the above polymer as a molecular aggregate. wherein R1 is a group independently selected from hydrogen, alkyl having a carbon atom number of 1 to 40, substituted or non-substituted aryl and substituted or non-substituted arylalkyl; in this alkyl having a carbon atom number of 1 to 40, optional hydrogens may be substituted with fluorine, and optional —CH2— may be substituted with —O—, —CH═CH—, cycloalkylene or cycloalkenylene; in alkylene in this arylalkyl, optional hydrogens may be substituted with fluorine, and optional —CH2— may be substituted with —O— or —CH═CH—; and A1 is a group having an α-haloester bond.
摘要翻译：本发明提供由式（1）表示的硅化合物和使用它的聚合物，不仅可以获得具有不同结构的有机 - 无机复合材料，而且可以控制上述结构聚合物作为分子聚集体。其中R 1是独立地选自氢，碳原子数为1至40的烷基，取代或未取代的芳基和取代或未取代的芳基烷基的基团; 在该碳原子数为1至40的烷基中，任选的氢可被氟取代，并且任选的-CH 2 - 可以被-O-，-CH-CH-，亚环烷基或环亚烯基在该芳烷基中的亚烷基中，任选的氢可以被氟取代，任选的-CH 2 - 可以被-O-或-CH-CH-取代; 且A 1是具有α-卤代酯键的基团。

33. 发明授权

US07053167B2 Silsesquioxane derivative having functional group 有权
标题翻译：具有官能团的倍半硅氧烷衍生物
公开(公告)号：US07053167B2
公开(公告)日：2006-05-30
申请号：US10661536
申请日：2003-09-15
申请人： Kenya Ito , Mikio Yamahiro , Kenichi Watanabe
发明人： Kenya Ito , Mikio Yamahiro , Kenichi Watanabe
IPC分类号： C08G77/24
CPC分类号： C08G77/06 , C08G77/045 , C08G77/38
摘要： A conventional silsesquioxane derivative has the problems that the functional groups are restricted and the chemical structure is not readily controlled and that it is expensive. The present inventors have developed a process for producing a silsesquioxane derivative at a high yield by a simple process in order to solve such problems. The novel silsesquioxane derivative according to the present invention is controlled in a structure thereof and has a functional group, which is excellent in reactivity with a target compound, to be modified. The present invention relates to a production process for a silsesquioxane derivative represented by Formula (2), characterized by using a silicon compound represented by Formula (1). In Formula (1) and Formula (2), R is a group selected from hydrogen, alkyl, aryl and arylalkyl; M is a monovalent alkaline metal atom; at least one of Y is a group represented by Formula (3), and the remainder of Y is hydrogen; R1 and R2 in Formula (3) represent the same group as defined for R; and Z is a functional group or a group having a functional group
摘要翻译：常规的倍半硅氧烷衍生物存在官能团受限并且化学结构不容易控制并且昂贵的问题。为了解决这些问题，本发明人通过简单的工艺开发了高产率的倍半硅氧烷衍生物的制备方法。根据本发明的新型倍半硅氧烷衍生物在其结构中被控制，并且具有与待改性的目标化合物的反应性优异的官能团。本发明涉及由式（2）表示的倍半硅氧烷衍生物的制备方法，其特征在于使用由式（1）表示的硅化合物。在式（1）和式（2）中，R是选自氢，烷基，芳基和芳基烷基的基团; M是一价碱性金属原子; Y中的至少一个为由式（3）表示的基团，Y的其余部分为氢; 式（3）中的R 1和R 2代表与R所定义的相同的基团; Z为官能团或具有官能团的基团

34. 发明授权

US09751286B2 Weather-resistant multilayer film 有权
公开(公告)号：US09751286B2
公开(公告)日：2017-09-05
申请号：US14129990
申请日：2012-07-02
申请人： Akiko Yoda , Kenya Ito , Koji Ohguma , Mikio Yamahiro
发明人： Akiko Yoda , Kenya Ito , Koji Ohguma , Mikio Yamahiro
IPC分类号： B32B27/18 , B32B27/30 , B32B27/08 , B32B27/36
CPC分类号： B32B27/18 , B32B27/08 , B32B27/308 , B32B27/36 , B32B2307/40 , B32B2307/71 , B32B2307/712 , B32B2457/20 , Y10T428/24975 , Y10T428/31797 , Y10T428/31928
摘要： Provided is a multi-layered weather-resistant multilayer film that exhibits good substrate adhesion, wherein curing problems are avoided, bleed-out is minimized, yellowing is reduced, and weather-resistance is improved. The weather-resistant multilayer film 10 is provided with the following: a transparent film-like substrate C; a UV-absorbing resin layer B laminated on the substrate C and containing a UV absorber; and a first cured resin layer A laminated on the UV-absorbing resin layer B. The first cured resin layer A has a thickness of 1.0 to 10 μm. The UV-absorbing resin layer B has a thickness of 0.5 to 5 μm. The UV-absorbing resin layer B has an absorption wavelength of 200 to 500 nm.

35. 发明授权

US09375867B2 Transfer film for in-mold molding and method for producing same 有权
标题翻译：模内成型用转印膜及其制造方法
公开(公告)号：US09375867B2
公开(公告)日：2016-06-28
申请号：US14127964
申请日：2012-06-18
申请人： Kenya Ito , Koji Ohguma , Takuro Tanaka , Yuka Takahashi , Aki Kuromatsu , Mikio Yamahiro
发明人： Kenya Ito , Koji Ohguma , Takuro Tanaka , Yuka Takahashi , Aki Kuromatsu , Mikio Yamahiro
IPC分类号： B29C45/14 , B32B27/16 , B44C1/17 , B32B7/06 , B32B38/00
CPC分类号： B29C45/14688 , B29C45/14 , B29C45/14811 , B29C45/14827 , B32B7/06 , B32B27/16 , B32B38/0036 , B32B2270/00 , B32B2451/00 , B44C1/1729 , Y10T428/24851 , Y10T428/31511 , Y10T428/31515 , Y10T428/31551 , Y10T428/31554 , Y10T428/31598 , Y10T428/31663 , Y10T428/31946
摘要： Provided is a transfer film for in-mold molding which is superior in solvent resistance, heat resistance, durability, blocking resistance, and moldability, and is capable of suppressing the generation of gate flow, and also provided is a method for producing such a film. The film is provided with: a transfer layer (11) which is to be transferred to an in-mold molded body and which is to be cured when irradiated with active energy rays after the transfer; and a film shaped substrate (L0). The transfer layer (11) comprises an IMD layer (L2) laminated on the substrate (L0) and to be arranged on the outermost surface of the molded body after the in-mold molding. The IMD layer (L2) is constituted by a mixture composition containing at least one active-energy curable resin and at least one thermosetting resin.
摘要翻译：提供了一种模内成型用转印膜，其耐溶剂性，耐热性，耐久性，耐粘连性和成型性优异，并且能够抑制栅极流动的产生，并且还提供了制造这种膜的方法。膜设置有：转印层（11），其被转印到模内成型体中，并且在转印后用活性能量射线照射时被固化; 和薄膜状基板（L0）。转印层（11）包括层叠在基板（L0）上的IMD层（L2），并且在模内成型之后布置在成形体的最外表面上。 IMD层（L2）由含有至少一种活性能量固化树脂和至少一种热固性树脂的混合物组合物构成。

36. 发明授权

US07563917B2 Silicon compound and a production process for silicon compound 有权
标题翻译：硅化合物和硅化合物的生产工艺
公开(公告)号：US07563917B2
公开(公告)日：2009-07-21
申请号：US11517457
申请日：2006-09-08
申请人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe
发明人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe
IPC分类号： C07F7/21
CPC分类号： C07F7/21 , C07F7/0876
摘要： The object of the present invention is to provide a new kind of silicon compound having an ester-type organic functional group and a new method for providing a T8-silsesquioxane compound having a hydroxyl group by using said silicon compound as the starting material.A silicon compound represented by formula (1) is obtained through the production process characterized by using a silicon compound represented by formula (2). wherein: in formula (1), each of seven R1 group is independently selected from the group consisting of hydrogen, alkyl, substituted or unsubstituted aryl, and substituted or unsubstituted arylalkyl and A2 is a hydroxyl-terminal organic functional group, and in formula (2), each of R1 group is the same as R1 in formula (1), and A1 is an organic functional group containing an acyloxy group.
摘要翻译：本发明的目的是提供一种具有酯型有机官能团的新型硅化合物和通过使用所述硅化合物作为起始原料提供具有羟基的T8-倍半硅氧烷化合物的新方法。通过以式（2）表示的硅化合物为特征的制造方法得到式（1）所示的硅化合物。其中：在式（1）中，七个R 1基团各自独立地选自氢，烷基，取代或未取代的芳基和取代或未取代的芳基烷基，A2是羟基末端有机官能团，并且在式 2）中，R 1基与式（1）中的R 1相同，且为含有酰氧基的有机官能团。

37. 发明申请

US20090143606A1 Production process for a silicon compound 有权
标题翻译：硅化合物的生产工艺
公开(公告)号：US20090143606A1
公开(公告)日：2009-06-04
申请号：US12318736
申请日：2009-01-07
申请人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Yasuhiro Yamamoto , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
发明人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Yasuhiro Yamamoto , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
IPC分类号： C07F7/07
CPC分类号： C08G77/04 , C07F7/21 , C08F10/00 , C08F30/08 , C08F2500/03
摘要： The present invention provides a silicon compound represented by Formula (1) and a polymer obtained by using the same, and this makes it possible not only to obtain an organic-inorganic composite material having a distinct structure but also to control the structure of the above polymer as a molecular aggregate. wherein R1 is a group independently selected from hydrogen, alkyl having a carbon atom number of 1 to 40, substituted or non-substituted aryl and substituted or non-substituted arylalkyl; in this alkyl having a carbon atom number of 1 to 40, optional hydrogens may be substituted with fluorine, and optional —CH2— may be substituted with —O—, —CH═CH—, cycloalkylene or cycloalkenylene; in alkylene in this arylalkyl, optional hydrogens may be substituted with fluorine, and optional —CH2— may be substituted with —O— or —CH═CH—; and A1 is a group having an α-haloester bond.
摘要翻译：本发明提供由式（1）表示的硅化合物和使用它的聚合物，不仅可以获得具有不同结构的有机 - 无机复合材料，而且可以控制上述结构聚合物作为分子聚集体。其中R1是独立地选自氢，碳原子数为1至40的烷基，取代或未取代的芳基和取代或未取代的芳基烷基的基团; 在该碳原子数为1至40的烷基中，任选的氢可以被氟取代，任选的-CH 2 - 可以被-O - ， - CH-CH-，亚环烷基或环亚烯基取代; 在该芳基烷基中的亚烷基中，任选的氢可以被氟取代，并且任选的-CH 2 - 可以被-O-或-CH-CH-取代; 并且A1是具有α-卤代酯键的基团。

38. 发明申请

US20090137765A1 Polymer obtained by addition-polymerization initiated by a silicon compound 有权
标题翻译：通过硅化合物引发的加成聚合得到的聚合物
公开(公告)号：US20090137765A1
公开(公告)日：2009-05-28
申请号：US12318733
申请日：2009-01-07
申请人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Yasuhiro Yamamoto , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
发明人： Mikio Yamahiro , Hisao Oikawa , Kenya Ito , Yasuhiro Yamamoto , Masami Tanaka , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
IPC分类号： C08F283/12
CPC分类号： C08G77/04 , C07F7/21 , C08F10/00 , C08F30/08 , C08F2500/03
摘要： The present invention provides a silicon compound represented by Formula (1) and a polymer obtained by using the same, and this makes it possible not only to obtain an organic-inorganic composite material having a distinct structure but also to control the structure of the above polymer as a molecular aggregate. wherein R1 is a group independently selected from hydrogen, alkyl having a carbon atom number of 1 to 40, substituted or non-substituted aryl and substituted or non-substituted arylalkyl; in this alkyl having a carbon atom number of 1 to 40, optional hydrogens may be substituted with fluorine, and optional —CH2— may be substituted with —O—, —CH═CH—, cycloalkylene or cycloalkenylene; in alkylene in this arylalkyl, optional hydrogens may be substituted with fluorine, and optional —CH2— may be substituted with —O— or —CH═CH—; and A1 is a group having an α-haloester bond.
摘要翻译：本发明提供由式（1）表示的硅化合物和使用它的聚合物，不仅可以获得具有不同结构的有机 - 无机复合材料，而且可以控制上述结构聚合物作为分子聚集体。其中R1是独立地选自氢，碳原子数为1至40的烷基，取代或未取代的芳基和取代或未取代的芳基烷基的基团; 在该碳原子数为1至40的烷基中，任选的氢可以被氟取代，任选的-CH 2 - 可以被-O - ， - CH-CH-，亚环烷基或环亚烯基取代; 在该芳基烷基中的亚烷基中，任选的氢可以被氟取代，并且任选的-CH 2 - 可以被-O-或-CH-CH-取代; 并且A1是具有α-卤代酯键的基团。

39. 发明授权

US07256243B2 Silicon compound 有权
标题翻译：硅化合物
公开(公告)号：US07256243B2
公开(公告)日：2007-08-14
申请号：US11121120
申请日：2005-05-04
申请人： Hisao Oikawa , Mikio Yamahiro , Kazuhiro Yoshida , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
发明人： Hisao Oikawa , Mikio Yamahiro , Kazuhiro Yoshida , Nobumasa Ootake , Kenichi Watanabe , Kohji Ohno , Yoshinobu Tsujii , Takeshi Fukuda
IPC分类号： C08F4/16 , C08G77/442
CPC分类号： C07F7/21
摘要： The present invention provides a novel silicon compound represented by Formula (1) having a living radical polymerization initiating ability for addition-polymerizable monomers and a polymer obtained using the same. The above polymer can provide an organic-inorganic composite material having a distinct structure. wherein R1 is hydrogen, alkyl, aryl or arylalkyl; R2 and R3 are alkyl, phenyl or cyclohexyl; and A is a group having an ability to initiate polymerization of a monomer.
摘要翻译：本发明提供一种由加成聚合性单体具有活性自由基聚合引发能力的式（1）表示的新型硅化合物和使用该硅化合物的聚合物。上述聚合物可以提供具有不同结构的有机 - 无机复合材料。其中R 1是氢，烷基，芳基或芳基烷基; R 2和R 3是烷基，苯基或环己基; 而A是具有引发单体聚合能力的基团。

40. 发明授权

US07235619B2 Silsesquioxane derivative 有权
标题翻译：倍半硅氧烷衍生物
公开(公告)号：US07235619B2
公开(公告)日：2007-06-26
申请号：US11121076
申请日：2005-05-04
申请人： Yoshitaka Morimoto , Kenya Ito , Hisaoi Oikawa , Mikio Yamahiro , Kenichi Watanabe , Nobumasa Ootake
发明人： Yoshitaka Morimoto , Kenya Ito , Hisaoi Oikawa , Mikio Yamahiro , Kenichi Watanabe , Nobumasa Ootake
IPC分类号： C08G77/16
CPC分类号： C08G77/04
摘要： A silsesquioxane derivative represented by Formula (2): wherein R is hydrogen, an alkyl, an aryl, or an arylalkyl; and X is hydrogen, chlorine, a functional group, or a group having a functional group.
摘要翻译：由式（2）表示的倍半硅氧烷衍生物：其中R是氢，烷基，芳基或芳基烷基; X为氢，氯，官能团或具有官能团的基团。

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