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1. 发明专利

JP2014087794A Method for producing carbon catalyst 有权
标题翻译：生产碳催化剂的方法
公开(公告)号：JP2014087794A
公开(公告)日：2014-05-15
申请号：JP2013244139
申请日：2013-11-26
申请人： Seizo Miyata , 清蔵宮田 , Masaharu Oshima , 正治尾嶋 , Gunma Univ , 国立大学法人群馬大学 , Nisshinbo Holdings Inc , 日清紡ホールディングス株式会社
发明人： MIYATA SEIZO , OSHIMA MASAHARU , OZAKI JUNICHI , SAITO KAZUO , MORIYA AKINORI , IIDA KYOSUKE , KISHIMOTO TAKEAKI
IPC分类号： B01J37/08 , B01J27/24 , B01J37/04 , H01M4/88 , H01M4/90 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a method for producing a carbon catalyst achieving a catalyst having sufficiently high catalytic activity and having high performance.SOLUTION: A carbon catalyst is produced through: a step of preparing a carbon precursor polymer using a polyacrylonitrile-polymethacrylic acid copolymer; a step of mixing the carbon precursor polymer with at least one kind of transition metal selected from cobalt (Co), iron (Fe) and nickel (Ni) or a compound of the transition metal(s) and nitrogen atoms as constituting elements; and a step of carbonizing the mixture of the carbon precursor compound, the transition metal(s) or the compound of the transition metal(s) and the carbon precursor polymer.
摘要翻译：要解决的问题：提供一种制备具有足够高催化活性和高性能的催化剂的碳催化剂的方法。解决方案：通过以下步骤制备碳催化剂：使用聚丙烯腈 - 聚甲基丙烯酸制备碳前体聚合物的步骤共聚物; 将碳前体聚合物与选自钴（Co），铁（Fe）和镍（Ni）或过渡金属的化合物和氮原子的至少一种过渡金属作为构成元素混合的步骤; 以及将碳前体化合物，过渡金属或过渡金属的化合物与碳前体聚合物的混合物碳化的步骤。

2. 发明专利

JP2012101155A Carbon catalyst and process for production thereof, and electrode and battery using the same 有权
标题翻译：碳催化剂及其生产方法，使用它的电极和电池
公开(公告)号：JP2012101155A
公开(公告)日：2012-05-31
申请号：JP2010250270
申请日：2010-11-08
申请人： Gunma Univ , Nisshinbo Holdings Inc , 国立大学法人群馬大学 , 日清紡ホールディングス株式会社
发明人： KISHIMOTO TAKEAKI , MIZUJIRI MAYUMI , OZAKI JUNICHI , SUDO YUSUKE , KAMINARI NAOKATSU
IPC分类号： B01J23/745 , B01J23/75 , H01M4/88 , H01M4/90 , H01M8/10
CPC分类号： H01M4/9041 , H01M4/96 , H01M2008/1095 , Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a carbon catalyst having an improved catalytic activity, a process for producing the carbon catalyst, and an electrode and a battery using the same.SOLUTION: The carbon catalyst is produced by carbonizing a raw material comprising an organic material containing a nitrogen atom and a metal, wherein iron and/or cobalt and copper are contained as the metal. The carbon catalyst has a crystallinity degree of 41.0% or less as determined by an X-ray diffraction method, a (nitrogen atom)/(carbon atom) ratio of 0.7 or more as determined by an X-ray photoelectron spectroscopy, and oxygen reduction onset potential of 0.774 V (vs. NHE) or more.
摘要翻译：要解决的问题：提供具有改善的催化活性的碳催化剂，制备碳催化剂的方法，以及使用其的电极和电池。解决方案：碳催化剂是通过碳化包含含有氮原子的有机材料和金属的金属制成的，其中包含铁和/或钴和铜作为金属。通过X射线衍射法测定的结晶度为41.0％以下，通过X射线光电子能谱测定的（氮原子）/（碳原子数）比为0.7以上，氧还原起始电位为0.774V（vs.NHE）以上。版权所有（C）2012，JPO＆INPIT

3. 发明专利

JP2011213586A Carbon material and method for producing the same 审中-公开
标题翻译：碳材料及其制造方法
公开(公告)号：JP2011213586A
公开(公告)日：2011-10-27
申请号：JP2011058865
申请日：2011-03-17
申请人： Gunma Univ , Nisshinbo Holdings Inc , Teijin Ltd , Tokyo Institute Of Technology , 国立大学法人東京工業大学 , 国立大学法人群馬大学 , 帝人株式会社 , 日清紡ホールディングス株式会社
发明人： KUWABARA HIROAKI , JOKAI MASAYUKI , MATSUBAYASHI KATSUYUKI , SHINODA TAKESHI , HAYAKAWA TERUAKI , NANBAE HIROTA , KUROKI SHIGEKI , KAKIMOTO MASAAKI , OZAKI JUNICHI , MIYATA SEIZO
IPC分类号： C01B31/02 , B01J27/24 , H01M4/88 , H01M4/90
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a carbon material not containing noble metal such as expensive platinum or platinum alloy and not containing the alloy of the noble metal and suitable for an electrode catalyst for a fuel cell and the like.SOLUTION: The carbon material is obtained by firing a polymer composition composed of: 100 pts.mass of an acrylonitrile-vinyl based boric acid monomer copolymer having an acrylonitrile component of ≥50 mol% and a vinyl based boric acid monomer component of ≥1 mol%; and 1 to 150 pts.mass of specific metal phthalocyanine containing metal ions selected from a group consisting of Fe, Co, Cuand Niat 500 to 1,500°C in an inert gas atmosphere.
摘要翻译：要解决的问题：提供不含贵金属的贵金属如不贵贵的铂或铂合金的碳材料，不含贵金属的合金，适用于燃料电池用电极催化剂等。解决方案：碳材料为通过焙烧由丙烯腈组分≥50摩尔％的丙烯腈 - 乙烯基系硼酸单体共聚物和乙烯基系硼酸单体成分≥1摩尔％组成的聚合物组合物得到的聚合物组合物; 以及在惰性气体气氛中，选自Fe，Co，Cu和Niat的500至1500℃的含有金属酞菁的1至150磅的金属酞菁。

4. 发明专利

JP2013113620A Reaction vessel for raman spectrophotometry and raman spectrophotometry method using the same 有权
标题翻译：用于拉曼光谱测定的反应容器和使用其的拉曼光谱测定方法
公开(公告)号：JP2013113620A
公开(公告)日：2013-06-10
申请号：JP2011257849
申请日：2011-11-25
申请人： Gunma Univ , 国立大学法人群馬大学 , Nisshinbo Holdings Inc , 日清紡ホールディングス株式会社
发明人： OZAKI JUNICHI , KANNARI NAOKATSU , HORIKAWA YUTA , KOBAYASHI RIEKO , SAITO NAOTO
IPC分类号： G01N21/65
CPC分类号： G01N21/75 , G01N21/03 , G01N21/09 , G01N21/65 , G01N2021/0325 , G01N2021/651
摘要： PROBLEM TO BE SOLVED: To provide a reaction vessel for Raman spectrophotometry suitable for observing electrochemical reactions on a solid surface in an electrolyte solution, and to provide a Raman spectrophotometry method using the reaction vessel.SOLUTION: The reaction vessel for Raman spectrophotometry includes: a housing part (10) which has a transparent window part (11), and in which a hollow part (12) for accommodating an electrolyte solution is formed; and a working electrode part (20) which is composed of a conductive material electrochemically inactive in the electrolyte solution, which is arranged in the hollow part, facing the window part, so that one part (21) of the working electrode part (20) holds a sample, and which is extended up to the outside of the housing part so that another part (22) of the working electrode part (20) is connected to an external power source.
摘要翻译：要解决的问题：提供一种适用于在电解质溶液的固体表面上观察电化学反应的拉曼分光光度法反应容器，并提供使用反应容器的拉曼分光光度法。解决方案：用于拉曼分光光度法的反应容器包括：具有透明窗部分（11）的壳体部分（10），其中形成用于容纳电解质溶液的中空部分（12）; 以及工作电极部（20），其由配置在所述中空部的电解液中的电化学惰性的导电性材料构成，与所述窗部相对，使得所述工作电极部（20）的一部分（21）保持样品，并且延伸到壳体部分的外部，使得工作电极部分（20）的另一部分（22）连接到外部电源。版权所有（C）2013，JPO＆INPIT

5. 发明专利

JP2011230099A Carbon catalyst and method of manufacturing the same 审中-公开
标题翻译：碳催化剂及其制备方法
公开(公告)号：JP2011230099A
公开(公告)日：2011-11-17
申请号：JP2010105491
申请日：2010-04-30
申请人： Gunma Univ , Nisshinbo Holdings Inc , Teijin Ltd , Tokyo Institute Of Technology , 国立大学法人東京工業大学 , 国立大学法人群馬大学 , 帝人株式会社 , 日清紡ホールディングス株式会社
发明人： JOKAI MASAYUKI , KIDO NOBUAKI , MORIYA AKINORI , MATSUBAYASHI KATSUYUKI , SHINODA TAKESHI , WU LIBIN , KIN ZAIKO , HAYAKAWA TERUAKI , NANBAE HIROTA , KUROKI SHIGEKI , KAKIMOTO MASAAKI , OZAKI JUNICHI , MIYATA SEIZO
IPC分类号： B01J23/745 , B01J35/10 , B01J37/08 , H01M4/88 , H01M4/90 , H01M4/96 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a carbon catalyst having high oxygen reduction capability without including noble metal such as expensive platinum or platinum alloy and suitable for an electrode catalyst for fuel cell or the like.SOLUTION: The carbon catalyst includes at least carbon, nitrogen, and hydrogen as constituent elements. The presence rate of carbon in the carbon catalyst is 80 mass% or more. The element ratio of hydrogen to carbon is 0.04 to 0.28. The element ratio of nitrogen to carbon is 0.005 to 0.06.
摘要翻译：要解决的问题：提供具有高氧还原能力的碳催化剂，而不包括昂贵的铂或铂合金等贵金属，适用于燃料电池等的电极催化剂。解决方案：碳催化剂至少包括碳，氮和氢作为组成元素。碳催化剂中碳的存在率为80质量％以上。氢与碳的元素比为0.04〜0.28。氮与碳的元素比为0.005〜0.06。版权所有（C）2012，JPO＆INPIT

6. 发明专利

JP2011115760A Carrier for supporting catalyst, catalyst carrier, electrode, and battery 有权
标题翻译：载体，用于支持催化剂，催化剂载体，电极和电池
公开(公告)号：JP2011115760A
公开(公告)日：2011-06-16
申请号：JP2009277825
申请日：2009-12-07
申请人： Gunma Univ , Nisshinbo Holdings Inc , 国立大学法人群馬大学 , 日清紡ホールディングス株式会社
发明人： KAKIMOTO ERINA , KISHIMOTO TAKEAKI , OZAKI JUNICHI
IPC分类号： B01J33/00 , B01J23/40 , H01M4/88 , H01M4/92 , H01M4/96 , H01M8/10
CPC分类号： H01M4/9083 , B82Y30/00 , C01B32/20 , H01M4/663 , H01M4/9008 , H01M4/926 , Y10T428/2982
摘要： PROBLEM TO BE SOLVED: To provide a carrier for supporting a catalyst, which can attain both of a durability and a facility of supporting the catalyst (catalyst support performance) at a high level. SOLUTION: The carrier for supporting the catalyst is obtained by carbonating a raw material containing a nitrogen-containing organic substance and a metal. In the carrier for supporting the catalyst, a peak in the vicinity of a diffraction angle 26° in an X-ray diffraction diagram may contain 20-45% structural components similar to black lead and 55-80% amorphous components. Further, in the carrier for supporting the catalyst, the intensity ratio (I 1,360 /I 1,580 ) of 1,360 cm -1 band in Raman spectrum to 1,580 cm -1 band may be ≥0.3 and ≤1.0 also. Furthermore, the carrier for supporting the catalyst can be also obtained by applying a metal removing treatment to the carbonated material obtained by the carbonation of the raw material, and further, applying a heat treatment. In this case, the metal may be a transition metal. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种用于支撑催化剂的载体，其能够以高水平实现催化剂（催化剂支撑性能）的耐久性和设备的两者。解决方案：用于负载催化剂的载体是通过对包含含氮有机物质和金属的原料进行碳酸化而获得的。在用于负载催化剂的载体中，X射线衍射图中衍射角26°附近的峰可以含有类似于黑铅和55-80％无定形组分的20-45％的结构组分。此外，在用于负载催化剂的载体中，拉曼光谱中的强度比（I 1,360 / I 1,580 ）为1360cm -1 SP波段到1,580厘米 -1 带也可以≥0.3和≤1.0。此外，用于负载催化剂的载体也可以通过对通过原料碳酸化获得的碳酸化材料进行金属去除处理，并进一步进行热处理来获得。在这种情况下，金属可以是过渡金属。版权所有（C）2011，JPO＆INPIT

7. 发明专利

JP2010184906A Method for oxidizing aromatic alcohol 审中-公开
标题翻译：氧化芳香醇的方法
公开(公告)号：JP2010184906A
公开(公告)日：2010-08-26
申请号：JP2009031092
申请日：2009-02-13
申请人： Gunma Univ , Nisshinbo Holdings Inc , Tokyo Institute Of Technology , 国立大学法人東京工業大学 , 国立大学法人群馬大学 , 日清紡ホールディングス株式会社
发明人： KAKIMOTO MASAAKI , HAYAKAWA TERUAKI , KUANG YONGBO , MIYATA SEIZO , OZAKI JUNICHI , IIDA KYOSUKE , OSHIMA YASUHIRO
IPC分类号： C07C45/38 , B01J21/18 , B01J27/22 , B01J35/10 , C07B61/00 , C07C45/39 , C07C47/54 , C07C47/546 , C07C47/55 , C07C47/575 , C07C49/76 , C07C49/78 , C07C49/786 , C07C51/235 , C07C63/06 , C07C63/10 , C07C63/36 , C07C65/21 , C07C201/12 , C07C205/44 , C07C205/57
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a method for oxidizing an aromatic alcohol by which an aldehyde or ketone can efficiently be produced without using a metallic oxidizing agent or catalyst. SOLUTION: The method for oxidizing the aromatic alcohol includes oxidizing the aromatic alcohol in the presence of a carbon material having ≥20 m 2 /g specific surface area, an oxygen-containing gas and nitric acid or alkali metal hydroxide. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：待解决的问题：提供氧化可以有效地制备醛或酮的芳族醇的方法，而不使用金属氧化剂或催化剂。解决方案：用于氧化芳族醇的方法包括在具有≥20m2 / SP / g比表面积的碳材料的存在下氧化芳族醇，含氧气体和硝酸或碱金属氢氧化物。版权所有（C）2010，JPO＆INPIT

8. 发明专利

JP2009291714A Catalyst and method for producing the same, membrane electrode assembly and method for producing the same, fuel cell member and method for producing the same, fuel cell and electric storage apparatus 有权
标题翻译：催化剂及其制造方法，膜电极组件及其制造方法，燃料电池组件及其制造方法，燃料电池及蓄电装置
公开(公告)号：JP2009291714A
公开(公告)日：2009-12-17
申请号：JP2008148387
申请日：2008-06-05
申请人： Gunma Univ , Seizo Miyata , Nisshinbo Holdings Inc , 国立大学法人群馬大学 , 清蔵宮田 , 日清紡ホールディングス株式会社
发明人： MIYATA SEIZO , OZAKI JUNICHI , SAITO KAZUO , MORIYA AKINORI , IIDA KYOSUKE , KISHIMOTO TAKEAKI
IPC分类号： B01J23/75 , B01J37/08 , H01M4/86 , H01M4/88 , H01M4/90 , H01M4/96 , H01M8/02 , H01M8/10
CPC分类号： H01M4/923 , H01M4/8807 , H01M4/8882 , H01M4/9008 , H01M4/96 , H01M2008/1095
摘要： PROBLEM TO BE SOLVED: To provide a catalyst constituted so that the catalyst is integrated with another member to be combined with the catalyst to reduce the number of components and decrease the contact resistance between them. SOLUTION: The catalyst is obtained by arranging an electrically conductive area in at least a part of a substrate 3 and forming a carbon catalyst 2 in the electrically conductive area. A carbon precursor polymer is stuck to the substrate, which is then carbonized to form the catalyst. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：提供一种催化剂，其构成为使催化剂与另一种与催化剂组合的构件一体化，以减少组分的数量并降低它们之间的接触电阻。解决方案：通过在导电区域中在衬底3的至少一部分中布置导电区域并形成碳催化剂2而获得催化剂。将碳前体聚合物粘附到基底上，然后将其碳化以形成催化剂。版权所有（C）2010，JPO＆INPIT

9. 发明专利

JP2009291707A Carbon catalyst, method for manufacturing the same, fuel cell, electric storage apparatus and method for using the catalyst 审中-公开
标题翻译：碳催化剂，其制造方法，燃料电池，电储存装置和使用催化剂的方法
公开(公告)号：JP2009291707A
公开(公告)日：2009-12-17
申请号：JP2008147402
申请日：2008-06-04
申请人： Gunma Univ , Seizo Miyata , Nisshinbo Holdings Inc , 国立大学法人群馬大学 , 清蔵宮田 , 日清紡ホールディングス株式会社
发明人： MIYATA SEIZO , OZAKI JUNICHI , SAITO KAZUO , MORIYA AKINORI , IIDA KYOSUKE , KISHIMOTO TAKEAKI
IPC分类号： B01J21/18 , B01J37/04 , B01J37/08 , C01B31/02 , H01M4/90 , H01M8/10
CPC分类号： H01M4/96 , C01B32/05 , H01M4/90 , H01M4/9083 , H01M8/1007 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a carbon catalyst having sufficiently high catalytic activity and high performance. SOLUTION: This invention relates to the carbon catalyst which contains oxygen, wherein the content of oxygen atoms on the surface has 0.02-0.4 atomic ratio to carbon atoms on the surface. COPYRIGHT: (C)2010,JPO&INPIT

10. 发明专利

JP2012115725A Carbon catalyst for hydrogen production, method for producing the same, and method for producing hydrogen using the same 有权
标题翻译：用于生产氢的碳催化剂，其生产方法和使用该方法生产氢的方法
公开(公告)号：JP2012115725A
公开(公告)日：2012-06-21
申请号：JP2010265334
申请日：2010-11-29
申请人： Gunma Univ , Nisshinbo Holdings Inc , 国立大学法人群馬大学 , 日清紡ホールディングス株式会社
发明人： OZAKI JUNICHI , KOBAYASHI RIEKO , FUJII CHIHIRO
IPC分类号： B01J23/745 , B01J21/18 , B01J23/34 , B01J23/75 , B01J23/755 , C01B3/26
CPC分类号： B01J23/755 , B01J21/18 , B01J23/02 , B01J23/34 , B01J23/74 , B01J23/745 , B01J23/75 , B01J23/78 , B01J37/06 , B01J37/084 , C01B3/22 , C01B3/26 , C01B2203/0277 , C01B2203/1041 , C01B2203/1211 , C01B2203/1217 , C01B2203/1223 , C01B2203/1229 , C01B2203/1235 , C01B2203/1241 , C01B2203/1247 , C01B2203/1252
摘要： PROBLEM TO BE SOLVED: To provide a carbon catalyst for hydrogen production which shows high catalytic activity, a method for producing the catalyst, and a method for producing hydrogen using the catalyst.SOLUTION: This carbon catalyst for hydrogen production is a carbon catalyst obtained by carbonization of a material containing an organic substance and a transition metal, and is used for hydrogen production by pyrolysis of a hydrocarbon compound and/or an oxygen-containing organic compound. Further, the carbon catalyst for hydrogen production may be obtained by allowing a carbonized material produced by the carbonization to support an alkaline earth metal.

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