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111. 发明申请

US20050236302A1 Process to manufacture low sulfur distillates 有权
标题翻译：制造低硫馏分的方法
公开(公告)号：US20050236302A1
公开(公告)日：2005-10-27
申请号：US11096498
申请日：2005-04-01
申请人： Stuart Soled , Sabato Miseo , Sonja Eijbouts
发明人： Stuart Soled , Sabato Miseo , Sonja Eijbouts
IPC分类号： B01J23/887 , B01J23/888 , B01J27/049 , B01J27/051 , B01J37/00 , B01J37/04 , C10G45/04 , C10G45/08 , C10G65/02
CPC分类号： C10G45/08 , B01J23/8877 , B01J23/888 , B01J37/0009 , B01J37/04 , C10G65/02
摘要： The instant invention relates to a process to produce low sulfur distillate products through the hydrotreating of distillate boiling range feedstreams in the presence of a bulk metal hydrotreating catalyst.
摘要翻译：本发明涉及通过在本体金属加氢处理催化剂存在下加热馏出馏出物沸程进料流来生产低硫馏分产物的方法。

112. 发明授权

US06712955B1 Slurry hydroprocessing using bulk multimetallic catalysts 有权
标题翻译：使用大量多金属催化剂的浆料加氢处理
公开(公告)号：US06712955B1
公开(公告)日：2004-03-30
申请号：US09869983
申请日：2001-08-22
申请人： Zhiguo Hou , Roby Bearden, Jr. , Ferrughelli Thomas David , Sabato Miseo , Martin Leo Gorbaty , Stuart Leon Soled
发明人： Zhiguo Hou , Roby Bearden, Jr. , Ferrughelli Thomas David , Sabato Miseo , Martin Leo Gorbaty , Stuart Leon Soled
IPC分类号： C10G4560
CPC分类号： B01J23/002 , B01J23/85 , B01J23/88 , B01J23/883 , B01J23/8878 , B01J23/888 , B01J23/8885 , B01J37/03 , B01J37/082 , B01J2523/00 , C07C29/16 , C08F8/00 , C08F8/04 , C08F8/50 , C10G45/08 , C10G45/16 , C10G47/04 , C10G65/04 , C10G65/08 , C10G65/12 , C10G2400/10 , C10G2400/14 , C08F240/00 , B01J2523/68 , B01J2523/69 , B01J2523/847 , B01J2523/842 , B01J2523/67 , B01J2523/31 , B01J2523/41
摘要： A slurry hydroprocessing process for upgrading a hydrocarbon feedstock containing nitrogen and sulfur using bulk multimetallic catalyst comprised of at least one Group VIII non-noble metal and at least two Group VIB metals wherein the ratio of Group VIB metal to Group VIII metal is about 10:1 to about 1:10.
摘要翻译：使用由至少一种VIII族非贵金属和至少两种VIB族金属组成的散装多金属催化剂来升级含有氮和硫的烃原料的浆料加氢处理方法，其中VIB族金属与VIII族金属的比例为约10： 1至约1:10。

113. 发明授权

US06652738B2 Process for preparing a mixed metal catalyst composition 有权
标题翻译：制备混合金属催化剂组合物的方法
公开(公告)号：US06652738B2
公开(公告)日：2003-11-25
申请号：US10346018
申请日：2003-01-16
申请人： Sonja Eijsbouts , Bob Gerardus Oogjen , Harmannus Willem Homan Free , Marinus Bruce Cerfontain , Kenneth Lloyd Riley , Stuart Leon Soled , Sabato Miseo
发明人： Sonja Eijsbouts , Bob Gerardus Oogjen , Harmannus Willem Homan Free , Marinus Bruce Cerfontain , Kenneth Lloyd Riley , Stuart Leon Soled , Sabato Miseo
IPC分类号： C10G4504
CPC分类号： B01J35/002 , B01J23/85 , B01J23/8885 , B01J35/0053 , B01J35/008 , B01J35/1019 , B01J35/1038 , B01J35/1061 , B01J37/0009 , B01J37/0236 , B01J37/031 , B01J37/20 , C10G49/04
摘要： The invention pertains to a process for the hydroprocessing of a hydrocarbon feedstock wherein said feedstock is contacted at hydroprocessing conditions with a catalyst composition which comprises bulk catalyst particles which comprise at least one Group VIII non-noble metal and at least two Group VIB metals. The Group VIII and Group VIB metals comprise from about 50 wt. % to about 100 wt. %, calculated as oxides, of the total weight of the bulk catalyst particles. The metals are present in the catalyst composition in their oxidic and/or sulfidic state. The catalyst composition has an X-ray diffraction pattern in which the characteristic full width at half maximum does not exceed 2.5° when the Group VIB metals are molybdenum, tungsten, and, optionally, chromium, or does not exceed 4.0° when the Group VIB metals are molybdenum and chromium or tungsten and chromium.
摘要翻译：本发明涉及烃原料的加氢处理方法，其中所述原料在加氢处理条件下与催化剂组合物接触，所述催化剂组合物包含包含至少一种VIII族非贵金属和至少两种VIB族金属的本体催化剂颗粒。 VIII族和VIB族金属包含约50wt。％至约100重量％以体积催化剂颗粒的总重量计算的氧化物％。金属以其氧化和/或硫化态存在于催化剂组合物中。催化剂组合物具有X射线衍射图，其中当VIB族金属为钼，钨和任选的铬时，半峰的特征全宽度不超过2.5°，当VIB族VIB金属为不超过4.0°时金属是钼和铬或钨和铬。

114. 发明授权

US06582590B1 Multistage hydroprocessing using bulk multimetallic catalyst 有权
标题翻译：使用大量多金属催化剂的多级加氢处理
公开(公告)号：US06582590B1
公开(公告)日：2003-06-24
申请号：US09869982
申请日：2001-08-22
申请人： Kenneth Lloyd Riley , Darryl Patrick Klein , Zhiguo Hou , Stuart Leon Soled , Michael Charles Kerby , Gary Brice McVicker , Edward Stanley Ellis , Michele Sue Touvelle , Sabato Miseo
发明人： Kenneth Lloyd Riley , Darryl Patrick Klein , Zhiguo Hou , Stuart Leon Soled , Michael Charles Kerby , Gary Brice McVicker , Edward Stanley Ellis , Michele Sue Touvelle , Sabato Miseo
IPC分类号： C10G4500
CPC分类号： B01J23/002 , B01J23/85 , B01J23/88 , B01J23/883 , B01J23/8878 , B01J23/888 , B01J23/8885 , B01J37/03 , B01J37/082 , B01J2523/00 , C07C29/16 , C08F8/00 , C08F8/04 , C08F8/50 , C10G45/08 , C10G45/16 , C10G47/04 , C10G65/04 , C10G65/08 , C10G65/12 , C10G2400/10 , C10G2400/14 , C08F240/00 , B01J2523/68 , B01J2523/69 , B01J2523/847 , B01J2523/842 , B01J2523/67 , B01J2523/31 , B01J2523/41
摘要： Sulfur content of distillate feedstock, which is greater than 3,000 wppm, is reduced using multi-stage hydrodesulfurization by reacting the feestream in stages with reaction zone(s) containing bulk multimetallic catalyst comprised of Group VIII non-noble metal(s) and at least two group VIB metals. The ratio of Group VIB to Group VIII non-noble metals is 10:1 to 1:10.
摘要翻译：通过使用多级加氢脱硫，通过使包含阶段的发泡与包含第VIII族非贵金属的多体金属催化剂和至少包含第一组的多元金属催化剂的反应区反应来减少大于3,000wppm的馏出物原料的硫含量两组VIB金属。 VIB族与VIII族非贵金属的比例为10：1〜1:10。

115. 发明授权

US5831138A Dispersed metal sulfide catalysts for hydroprocessing 失效
公开(公告)号：US5831138A
公开(公告)日：1998-11-03
申请号：US912895
申请日：1997-08-15
申请人： Teh Chung Ho , Stuart Leon Soled , Sabato Miseo , Gary Brice McVicker , Michel Daage , Viktor Buchholz
发明人： Teh Chung Ho , Stuart Leon Soled , Sabato Miseo , Gary Brice McVicker , Michel Daage , Viktor Buchholz
IPC分类号： B01J31/22 , B01J23/887 , B01J23/889 , B01J27/051 , B01J37/08 , B01J37/20 , C07B35/02 , C10G45/46 , C10G45/50 , C07C5/10
CPC分类号： B01J37/086 , B01J23/887 , B01J23/8878 , B01J23/8892 , B01J27/051 , B01J37/20 , C10G45/46 , C10G45/50
摘要： The present invention is directed toward a catalyst composition comprising a catalyst prepared by a process comprising: (a) impregnating an oxide precursor selected from the group consisting of rare earth oxide precursors, yttria precursors and mixtures thereof, onto an inorganic refractory oxide support; (b) drying said support at a temperature of about 100.degree. to about 120.degree. C. followed by calcining said support at a temperature of about 400.degree. to about 600.degree. C.; and (c) compositing or depositing on said support of step (b), a catalyst precursor salt represented by (ML)(Mo.sub.y W.sub.1-y O.sub.4).sub.a wherein M comprises Cr and/or one or more divalent promoter metals selected from the group consisting of Mn, Fe, Co, Ni, Cu, Zn and mixtures thereof, wherein y is any value ranging from 0 to 1, and wherein L is one or more neutral, nitrogen-containing ligands at least one of which is a chelating polydentate ligand; a=1 when chromium is not one of the promoter metals and 0.5.ltoreq.a.ltoreq.3 when Cr is one of the promoter metals. (d) sulfiding said deposited or composited supports of step (c) with an excess amount of sulfur in the form of one or more sulfur bearing compounds and at a temperature of at least about 250.degree. C. to form catalysts. In a preferred embodiment, the process will further comprise decomposing the composited or deposited supports of step (c) in a nonoxidizing atmosphere at a temperature of at least about 250.degree. C. prior to said sulfiding step (d). In a second aspect of the invention there is provided an improved aromatics hydrogenation process.

116. 发明授权

US5648577A Dispersed metal sulfide catalysts for hydroprocessing (LAW105) 失效
标题翻译：用于加氢处理的分散金属硫化物催化剂（LAW105）
公开(公告)号：US5648577A
公开(公告)日：1997-07-15
申请号：US460410
申请日：1995-06-02
申请人： Teh Chung Ho , Stuart Leon Soled , Sabato Miseo , Gary Brice McVicker , Michel Daage , Viktor Buchholz
发明人： Teh Chung Ho , Stuart Leon Soled , Sabato Miseo , Gary Brice McVicker , Michel Daage , Viktor Buchholz
IPC分类号： B01J31/22 , B01J23/887 , B01J23/889 , B01J27/051 , B01J37/08 , B01J37/20 , C07B35/02 , C10G45/46 , C10G45/50 , C07C5/10
CPC分类号： B01J37/086 , B01J23/887 , B01J23/8878 , B01J23/8892 , B01J27/051 , B01J37/20 , C10G45/46 , C10G45/50
摘要： The present invention is directed toward a catalyst composition prepared by a process comprising: (a) impregnating an oxide precursor selected from the group consisting of rare earth oxide precursors, yttria precursors and mixtures thereof, onto an inorganic refractory oxide support; (b) drying said support at a temperature of about 100.degree. to about 120.degree. C. followed by calcining said support at a temperature of about 400.degree. to about 600.degree. C.; and (c) compositing or depositing on said support of step (b), a catalyst precursor salt represented by (ML)(Mo.sub.y W.sub.1-y O.sub.4).sub.a wherein M comprises Cr and/or one or more divalent promoter metals selected from the group consisting of Mn, Fe, Co, Ni, Cu, Zn and mixtures thereof, wherein y is any value ranging from 0 to 1, and wherein L is one or more neutral, nitrogen-containing ligands at least one of which is a chelating polydentate ligand; a=1 when chromium is not one of the promoter metals and 0.5.ltoreq.a.ltoreq.3 when Cr is one of the promoter metals. (d) sulfiding said deposited or composited support of step (c) with an excess amount of sulfur in the form of one or more sulfur bearing compounds and at a temperature of at least about 250.degree. C. to form catalysts. In a preferred embodiment, the the composited or deposited supports of step (c) may be decomposed in a nonoxidizing atmosphere at a temperature of at least about 250.degree. C. prior to said sulfiding step (d). In a second aspect of the invention there is provided an improved aromatics hydrogenation process.
摘要翻译：本发明涉及通过包括以下步骤的方法制备的催化剂组合物：（a）将选自稀土氧化物前体，氧化钇前体及其混合物的氧化物前体浸渍到无机难熔氧化物载体上; （b）在约100至约120℃的温度下干燥所述载体，然后在约400至约600℃的温度下煅烧所述载体; 和（c）在步骤（b）的所述载体上合成或沉积由（ML）（MoyW1-yO4）a表示的催化剂前体盐，其中M包含Cr和/或一种或多种选自以下的二价助催化剂金属： Mn，Fe，Co，Ni，Cu，Zn及其混合物，其中y是0至1的任何值，并且其中L是一种或多种中性含氮配体，其中至少一种是螯合多齿配体; 当Cr不是助催化剂金属之一时，a = 1，当Cr是助催化剂金属之一时，a = 1。（d）将步骤（c）的沉积或复合载体用一种或多种含硫化合物形式的过量的硫硫化并在至少约250℃的温度下硫化以形成催化剂。在优选的实施方案中，在所述硫化步骤（d）之前，步骤（c）的复合或沉积的载体可以在非氧化气氛中在至少约250℃的温度下分解。在本发明的第二方面，提供了一种改进的芳族化合物氢化方法。

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