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21. 发明授权

US5277792A Production of hydrocracked lubricants 失效
标题翻译：生产加氢裂化润滑剂
公开(公告)号：US5277792A
公开(公告)日：1994-01-11
申请号：US734971
申请日：1991-07-24
申请人： David O. Marler , Dominick N. Mazzone
发明人： David O. Marler , Dominick N. Mazzone
IPC分类号： B01J29/04 , C10G47/16 , C10G47/02 , C10G47/04 , C10G47/20
CPC分类号： B01J29/04 , C10G47/16
摘要： A lube hydrocracking process uses a catalyst which is based on an ultra-large pore crystalline material. The crystalline material exhibits unusually large pores of at least 13 .ANG. diameter and a high sorption capacity demonstrated by its benzene adsorption capacity of greater than about 15 grams benzene/100 grams at 50 torr and 25.degree. C. The crystalline material is characterized by an X-ray diffraction pattern with at least one d-spacing greater than about 18 .ANG. and in a particularly preferred form, a hexagonal arrangement of pores of at least 13 .ANG. diameter which can be indexed with a d.sub.100 value greater than about 18 .ANG.. The hydrocracking catalysts based on these materials are capable of producing hydrocracked lube products of good viscosity index in high yields without the use of fluorine or other promoters.
摘要翻译：润滑油加氢裂化方法使用基于超大孔结晶材料的催化剂。结晶材料表现出非常大的至少13（Aangstroem）直径的大孔，并且在50托和25摄氏度下其苯吸附能力大于约15克苯/ 100克证明具有高吸附能力。结晶材料的特征在于具有大于约18（Aangstroem）的至少一个d-间距的X射线衍射图案，并且在特别优选的形式中，具有至少13（Aangstroem）直径的孔的六边形排列，其可以以大于约18（Aangstroem）。基于这些材料的加氢裂化催化剂能够在不使用氟或其它促进剂的情况下以高产率生产粘度指数高的加氢裂化润滑油产品。

22. 发明授权

US5183557A Hydrocracking process using ultra-large pore size catalysts 失效
标题翻译：使用超大孔径催化剂的加氢裂化工艺
公开(公告)号：US5183557A
公开(公告)日：1993-02-02
申请号：US734983
申请日：1991-07-24
申请人： Thomas F. Degnan, Jr. , Kathleen M. Keville , Michael E. Landis , David O. Marler , Dominick N. Mazzone
发明人： Thomas F. Degnan, Jr. , Kathleen M. Keville , Michael E. Landis , David O. Marler , Dominick N. Mazzone
IPC分类号： B01J29/00 , B01J29/03 , B01J29/04 , B01J29/08 , B01J29/40 , B01J29/70 , B01J29/76 , B01J29/78 , B01J29/80 , C10G47/16
CPC分类号： B01J29/041 , B01J29/005 , B01J29/04 , B01J29/044 , B01J29/045 , B01J29/08 , B01J29/40 , B01J29/70 , B01J29/76 , B01J29/78 , B01J29/80 , C10G47/16 , B01J2229/26 , B01J2229/36 , B01J2229/42 , B01J29/0308 , B01J29/084
摘要： A hydrocracking catalyst with improved distillate selectivity comprises, in addition to a metal component, a mesoporous crystalline material together with a molecular sieve component of relatively smaller pore size. The metal component of the catalyst is preferably associated with the high-surface area mesoporous component and high-metal loadings can be achieved in order to give good hydrogenation activity to the catalyst. The relatively smaller pore size component is preferably a large pore size zeolite such as zeolite Y or an intermediate pore size zeolite such as ZSM-5; this component provides a higher level of acidic functionality than the mesoporous component, achieving a functional separation in the hydrocracking process, permitting the metals loading and acidic activities to be optimized for good catalyst selectivity and activity. The catalysts enable the distillate selectivities comparable to amorphous catalyst to be achieved with improved conversion activity.
摘要翻译：具有改进的馏出物选择性的加氢裂化催化剂除了金属组分之外还包括介孔结晶材料以及具有相对较小孔径的分子筛组分。催化剂的金属组分优选与高表面积介孔组分相关，并且可以实现高金属负载量，以便为催化剂提供良好的氢化活性。相对较小的孔径成分优选为大孔分子沸石，例如沸石Y或中等孔径沸石如ZSM-5; 该组分提供比介孔组分更高水平的酸性官能度，在加氢裂化过程中实现功能性分离，允许金属负载和酸性活性被优化以获得良好的催化剂选择性和活性。催化剂使得能够通过改进的转化活性实现与无定形催化剂相当的馏出物选择性。

23. 发明授权

US5144084A Process for the conversion of olefins to alcohols and/or ethers 失效
标题翻译：将烯烃转化为醇和/或醚的方法
公开(公告)号：US5144084A
公开(公告)日：1992-09-01
申请号：US798017
申请日：1991-11-20
申请人： Charles M. Sorensen , Philip Varghese , David O. Marler
发明人： Charles M. Sorensen , Philip Varghese , David O. Marler
IPC分类号： B01J29/06 , C07C29/04 , C07C41/06
CPC分类号： C07C41/06 , C07C29/04 , C07C41/09 , B01J2229/42 , B01J29/06
摘要： Olefins are converted to alcohols and/or ethers employing, as catalyst, an acidic zeolite which has been bound with an essentially non-acidic refractory oxide of at least one metal of Group IVA and/or IVB of the Period Table of the Elements, e.g., silica, titania, zirconia and/or germania.
摘要翻译：使用已经与元素周期表中IVA族和/或IVB族的至少一种金属的基本上非酸性耐火氧化物结合的酸性沸石作为催化剂将烯烃转化为醇和/或醚，例如，二氧化硅，二氧化钛，氧化锆和/或锗酸盐。

24. 发明授权

US4992606A Process for preparing short chain alkyl aromatic compounds 失效
标题翻译：制备短链烷基芳族化合物的方法
公开(公告)号：US4992606A
公开(公告)日：1991-02-12
申请号：US469998
申请日：1990-01-25
申请人： John D. Kushnerick , David O. Marler , John P. McWilliams , Charles M. Smith
发明人： John D. Kushnerick , David O. Marler , John P. McWilliams , Charles M. Smith
IPC分类号： B01J29/04 , C07C2/12
CPC分类号： C07C2/12 , B01J29/04 , C07C2529/06 , C07C2529/70
摘要： Relatively short chain alkyl aromatic compounds are prepared by alkylating an alkylatable aromatic compound with a relatively short chain alkylating agent under alkylation reaction conditions in the presence of catalyst comprising a synthetic porous crystalline material characterized by an X-ray diffraction pattern including interplanar d-spacings at 12.36.+-.0.4, 11.03.+-.0.2, 8.83.+-.0.14, 6.18.+-.0.12, 6.00.+-.0.10, 4.06.+-.0.07, 3.91.+-.0.07 and 3.42.+-.0.06 Angstroms.
摘要翻译：通过在烷基化反应条件下，在催化剂存在下，在烷基化反应条件下，使烷基化芳族化合物与相对短链烷基化剂进行烷基化，制备相对短链烷基芳族化合物，所述催化剂包含合成多孔结晶材料，其特征在于X射线衍射图包括在 12.36 +/- 0.4,11.03 +/- 0.2,8.83±0.14 6.18 +/- 0.12,6.00 +/- 0.10,4.06 +/- 0.07,3.91 +/- 0.07和3.42 +/- 0.06埃。

25. 发明授权

US4954663A Process for preparing long chain alkyl phenols 失效
标题翻译：制备长链烷基酚的方法
公开(公告)号：US4954663A
公开(公告)日：1990-09-04
申请号：US470015
申请日：1990-01-25
申请人： David O. Marler , John P. McWilliams
发明人： David O. Marler , John P. McWilliams
IPC分类号： B01J29/04 , C07C2/12
CPC分类号： C07C2/12 , B01J29/04 , C07C2529/06 , C07C2529/70
摘要： Long chain alkyl phenols are prepared by alkylating an alkylatable phenolic compound with a long chain alkylating agent under alkylation reaction conditions in the presence of catalyst comprising a synthetic porous crystalline material characterized by an X-ray diffraction pattern including interplanar d-spacings at 12.36.+-.0.4, 11.03.+-.0.2, 8.83.+-.0.14, 6.18.+-.0.12, 6.00.+-.0.10, 4.06.+-.0.07; 3.91.+-.0.07 and 3.42.+-.0.06 Angstroms.
摘要翻译：长链烷基酚通过在烷基化反应条件下在烷基化反应条件下在催化剂存在下烷基化制备，所述催化剂包含合成多孔结晶材料，其特征在于X射线衍射图包括在12.36±/ -0.4,11.03 +/- 0.2,8.83±0.14,6.18±0.12,6.00±0.10,4.06±0.07; 3.91 +/- 0.07和3.42 +/- 0.06埃。

26. 发明申请

US20110152062A1 DRYING DEVICE FOR PRODUCING SMALL QUANTITIES OF CONTROLLED PARTICLE SIZE CATALYSTS WHICH ARE APPROPRIATE FOR USE IN FLUIDIZED BED OPERATIONS SUCH AS FLUID CATALYTIC CRACKING 审中-公开
标题翻译：用于生产适用于流化床操作的受控粒度催化剂的小量数量的干燥装置，如流体催化裂化
公开(公告)号：US20110152062A1
公开(公告)日：2011-06-23
申请号：US12957817
申请日：2010-12-01
申请人： William A. Wachter , Brenda A. Raich , Theodore E. Datz , David O. Marler , Nicholas Rollman , Jeffrey T. Elks , Gordon F. Stuntz
发明人： William A. Wachter , Brenda A. Raich , Theodore E. Datz , David O. Marler , Nicholas Rollman , Jeffrey T. Elks , Gordon F. Stuntz
IPC分类号： B01J37/08 , B01J37/10 , B01J35/10 , B01J31/06 , B01J29/04
CPC分类号： B01J29/06 , B01J29/70 , B01J37/0018 , B01J37/0072 , B01J37/0236 , B01J37/08 , B01J2229/36 , B01J2229/42 , C10G11/05
摘要： Catalysts for experimentation are produced having a controlled matrix pore structure. The manufacturing process utilizes tape casting in the drying procedure in which a catalyst slurry is cast on a substrate and dried at a temperature of between about 50° C. to 200° C. for a period of time of about 0.1 to 1.0 hour. The dried catalyst particles can be removed from the substrate by several techniques, including scraping, burning, and deforming the substrate material, The resulting catalytic particles can be produced in an amount of about ca. 3 g to 300 g from slurries with volumes between 5 cc to 500 cc, which are suitable for small scale FCC reactors and for high throughput experimentation.
摘要翻译：生产具有受控矩阵孔结构的用于实验的催化剂。制造方法在干燥过程中使用带铸造，其中将催化剂浆料浇铸在基材上并在约50℃至200℃的温度下干燥约0.1至1.0小时的时间。干燥的催化剂颗粒可以通过几种技术从基材中除去，包括刮擦，燃烧和使基材变形。所得到的催化剂颗粒可以以约约 3克至300克，体积在5毫升至500毫升之间的浆料，适用于小规模的FCC反应器和高通量实验。

27. 发明授权

US07361619B2 Fischer-Tropsch catalyst production 有权
标题翻译：费 - 托催化剂生产
公开(公告)号：US07361619B2
公开(公告)日：2008-04-22
申请号：US10819379
申请日：2004-04-06
申请人： Andrzej M. Malek , Stephen C. Leviness , Horacio M. Trevino , Weldon K. Bell , David O. Marler
发明人： Andrzej M. Malek , Stephen C. Leviness , Horacio M. Trevino , Weldon K. Bell , David O. Marler
IPC分类号： B01J20/34 , B01J21/20 , B01J23/00 , B01J25/04 , B01J27/28
CPC分类号： C10G2/33 , B01J23/75 , B01J23/8896 , B01J37/12 , B01J37/18
摘要： Dispersed Active Metal catalyst for hydrogenation reactions is produced by treating a substantially catalytically inactive metal particulate with a solution capable of oxidizing the metal particulate and comprising of at least one compound of a hydrogenation catalyst metal thereby forming a layer of at least one of hydroxides and oxides thereon. The metal particulate is activated by treatment with a hydrogen-containing gas at elevated temperatures to form a porous layer of Dispersed Active Metal catalyst. Preferably, the treated metal particulate is dried prior to activation, and also preferably calcined in an oxidant-containing atmosphere prior to activation. The treatment solution may advantageously contain a compound of at least one promoter metal for the added catalyst metal. The porosity of the layer provides enhanced catalyst activity as well as improved methane selectivity in the Fischer-Tropsch process.
摘要翻译：用于氢化反应的分散活性金属催化剂通过用能够氧化金属颗粒并且包含至少一种氢化催化剂金属的化合物的溶液处理基本上催化惰性的金属颗粒而产生，从而形成氢氧化物和氧化物中的至少一种的层上。通过在高温下用含氢气体处理来活化金属颗粒以形成分散活性金属催化剂的多孔层。优选地，处理的金属颗粒在活化之前被干燥，并且还优选在活化之前在含氧化剂的气氛中煅烧。处理溶液可以有利地含有用于加入的催化剂金属的至少一种助催化剂金属的化合物。该层的孔隙率提高了催化剂活性以及在费 - 托工艺中提高的甲烷选择性。

28. 发明授权

US5705724A Aromatics alkylation with cracked recycled plastics 失效
标题翻译：用裂解的再生塑料进行芳烃烷基化
公开(公告)号：US5705724A
公开(公告)日：1998-01-06
申请号：US548850
申请日：1995-10-26
申请人： Nick A. Collins , Larry A. Green , Anagha A. Gupte , David O. Marler , William J. Tracy, III
发明人： Nick A. Collins , Larry A. Green , Anagha A. Gupte , David O. Marler , William J. Tracy, III
IPC分类号： C07C2/66 , C07C2/68 , C07C2/70 , C10G1/00 , C10G1/10 , C10G29/20 , C10G50/00
CPC分类号： C10G29/205 , C07C2/66 , C07C2/68 , C07C2/70 , C10G1/002 , C10G1/10 , C10G50/00 , C07C2521/12 , C07C2527/054 , C07C2527/1206 , C07C2527/1213 , C07C2527/126 , C07C2527/128 , C07C2527/135 , C07C2527/138 , C07C2527/16 , C07C2529/08 , C07C2529/18 , C07C2529/40 , C07C2529/65 , C07C2529/70
摘要： A process is disclosed for the production of alkylaromatic compounds employing olefinic liquid from thermally or catalytically cracked plastics as alkylating agent. The process comprises contacting a feedstream comprising alkylatable aromatics and the olefinic liquid with acidic alkylation catalyst under alkylation conditions in an alkylation zone; and recovering an effluent stream comprising alkylaromatic compounds. The alkylation can be performed with the product of plastics pyrolysis or with non-degraded plastic feedstock in-situ with thermal/catalytic degradation of the plastic.
摘要翻译：公开了用于使用来自热或催化裂化塑料的烯烃液体作为烷基化剂生产烷基芳族化合物的方法。该方法包括在烷基化区域的烷基化条件下将包含可烷基化芳族化合物和烯烃液体的进料流与酸性烷基化催化剂接触; 并回收包含烷基芳族化合物的流出物流。烷基化可以用塑料热分解产物或非降解塑料原料进行原位与塑料的热/催化降解进行。

29. 发明授权

US5583276A Process for producing low aromatic diesel fuel with high cetane index 失效
标题翻译：具有高十六烷指数的低芳烃柴油的生产工艺
公开(公告)号：US5583276A
公开(公告)日：1996-12-10
申请号：US442549
申请日：1995-05-16
申请人： Stuart D. Hellring , Charles T. Kresge , David O. Marler , Ernest W. Valyocsik
发明人： Stuart D. Hellring , Charles T. Kresge , David O. Marler , Ernest W. Valyocsik
IPC分类号： B01J29/04 , B01J29/70 , C01B39/12 , C01B39/46 , C01B39/48 , C07C2/58
CPC分类号： C01B39/12 , B01J29/04 , C01B39/48 , C07C2/58 , C07C2529/70
摘要： A process for converting at least one olefin and at least one isoparaffin to a diesel fuel blending component comprising the steps of contacting the olefin and the isoparaffin with a catalyst comprising MCM-58 to provide a diesel fuel. Process conditions can be varied to favor the formation of gasoline, distillate, lube range products or mixtures thereof.
摘要翻译：一种将至少一种烯烃和至少一种异链烷烃转化为柴油燃料共混组分的方法，包括使烯烃和异链烷烃与包含MCM-58的催化剂接触以提供柴油燃料的步骤。工艺条件可以变化以有利于形成汽油，馏出物，润滑剂产品或其混合物。

30. 发明授权

US5552357A Catalyst modification for shape selective hydrocarbon conversions 失效
标题翻译：用于形状选择性烃转化的催化剂改性
公开(公告)号：US5552357A
公开(公告)日：1996-09-03
申请号：US294801
申请日：1994-08-25
申请人： Rudolph M. Lago , David O. Marler , Sharon B. McCullen , David H. Olson
发明人： Rudolph M. Lago , David O. Marler , Sharon B. McCullen , David H. Olson
IPC分类号： B01J29/40 , B01J31/02 , B01J31/12 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/27 , C07C5/41 , C07C6/12 , C10G45/64 , B01J29/06
CPC分类号： C10G45/64 , B01J29/40 , B01J31/123 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/2708 , C07C5/41 , C07C6/123 , C07C6/126 , B01J2229/12 , B01J2229/26 , B01J2229/32 , B01J2229/36 , B01J2229/42 , C07C2529/06 , C07C2529/064 , Y02P20/52
摘要： A process for shape selective hydrocarbon conversion involves contacting a hydrocarbon feedstream under conversion conditions with a catalytic molecular sieve which has been modified by treatment with an amino silane polymer while molecular sieve acid sites are protected. When the process is toluene disproportionation, a toluene feedstream may also contain a second silicon source which is a high p-xylene selectivating agent. The invention also includes the modification method and the shape selective catalyst which results from the modification.
摘要翻译：用于形状选择性烃转化的方法包括在转化条件下使烃进料流与催化分子筛接触，催化分子筛在分子筛酸性位点受到保护时已用氨基硅烷聚合物进行改性。当该方法是甲苯歧化反应时，甲苯进料流还可含有作为高对二甲苯选择性试剂的第二硅源。本发明还包括由改性产生的改性方法和形状选择性催化剂。

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