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1. 发明公开

EP1209173A1 BRANCHED OLEFINIC MACROMONOMER, OLEFIN GRAFT COPOLYMER, AND OLEFIN RESIN COMPOSITION 审中-公开
标题翻译： VERZWEIGTE OLEFINISCHE MAKROMONOMERE，OLEFINISCHES PFROPFPOLYMER UND POLYOLEFINMISCHUNG
公开(公告)号：EP1209173A1
公开(公告)日：2002-05-29
申请号：EP00946378.7
申请日：2000-07-18
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： MACHIDA, Shuji , SATO, Kazuo , TATSUMI, Tomio , GOTO, Yasuhiro
IPC分类号： C08F10/00 , C08F290/04 , C08L101/00
CPC分类号： C08F290/04 , C08F290/042 , C08F290/14 , C08F290/141
摘要： The invention relates to olefin branched macromonomers, olefin graft copolymers and olefin resin compositions having the advantages of good compatibility with polyolefin resins and good moldability and workability. The olefin branched macromonomer satisfies the following (a) and (b):

(a) its weight-average molecular weight (Mw) measured through gel permeation chromatography (GPC) falls between 400 and 200000;
(b) its vinyl content is at least 70 mol% of all the unsaturated groups in the macromonomer.
摘要翻译：本发明涉及烯烃支化大分子单体，烯烃接枝共聚物和烯烃树脂组合物，其具有与聚烯烃树脂的良好相容性和良好的成型性和可加工性。烯烃支化大分子单体满足以下（a）和（b）：（a）通过凝胶渗透色谱法（GPC）测定的重均分子量（Mw）为400〜200000; （b）其乙烯基含量为大分子单体中所有不饱和基团的至少70摩尔％。

2. 发明公开

EP1375585A1 PROPYLENE POLYMER COMPOSITION, MOLDED OBJECT, AND POLYOLEFIN COPOLYMER 有权
标题翻译：丙烯酸树脂，丙烯腈聚合物，聚对苯二甲酸乙二醇酯
公开(公告)号：EP1375585A1
公开(公告)日：2004-01-02
申请号：EP02708707.1
申请日：2002-03-28
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： GOTO, Yasuhiro , NAKAGAWA, Masaru , TATSUMI, Tomio , MACHIDA, Shuji
IPC分类号： C08L23/10 , C08L53/00 , C08F255/00 , C08F210/16
CPC分类号： C08L23/10 , C08F210/06 , C08F297/08 , C08F297/083 , C08L23/02 , C08L23/16 , C08L53/00 , C08L2666/06 , C08L2666/04 , C08L2666/24 , C08L2666/02 , C08F210/16 , C08F2500/03 , C08F2500/17
摘要： The present invention provides a propylene polymer composition containing a component (A) which is either a propylene block copolymer or a composition containing a propylene polymer and a rubber ingredient; and a component (B) which is a polyolefin copolymer that contains a fraction eluting at 101°C or higher through temperature rising elution fractionation chromatography, the fraction exhibiting a 13 C-NMR peak attributed to an ethylene chain, the polyolefin copolymer having an intrinsic viscosity falling within a range of 0.5 to 10.0 deciliter/g as measured at 135°C in decalin; a molded product formed from the composition; and a polyolefin copolymer formed of the component (B) in which a propylene polymer segment and an ethylene copolymer segment are chemically linked. According to the invention, a propylene block copolymer or a composition containing a propylene polymer and a rubber ingredient that are excellent in impact strength and tensile strength, while maintaining high rigidity thereof can be produced.
摘要翻译：本发明提供了含有作为丙烯嵌段共聚物的组分（A）或含有丙烯聚合物和橡胶组分的组合物的丙烯聚合物组合物; 以及作为聚烯烃共聚物的成分（B），其含有通过升温洗脱分级分离色谱法在101℃以上洗脱的部分，所述馏分呈现归因于乙烯链的13 C-NMR峰，所述聚烯烃共聚物具有在135℃下在十氢化萘中测定的特性粘度在0.5至10.0分升/克的范围内; 由该组合物形成的模制品; 和由丙烯聚合物链段和乙烯共聚物链段化学连接的组分（B）形成的聚烯烃共聚物。根据本发明，可以制造出具有优异冲击强度和拉伸强度同时保持其高刚性的丙烯嵌段共聚物或含有丙烯聚合物和橡胶成分的组合物。

3. 发明公开

EP1375538A1 PROCESS FOR PRODUCING POLYOLEFIN RESIN COMPOSITION AND POLYPROPYLENE COMPOSITION 有权
标题翻译：生产聚烯烃树脂组合物和聚丙烯组合物的方法
公开(公告)号：EP1375538A1
公开(公告)日：2004-01-02
申请号：EP02702904.0
申请日：2002-03-12
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： MACHIDA, Shuji , SHINOHARA, Masayuki , HOUSAKI, Tatsuya
IPC分类号： C08F210/16 , C08L23/16 , C08F4/64 , C08F297/06
CPC分类号： C08L23/10 , C08F4/65904 , C08F4/65912 , C08F4/65927 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06 , C08F212/08 , C08F255/00 , C08F257/02 , C08F297/06 , C08F297/08 , C08L23/02 , C08L51/06 , C08L2205/02 , C08L2205/025 , C08L2308/00 , C08F4/65916 , C08F2/001 , C08L2666/06 , C08L2666/04 , C08L2666/02 , C08F2500/12 , C08F2500/18 , C08F2500/11 , C08F2500/17 , C08F210/08 , C08F210/14 , C08F2500/09 , C08F236/20 , C08F210/18 , C08F210/16
摘要： A process for producing a polyolefin-based resin composition comprises, in the first polymerization stage, polymerizing an α-olefin having 4 to 20 carbon atoms, a styrene or a cyclic olefin in the presence of a specific catalyst and, in the second polymerization stage, copolymerizing the obtained polymer with an α-olefin having 2 to 20 carbon atoms, a styrene or a cyclic olefin in the presence of a polyene. A polypropylene composition has a branching parameter a and a branching index g in specific ranges. The curve showing the change in viscosity under elongation with time, the degradation parameter D or the content of a high molecular weight component is specified. The polyolefin-based resin composition exhibits excellent uniformity and improved workability in melting due to improved tension in melted condition. The polypropylene composition exhibits excellent melting elasticity and secondary workability and provides foamed molded articles, sheets and blow molded articles.
摘要翻译：在第一聚合阶段中，聚烯烃基树脂组合物的制备方法包括在特定催化剂存在下使具有4至20个碳原子的α-烯烃，苯乙烯或环烯烃聚合，并且在第二聚合阶段将所得到的聚合物与碳原子数2〜20的α-烯烃，苯乙烯或环状烯烃在多烯存在下进行共聚。聚丙烯组合物在特定范围内具有支化参数α和支化指数g。规定了伸长随时间的粘度变化，降解参数D或高分子量组分含量的曲线。由于熔融条件下的张力改善，聚烯烃基树脂组合物表现出优异的均匀性和改进的熔化可加工性。该聚丙烯组合物表现出优异的熔融弹性和二次加工性，并提供发泡模塑制品，片材和吹塑制品。

4. 发明公开

EP1408080A1 POLYOLEFIN RESIN COMPOSITION 有权
标题翻译： POLYOLEFINHARZZUSAMMENSETZUNG
公开(公告)号：EP1408080A1
公开(公告)日：2004-04-14
申请号：EP02741396.2
申请日：2002-07-02
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： MACHIDA, Shuji , KOBAYASHI, Yutaka , KUSUYAMA, Hideo , TANAKA, Akira
IPC分类号： C08L23/10
CPC分类号： C08L23/10 , C08L23/14 , C08L51/06 , C08L53/00 , C08L2205/02 , C08L2666/24 , C08L2666/04
摘要： The polyolefin-based resin composition (I) of the present invention comprises (A) 99.9 to 80% by mass of a propylene (co)polymer having (a) a melt flow rate (MFR) of 0.1 to 200 g/10 min, (b) a meso-pentad fraction [mmmm] of an ordinary temperature (25°C) xylene-insoluble component of 97.0% or higher, and (c) a content of an ordinary temperature (25°C) xylene-soluble component of 4 to 50% by mass; and (B) 0.1 to 20% by mass of a copolymer containing propylene chains of an isotactic structure, and copolymer chains constituted from at least two monomer units selected from the group consisting of ethylene, C 3 to C 20 α-olefins, cyclic olefins and aromatic vinyl monomers which are graft-bonded and/or block-bonded to said copolymer, and exhibits not only a high rigidity but also a highly enhanced impact strength and is well-balanced between the physical properties thereof.
摘要翻译：聚烯烃树脂组合物（I）含有99.9-80重量％的（A）丙烯（共）聚合物和0.1-20重量％的（B）共聚物，其中共聚物链由> = 2组成，选自乙烯，3- 20Cα-烯烃，环烯烃和芳族乙烯基单体与全同立构丙烯链接枝和/或嵌段键合。聚烯烃树脂组合物（I）含有99.9-80重量％的（A）丙烯（共）聚合物，其具有（a）熔体流动速率（MFR）为0.1-200g / 10分钟，（b）中孔部分（mmmm））常压（25℃）> 97％的二甲苯不溶物和（c）4-50重量％的常温（25℃）下的二甲苯可溶物含量; 和（B）共聚物的0.1-20重量％共聚物，其中选自乙烯，3-20℃的α-烯烃，环烯烃和芳族乙烯基单体的= 2的共聚物链与...共聚链被接枝和/或嵌段键合全同立构丙烯链。

5. 发明公开

EP1367093A1 POLYOLEFIN RESIN COMPOSITION 有权
标题翻译：聚烯烃树脂组合物
公开(公告)号：EP1367093A1
公开(公告)日：2003-12-03
申请号：EP02711323.2
申请日：2002-02-06
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： MACHIDA, Shuji , SATO, Kazuo
IPC分类号： C08L23/02 , C08L25/00 , C08L45/00 , C08L51/06
CPC分类号： C08L23/02 , C08F255/00 , C08L23/06 , C08L23/0815 , C08L23/0823 , C08L23/12 , C08L23/142 , C08L25/04 , C08L25/06 , C08L51/06 , C08L65/00 , C08L2205/02 , C08L2205/025 , C08L2205/03 , C08L2207/12 , C08L2666/02 , C08L2666/24 , C08L2666/04
摘要： The present invention provides a polyolefin-based resin composition, comprising (A) a polyolefin I produced from at least one monomer selected from the group consisting of α-olefins, cyclic olefins and styrenes; (B) a polyolefin II produced from said at least one monomer, which differs in composition or properties from said polyolefin I; and (C) a graft copolymer produced by bonding said polyolefins I and II to each other through a polyene, wherein (a) a ratio [(1/R 1 )/(1/R 1 )0] of a relaxation velocity (1/R 1 ) of a long-term relaxation component measured by a solid 1 H-NMR method about the composition to a relaxation velocity (1/R 1 ) 0 of a long-term relaxation component measured by a solid 1 H-NMR method about a resin mixture of only the components (A) and (B) is 1.01 or higher; and (b) an intrinsic viscosity [η] of the composition is in the range of 0.1 to 10 deciliter/g as measured in decalin at 135°C. The resin composition is readily controlled in property-determining factors such as morphology and interfacial strength, and is capable of providing a composite material composed of polyolefin-based resins according to properties as required.
摘要翻译：本发明提供了一种聚烯烃基树脂组合物，其包含（A）由选自α-烯烃，环烯烃和苯乙烯的至少一种单体制备的聚烯烃I; （B）由所述至少一种单体生产的聚烯烃II，其与所述聚烯烃I的组成或性能不同; 和（C）通过多烯将所述聚烯烃I和II彼此粘合而制得的接枝共聚物，其中（a）松弛速度（1 / R1）/（1 / R1））通过固体1 H-NMR法测定的关于该组成的长期松弛成分与仅通过固体1 H-NMR法测定的长期松弛成分的松弛速度（1 / R1）0 组分（A）和（B）为1.01或更高; 和（b）该组合物的特性粘度[η]在135℃萘烷中测得为0.1至10分升/克。树脂组合物容易控制诸如形态和界面强度等性能决定因素，并且能够根据需要提供由聚烯烃基树脂组成的复合材料。

6. 发明公开

EP1312620A1 PROPYLENE HOMOPOLYMER AND PROPYLENE COPOLYMER 有权
标题翻译：丙烯均和共聚
公开(公告)号：EP1312620A1
公开(公告)日：2003-05-21
申请号：EP01951943.8
申请日：2001-07-19
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： MACHIDA, Shuji , SAEKI, Takashi , TATSUMI, Tomio
IPC分类号： C08F10/06 , C08L23/10 , C08J5/00
CPC分类号： C08F110/06 , C08F210/06 , C08L23/02 , C08L23/10 , C08L23/12 , C08L2666/04 , C08F2500/11 , C08F2500/12
摘要： Provided are a propylene homopolymer in which a melt tension (MT), a Z average molecular weight (Mz) and a melt index (MI) (g/10 minutes) are specifically related and in which a difference in eluting temperatures and a maximum eluting temperature in programmed temperature fractional chromatography and a propylene copolymer in which a comonomer is specific α-olefin and a content thereof falls in a specific range and in which a melt tension (MT), a Z average molecular weight (Mz) and a melt index (MI) (g/10 minutes) are specifically related.
The propylene homopolymer or the propylene copolymer of the present invention has physical properties equivalent to or not lower than those of conventional propylene polymers, and it can be controlled in a melt tension and is suited to foaming molding, sheet molding and blow molding. Further, it is excellent in melt-processing characteristics, molding stability and a recycling property and can be applied to molding methods which are restricted in use in conventional propylene polymers, for example, large size blow molding and extrusion foaming molding.

7. 发明公开

EP0987279A1 OLEFINIC POLYMER 失效
标题翻译： VERZWEIGTES POLYPROPYLEN
公开(公告)号：EP0987279A1
公开(公告)日：2000-03-22
申请号：EP98923126.1
申请日：1998-06-04
申请人： IDEMITSU PETROCHEMICAL CO., LTD.
发明人： TATSUMI, Tomio , MACHIDA, Shuji , KANZAWA, Mitsugu , MINAMI, Yutaka , GOTO, Yasuhiro , KIJIMA, Masato
IPC分类号： C08F10/06 , C08F255/02 , C08L23/10
CPC分类号： C08F10/06 , C08F110/06 , C08F210/06 , C08F290/042 , C08L2205/08 , C08F2500/03 , C08F2500/17 , C08F2500/11 , C08F2500/12 , C08F2500/09 , C08F210/14 , C08F210/16
摘要： Long-chain, branched, propylene-based polymers, of which the melt index and the molecular weight distribution and the melt tension and the limiting viscosity both satisfy specific requirements, have good physical properties that are comparable to or better than those of conventional propylene-based polymers. They have good melt workability and are favorable to large-size blow molding and extrusion foaming. They are favorably used as miscibility improvers for propylene homopolymers and propylene-based copolymers.
摘要翻译：长链，支链，丙烯基聚合物，其熔体指数和分子量分布以及熔体张力和极限粘度都满足特定要求，具有与常规丙烯类聚合物相当或更好的物理性能，基聚合物。它们具有良好的熔融加工性，并且有利于大型吹塑和挤出发泡。它们有利地用作丙烯均聚物和丙烯基共聚物的混溶性改进剂。

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