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1. 发明授权

US08951646B2 Layered structure comprising a layer containing a conjugated polymer compound 有权
标题翻译：包含含有共轭高分子化合物的层的层状结构
公开(公告)号：US08951646B2
公开(公告)日：2015-02-10
申请号：US12921108
申请日：2009-03-05
申请人： Masanobu Tanaka , Kenta Tanaka , Shohgo Yamauchi , Hideyuki Higashimura
发明人： Masanobu Tanaka , Kenta Tanaka , Shohgo Yamauchi , Hideyuki Higashimura
IPC分类号： H01L51/54 , C09K11/06 , C08G63/00 , H01L51/00 , C08G61/02 , C08G61/12 , H01L51/50
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/124 , C08G2261/1426 , C08G2261/3142 , C08G2261/316 , C08G2261/3221 , C08G2261/5222 , C08G2261/80 , H01L51/5048 , Y02E10/549 , Y10S428/917
摘要： A layered structure including a first electrode and a second electrode, a light-emitting layer or a charge separation layer between the first electrode and the second electrode, and a layer containing a conjugated polymer compound between the light-emitting layer or the charge separation layer and the first electrode, wherein the conjugated polymer compound contains a repeating unit selected from the group consisting of a repeating unit of formula (1).
摘要翻译：包括第一电极和第二电极的层状结构，在第一电极和第二电极之间的发光层或电荷分离层，以及在发光层或电荷分离层之间含有共轭高分子化合物的层和第一电极，其中共轭高分子化合物含有选自式（1）的重复单元的重复单元。

2. 发明申请

US20110006294A1 LAYERED STRUCTURE 有权
标题翻译：层状结构
公开(公告)号：US20110006294A1
公开(公告)日：2011-01-13
申请号：US12921108
申请日：2009-03-05
申请人： Masanobu Tanaka , Kenta Tanaka , Shohgo Yamauchi , Hideyuki Higashimura
发明人： Masanobu Tanaka , Kenta Tanaka , Shohgo Yamauchi , Hideyuki Higashimura
IPC分类号： H01L51/54 , C08G63/00
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/124 , C08G2261/1426 , C08G2261/3142 , C08G2261/316 , C08G2261/3221 , C08G2261/5222 , C08G2261/80 , H01L51/5048 , Y02E10/549 , Y10S428/917
摘要： Disclosed is a layered structure including a first electrode and a second electrode, a light-emitting layer or a charge separation layer between the first electrode and the second electrode, and a layer containing a conjugated polymer compound between the light-emitting layer or the charge separation layer and the first electrode, wherein the conjugated polymer compound contains a repeating unit selected from the group consisting of a repeating unit represented by formula (1): wherein Ar1 represents a divalent aromatic group, R1 represents a substituent group having a group represented by formula (2), Ar1 may have a substituent group other than R1, and n1 represents an integer of 1 or more; -(R2)c1-(Q1)n2-Y1(M1)a1(Z1)b1 (2) wherein R2 represents a divalent aromatic group which may have a substituent group, Q1 represents a divalent organic group which may have a substituent group, Y1 represents a carbocation, an ammonium cation, a phosphonyl cation or a sulfonyl cation, M1 represents F−, Cl−, Br−, I−, OH−, RaSO3−, RaCOO−, ClO−, ClO2−, ClO3−, ClO4−, SCN−, CN−, NO3−, SO42−, HSO4−, PO43−, HPO42−, H2PO4−, BF4− or PF6−, Z1 represents a metal ion or an ammonium ion which may have a substituent group, c1 represents 0 or 1, n2 represents an integer of 0 or more, provided that n2 is 0 when c1 is 0, a1 represents an integer of 1 or more, b1 represents an integer of 0 or more, a1 and b1 are selected so that the charge of the substituent group represented by formula (2) is 0, Ra represents an alkyl group having 1 to 30 carbon atoms, which may have a substituent group, or an aryl group having 6 to 50 carbon atoms, which may have a substituent group.
摘要翻译：公开了一种层状结构，其包括第一电极和第二电极，在第一电极和第二电极之间的发光层或电荷分离层，以及在发光层或电荷之间含有共轭高分子化合物的层分离层和第一电极，其中共轭高分子化合物含有选自由式（1）表示的重复单元的重复单元：其中Ar1表示二价芳族基团，R1表示具有由式（2）中，Ar 1可以具有除了R1以外的取代基，n1表示1以上的整数。 - （R2）c1-（Q1）n2-Y1（M1）a1（Z1）b1（2）其中R2表示可以具有取代基的二价芳族基团，Q1表示可以具有取代基的二价有机基团， Y1表示碳阳离子，铵阳离子，膦酰基阳离子或磺酰基阳离子，M1表示F-，Cl-，Br-，I-，OH-，RaSO 3 - ，RaCOO-，ClO-，ClO 2 - ，ClO 3 - ，ClO 4 - ，SCN-，CN-，NO3-，SO42-，HSO4-，PO43-，HPO42-，H2PO4-，BF4-或PF6-，Z1表示可具有取代基的金属离子或铵离子，c1表示 0或1，n2表示0以上的整数，条件是当c1为0时，n2为0，a1表示1以上的整数，b1表示0以上的整数，a1和b1选择为电荷由式（2）表示的取代基为0，R a表示可以具有取代基的碳原子数1〜30的烷基或碳原子数6〜50的芳基，可以具有取代基 ent组。

3. 发明授权

US09455408B2 Layered structure, polymer, electroluminescent device, and photoelectric conversion device 有权
标题翻译：分层结构，聚合物，电致发光器件和光电转换器件
公开(公告)号：US09455408B2
公开(公告)日：2016-09-27
申请号：US13499631
申请日：2010-09-28
申请人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
发明人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
IPC分类号： H01L51/54 , C08G63/685 , C08G63/66 , H01L51/00 , C08G61/02 , C08G61/12 , H01L51/50
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/1424 , C08G2261/1426 , C08G2261/146 , C08G2261/312 , C08G2261/3142 , C08G2261/3162 , C08G2261/344 , C08G2261/91 , C08G2261/95 , H01L51/0038 , H01L51/0043 , H01L51/5056 , H01L51/5072 , Y02E10/549
摘要： Provided is a layered structure having a first electrode, a second electrode, a light emitting layer or a charge separation layer located between the first electrode and the second electrode, and a layer located between the light emitting layer or the charge separation layer and the first electrode and containing a polymer having a repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups. Also provided is a polymer having, as the repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups, one or more repeating units selected from four specific repeating units containing an aromatic group. The layered structure of the present invention provides an electroluminescent device capable of emitting light at a high luminance and a photoelectric conversion device having a high photoelectric conversion efficiency.
摘要翻译：提供一种分层结构，其具有位于第一电极和第二电极之间的第一电极，第二电极，发光层或电荷分离层，以及位于发光层或电荷分离层之间的层和第一并且含有具有重复单元的聚合物，所述重复单元含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团。还提供了作为含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团的重复单元的聚合物，一个或多个选自含有芳族基团的四个特定重复单元的重复单元。本发明的分层结构提供了能够以高亮度发光的电致发光器件和具有高光电转换效率的光电转换器件。

4. 发明申请

US20120181529A1 LAYERED STRUCTURE, POLYMER, ELECTROLUMINESCENT DEVICE, AND PHOTOELECTRIC CONVERSION DEVICE 有权
标题翻译：层状结构，聚合物，电致发光器件和光电转换器件
公开(公告)号：US20120181529A1
公开(公告)日：2012-07-19
申请号：US13499631
申请日：2010-09-28
申请人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
发明人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
IPC分类号： H01L51/54 , C08G63/685 , C08G63/66
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/1424 , C08G2261/1426 , C08G2261/146 , C08G2261/312 , C08G2261/3142 , C08G2261/3162 , C08G2261/344 , C08G2261/91 , C08G2261/95 , H01L51/0038 , H01L51/0043 , H01L51/5056 , H01L51/5072 , Y02E10/549
摘要： Provided is a layered structure having a first electrode, a second electrode, a light emitting layer or a charge separation layer located between the first electrode and the second electrode, and a layer located between the light emitting layer or the charge separation layer and the first electrode and containing a polymer having a repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups. Also provided is a polymer having, as the repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups, one or more repeating units selected from four specific repeating units containing an aromatic group. The layered structure of the present invention provides an electroluminescent device capable of emitting light at a high luminance and a photoelectric conversion device having a high photoelectric conversion efficiency.
摘要翻译：提供一种分层结构，其具有位于第一电极和第二电极之间的第一电极，第二电极，发光层或电荷分离层，以及位于发光层或电荷分离层之间的层和第一并且含有具有重复单元的聚合物，所述重复单元含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团。还提供了作为含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团的重复单元的聚合物，一个或多个选自含有芳族基团的四个特定重复单元的重复单元。本发明的分层结构提供了能够以高亮度发光的电致发光器件和具有高光电转换效率的光电转换器件。

5. 发明申请

US20130099224A1 LIGHT-EMITTING DEVICE AND PHOTOVOLTAIC CELL, AND METHOD FOR MANUFACTURING THE SAME 有权
标题翻译：发光装置和光电池及其制造方法
公开(公告)号：US20130099224A1
公开(公告)日：2013-04-25
申请号：US13807226
申请日：2011-06-24
申请人： Takayuki Iljima , Kenta Tanaka , Masanobu Tanaka , Hideyuki Higashimura
发明人： Takayuki Iljima , Kenta Tanaka , Masanobu Tanaka , Hideyuki Higashimura
IPC分类号： H01L51/50 , H01L51/00 , H01L51/42
CPC分类号： H01L51/5012 , C07D471/04 , C08G61/02 , C08G2261/1424 , C08G2261/1426 , C08G2261/149 , C08G2261/3142 , C08G2261/411 , C08G2261/412 , C08G2261/95 , H01L51/0002 , H01L51/0003 , H01L51/0037 , H01L51/0039 , H01L51/42 , H01L51/424 , H01L51/4253 , H01L51/5076 , H01L51/5092 , H05B33/22 , Y02E10/549 , Y02P70/521
摘要： Provided are a light-emitting device and a photovoltaic cell having excellent characteristics. A light-emitting device (10) includes a cathode (34), an anode (32), a light-emitting layer (50) interposed between the cathode (34) and the anode (32), and an electron injection layer (44) provided between the cathode (34) and the light-emitting layer (50) and connected to the cathode (34), in which at least one of the anode (32) and the cathode (34) contains a conductive material having an aspect ratio of 1.5 or more, and the electron injection layer (44) contains an organic compound having at least one of an ionic group and a polar group.
摘要翻译：提供了具有优异特性的发光器件和光伏电池。发光装置（10）包括阴极（34），阳极（32），介于阴极（34）和阳极（32）之间的发光层（50）和电子注入层（44））设置在阴极（34）和发光层（50）之间并连接到阴极（34），其中阳极（32）和阴极（34）中的至少一个包含具有一方面的导电材料比例为1.5以上，电子注入层（44）含有具有离子性基团和极性基团中的至少一种的有机化合物。

6. 发明授权

US08866134B2 Light-emitting device and photovoltaic cell, and method for manufacturing the same 有权
标题翻译：发光装置和光伏电池及其制造方法
公开(公告)号：US08866134B2
公开(公告)日：2014-10-21
申请号：US13807226
申请日：2011-06-24
申请人： Takayuki Iljima , Kenta Tanaka , Masanobu Tanaka , Hideyuki Higashimura
发明人： Takayuki Iljima , Kenta Tanaka , Masanobu Tanaka , Hideyuki Higashimura
IPC分类号： H01L29/06 , H01L51/52 , C08G61/02 , C07D471/04 , H01L51/00 , H01L51/50 , H01L51/42
CPC分类号： H01L51/5012 , C07D471/04 , C08G61/02 , C08G2261/1424 , C08G2261/1426 , C08G2261/149 , C08G2261/3142 , C08G2261/411 , C08G2261/412 , C08G2261/95 , H01L51/0002 , H01L51/0003 , H01L51/0037 , H01L51/0039 , H01L51/42 , H01L51/424 , H01L51/4253 , H01L51/5076 , H01L51/5092 , H05B33/22 , Y02E10/549 , Y02P70/521
摘要： Provided are a light-emitting device and a photovoltaic cell having excellent characteristics. A light-emitting device (10) includes a cathode (34), an anode (32), a light-emitting layer (50) interposed between the cathode (34) and the anode (32), and an electron injection layer (44) provided between the cathode (34) and the light-emitting layer (50) and connected to the cathode (34), in which at least one of the anode (32) and the cathode (34) contains a conductive material having an aspect ratio of 1.5 or more, and the electron injection layer (44) contains an organic compound having at least one of an ionic group and a polar group.
摘要翻译：提供了具有优异特性的发光器件和光伏电池。发光装置（10）包括阴极（34），阳极（32），介于阴极（34）和阳极（32）之间的发光层（50）和电子注入层（44））设置在阴极（34）和发光层（50）之间并连接到阴极（34），其中阳极（32）和阴极（34）中的至少一个包含具有一方面的导电材料比例为1.5以上，电子注入层（44）含有具有离子性基团和极性基团中的至少一种的有机化合物。

7. 发明授权

US09306169B2 Electronic device, polymer compound, organic compound, and method of producing polymer compound 有权
标题翻译：电子器件，高分子化合物，有机化合物，以及高分子化合物的制造方法
公开(公告)号：US09306169B2
公开(公告)日：2016-04-05
申请号：US14007668
申请日：2012-03-27
申请人： Masanobu Tanaka , Rui Ishikawa , Ken Sakakibara , Hideyuki Higashimura
发明人： Masanobu Tanaka , Rui Ishikawa , Ken Sakakibara , Hideyuki Higashimura
IPC分类号： H01L51/00 , C07C69/94 , C08G61/02 , C08G61/12 , C07C69/76 , H01L51/50
CPC分类号： H01L51/0039 , C07C69/76 , C07C69/94 , C07C2603/18 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/124 , C08G2261/142 , C08G2261/1424 , C08G2261/1426 , C08G2261/3142 , C08G2261/3221 , C08G2261/411 , C08G2261/512 , H01L51/0035 , H01L51/0043 , H01L51/5056 , H01L51/5088
摘要： An electronic device that serves as a high-brightness electroluminescent device includes a layer containing a polymer compound having one or more structural units selected from a structural unit represented by formula (1) and a structural unit represented by formula (7) as a charge injection layer and/or a charge transport layer: Wherein R1, R2, R6 and R7 represent certain groups; m1 and m5 represent an integer of 0 or more; when R2 and R7 are plurally present, they may be the same or different; and a hydrogen atom in formula (1) or (7) may be replaced with a substituent other than the certain groups.
摘要翻译：用作高亮度电致发光器件的电子器件包括含有具有一个或多个选自式（1）表示的结构单元和由式（7）表示的结构单元作为电荷注入的结构单元的高分子化合物的层层和/或电荷传输层：其中R1，R2，R6和R7表示某些基团; m1和m5表示0以上的整数，当R2和R7多个存在时，它们可以相同或不同; 式（1）或（7）中的氢原子可以被除了某些基团以外的取代基取代。

8. 发明授权

US09184388B2 Layered structure, electronic device using same, aromatic compound, and method for manufacturing said compound 有权
标题翻译：层状结构，使用其的电子器件，芳族化合物，以及所述化合物的制造方法
公开(公告)号：US09184388B2
公开(公告)日：2015-11-10
申请号：US13812678
申请日：2011-07-29
申请人： Arihiro Yashiro , Hideyuki Higashimura , Rui Ishikawa , Masanobu Tanaka
发明人： Arihiro Yashiro , Hideyuki Higashimura , Rui Ishikawa , Masanobu Tanaka
IPC分类号： H01L51/50 , H01L51/00 , C07C211/56 , C07C211/63 , C07F9/54 , C07F9/572 , C08G61/12 , C07D209/86 , C07F5/02
CPC分类号： H01L51/0035 , C07C211/56 , C07C211/63 , C07D209/86 , C07F5/025 , C07F9/5407 , C07F9/5442 , C07F9/5456 , C07F9/5728 , C08G61/12 , C08G2261/1424 , C08G2261/312 , C08G2261/3162 , C08G2261/411 , C08G2261/512 , C08G2261/91 , C08G2261/92 , C08G2261/95 , H01L51/5056 , Y02E10/549 , Y02P70/521
摘要： The present invention provides: a layered structure having a substrate and a hole injection and/or hole transport layer comprising an aromatic compound having, on a side chain, at least one type of group having a cationic center; an electronic device having the layered structure; an aromatic compound having, on a hydrocarbon side chain, at least one type of group having a cationic center; an aromatic compound having a leaving group on a hydrocarbon side chain; and a method for manufacturing the aromatic compound having, on a hydrocarbon side chain, at least one type of group having a cationic center, the method comprising reacting the aromatic compound having a leaving group on a hydrocarbon side chain with a specific nitrogen compound, phosphorus compound, sulfur compound, or a combination of two or more of these compounds, thereby converting the aromatic compound into an onium salt thereof. When used as an electronic device material, and particularly as a hole transport and/or hole injection material, the aromatic compound can achieve a higher current density at a given voltage.
摘要翻译：本发明提供：具有基材和空穴注入和/或空穴传输层的层状结构，所述空穴注入和/或空穴传输层包含芳族化合物，所述芳族化合物在侧链上具有至少一种具有阳离子中心的基团; 具有层状结构的电子设备; 在烃侧链上具有至少一种具有阳离子中心的基团的芳族化合物; 在烃侧链上具有离去基团的芳族化合物; 以及在烃侧链具有至少一种具有阳离子中心的基团的芳香族化合物的制造方法，其特征在于，使烃侧链上具有离去基团的芳香族化合物与特定的氮化合物反应，化合物，硫化合物或两种或更多种这些化合物的组合，从而将芳族化合物转化成其鎓盐。当用作电子器件材料，特别是用作空穴传输和/或空穴注入材料时，芳族化合物可以在给定电压下实现更高的电流密度。

9. 发明授权

US09306170B2 Electronic device and polymer compound 有权
标题翻译：电子器件和高分子化合物
公开(公告)号：US09306170B2
公开(公告)日：2016-04-05
申请号：US14007854
申请日：2012-03-27
申请人： Masanobu Tanaka , Rui Ishikawa , Norifumi Kobayashi , Ken Sakakibara , Hideyuki Higashimura
发明人： Masanobu Tanaka , Rui Ishikawa , Norifumi Kobayashi , Ken Sakakibara , Hideyuki Higashimura
IPC分类号： H01L51/00 , C08G61/10 , C08G61/12 , H01L51/50
CPC分类号： H01L51/0043 , C08G61/10 , C08G61/12 , C08G2261/1424 , C08G2261/1426 , C08G2261/314 , C08G2261/3142 , C08G2261/3162 , C08G2261/514 , C08G2261/95 , H01L51/0035 , H01L51/0039 , H01L51/5056 , H01L51/5088
摘要： An electronic device that serves as a high-brightness electroluminescent device includes a layer containing a polymer compound having one or more structural units selected from a structural unit represented by formula (1) and a structural unit represented by formula (14) as a charge injection layer and/or a charge transport layer: wherein Ar1 and Ar2 represent certain fused polycyclic aromatic groups; R1, R2, R6 and R7 represent certain organic groups; m1, m2 and m6 represent an integer of 1 or more; m7 represents an integer of 0 or more; and when R1, R2, R6 and R7 are each plurally present, they each may be the same or different.
摘要翻译：用作高亮度电致发光器件的电子器件包括含有具有一个或多个选自由式（1）表示的结构单元和由式（14）表示的结构单元作为电荷注入的结构单元的聚合物化合物的层层和/或电荷传输层：其中Ar1和Ar2表示某些稠合多环芳族基团; R1，R2，R6和R7表示某些有机基团; m1，m2，m6表示1以上的整数， m7表示0以上的整数，当R1，R2，R6和R7各自存在时，它们各自可以相同或不同。

10. 发明申请

US20140039131A1 ELECTRONIC DEVICE AND POLYMER COMPOUND 有权
标题翻译：电子器件和聚合物化合物
公开(公告)号：US20140039131A1
公开(公告)日：2014-02-06
申请号：US14007854
申请日：2012-03-27
申请人： Masanobu Tanaka , Rui Ishikawa , Norifumi Kobayashi , Ken Sakakibara , Hideyuki Higashimura
发明人： Masanobu Tanaka , Rui Ishikawa , Norifumi Kobayashi , Ken Sakakibara , Hideyuki Higashimura
IPC分类号： H01L51/00
CPC分类号： H01L51/0043 , C08G61/10 , C08G61/12 , C08G2261/1424 , C08G2261/1426 , C08G2261/314 , C08G2261/3142 , C08G2261/3162 , C08G2261/514 , C08G2261/95 , H01L51/0035 , H01L51/0039 , H01L51/5056 , H01L51/5088
摘要： An electronic device that serves as a high-brightness electroluminescent device includes a layer containing a polymer compound having one or more structural units selected from a structural unit represented by formula (1) and a structural unit represented by formula (14) as a charge injection layer and/or a charge transport layer: wherein Ar1 and Ar2 represent certain fused polycyclic aromatic groups; R1, R2, R6 and R7 represent certain organic groups; m1, m2 and m6 represent an integer of 1 or more; m7 represents an integer of 0 or more; and when R1, R2, R6 and R7 are each plurally present, they each may be the same or different.
摘要翻译：用作高亮度电致发光器件的电子器件包括含有具有一个或多个选自由式（1）表示的结构单元和由式（14）表示的结构单元作为电荷注入的结构单元的聚合物化合物的层层和/或电荷传输层：其中Ar1和Ar2表示某些稠合多环芳族基团; R1，R2，R6和R7表示某些有机基团; m1，m2，m6表示1以上的整数， m7表示0以上的整数，当R1，R2，R6和R7各自存在时，它们各自可以相同或不同。

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