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11. 发明申请

US20120012797A1 SYNTHESIS OF LITHIUM-IRON-PHOSPHATES UNDER HYDROTHERMAL CONDITIONS 有权
标题翻译：氢氧条件下的锂铁磷酸盐的合成
公开(公告)号：US20120012797A1
公开(公告)日：2012-01-19
申请号：US13257137
申请日：2010-03-16
申请人： Kirill Bramnik , Hartmut Hibst , Jordan Keith Lampert
发明人： Kirill Bramnik , Hartmut Hibst , Jordan Keith Lampert
IPC分类号： H01B1/02 , H01B1/04 , B82Y30/00
CPC分类号： C01B25/45 , H01M4/5825
摘要： The present invention relates to a process for the preparation of compounds of general formula (I) Lia-bMb1Fe1-cMc2Pd-eMe3Ox, wherein Fe has the oxidation state +2 and M1, M2, M3, a, b, c, d, e and x are: M1: Na, K, Rb and/or Cs, M2: Mn, Mg, Al, Ca, Ti, Co, Ni, Cr, V, M3: Si, S, F a: 0.8-1.9, b: 0-0.3, c: 0-0.9, d: 0.8-1.9, e: 0-0.5, x: 1.0-8, depending on the amount and oxidation state of Li, M1, M2, P, M3, wherein compounds of general formula (I) are neutrally charged, comprising the following steps (A) providing a mixture comprising at least one lithium-comprising compound, at least one iron-comprising compound, in which iron has the oxidation state 0, and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and/or least one M3-comprising compound, if present, and at least one compound comprising at least one phosphorous atom in oxidation state +5, and (B) heating the mixture obtained in step (A) at a temperature of 100 to 500° C. and at an autogeneous pressure to obtain a compound of general formula (I).
摘要翻译：本发明涉及制备通式（I）Lia-bMb1Fe1-cMc2Pd-eMe3Ox的化合物的方法，其中Fe具有氧化态+2和M1，M2，M3，a，b，c，d，e 和x为：M1：Na，K，Rb和/或Cs，M2：Mn，Mg，Al，Ca，Ti，Co，Ni，Cr，V，M3：Si，S，Fa：0.8-1.9，b ：0-0.3，c：0-0.9，d：0.8-1.9，e：0-0.5，x：1.0-8，这取决于Li，M1，M2，P，M3的量和氧化态，其中化合物通式（I）是中性带电的，包括以下步骤（A），提供包含至少一种含锂化合物，至少一种含铁化合物的混合物，其中铁具有氧化态0，和至少一种M1 和/或至少一种含M2的化合物（如果存在）和/或至少一种含M3的化合物（如果存在）和至少一种包含至少一个氧化态的磷原子的化合物+5 ，（B）在100〜500℃的温度下加热步骤（A）中得到的混合物。和自动压力下，得到通式（I）的化合物。

12. 发明申请

US20100301281A1 PROCESS FOR THE PREPARATION OF POROUS CRYSTALLINE LITHIUM-, VANADIUM AND PHOSPHATE-COMPRISING MATERIALS 审中-公开
标题翻译：制备多晶硅酸锂，钒和磷酸盐包覆材料的方法
公开(公告)号：US20100301281A1
公开(公告)日：2010-12-02
申请号：US12681193
申请日：2008-09-18
申请人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
发明人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
IPC分类号： H01B1/04 , H01M4/88 , H01B1/02
CPC分类号： C01B25/45 , H01M4/136 , H01M4/5825
摘要： The present invention relates to a process for the preparation of compounds of general formula (I): Lia−bM1bV2-cM2c(PO4)x; wherein M1, M2, a, b, c and x have the following meanings: M1: Na, K, Rb and/or Cs, M2: Ti, Zr, Nb, Cr, Mn, Fe, Co, Ni, Al, Mg and/or Sc, a: 1.5-4.5, b: 0-0.6, c: 0-1.98 and x: number to equalize the charge of Li and V and M1 and/or M2, if present, wherein a−b is >0, to a compound according to general formula (I) as defined above, to spherical agglomerates and/or particles comprising at least one compound of general formula (I) as defined above, to the use of such a compound for the preparation of a cathode of a lithium ion battery or an electrochemical cell, and to a cathode for a lithium ion battery, comprising at least one compound as defined above.
摘要翻译：本发明涉及制备通式（I）的化合物的方法：Lia-bM1bV2-cM2c（PO4）x; 其中M1，M2，a，b，c和x具有以下含义：M1：Na，K，Rb和/或Cs，M2：Ti，Zr，Nb，Cr，Mn，Fe，Co，Ni，和/或Sc，a：1.5-4.5，b：0-0.6，c：0-1.98和x：数，以均衡Li和V以及M1和/或M2的电荷（如果存在），其中a-b> 0的至少一种如上定义的通式（I）的化合物与包含至少一种如上所定义的通式（I）的化合物的球形聚集体和/或颗粒结合使用这种化合物来制备锂离子电池或电化学电池的阴极，以及包含至少一种如上所定义的化合物的锂离子电池用阴极。

13. 发明申请

US20100283012A1 PROCESS FOR THE PREPARATION OF CRYSTALLINE LITHIUM-, VANADIUM-AND PHOSPHATE-COMPRISING MATERIALS 失效
标题翻译：制备晶体锂，钒和磷酸盐包覆材料的方法
公开(公告)号：US20100283012A1
公开(公告)日：2010-11-11
申请号：US12680797
申请日：2008-09-18
申请人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
发明人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
IPC分类号： H01B1/04 , H01M4/88 , H01B1/02
CPC分类号： C01B25/45 , H01M4/5825 , H01M10/0525
摘要： The present invention relates to a process for the preparation of compounds of general formula (I) Lia-bM1bV2-cM2c(PO4)x (I) with M1: Na, K, Rb and/or Cs, M2: Ti, Zr, Nb, Cr, Mn, Fe, Co, Ni, Al, Mg and/or Sc, a: 1.5-4.5, b: 0-0.6, c: 0-1.98 and x: number to equalize the charge of Li and V and M1 and/or M2, if present, wherein a−b is >0, by providing an essentially aqueous mixture comprising at least one lithium-comprising compound, at least one vanadium-comprising compound in which vanadium has the oxidation state +5 and/or +4, and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and at least one reducing agent which is oxidized to at least one compound comprising at least one phosphorous atom in oxidation state +5, drying and calcining.
摘要翻译：本发明涉及制备具有M1：Na，K，Rb和/或Cs，M2：Ti，Zr，Nb的通式（I）Lia-bM1bV2-cM2c（PO4）x（Ⅰ）的化合物的方法，Cr，Mn，Fe，Co，Ni，Al，Mg和/或Sc，a：1.5-4.5，b：0-0.6，c：0-1.98和x：等于Li和V和M1 和/或M2，如果存在，其中a-b为> 0，通过提供基本上含水的混合物，其包含至少一种含锂化合物，至少一种含钒化合物，其中钒具有+5和/或 +4，和至少一种含M1化合物（如果存在）和/或至少一种含M2化合物（如果存在）和至少一种还原剂被氧化成至少一种包含至少一个磷原子的化合物氧化态+5，干燥和煅烧。

14. 发明授权

US08506847B2 Process for the preparation of crystalline lithium-, vanadium-and phosphate-comprising materials 失效
标题翻译：用于制备结晶的含锂，钒和磷酸盐的材料的方法
公开(公告)号：US08506847B2
公开(公告)日：2013-08-13
申请号：US12680797
申请日：2008-09-18
申请人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
发明人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
IPC分类号： H01B1/06 , H05B7/085 , H01M4/88
CPC分类号： C01B25/45 , H01M4/5825 , H01M10/0525
摘要： The present invention relates to a process for the preparation of compounds of general formula (I) Lia-bM1bV2-cM2c(PO4)x (I) with M1: Na, K, Rb and/or Cs, M2: Ti, Zr, Nb, Cr, Mn, Fe, Co, Ni, Al, Mg and/or Sc, a: 1.5-4.5, b: 0-0.6, c: 0-1.98 and x: number to equalize the charge of Li and V and M1 and/or M2, if present, wherein a−b is >0, by providing an essentially aqueous mixture comprising at least one lithium-comprising compound, at least one vanadium-comprising compound in which vanadium has the oxidation state +5 and/or +4, and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and at least one reducing agent which is oxidized to at least one compound comprising at least one phosphorous atom in oxidation state +5, drying and calcining.
摘要翻译：本发明涉及制备具有M1：Na，K，Rb和/或Cs，M2：Ti，Zr，Nb的通式（I）Lia-bM1bV2-cM2c（PO4）x（Ⅰ）的化合物的方法，Cr，Mn，Fe，Co，Ni，Al，Mg和/或Sc，a：1.5-4.5，b：0-0.6，c：0-1.98和x：等于Li和V和M1的电荷和/或M2，如果存在，其中ab> 0，通过提供基本上含水的混合物，其包含至少一种含锂化合物，至少一种含钒化合物，其中钒具有+5和/或+4的氧化态和至少一种含M1化合物（如果存在）和/或至少一种含M2化合物（如果存在）和至少一种还原剂被氧化成至少一种包含至少一个氧化态磷原子的化合物 +5，干燥和煅烧。

15. 发明申请

US20110049443A1 PROCESS FOR THE PREPARATION OF CRYSTALLINE LITHIUM-, IRON- AND PHOSPHATE-COMPRISING MATERIALS 审中-公开
标题翻译：制备结晶锂，铁和磷酸盐包覆材料的方法
公开(公告)号：US20110049443A1
公开(公告)日：2011-03-03
申请号：US12988418
申请日：2009-04-16
申请人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
发明人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
IPC分类号： H01B1/08 , H01B1/10
CPC分类号： H01M4/48 , C01B25/30 , C01B25/45 , C01P2006/40 , H01B1/02 , H01B1/08 , H01M4/525 , H01M4/5825 , H01M4/625 , H01M10/0525
摘要： The present application relates to a process for the preparation of compounds of general formula (I) Lia-bM1bFe1-cM2cPd-eM3eOx (I), wherein M1, M2, M3, a, b, c, d, e and x: M1: Na, K, Rb and/or Cs, M2: Mn, Mg, Ca, Ti, Co, Ni, Cr, V, M3: Si, S, a: 0.8-1.9, b: 0-0.3, c: 0-0.9, d: 0.8-1.9, e: 0-0.5, x: 1.0-8, depending on the amount and oxidation state of L1, M1, Fe, M2, P, M3, wherein compounds of general formula (I) are neutrally charged, comprising the following steps (A) providing an essentially aqueous mixture comprising at least one lithium-comprising compound, FeOOH as iron-comprising compound and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and/or least one M3-comprising compound, if present, at least one compound comprising at least one phosphorous atom and at least one reducing agent, (B) drying the mixture provided in step (A), in order to obtain a solid compound and (C) calcining the solid compound obtained from step (A) or (B) at a temperature of 300 to 950° C.
摘要翻译：本申请涉及制备通式（I）Lia-bM1bFe1-cM2cPd-eM3eOx（Ⅰ）的化合物的方法，其中M1，M2，M3，a，b，c，d，e和x：M1： Na，K，Rb和/或Cs，M2：Mn，Mg，Ca，Ti，Co，Ni，Cr，V，M3：Si，S，a：0.8-1.9，b：0-0.3，c： 0.9，d：0.8-1.9，e：0-0.5，x：1.0-8，取决于L1，M1，Fe，M2，P，M3的量和氧化态，其中通式（I）的化合物是中性的包括以下步骤（A），其提供基本上含水的混合物，其包含至少一种含锂化合物，作为含铁化合物的FeOOH和至少一种含M1化合物（如果存在）和/或至少一种含M2的化合物化合物（如果存在）和/或至少一种含M3化合物（如果存在）至少一种包含至少一个磷原子和至少一种还原剂的化合物，（B）按顺序干燥步骤（A）中提供的混合物得到固体化合物，（C）煅烧由步骤获得的固体化合物（A）或（B）在300〜950℃的温度下进行。

16. 发明授权

US08709298B2 Electrode material and use thereof for production of electrochemical cells 失效
标题翻译：电极材料及其用于生产电化学电池的用途
公开(公告)号：US08709298B2
公开(公告)日：2014-04-29
申请号：US13111263
申请日：2011-05-19
申请人： Martin Schulz-Dobrick , Hartmut Hibst , Jordan Keith Lampert , Robert Glaum , Helmut Ehrenberg , Katharina Gerber , Markus Herklotz , Frieder Scheiba
发明人： Martin Schulz-Dobrick , Hartmut Hibst , Jordan Keith Lampert , Robert Glaum , Helmut Ehrenberg , Katharina Gerber , Markus Herklotz , Frieder Scheiba
IPC分类号： H01B1/02 , C01B15/16 , H01M4/13 , H01M4/48
CPC分类号： H01B1/24 , C01B25/45 , H01M4/0404 , H01M4/136 , H01M4/505 , H01M4/525 , H01M4/5825 , H01M10/0525 , H01M10/0568 , H01M10/0569
摘要： A compound of the general formula (I) AaMbPcOd (I) in which the variables are each defined as follows: M is at least one transition metal selected from Co, Ni, Mn, Fe and Cr, A is Li or LixNa1-x where x is in the range from 0.2 to 1.0, a is in the range from 3.5 to 4.5, b is in the range from 0.8 to 1.2, c is in the range from 1.8 to 2.2 and d is in the range from 7.2 to 8.8.
摘要翻译：通式（I）AaMbPcOd（I）的化合物，其变量各自定义如下：M是选自Co，Ni，Mn，Fe和Cr中的至少一种过渡金属，A是Li或Li x Na 1-x，其中 x在0.2至1.0的范围内，a在3.5至4.5的范围内，b在0.8至1.2的范围内，c在1.8至2.2的范围内，d在7.2至8.8的范围内。

17. 发明申请

US20110147671A1 SYNTHESIS OF LIFEPO4 UNDER HYDROTHERMAL CONDITIONS 失效
标题翻译： LIFEPO4在水热条件下的合成
公开(公告)号：US20110147671A1
公开(公告)日：2011-06-23
申请号：US13060976
申请日：2009-08-25
申请人： Kirill Bramnik , Hartmut Hibst , Jordan Keith Lampert
发明人： Kirill Bramnik , Hartmut Hibst , Jordan Keith Lampert
IPC分类号： H01B1/02 , H01M4/88 , H01B1/04 , B82Y30/00
CPC分类号： H01M4/131 , C01B25/45 , H01M4/1391 , H01M4/5825
摘要： The present invention relates to a process for the preparation of compounds of general Formula (I) La−bM1bFe1−cM2cPd−eM3eOx (I), wherein Fe has the oxidation state +2 and M1, M2, M3, a, b, c, d, e and x are: M1: Na, K, Rb and/or Cs, M2: Mn, Mg, Al Ca, Ti Co, Ni, Cr, V, M3: Si, S, F a: 0.8-1.9, b: 0-0.3, c: 0-0.9, 15 d: 0.8-1.9, e: 0-0.5, x: 1.0-8, depending on the amount and oxidation state of Li, M1, M2, P, M3, wherein compounds of general Formula (I) are neutrally charged, comprising the following steps (A) providing a mixture comprising at least one lithium-comprising compound, at least one iron-comprising compound, in which iron has the oxidation state +3, and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and/or least one M3-comprising compound, if present, and at least one reducing agent which is oxidized to at least one compound comprising at least one phosphorous atom in oxidation state +5, and (B) heating the mixture obtained in step (A) at a temperature of 100 to 500° C. and at an autogeneous pressure to reduce Fe to oxidation state +2 and to obtain a compound of general Formula (I).
摘要翻译：本发明涉及制备通式（I）化合物La-bM1bFe1-cM2cPd-eM3eOx（Ⅰ）的方法，其中Fe具有氧化态+2和M1，M2，M3，a，b，c， d，e和x是：M1：Na，K，Rb和/或Cs，M2：Mn，Mg，Al Ca，Ti Co，Ni，Cr，V，M3：Si，S，F a：0.8-1.9， b：0-0.3，c：0-0.9,15d：0.8-1.9，e：0-0.5，x：1.0-8，这取决于Li，M1，M2，P，M3的量和氧化态，其中通式（I）的化合物是中性带电的，包括以下步骤（A），提供包含至少一种含锂化合物，至少一种含铁化合物的混合物，其中铁具有+3的氧化态，至少一种含M1化合物（如果存在）和/或至少一种含M2化合物（如果存在）和/或至少一种含M3化合物（如果存在）和至少一种被氧化成至少一种包含至少一个氧化态+5的磷原子的化合物，和（B）加热混合物在步骤（A）中，在100-500℃的温度和自发压力下将Fe还原成氧化态+2，得到通式（I）的化合物。

18. 发明授权

US09023523B2 Synthesis of lithium-iron-phosphates under hydrothermal conditions 有权
标题翻译：在水热条件下合成磷酸铁锂
公开(公告)号：US09023523B2
公开(公告)日：2015-05-05
申请号：US13257137
申请日：2010-03-16
申请人： Kirill Bramnik , Hartmut Hibst , Jordan Keith Lampert
发明人： Kirill Bramnik , Hartmut Hibst , Jordan Keith Lampert
IPC分类号： H01M4/58 , C01B25/30 , C01B25/45
CPC分类号： C01B25/45 , H01M4/5825
摘要： The present invention relates to a process for the preparation of compounds of general formula (I) Lia-bMb1Fe1-cMc2Pd-eMe3Ox, wherein Fe has the oxidation state +2 and M1, M2, M3, a, b, c, d, e and x are: M1: Na, K, Rb and/or Cs, M2: Mn, Mg, Al, Ca, Ti, Co, Ni, Cr, V, M3: Si, S, F a: 0.8-1.9, b: 0-0.3, c: 0-0.9, d: 0.8-1.9, e: 0-0.5, x: 1.0-8, depending on the amount and oxidation state of Li, M1, M2, P, M3, wherein compounds of general formula (I) are neutrally charged, comprising the following steps (A) providing a mixture comprising at least one lithium-comprising compound, at least one iron-comprising compound, in which iron has the oxidation state 0, and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and/or least one M3-comprising compound, if present, and at least one compound comprising at least one phosphorous atom in oxidation state +5, and (B) heating the mixture obtained in step (A) at a temperature of 100 to 500° C. and at an autogeneous pressure to obtain a compound of general formula (I).
摘要翻译：本发明涉及制备通式（I）Lia-bMb1Fe1-cMc2Pd-eMe3Ox的化合物的方法，其中Fe具有氧化态+2和M1，M2，M3，a，b，c，d，e 和x为：M1：Na，K，Rb和/或Cs，M2：Mn，Mg，Al，Ca，Ti，Co，Ni，Cr，V，M3：Si，S，F a：0.8-1.9，b ：0-0.3，c：0-0.9，d：0.8-1.9，e：0-0.5，x：1.0-8，这取决于Li，M1，M2，P，M3的量和氧化态，其中化合物通式（I）是中性带电的，包括以下步骤（A），提供包含至少一种含锂化合物，至少一种含铁化合物的混合物，其中铁具有氧化态0，和至少一种M1 和/或至少一种含M2的化合物（如果存在）和/或至少一种含M3的化合物（如果存在）和至少一种包含至少一个氧化态的磷原子的化合物+5 ，（B）在100〜500℃的温度下加热步骤（A）中得到的混合物。和自动压力下，得到通式（I）的化合物。

19. 发明授权

US08673497B2 Process for the preparation of crystalline lithium-, iron- and phosphate-comprising materials 有权
标题翻译：制备结晶的含锂，铁和磷酸盐的材料的方法
公开(公告)号：US08673497B2
公开(公告)日：2014-03-18
申请号：US12988222
申请日：2009-04-16
申请人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
发明人： Hartmut Hibst , Brian Roberts , Jordan Keith Lampert , Kirill Bramnik
IPC分类号： H01M4/58 , C01B25/30
CPC分类号： C01B25/45 , H01M4/136 , H01M4/5825 , H01M10/052
摘要： The present invention relates to a Process for the preparation of compounds of general formula (I), Lia-bM1bFe1-cM2cPd-eM3eOx, wherein M1, M2, M3, a, b, c, d and e: M1: Na, K, Rb and/or Cs, M2: Mn, Mg, Ca, Ti, Co, Ni, Cr, V, M3: Si, S, a: 0.8-1.9, b: 0-0.3, c: 0-0.9, d: 0.8-1.9, e: 0-0.5, x: 1.0-8, depending on the amount and oxidation state of Li, M1, Fe, M2, P, M3, wherein compounds of general formula (I) are neutrally charged, comprising the following steps (A) providing a mixture comprising at least one lithium-comprising compound, at least one iron-comprising compound, in which iron has the oxidation state +3, and at least one M1-comprising compound, if present, and/or at least one M2-comprising compound, if present, and/or least one M3-comprising compound, if present, and at least one reducing agent which is oxidized to at least one compound comprising at least one phosphorous atom in oxidation state +5, (B) optionally drying the mixture provided in step (A), in order to obtain a solid compound and (C) calcining the solid compound obtained from step (A) or (B) at a temperature of 300 to 1000° C.
摘要翻译：本发明涉及制备通式（I）化合物Lia-bM1bFe1-cM2cPd-eM3eOx的方法，其中M1，M2，M3，a，b，c，d和e：M1：Na，K， Rb和/或Cs，M2：Mn，Mg，Ca，Ti，Co，Ni，Cr，V，M3：Si，S，a：0.8-1.9，b：0-0.3，c：0-0.9，d： 0.8-1.9，e：0-0.5，x：1.0-8，这取决于Li，M1，Fe，M2，P，M3的量和氧化态，其中通式（I）的化合物是中性带电的，提供包含至少一种含锂化合物的混合物的步骤（A），至少一种含铁化合物，其中铁具有+3的氧化态和至少一种含M1化合物（如果存在）和/或至少一种含M2的化合物（如果存在）和/或至少一种含M3化合物（如果存在）和至少一种还原剂被氧化成至少一种包含至少一个氧化态的磷原子+5的化合物，（B）任选地干燥步骤（A）中提供的混合物，以获得a 固体化合物和（C）在300〜1000℃的温度下煅烧由步骤（A）或（B）得到的固体化合物。

20. 发明申请

US20110284806A1 ELECTRODE MATERIAL AND USE THEREOF FOR PRODUCTION OF ELECTROCHEMICAL CELLS 失效
标题翻译：电极材料及其生产电化学电池的用途
公开(公告)号：US20110284806A1
公开(公告)日：2011-11-24
申请号：US13111263
申请日：2011-05-19
申请人： Martin SCHULZ-DOBRICK , Hartmut Hibst , Jordan Keith Lampert , Robert Glaum , Helmut Ehrenberg , Katharina Gerber , Markus Herklotz , Frieder Scheiba
发明人： Martin SCHULZ-DOBRICK , Hartmut Hibst , Jordan Keith Lampert , Robert Glaum , Helmut Ehrenberg , Katharina Gerber , Markus Herklotz , Frieder Scheiba
IPC分类号： H01B1/18 , H01M4/525 , H01M4/485 , H01M4/505
CPC分类号： H01B1/24 , C01B25/45 , H01M4/0404 , H01M4/136 , H01M4/505 , H01M4/525 , H01M4/5825 , H01M10/0525 , H01M10/0568 , H01M10/0569
摘要： A compound of the general formula (I) AaMbPcOd (I) in which the variables are each defined as follows: M is at least one transition metal selected from Co, Ni, Mn, Fe and Cr, A is Li or LixNa1-x where x is in the range from 0.2 to 1.0, a is in the range from 3.5 to 4.5, b is in the range from 0.8 to 1.2, c is in the range from 1.8 to 2.2 and d is in the range from 7.2 to 8.8.
摘要翻译：通式（I）AaMbPcOd（I）的化合物，其变量各自定义如下：M是选自Co，Ni，Mn，Fe和Cr中的至少一种过渡金属，A是Li或Li x Na 1-x，其中 x在0.2至1.0的范围内，a在3.5至4.5的范围内，b在0.8至1.2的范围内，c在1.8至2.2的范围内，d在7.2至8.8的范围内。

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