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11. 发明公开

EP2416176A1 RADIOGRAPHIC IMAGE DETECTOR 审中-公开
标题翻译： RÖNTGENBILDDETEKTOR
公开(公告)号：EP2416176A1
公开(公告)日：2012-02-08
申请号：EP10758456.7
申请日：2010-03-19
申请人： Tokuyama Corporation , Tohoku University , Kyoto University , The University of Tokyo
发明人： FUKUDA, Kentaro , ISHIZU, Sumito , KAWAGUCHI, Noriaki , SUYAMA, Toshihisa , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , KUBO, Hidetoshi , TANIMORI, Toru , SEKIYA, Hiroyuki
IPC分类号： G01T1/18 , G01T1/20 , H01J31/50
CPC分类号： G01T1/28 , H01J31/49 , H01J47/02
摘要： [Problems to be Solved] It is an object of the present invention to provide a novel radiographic image detector which can detect radiation, such as hard X-rays or γ-rays, with high sensitivity and which is excellent in position resolution and count rate characteristic.
[Means to Solve the Problems] A radiographic image detector comprises a combination of a scintillator, such as a lanthanum fluoride crystal containing neodymium, for converting incident radiation into ultraviolet rays; and a gas multiplication ultraviolet image detector for converting ultraviolet rays into electrons, amplifying such electrons by use of a gas electron avalanche phenomenon, and detecting the electrons. The radiographic image detector is characterized in that the gas multiplication ultraviolet image detector is basically constituted by a photoelectric conversion substance, such as cesium iodide or cesium telluride, for converting ultraviolet rays into electrons; a gas electron multiplier for amplifying electrons by use of the gas electron avalanche phenomenon; and a pixel electrode having an amplification function and a detection function.
摘要翻译： [待解决的问题]本发明的目的是提供一种能够以高灵敏度检测诸如硬X射线或³射线等辐射的新型放射线图像检测器，其位置分辨率和计数率优异特性。解决问题的手段放射线图像检测器包括闪烁体，例如含有钕的氟化镧晶体，用于将入射辐射转换为紫外线的组合; 以及用于将紫外线转换成电子的气体倍增紫外线图像检测器，利用气体电子雪崩现象来放大这些电子，并检测电子。射线照相图像检测器的特征在于，气相色谱紫外图像检测器基本上由诸如碘化铯或碲化铯的光电转换物质构成，用于将紫外线转换成电子; 用于通过使用气体电子雪崩现象来放大电子的气体电子倍增器; 以及具有放大功能和检测功能的像素电极。

12. 发明授权

EP2636647B1 METAL FLUORIDE EUTECTIC BODY AND NEUTRON SCINTILLATOR 有权
标题翻译：金属氟化物共晶体和中子闪烁体
公开(公告)号：EP2636647B1
公开(公告)日：2017-06-28
申请号：EP11838044.3
申请日：2011-11-01
申请人： Tokuyama Corporation , Tohoku University
发明人： FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： C01F17/00 , C01D3/02 , C01F11/22 , C09K11/00 , C09K11/61 , G01T3/06 , G21K4/00 , C30B29/12 , C01D15/04 , C30B21/00 , C09K11/77
CPC分类号： C09K11/616 , C01D15/04 , C01F11/22 , C09K11/772 , C30B21/00 , C30B29/12 , G01T3/06 , G21K4/00 , G21K2004/06 , Y10T428/24975

13. 发明公开

EP2843088A1 METAL FLUORIDE CRYSTAL, LIGHT EMITTING ELEMENT, SCINTILLATOR, METHOD FOR DETECTING NEUTRONS, AND METHOD FOR PRODUCING METAL FLUORIDE CRYSTAL 审中-公开
标题翻译：金属氟化物结晶，发光元件闪烁体METHOD FOR中子用于生产金属氟化物结晶DETECTION AND METHOD
公开(公告)号：EP2843088A1
公开(公告)日：2015-03-04
申请号：EP13782368.8
申请日：2013-04-18
申请人： Tokuyama Corporation , Tohoku University
发明人： ISHIZU, Sumito , FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： C30B29/12 , C01F17/00 , C09K11/00 , C09K11/61 , G01T1/20 , G01T3/06
CPC分类号： C09K11/7733 , C30B15/08 , C30B29/12 , G01T3/06 , G21K4/00
摘要： [Object] To provide: a metal fluoride crystal which has a large amount of light emission; a method for producing the metal fluoride crystal; a light emitting element; a scintillator; and a method for detecting neutrons with use of the metal fluoride crystal.
[Solving Means] A light emitting element according to one embodiment of the present invention is configured of a metal fluoride crystal which is represented by chemical formula LiM 1 M 2 F 6 (wherein Li includes 6 Li; M 1 represents at least one alkaline earth metal element selected from among Mg, Ca, Sr and Ba; and M 2 represents at least one metal element selected from among Al, Ga and Sc), said metal fluoride crystal containing 0.02% by mole or more of Eu and having an Eu 2+ concentration of less than 0.01% by mole.
摘要翻译：本发明的课题提供：一种金属氟化物晶体具有大的发光量的; 用于制造金属氟化物结晶的方法; 一个发光元件; 闪烁; 和用于在使用该金属氟化物结晶的检测中子的方法。 [解决手段]发光元件雅丁到本发明的一个实施例的光被配置成在金属氟化物结晶的所有这是由化学式的LiM 1 M 2 F 6代表（worin李包括的6 Li，M 1个darstellt至少一种碱土选自Mg，Ca，Sr和Ba中选择的金属元素;和M 2 darstellt选自Al，Ga和Sc）中的至少一种金属元素，所述金属氟化物结晶含有12：02摩尔％或更多的Eu和具有与Eu 2 摩尔+小于0.01％的浓度。

14. 发明公开

EP2695928A1 SCINTILLATOR, RADIATION DETECTOR, AND METHOD FOR DETECTING RADIATION 有权
标题翻译：斯德哥尔摩公司（STRAHLUNGSDETEKTOR UND STRAHLUNGSDETEKTIONSVERFAHREN）
公开(公告)号：EP2695928A1
公开(公告)日：2014-02-12
申请号：EP12768181.5
申请日：2012-04-02
申请人： Tokuyama Corporation , Tohoku University
发明人： FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui
IPC分类号： C09K11/64 , C09K11/00 , G01T1/20 , G01T1/202 , G01T3/06
CPC分类号： C09K11/7733 , C09K11/772 , C09K11/7732 , G01T1/2023 , G01T3/06 , G21K4/00
摘要： The present invention aims at providing a scintillator for high temperature environments which has satisfactory light emission characteristics under high temperature environments; and a method for measuring radiation under high temperature environments. The scintillator for high temperature environments comprises a colquiriite-type crystal represented by the chemical formula LiM 1 M 2 X 6 (where M 1 is at least one alkaline earth metal element selected from Mg, Ca, Sr and Ba, M 2 is at least one metal element selected from Al, Ga and Sc, and X is at least one halogen element selected from F, Cl, Br and I), for example, typified by LiCaAlF 6 , and the crystal optionally containing a lanthanoid element such as Ce or Eu. The method for measuring radiation under high temperature environments uses the scintillator.
摘要翻译：本发明旨在提供一种在高温环境下具有令人满意的发光特性的高温环境的闪烁体; 以及在高温环境下测量辐射的方法。用于高温环境的闪烁体包括由化学式LiM 1 M 2 X 6（其中M 1是至少一种选自Mg，Ca，Sr和Ba的碱土金属元素，M 2至少为1 一种选自Al，Ga和Sc的金属元素，X是选自F，Cl，Br和I中的至少一种卤素元素），例如以LiCaAlF 6为代表的晶体，以及任选地含有镧系元素如Ce或欧洲联盟。在高温环境下测量辐射的方法使用闪烁体。

15. 发明公开

EP2636772A1 COLQUIRIITE-TYPE CRYSTAL, SCINTILLATOR FOR NEUTRON DETECTION, AND NEUTRON RADIATION DETECTOR 有权
标题翻译：中国科学院学报（社会科学版），，TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR TOR
公开(公告)号：EP2636772A1
公开(公告)日：2013-09-11
申请号：EP11838031.0
申请日：2011-11-01
申请人： Tokuyama Corporation , Tohoku University
发明人： ISHIZU, Sumito , FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： C30B29/12 , C09K11/00 , C09K11/64 , G01T3/06
CPC分类号： G01T3/06 , C09K11/7721 , C30B15/00 , C30B15/08 , C30B29/12
摘要： [Problems to be Solved] A colquiriite-type crystal preferred for a scintillator for neutron detection, which has high sensitivity to neutron and which is reduced in background noise attributed to γ rays; a scintillator for neutron detection which comprises this crystal; and a neutron detector are provided.
[Means to Solve the Problems] A colquiriite-type crystal represented by the chemical formula LiM 1 M 2 X 6 , such as LiCaAlF 6 , containing Na and Ce, for example, the colquiriite-type crystal containing at least one alkali metal element selected from the group consisting of Na, K, Rb and Cs, and a lanthanoid element selected from the group consisting of Ce, Pr and Nd, and having an isotopic ratio of 6 Li of 20 mol% or more, preferably 50 mol% or more; a scintillator for neutron detection comprising the colquiriite-type crystal; and a neutron detector.
摘要翻译： [待解决的问题]优选用于中子检测的闪烁体的colquiriite型晶体，其对中子具有高灵敏度，并且由于³射线而降低背景噪声; 包含该晶体的中子检测用闪烁体; 并提供中子探测器。解决问题的方法由含有Na和Ce的LiCaAlF 6等化学式LiM 1 M 2 X 6表示的扁桃体型晶体，例如含有至少一种选自碱金属元素的扁桃体型晶体来自由Na，K，Rb和Cs组成的组和选自Ce，Pr和Nd的镧系元素，同位素比为6Li为20mol％以上，优选为50mol％以上 ; 一种用于中子检测的闪烁体，包括该共挤出型晶体; 和中子探测器。

16. 发明公开

EP2573590A1 NEUTRON BEAM DETECTOR, NEUTRON BEAM DETECTION SCINTILLATOR, AND METHOD FOR DISCRIMINATION BETWEEN NEUTRON BEAM AND BEAM 审中-公开
标题翻译：中子束检测器，用于中子之间的射线和γ射线的区别闪烁体中子束检测和方法
公开(公告)号：EP2573590A1
公开(公告)日：2013-03-27
申请号：EP11783585.0
申请日：2011-05-18
申请人： Tokuyama Corporation , National University Corporation Nagoya University , Tohoku University
发明人： WATANABE, Kenichi , YAMAZAKI, Atsushi , URITANI, Akira , KONDO, Yoshiyuki , KAWAGUCHI, Noriaki , FUKUDA, Kentaro , SUYAMA, Toshihisa , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , IGUCHI, Tetsuo
IPC分类号： G01T3/06 , C09K11/00 , C09K11/64 , G01T1/17 , G01T3/00
CPC分类号： G01T3/06 , C09K11/7734 , C30B15/00 , C30B29/12
摘要： Disclosed are: a neutron beam detector which comprises a material having low deliquescent properties and can discriminate between a neutron beam and a γ beam; a neutron beam detection scintillator; and a method for discriminating between a neutron beam and a γ beam. Specifically disclosed are: a neutron beam detection scintillator for use in the discrimination between a neutron beam and a γ beam based on the difference in waveforms of light detection signals, and which comprises Ce-containing LiCaAlF6 single crystals; a neutron beam detector which has a function of discriminating between a neutron beam and a γ beam based on the difference in waveforms of light detection signals from a neutron beam detection scintillator, and which is characterized by using a neutron beam detection scintillator comprising Ce-containing LiCaAlF6 single crystals as a neutron beam detection scintillator; and a method for discriminating between a neutron beam and a γ beam.
摘要翻译：公开的是：中子束检测器，其包括具有低潮解性质并且可以中子束和光束³区分的材料; 中子束检测闪烁体; 和中子束和光束³区分的方法。具体地说游离缺失盘是：用于在中子束和基于在光检测信号的波形的差的光束³之间的区分使用中子束检测闪烁体，并且其包含含Ce的LiCaAlF6单晶; 它是通过使用中子束检测闪烁体包括为特征的中子束检测器，它具有一个中子束并且基于来自中子束检测闪烁体中的光检测信号的波形的差的³光束之间进行鉴别的功能，并且所有含Ce LiCaAlF6晶体作为单个中子束检测闪烁体; 和中子束和光束³区分的方法。

17. 发明授权

EP2636646B1 METAL FLUORIDE EUTECTIC, SCINTILLATOR FOR NEUTRONS, AND NEUTRON IMAGING DEVICE 有权
标题翻译：共晶金属氟化物BODY NEUTRONENSZINTILLATOR和中子成像装置
公开(公告)号：EP2636646B1
公开(公告)日：2017-04-12
申请号：EP11838045.0
申请日：2011-11-01
申请人： Tokuyama Corporation , Tohoku University
发明人： FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： C01F17/00 , C01D3/02 , C01F11/22 , C09K11/00 , C09K11/61 , G01T3/06 , G21K4/00 , C30B29/12 , C01D15/04 , C30B21/00 , C09K11/77
CPC分类号： C09K11/616 , C09K11/772 , C30B21/00 , C30B29/12 , G01T3/06 , G21K4/00 , G21K2004/06

18. 发明授权

EP2636772B1 COLQUIRIITE-TYPE CRYSTAL, SCINTILLATOR FOR NEUTRON DETECTION, AND NEUTRON RADIATION DETECTOR 有权
标题翻译： Colquiriite水晶，闪烁的中子检测和中子辐射探测器
公开(公告)号：EP2636772B1
公开(公告)日：2017-02-01
申请号：EP11838031.0
申请日：2011-11-01
申请人： Tokuyama Corporation , Tohoku University
发明人： ISHIZU, Sumito , FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： C30B29/12 , C09K11/00 , C09K11/64 , G01T3/06 , C09K11/77 , C30B15/00 , C30B15/08
CPC分类号： G01T3/06 , C09K11/7721 , C30B15/00 , C30B15/08 , C30B29/12

19. 发明公开

EP2685286A1 NEUTRON BEAM DETECTION DEVICE 审中-公开
标题翻译：中子束检测装置
公开(公告)号：EP2685286A1
公开(公告)日：2014-01-15
申请号：EP12754361.9
申请日：2012-03-08
申请人： Tokuyama Corporation , Tohoku University
发明人： KAWAGUCHI, Noriaki , FUKUDA, Kentaro , SUYAMA, Toshihisa , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： G01T3/06
CPC分类号： G01T3/06 , C09K11/7733 , C09K11/7734 , C30B15/00 , C30B29/12 , G21K4/00
摘要： The present invention is a neutron detection device comprising a neutron detection scintillator composed of a colquiriite-type fluoride single crystal, and a silicon photodiode, characterized in that the single crystal contains only Eu as a lanthanoid and contains 0.80 atom/nm 3 or more of 6 Li, the content of Eu is 0.0025 to 0.05 mol%, and the thickness of the scintillator exceeds 1 mm. The present invention provides a neutron detection device which has a sufficiently high neutron detection efficiency, is equipped with a neutron detection unit minimally affected by gamma rays, and is compact as a whole and lightweight.
摘要翻译：本发明是一种中子检测装置，其特征在于，包含由铬绿石型氟化物单晶构成的中子检测闪烁体和硅光电二极管，其特征在于，所述单晶仅含有作为镧系元素的Eu，且含有0.80原子/ nm 3以上的6Li ，Eu的含量为0.0025〜0.05摩尔％，闪烁体的厚度超过1mm。本发明提供一种中子检测装置，该中子检测装置具有足够高的中子检测效率，装备有受γ射线影响最小的中子检测单元，并且整体上紧凑并且重量轻。

20. 发明公开

EP2636773A1 METAL FLUORIDE CRYSTAL, AND LIGHT-EMITTING ELEMENT 审中-公开
标题翻译： METALLFLUORIDKRISTALL UND LICHTEMITTIERENDES ELEMENT
公开(公告)号：EP2636773A1
公开(公告)日：2013-09-11
申请号：EP11838032.8
申请日：2011-11-01
申请人： Tokuyama Corporation , Tohoku University
发明人： ISHIZU, Sumito , FUKUDA, Kentaro , KAWAGUCHI, Noriaki , YOSHIKAWA, Akira , YANAGIDA, Takayuki , YOKOTA, Yui , FUJIMOTO, Yutaka
IPC分类号： C30B29/12 , C09K11/00 , C09K11/64 , H01J47/12 , G01T3/06
CPC分类号： C09K11/7733 , C09K11/7734 , C30B11/00 , C30B15/00 , C30B15/08 , C30B29/12 , G01T3/06
摘要： [Problems to be Solved] To provide a neutron scintillator which shows a large amount of luminescence in response to neutrons and which is excellent in neutron detection efficiency and n/γ discrimination ability; and a metal fluoride crystal suitable for the neutron scintillator.
[Means to Solve the Problems] A metal fluoride crystal, as a parent crystal, represented by the chemical formula LiM 1 M 2 F 6 (where M 1 represents at least one alkaline earth metal element selected from the group consisting of Mg, Ca, Sr and Ba, and M 2 represents at least one metal element selected from the group consisting of Al, Ga and Sc), such as lithium calcium aluminum fluoride, lithium strontium aluminum fluoride, or lithium magnesium aluminum fluoride, the metal fluoride crystal containing at least one alkali metal element selected from the group consisting of Na, K, Rb and Cs, and also containing Eu; and a light-emitting device comprising the crystal, such as a neutron scintillator.
摘要翻译： [待解决的问题]提供响应中子显示大量发光并且中子检测效率和n /³辨别能力优异的中子闪烁体; 和适用于中子闪烁体的金属氟化物晶体。解决问题的方法以化学式LiM 1 M 2 F 6表示的母体晶体的金属氟化物晶体（其中M 1表示选自Mg，Ca， Sr和Ba，M 2表示选自Al，Ga和Sc中的至少一种金属元素，例如氟化锂钙铝，氟化锂铝锂或氟化锂铝镁，所述金属氟化物晶体含有选自Na，K，Rb和Cs中的至少一种碱金属元素，并且还含有Eu; 以及包括晶体的发光器件，例如中子闪烁体。

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