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21. 发明申请

US20110257450A1 Method of Coupling a Carbon Source with Toluene to Form a Styrene Ethylbenzene 失效
标题翻译：将碳源与甲苯偶联以形成苯乙烯乙苯的方法
公开(公告)号：US20110257450A1
公开(公告)日：2011-10-20
申请号：US12763234
申请日：2010-04-20
申请人： Sivadinarayana Chinta , Joseph Thorman , James Butler
发明人： Sivadinarayana Chinta , Joseph Thorman , James Butler
IPC分类号： C07C1/207
CPC分类号： C07C2/862 , C07C2/864 , C07C2/867 , C07C2529/08 , C07C2529/60 , C07C15/46 , C07C15/073
摘要： A process is disclosed for making styrene or ethylbenzene by reacting toluene with a C1 source that is selected from the group consisting of methanol, formaldehyde, formalin, trioxane, methylformcel, paraformaldehyde, methylal, and combinations thereof.
摘要翻译：公开了通过使甲苯与选自甲醇，甲醛，福尔马林，三恶烷，甲基甲缩醛，多聚甲醛，甲缩醛及其组合的C1源反应制备苯乙烯或乙苯的方法。

22. 发明申请

US20070244273A1 Catalyst Deactivation Agents and Methods for Use of Same 失效
标题翻译：催化剂灭活剂及其使用方法
公开(公告)号：US20070244273A1
公开(公告)日：2007-10-18
申请号：US11279603
申请日：2006-04-13
申请人： Kenneth Blackmon , Joseph Thorman
发明人： Kenneth Blackmon , Joseph Thorman
IPC分类号： C08F2/38
CPC分类号： C08F10/00 , C08F110/06 , C08F2/42 , C08F2/14
摘要： A method of deactivating a polymerization catalyst system comprising contacting the catalyst system with a catalyst deactivation agent wherein the catalyst system comprises an alkyl aluminum cocatalyst and the reaction of the catalyst system and catalyst deactivation agent produces reaction products that are noncorrosive, nongelatinous, or both. A method of inhibiting the polymerization of propylene comprising contacting a polymerization catalyst system with a catalyst deactivation agent wherein the catalyst system comprises an alkyl aluminum cocatalyst and the reaction of the cocatalyst and the catalyst deactivation agent produces reaction products that are noncorrosive, nongelatinous, or both. A method of deactivating a polymerization catalyst system having an alkyl aluminum cocatalyst, comprising contacting the catalyst system with an alcohol, a carboxylic acid, an alkylene glycol, or combinations thereof.
摘要翻译：一种使聚合催化剂体系失活的方法，包括使催化剂体系与催化剂失活剂接触，其中催化剂体系包含烷基铝助催化剂，并且催化剂体系和催化剂失活剂的反应产生非腐蚀性，非皂化性或两者的反应产物。一种抑制丙烯聚合的方法，包括使聚合催化剂体系与催化剂失活剂接触，其中催化剂体系包含烷基铝助催化剂，并且助催化剂和催化剂失活剂的反应产生非腐蚀性，非皂化性或两者的反应产物。一种使具有烷基铝助催化剂的聚合催化剂体系失活的方法，包括使催化剂体系与醇，羧酸，亚烷基二醇或其组合物接触。

23. 发明申请

US20060142509A1 Polymerization catalyst system using di-se-butyl dimethyoxysilane for preparation of polypropylene 失效
标题翻译：使用二异丁基二甲氧基硅烷制备聚丙烯的聚合催化剂体系
公开(公告)号：US20060142509A1
公开(公告)日：2006-06-29
申请号：US11359818
申请日：2006-02-22
申请人： Joseph Thorman
发明人： Joseph Thorman
IPC分类号： C08F4/44
CPC分类号： B01J31/122 , B01J31/128 , B01J2231/122 , C08F10/00 , C08F10/06 , C08F110/06 , Y02P20/52 , C08F2500/15 , C08F2500/12 , C08F2500/04 , C08F2500/18 , C08F4/6465
摘要： It has been discovered that using di-sec-butyldialkoxysilanes, such as di-sec-butyldimethoxysilane (DSBDMS), as external electron donors for Ziegler-Natta catalysts can provide a catalyst system that may prepare polypropylene films with improved properties and processing. The catalyst systems of the invention provide high activity, high bulk density, moderate hydrogen response, moderate donor response and high polydispersity (MWD). Suitable di-sec-butyldialkoxysilanes have the formula (sBu)2Si(OR″)2, where R″ is independently a straight or branched alkyl group of 1-5 carbon atoms.
摘要翻译：已经发现，使用二仲丁基二烷氧基硅烷如二仲丁基二甲氧基硅烷（DSBDMS）作为齐格勒 - 纳塔催化剂的外部电子供体可以提供可制备具有改进的性能和加工性的聚丙烯膜的催化剂体系。本发明的催化剂体系提供高活性，高堆积密度，中等氢响应，中等供体响应和高多分散性（MWD）。合适的二仲丁基二烷氧基硅烷具有式（其中R“独立地为 1-5个碳原子的直链或支链烷基。

24. 发明授权

US09089832B2 Catalysts for oxidative coupling of hydrocarbons 有权
标题翻译：用于烃类氧化偶联的催化剂
公开(公告)号：US09089832B2
公开(公告)日：2015-07-28
申请号：US12494088
申请日：2009-06-29
申请人： Sivadinarayana Chinta , Joseph Thorman , James Butler
发明人： Sivadinarayana Chinta , Joseph Thorman , James Butler
IPC分类号： B01J23/00 , B01J23/10 , B01J23/02 , B01J23/06 , B01J23/04 , B01J23/36 , C07C2/84
CPC分类号： B01J23/04 , B01J23/002 , B01J23/10 , B01J23/36 , B01J2523/00 , C07C2/84 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/10 , C07C2523/36 , Y02P20/52 , C07C15/073 , C07C15/46 , C07C11/04 , C07C9/06 , B01J2523/22 , B01J2523/23 , B01J2523/3706 , B01J2523/24 , B01J2523/12 , B01J2523/15 , B01J2523/74
摘要： A catalyst includes: (A) at least one element selected from the group consisting of the Lanthanoid group, Mg, Ca, and the elements of Group 4 of the periodic table (Ti, Zr, and Hf); (B) at least one element selected from the group consisting of the Group 1 elements of Li, Na, K, Rb, Cs, and the elements of Group 3 (including La and Ac) and Groups 5-15 of the periodic table; (C) at least one element selected from the group consisting of the Group 1 elements of Li, Na, K, Rb, Cs, and the elements Ca, Sr, and Ba; and (D) oxygen.
摘要翻译：催化剂包括：（A）选自镧系元素，Mg，Ca和元素周期表第4族元素中的至少一种元素（Ti，Zr和Hf）; （B）选自Li，Na，K，Rb，Cs的第1族元素和第3族元素（包括La和Ac）和元素周期表第5-15族中的至少一种元素; （C）选自Li，Na，K，Rb，Cs族元素和元素Ca，Sr和Ba中的至少一种元素; 和（D）氧气。

25. 发明申请

US20120277509A1 Alkylation of Toluene to Form Styrene and Ethylbenzene 审中-公开
标题翻译：甲苯的烷基化形成苯乙烯和乙苯
公开(公告)号：US20120277509A1
公开(公告)日：2012-11-01
申请号：US13547605
申请日：2012-07-12
申请人： Joseph Thorman , James Butler , Sivadinarayana Chinta
发明人： Joseph Thorman , James Butler , Sivadinarayana Chinta
IPC分类号： C07C1/20
CPC分类号： C07C2/867 , C07C2/862 , C07C2/864 , C07C2529/068 , C07C2529/076 , C07C2529/08 , C07C2529/60 , C07C15/073 , C07C15/46
摘要： A process is disclosed for making styrene and/or ethylbenzene by reacting toluene with a C1 source over a catalyst in one or more reactors to form a product stream comprising styrene and/or ethylbenzene where the catalyst time on stream prior to regeneration is less than 1 hour.
摘要翻译：公开了一种用于通过在一个或多个反应器中的催化剂上使甲苯与C1源反应制备苯乙烯和/或乙苯以形成包含苯乙烯和/或乙苯的产物流的方法，其中再生之前的催化剂时间小于1 小时。

26. 发明授权

US08258359B2 Alkylation of toluene to form styrene and ethylbenzene 失效
标题翻译：甲苯的烷基化形成苯乙烯和乙苯
公开(公告)号：US08258359B2
公开(公告)日：2012-09-04
申请号：US12763235
申请日：2010-04-20
申请人： Joseph Thorman , James Butler , Sivadinarayana Chinta
发明人： Joseph Thorman , James Butler , Sivadinarayana Chinta
IPC分类号： C07C2/66
CPC分类号： C07C2/867 , C07C2/862 , C07C2/864 , C07C2529/068 , C07C2529/076 , C07C2529/08 , C07C2529/60 , C07C15/073 , C07C15/46
摘要： A process is disclosed for making styrene and/or ethylbenzene by reacting toluene with a C1 source over a catalyst in one or more reactors to form a product stream comprising styrene and/or ethylbenzene where the catalyst time on stream prior to regeneration is less than 1 hour.
摘要翻译：公开了一种用于通过在一个或多个反应器中的催化剂上使甲苯与C1源反应制备苯乙烯和/或乙苯以形成包含苯乙烯和/或乙苯的产物流的方法，其中再生之前的催化剂时间小于1 小时。

27. 发明申请

US20110257451A1 Alkylation of Toluene to Form Styrene and Ethylbenzene 失效
标题翻译：甲苯的烷基化形成苯乙烯和乙苯
公开(公告)号：US20110257451A1
公开(公告)日：2011-10-20
申请号：US12763235
申请日：2010-04-20
申请人： Joseph Thorman , James Butler , Sivadinarayana Chinta
发明人： Joseph Thorman , James Butler , Sivadinarayana Chinta
IPC分类号： C07C1/207 , C07C15/46
CPC分类号： C07C2/867 , C07C2/862 , C07C2/864 , C07C2529/068 , C07C2529/076 , C07C2529/08 , C07C2529/60 , C07C15/073 , C07C15/46
摘要： A process is disclosed for making styrene and/or ethylbenzene by reacting toluene with a C1 source over a catalyst in one or more reactors to form a product stream comprising styrene and/or ethylbenzene where the catalyst time on stream prior to regeneration is less than 1 hour.
摘要翻译：公开了一种用于通过在一个或多个反应器中的催化剂上使甲苯与C1源反应制备苯乙烯和/或乙苯以形成包含苯乙烯和/或乙苯的产物流的方法，其中再生之前的催化剂时间小于1 小时。

28. 发明申请

US20070093378A1 Process for forming a Ziegler-Natta catalyst system having a controlled morphology 审中-公开
标题翻译：形成具有受控形态的齐格勒 - 纳塔催化剂体系的方法
公开(公告)号：US20070093378A1
公开(公告)日：2007-04-26
申请号：US11638117
申请日：2006-12-13
申请人： Joseph Thorman
发明人： Joseph Thorman
IPC分类号： B01J31/00
CPC分类号： C08F10/00 , C08F110/02 , C08F110/06 , C08F4/6546 , C08F4/6541 , C08F4/651 , C08F2500/12 , C08F2500/18 , C08F2500/04 , C08F2500/24
摘要： A pre-catalyst is formed by reacting butylethylmagnesium with an alcohol to form a magnesium alkoxide compound, followed by contacting the magnesium alkoxide compound with a phosphorous compound to form a magnesium alkoxide phosphorous compound mixture. The magnesium alkoxide phosphorous compound mixture is subsequently reacted with TiCl4 to form a MgCl2 support. The MgCl2 support is then contacted with an internal donor while being heated to form a first catalyst slurry, which is then contacted with TiCl4 while being heated to form a second catalyst slurry. The second catalyst slurry is next contacted with TiCl4 while being heated to form a third catalyst slurry, which is washed and dried, resulting in a highly active pre-catalyst with controlled morphology. The pre-catalyst may be combined with one or more co-catalysts and optionally one or more external electron donors to form an active catalyst system, which may be used for the polymerization of olefins.
摘要翻译：通过使丁基乙基镁与醇反应以形成烷氧基镁化合物形成预催化剂，然后使烷氧基化镁与磷化合物接触以形成烷氧基镁磷化合物混合物。随后使烷氧基镁磷化合物混合物与TiCl 4反应形成MgCl 2载体。然后将MgCl 2载体与内部供体接触，同时被加热以形成第一催化剂浆料，然后在加热下与TiCl 4接触以形成第二催化剂泥浆。接着第二催化剂浆料与TiCl 4同时加热，形成第三催化剂浆料，将其洗涤和干燥，得到具有受控形态的高活性预催化剂。预催化剂可以与一种或多种助催化剂和任选的一种或多种外部电子给体结合以形成可用于烯烃聚合的活性催化剂体系。

29. 发明申请

US20050004329A1 Process for forming a ziegler-natta catalyst system having a controlled morphology 失效
标题翻译：用于形成具有受控形态的齐格勒 - 纳塔催化剂体系的方法
公开(公告)号：US20050004329A1
公开(公告)日：2005-01-06
申请号：US10898739
申请日：2004-07-26
申请人： Joseph Thorman
发明人： Joseph Thorman
IPC分类号： C08F10/00 , C08F110/02 , C08F110/06 , C09K8/62 , C09K8/68 , C08F4/44 , B01J31/00
CPC分类号： C08F10/00 , C08F110/02 , C08F110/06 , C08F4/6546 , C08F4/6541 , C08F4/651 , C08F2500/12 , C08F2500/18 , C08F2500/04 , C08F2500/24
摘要： A pre-catalyst is formed by reacting butylethylmagnesium with an alcohol to form a magnesium alkoxide compound, followed by contacting the magnesium alkoxide compound with a phosphorous compound to form a magnesium alkoxide phosphorous compound mixture. The magnesium alkoxide phosphorous compound mixture is subsequently reacted with TiCl4 to form a MgCl2 support. The MgCl2 support is then contacted with an internal donor while being heated to form a first catalyst slurry, which is then contacted with TiCl4 while being heated to form a second catalyst slurry. The second catalyst slurry is next contacted with TiCl4 while being heated to form a third catalyst slurry, which is washed and dried, resulting in a highly active pre-catalyst with controlled morphology. The pre-catalyst may be combined with one or more co-catalysts and optionally one or more external electron donors to form an active catalyst system, which may be used for the polymerization of olefins.
摘要翻译：通过使丁基乙基镁与醇反应以形成烷氧基镁化合物形成预催化剂，然后使烷氧基化镁与磷化合物接触以形成烷氧基镁磷化合物混合物。随后将烷氧基镁磷化合物混合物与TiCl 4反应形成MgCl 2载体。然后将MgCl 2载体与内部供体接触，同时被加热以形成第一催化剂浆料，然后将其与TiCl 4接触，同时加热形成第二催化剂浆料。接着第二催化剂浆料与TiCl 4接触，同时被加热以形成第三催化剂浆液，将其洗涤和干燥，得到具有受控形态的高活性预催化剂。预催化剂可以与一种或多种助催化剂和任选的一种或多种外部电子给体结合以形成可用于烯烃聚合的活性催化剂体系。

30. 发明申请

US20110257453A1 Reactors and Processes for the Oxidative Coupling of Hydrocarbons 有权
标题翻译：碳氢化合物的氧化偶联反应器和工艺
公开(公告)号：US20110257453A1
公开(公告)日：2011-10-20
申请号：US12763233
申请日：2010-04-20
申请人： Sivadinarayana Chinta , Joseph Thorman
发明人： Sivadinarayana Chinta , Joseph Thorman
IPC分类号： C07C15/46 , B01J8/02 , C07C1/20
CPC分类号： C07C2/84 , B01J8/02 , B01J8/18 , B01J19/02 , B01J23/002 , B01J23/02 , B01J23/34 , B01J37/0201 , B01J37/031 , B01J2219/00006 , B01J2219/0209 , B01J2219/0218 , B01J2219/025 , B01J2523/00 , C07C2/64 , C07C5/327 , C07C2521/10 , C07C2523/02 , C07C2523/30 , C07C2523/34 , Y02P20/52 , B01J2523/12 , B01J2523/22 , B01J2523/69 , B01J2523/72 , C07C15/46
摘要： A method for the oxidative coupling of hydrocarbons includes providing an oxidative catalyst inside a reactor and carrying out the oxidative coupling reaction under a set of reaction conditions. The reactor surfaces that contact the reactants and products do not provide a significant detrimental catalyzing effect. In an embodiment the reactor contains an inert lining or a portion of the reactor inner surface is treated to reduce the detrimental catalytic effects. In an embodiment the reactor contains a lining that includes an oxidative catalyst.
摘要翻译：烃的氧化偶合的方法包括在反应器内提供氧化催化剂，并在一组反应条件下进行氧化偶联反应。与反应物和产物接触的反应器表面不会产生显着的不利的催化作用。在一个实施方案中，反应器包含惰性衬里或处理反应器内表面的一部分以减少有害的催化作用。在一个实施方案中，反应器含有包含氧化催化剂的衬里。

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