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21. 发明申请

US20070099053A1 High durability fuel cell components with cerium salt additives 有权
标题翻译：高耐久性燃料电池组件与铈盐添加剂
公开(公告)号：US20070099053A1
公开(公告)日：2007-05-03
申请号：US11262268
申请日：2005-10-28
申请人： Matthew Frey , Daniel Pierpont , Steven Hamrock
发明人： Matthew Frey , Daniel Pierpont , Steven Hamrock
IPC分类号： H01M8/10 , C08J5/22
CPC分类号： H01M8/1051 , C08J5/2237 , C08J2327/18 , H01M8/1004 , H01M8/1023 , H01M8/1027 , H01M8/1032 , H01M8/1039 , H01M8/1058 , H01M8/1072 , H01M8/1081 , H01M2300/0091 , Y02E60/521 , Y02P70/56
摘要： A fuel cell membrane electrode assembly is provided comprising a polymer electrolyte membrane which comprises a polymer that comprises bound anionic functional groups, wherein the polymer electrolyte membrane additionally comprises cerium cations. In another aspect, a fuel cell membrane electrode assembly is provided comprising a polymer electrolyte membrane which comprises a polymer that comprises bound anionic functional groups, wherein at least a portion of the anionic functional groups are in acid form and at least a portion of the anionic functional groups are neutralized by cerium cations. In another aspect, a polymer electrolyte membrane is provided which comprises a polymer that comprises bound anionic functional groups, wherein the polymer electrolyte membrane additionally comprises cerium cations, and wherein the amount of cerium cations present is between 0.001 and 0.5 charge equivalents based on the molar amount of acid functional groups present in the polymer electrolyte, more typically between 0.005 and 0.2, more typically between 0.01 and 0.1, and more typically between 0.02 and 0.05.
摘要翻译：提供一种燃料电池膜电极组件，其包括聚合物电解质膜，其包含含有结合的阴离子官能团的聚合物，其中所述聚合物电解质膜另外包含铈阳离子。在另一方面，提供一种燃料电池膜电极组件，其包括聚合物电解质膜，其包含含有结合的阴离子官能团的聚合物，其中至少一部分阴离子官能团为酸形式，并且至少部分阴离子官能团被铈阳离子中和。在另一方面，提供了一种聚合物电解质膜，其包含含有结合的阴离子官能团的聚合物，其中所述聚合物电解质膜另外包含铈阳离子，并且其中存在的铈阳离子的量为0.001至0.5当量，基于摩尔存在于聚合物电解质中的酸官能团的量更多，通常在0.005至0.2之间，更典型地在0.01至0.1之间，更典型地在0.02至0.05之间。

22. 发明申请

US20070099052A1 High durability fuel cell components with cerium oxide additives 有权
标题翻译：高耐久性燃料电池组件与氧化铈添加剂
公开(公告)号：US20070099052A1
公开(公告)日：2007-05-03
申请号：US11261053
申请日：2005-10-28
申请人： Matthew Frey , Daniel Pierpont , Steven Hamrock
发明人： Matthew Frey , Daniel Pierpont , Steven Hamrock
IPC分类号： H01M8/10
CPC分类号： C08J5/2237 , C08J2327/12 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M8/1051 , H01M8/1058 , H01M2300/0091 , Y02P70/56 , Y10T29/49115
摘要： A fuel cell membrane electrode assembly is provided comprising a polymer electrolyte membrane which comprises a highly fluorinated polymer electrolyte and at least one cerium oxide compound dispersed therein. In addition, a method of making a fuel cell polymer electrolyte membrane is provided comprising the steps of: a) providing a highly fluorinated polymer electrolyte comprising acidic functional groups; b) dispersing therein at least one cerium oxide in an amount so as to provide between 0.01 and 5 percent of the total weight of the polymer electrolyte membrane; and c) thereafter forming a polymer electrolyte membrane comprising said polymer electrolyte.
摘要翻译：提供一种燃料电池膜电极组件，其包括聚合物电解质膜，其包含高度氟化的聚合物电解质和分散在其中的至少一种氧化铈化合物。此外，提供了制造燃料电池聚合物电解质膜的方法，包括以下步骤：a）提供包含酸性官能团的高氟化聚合物电解质; b）在其中分散至少一种氧化铈，以提供聚合物电解质膜总重量的0.01％至5％; 和c）之后形成包含所述聚合物电解质的聚合物电解质膜。

23. 发明申请

US20070065699A1 Fuel cell electrolyte membrane with basic polymer 有权
标题翻译：具有碱性聚合物的燃料电池电解质膜
公开(公告)号：US20070065699A1
公开(公告)日：2007-03-22
申请号：US11230091
申请日：2005-09-19
申请人： James Larson , Phat Pham , Matthew Frey , Steven Hamrock , Gregory Haugen , William Lamanna
发明人： James Larson , Phat Pham , Matthew Frey , Steven Hamrock , Gregory Haugen , William Lamanna
IPC分类号： H01M8/10
CPC分类号： C08J5/22 , C08J2379/06 , H01M8/1027 , H01M8/103 , H01M8/1048 , H01M8/1051 , H01M8/106 , H01M8/1062 , H01M8/1081 , H01M8/1093 , Y02P70/56
摘要： The present invention is an electrolyte membrane comprising an acid and a basic polymer, where the acid is a low-volatile acid that is fluorinated and is either oligomeric or non-polymeric, and where the basic polymer is protonated by the acid and is stable to hydrolysis.
摘要翻译：本发明是一种包含酸和碱性聚合物的电解质膜，其中酸是氟化的低分子或低聚物的低挥发性酸，其中碱性聚合物被酸质子化并且稳定于水解。

24. 发明申请

US20060063054A1 Durable fuel cell 有权
标题翻译：耐用燃料电池
公开(公告)号：US20060063054A1
公开(公告)日：2006-03-23
申请号：US10944998
申请日：2004-09-20
申请人： Matthew H. Frey , Steven Hamrock , Gregory Haugen , Phat Pham
发明人： Matthew H. Frey , Steven Hamrock , Gregory Haugen , Phat Pham
IPC分类号： H01M8/00
CPC分类号： B01D71/32 , B01D67/0079 , B01D69/141 , B01D2323/12 , H01M8/1023 , H01M8/1039 , H01M8/1051 , H01M8/1081 , Y02P70/56
摘要： Fuel cell membrane electrode assemblies and fuel cell polymer electrolyte membranes are provided comprising manganese oxides which demonstrate increased durability. Methods of making same are provided.
摘要翻译：提供燃料电池膜电极组件和燃料电池聚合物电解质膜，其包含显示出增加的耐久性的氧化锰。提供了制备方法。

25. 发明申请

US20050131096A1 Crosslinked polymer 有权
标题翻译：交联聚合物
公开(公告)号：US20050131096A1
公开(公告)日：2005-06-16
申请号：US10730238
申请日：2003-12-08
申请人： Naiyong Jing , Steven Hamrock
发明人： Naiyong Jing , Steven Hamrock
IPC分类号： C08J3/24 , C08J5/22 , C08G2/00
CPC分类号： C08J5/225 , C08J3/24 , C08J2327/12
摘要： A method is provided for obtaining crosslinked polymers, particularly fluorinated polymers having pendent sulfonic acid groups, by crosslinking through pendent groups which include a sulfonyl chloride group (—SO2Cl). The sulfonyl chloride group may be removed by application of electromagnetic radiation, typically in the ultraviolet band, or a radical initiator, leaving behind a radical which readily binds covalently to other polymer strands or to crosslinking agents to form crosslinks. Typically, the polymer is made by providing a polymer comprising pendent groups which include a group according to the formula —SO2F and converting at least a portion of the —SO2F groups to —SO2Cl. After crosslinking, the remaining —SO2F groups may be converted to sulfonic acid groups, yielding a crosslinked polymer electrolyte. Such crosslinked polymer electrolytes may be used to make polymer electrolyte membranes (PEM's) that may be used in electrolytic cells such as fuel cells.
摘要翻译：提供一种用于获得交联聚合物，特别是具有侧链磺酸基的氟化聚合物的方法，通过通过包括磺酰氯基团（-SO 2 Cl）的侧基进行交联。可以通过施加通常在紫外线带中的电磁辐射或自由基引发剂来除去磺酰氯基团，留下易于与其它聚合物链或交联剂共价结合以形成交联的基团。通常，通过提供包含侧基的聚合物制备聚合物，所述侧基包括根据式-SO 2 F的基团，并将至少一部分-SO 2 F基团取代-SO 2 Cl。交联后，剩余的-SO 2 F基团可以转化为磺酸基团，得到交联聚合物电解质。这种交联聚合物电解质可用于制备可用于电解池如燃料电池的聚合物电解质膜（PEM）。

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