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21. 发明授权

US06562905B1 High density polyethylene compositions, a process for the production thereof and films prepared 有权
标题翻译：高密度聚乙烯组合物，其制备方法和制备的薄膜
公开(公告)号：US06562905B1
公开(公告)日：2003-05-13
申请号：US09647846
申请日：2000-11-09
申请人： Auli Nummila-Pakarinen , Ole Jan Myhre , Jarmo Lindroos , Solveig Johansson
发明人： Auli Nummila-Pakarinen , Ole Jan Myhre , Jarmo Lindroos , Solveig Johansson
IPC分类号： C08F1002
CPC分类号： C08F10/00 , C08L23/04 , C08L23/06 , C08L2205/02 , C08L2314/02 , Y10T428/13 , Y10T428/1334 , Y10T428/1345 , Y10T428/1352 , Y10T428/1397 , C08F4/6555 , C08L2666/04
摘要： The present invention concerns a bimodal film-making HDPE composition, a process for the preparation thereof, a film prepared thereof and a film-making process. The composition comprises at least one polyethylene component having a relatively low molecular weight and another polyethylene component having a relatively high molecular weight. The composition has a shear thinning index defined by the relationship: SHI5/300≦0.00014 &eegr;5kPa+78 wherein &eegr;5kPa is the complex viscosity at G*=5 Pa and SHI5/300 is the ratio of complex viscosity at G*=5 kPa to the complex viscosity at G*=300 kPa. By means of the invention it is possible to produce material for making HDPE blown films with good mechanical properties in a process where the whole range of PE products from LLD to HD can be produced.
摘要翻译：本发明涉及双峰成膜HDPE组合物，其制备方法，其制备的膜和成膜方法。组合物包含至少一种具有较低分子量的聚乙烯组分和另一种具有相对较高分子量的聚乙烯组分。该组合物具有由以下关系式定义的剪切稀化指数：其中η5kPa是G * = 5Pa时的复数粘度，SHI5 / 300是G * = 5kPa下的复数粘度与G * = 300kPa下的复数粘度的比率.By 在本发明的方法中，可以生产用于制造具有良好机械性能的HDPE吹塑薄膜的材料，其中可以生产从LLD到HD的全部范围的PE产品。

22. 发明授权

US06552150B1 Polymer films and a process for the production thereof 有权
标题翻译：聚合物膜及其生产方法
公开(公告)号：US06552150B1
公开(公告)日：2003-04-22
申请号：US09601366
申请日：2000-09-14
申请人： Auli Nummila-Pakarinen , Ole Jan Myhre , Bjarne Jansen
发明人： Auli Nummila-Pakarinen , Ole Jan Myhre , Bjarne Jansen
IPC分类号： C08F1002
CPC分类号： C08F10/02 , C08L23/04 , C08L23/0815 , C08L2205/02 , C08F2/001 , C08L2666/04
摘要： The present invention concerns a polyethylene composition particularly suitable for film blowing. The invention also concerns a process for the production thereof. The composition comprises a low molecular weight portion having a density of more than 960 kg/m3 and a high molecular weight portion. The polyethylene composition has a density of about 925-940 kg/m3 and a melt flow rate in the range of MFR21, from 5 to 40 g/10 min. A polyethylene film blown from the polyethylene composition exhibits a tensile strength at yield in transverse direction at least 15 MPa, a 1% secant modulus in machine direction at least 300 MPa and in transverse direction at least 400 MPa, and a dart drop of at least 5 g/&mgr;m.
摘要翻译：本发明涉及特别适用于吹膜的聚乙烯组合物。本发明还涉及其生产方法。组合物包含密度高于960kg / m 3的高分子量部分的低分子量部分。聚乙烯组合物的密度为约925-940kg / m 3，熔体流动速率在MFR 21范围内，为5至40g / 10min。从聚乙烯组合物吹出的聚乙烯薄膜在横向收缩率表现出拉伸强度至少为15MPa，机器方向上的1％割草模数至少为300MPa，横向为至少400MPa，并且至少具有飞镖滴 5g / mum。

23. 发明授权

US06462161B1 Polyolefin composition with molecular weight maximum occurring in that part of the composition that has the highest comonomer content 有权
标题翻译：具有分子量最大值的聚烯烃组合物出现在具有最高共聚单体含量的该组合物的该部分中
公开(公告)号：US06462161B1
公开(公告)日：2002-10-08
申请号：US09180414
申请日：1998-11-06
申请人： Larry D. Cady , Christopher J. Frye , Philip Howard , Teresa P. Karjala , Peter J. Maddox , Ian M. Munro , Deepak R. Parikh , S. Roy Partington , Kevin P. Peil , Lee Spencer , William R. Van Volkenburgh , Peter S. Williams , David R. Wilson , J. Mark Winter
发明人： Larry D. Cady , Christopher J. Frye , Philip Howard , Teresa P. Karjala , Peter J. Maddox , Ian M. Munro , Deepak R. Parikh , S. Roy Partington , Kevin P. Peil , Lee Spencer , William R. Van Volkenburgh , Peter S. Williams , David R. Wilson , J. Mark Winter
IPC分类号： C08F1002
CPC分类号： C08F210/00 , C08F4/65908 , C08F4/65912 , C08F4/65916 , C08F4/6592 , C08F4/65927 , C08F210/16 , C08F2410/02 , C08J5/18 , C08J2323/08 , C08L23/06 , C08L23/0815 , C08L2205/02 , C08L2205/025 , C08L2207/07 , C08L2308/00 , C08L2314/06 , Y10S526/901 , Y10S526/916 , Y10S526/943 , C08L2666/06 , C08F210/14 , C08F2500/09 , C08F2500/20 , C08L2666/04
摘要： The invention relates to a polyolefin copolymer composition produced with a catalyst having a metallocene, complex in a single reactor for the polymer of an &agr;-olefin monomer with one or more olefin comonomers, and a molecule weight maximum which occurs in that 50 percent by weight of the composition which has the highest weight percent comonomer content. Preferably, the composition has a comonomer partitioning fact Cpf which is equal to or greater than 1.10 or molecule weight partitioning fact Mpf which is equal to or greater than 1.15. Preferred composition also have at least 0.01 long chain branches per 1000 carbon atoms along the polymer backbone. These compositions with reverse molecular engineering have. superior properties and are easily processable due to the simultaneous presence of the association of high molecular weight with high comonomer content and of long chain branching.
摘要翻译：本发明涉及一种聚烯烃共聚物组合物，该聚烯烃共聚物组合物由具有茂金属的催化剂制备，在具有一种或多种烯烃共聚单体的α-烯烃单体的聚合物的单个反应器中为复合物，分子量最大值为50重量％具有最高重量百分比共聚单体含量的组合物。优选地，组合物具有等于或大于1.10的共聚单体分配事实Cpf或等于或大于1.15的分子量分配事实Mpf。优选的组合物也沿着聚合物主链每1000个碳原子具有至少0.01个长链分支。这些具有反向分子工程的组合物具有。优异的性能并且由于高分子量与高共聚单体含量和长链支化的结合的同时存在而容易加工。

24. 发明授权

US06403666B1 Polyolefin base porous film 失效
标题翻译：聚烯烃基多孔膜
公开(公告)号：US06403666B1
公开(公告)日：2002-06-11
申请号：US09443467
申请日：1999-11-19
申请人： Nobuhiko Nakayama , Masaji Enokuchi
发明人： Nobuhiko Nakayama , Masaji Enokuchi
IPC分类号： C08F1002
CPC分类号： C08J5/18 , A61F13/514 , C08J2323/02 , C08J2323/08 , C08K3/26 , Y10T442/60 , C08L23/02
摘要： Provided is a polyolefin base porous film comprising a polyolefin composition in which calcium carbonate particles, preferably calcium carbonate particles subjected to surface treatment with chain carboxylic acid having 3 to 6 carbon atoms are dispersed. This polyolefin base porous film is characterized by that the leached solution with water has a pH which falls in the vicinity of neutrality and has a low stimulation to the skin, and therefore it is useful for goods contacting human bodies, particularly a back sheet for a sanitary napkin.
摘要翻译：提供了一种聚烯烃基多孔膜，其包含分散有碳原子数为3〜6的链状羧酸表面处理的碳酸钙粒子，优选碳酸钙粒子的聚烯烃组合物。该聚烯烃基多孔膜的特征在于，具有水的浸出溶液的pH值落在中性附近，对皮肤的刺激性低，因此对于与人体接触的物品，特别是用于卫生巾。

25. 发明授权

US06346576B1 Ethylene resin packaging films 有权
标题翻译：乙烯树脂包装膜
公开(公告)号：US06346576B1
公开(公告)日：2002-02-12
申请号：US09646475
申请日：2000-09-19
申请人： Mamoru Takahashi
发明人： Mamoru Takahashi
IPC分类号： C08F1002
CPC分类号： C08J5/18 , C08J2323/08 , C08L23/06 , C08L23/0815 , C08L2666/04
摘要： The present invention provides a packaging film which exhibits excellent mechanical strength properties such as high dart impact strength with retaining properties of transparency and film surface smoothness. The ethylene resin packaging film comprises an ethylene/&agr;-olefin copolymer having the following properties: the density is in the range of 0.918 to 0.935 g/cm3; the melt flow rate (MFR) at 190° C. under a load of 2.16 kg is in the range of 0.05 to 1.0 g/10 min; the decane-soluble component fraction (W) at room temperature and the density (d) satisfy the relation W 75×MFR; and the melt tension (MT) at 190° C. and MFR satisfy the relation MT>2.2×MFR−0.84.
摘要翻译：本发明提供一种具有优异的机械强度性能的包装膜，例如具有高的飞镖冲击强度，并且具有透明性和膜表面光滑度的保持性能。乙烯树脂包装膜包含具有以下特性的乙烯/α-烯烃共聚物：密度在0.918至0.935g / cm3的范围内; 在2.16kg载荷下190℃下的熔体流动速率（MFR）在0.05-1.0g / 10min的范围内; 室温下的癸烷可溶性成分馏分（W）和密度（d）满足W <80×exp（-100（d-0.88））+ 0.1的关系。流动指数（FI）被定义为在190℃的熔融状态下所述共聚物的剪切应力达到2.4×10 6达因/ cm 2的剪切速率，MFR满足关系FI> 75xMFR; 并且在190℃下的熔体张力（MT）和MFR满足MT> 2.2×MFR-0.84的关系。

26. 发明授权

US06316511B1 Polyethylene closure for a container 失效
标题翻译：聚乙烯封闭容器
公开(公告)号：US06316511B1
公开(公告)日：2001-11-13
申请号：US09463899
申请日：2000-04-18
申请人： Kelvin Allan Davies , Roland David South
发明人： Kelvin Allan Davies , Roland David South
IPC分类号： C08F1002
CPC分类号： B29C44/425 , B29C44/3415 , B65D39/00 , B65D39/0011
摘要： A polymeric closure for a container comprising a foamed polyethylene, wherein said polyethylene prior to foaming has: 1) a density of between 0.910 g/cm3 and 0.885 g/cm3; ii) a molecular weight distribution of 2 or less; and iii) a melt index of between 2 and 10. Closure can be used as a replacement of natural cork for wine bottles.
摘要翻译：一种用于包含发泡聚乙烯的容器的聚合物封闭物，其中所述发泡前的聚乙烯具有：1）0.910g / cm 3至0.885g / cm 3之间的密度; ii）分子量分布为2以下; 和iii）熔体指数在2和10之间。封闭可以用来替代葡萄酒瓶的天然软木塞。

27. 发明授权

US06310167B1 Ethylene homopolymer and its molded article 失效
标题翻译：乙烯均聚物及其模塑制品
公开(公告)号：US06310167B1
公开(公告)日：2001-10-30
申请号：US09373194
申请日：1999-08-12
申请人： Mitsugu Kanzawa , Fumio Okuda , Tatsuya Housaki , Tomio Tatsumi
发明人： Mitsugu Kanzawa , Fumio Okuda , Tatsuya Housaki , Tomio Tatsumi
IPC分类号： C08F1002
CPC分类号： C08F110/02 , C08F10/00 , C08F2500/10 , C08F2500/12 , C08F2500/08 , C08F4/7006
摘要： Provided are an ethylene homopolymer having well-balanced properties of good heat resistance, good heat-sealability and good moldability, and its molded articles. The ethylene homopolymer is characterized in that the number of butyl branches per 100 methyl branches therein falls between 1 and 20, as measured through 13C-NMR, that its density, d (kg/m3), falls between 880 and 980, and that the density, d, and its melting point, Tm (° C.) , satisfy the conditions defined by the following formulae (1) to (3): Tm≧1.2×d−982 (980≧d≧925) (1), Tm≧0.6×d−430 (925>d≧915) (2), Tm≧0.16×d−28.4 (915>d≧880) (3). The ethylene homopolymer is molded into moldings.
摘要翻译：提供具有良好的耐热性，良好的热封性和良好的成型性的良好平衡性的乙烯均聚物及其模塑制品。乙烯均聚物的特征在于，通过13 C-NMR测量，其每100个甲基支链中的丁基支链数目在1和20之间，其密度d（kg / m 3）在880和980之间，密度d及其熔点Tm（℃）满足由下式（1）至（3）定义的条件：将乙烯均聚物模塑成型。

28. 发明授权

US06207754B1 Low modulus thermoplastic olefin compositions 失效
标题翻译：低模量热塑性烯烃组合物
公开(公告)号：US06207754B1
公开(公告)日：2001-03-27
申请号：US08864954
申请日：1997-05-29
申请人： Thomas Chen-Chi Yu
发明人： Thomas Chen-Chi Yu
IPC分类号： C08F1002
CPC分类号： C08L23/10 , C08L23/0815 , C08L23/16 , Y10T428/31938 , C08L2666/04
摘要： This invention relates to thermoplastic olefin compositions of a low modulus which are suitable for fabrication into flexible skins and liners for applications which heretofore have been serviced by skins and liners produced essentially only from plasticized polyvinyl chloride resin compositions. TPO compositions of this invention comprise an impact modified polypropylene resin and a “plastomer” resin intimately blended in proportions with respect of one to another to provide a blend composition having a 1% secant modulus of less than 40,000 psi, and preferably less than 30,000 psi. Optionally, and preferably, the blend also comprises as a discrete component apart from the impact modified polypropylene an olefin copolymer elastomer or a cross-linked elastomer concentrate. Optionally the blend may contain other polyolefin components to alter its stiffness in desirable ways. In addition to the olefin based polymer components, the blend may further comprise, and preferably does comprise, a coupling agent and activator compound which, during melt compounding of the blend components causes the plastomer to extend to its dimer form and, when a discrete OCE component is present to couple the plastomer thereto.
摘要翻译：本发明涉及低模量的热塑性烯烃组合物，其适于制造用于迄今为止仅由增塑的聚氯乙烯树脂组合物生产的表皮和衬里所提供的应用的柔性表皮和衬里。本发明的TPO组合物包含冲击改性的聚丙烯树脂和“塑性体”树脂，其按相对于彼此的比例密切混合，以提供具有小于40,000psi，优选小于30,000psi的1％割线模量的共混组合物。并且优选地，并且优选地，共混物还包括作为分散组分，除了抗冲改性聚丙烯之外，烯烃共聚物弹性体或交联的弹性体浓缩物。任选地，共混物可以含有其它聚烯烃组分以以期望的方式改变其刚度。除了基于烯烃的聚合物组分之外，共混物可以进一步包含并且优选地包含偶联剂和活化剂化合物，其在共混组分的熔融混合期间使塑性体延伸至其二聚体形式，并且当离散的OCE 存在组分以将塑性体连接到其上。

29. 发明授权

US06191227B1 Polyethylene resin, and pipes and pipe joints using same 失效
标题翻译：聚乙烯树脂，管道和管接头使用相同
公开(公告)号：US06191227B1
公开(公告)日：2001-02-20
申请号：US08875845
申请日：1997-08-06
申请人： Tohru Matsuoka , Kiyofumi Matsuoka , Fumiaki Naka , Kiyonobu Sato
发明人： Tohru Matsuoka , Kiyofumi Matsuoka , Fumiaki Naka , Kiyonobu Sato
IPC分类号： C08F1002
CPC分类号： C08F10/02 , C08F210/16 , C08L23/0815 , C08L2205/02 , C08L2666/06 , C08F210/14 , C08F2500/12 , C08F2500/17 , C08F2500/01 , C08F2500/02
摘要： A polyethylene resin superior in both moldability and long-term physical properties and suitable for both pipe and pipe joint, the polyethylene resin having a density of 0.915 to 0.955 g·cm−3, a melt flow rate of not more than 0.20 dg·min as measured at 190° C. and at a load of 2.16 kgf, a melt flow rate of 17.0 to 70.0 dg·min−1 as measured at 190° C. and at a load of 21.6 kgf, a zero shear viscosity (&eegr;0) of 200,000 to 2,000,000 Pa·s, a characteristic time constant (&tgr;0) of 50 to 500 sec., and a ratio (&tgr;0/&eegr;0) of 1.0×10−4 to 4.0×10−4 Pa−1, the zero shear viscosity (&eegr;0) being obtained by approximating a dynamic melt viscosity (&eegr;*, unit: Pa·s) with equation [1], the dynamic melt viscosity (&eegr;*) being obtained by measurement using a rheometer at 190° C., at a parallel plate spacing of 1.5 mm, at a distortion of 10% to 15% and in the frequency (&ohgr;) range of 100 to 0.01 rad·s−1: η * = η 0 1 + ( τ 0 · ω ) n [ 1 ] where ⁢ ⁢ n ⁢ ⁢ is ⁢ ⁢ a ⁢ ⁢ parameter .
摘要翻译：聚乙烯树脂的成型性和长期物理性能均优于管接头，聚乙烯树脂的密度为0.915〜0.955g·cm-3，熔体流动速率不大于0.20dg·min 在190℃和2.16kgf的负荷下测量的熔体流动速率为在190℃和21.6kgf的负荷下测得的17.0至70.0dg.min-1，零剪切粘度（eta0） 20,000至2,000,000Pa.s，特征时间常数（＆tgr; 0）为50至500秒，比率（＆tgr; 0 / eta0）为1.0x10-4至4.0x10-4 Pa-1，零通过用等式[1]逼近动态熔体粘度（eta *，单位：Pa.s）获得的剪切粘度（eta0），通过使用流变仪在190℃测量获得的动态熔体粘度（η）平行板间距为1.5mm，畸变为10％至15％，频率（ω）范围为100至0.01rad.s -1：

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