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41. 发明申请

US20110201769A1 Copolymers Of Ethylene And At Least One Other 1-Olefin, And Process For Their Preparation 审中-公开
标题翻译：乙烯和至少一种其他1-烯烃的共聚物及其制备方法
公开(公告)号：US20110201769A1
公开(公告)日：2011-08-18
申请号：US12223233
申请日：2007-01-24
申请人： Chistoph Kiener , Rainer Karer , Jens Wiesecke , Gerhardus Meier
发明人： Chistoph Kiener , Rainer Karer , Jens Wiesecke , Gerhardus Meier
IPC分类号： C08F210/16
CPC分类号： C08F210/16 , C08F4/24 , C08F2/34 , C08F210/14 , C08F2500/12 , C08F2500/17 , C08F2500/04 , C08F2500/07 , C08F2500/11 , C08F2500/13
摘要： Ethylene copolymers composed of ethylene units and units composed of at least one other 1-olefin whose density is from 0.940 to 0.955 g/cm3, whose vinyl end group content is at least 0.5 end groups, based on 1000 carbon atoms, whose tensile impact strength atn, measured to ISO 8256 (1997)/1A at −30° C., is greater than or equal to 145 kJ/m2, and whose content of comonomer side chains per 1000 carbon atoms Cx is above a value defined via equation I, Cx=128.7−134.62 d′ (I), where d′ is the density d of the copolymer in g/cm3, and a process for their preparation, and their use as blow-molded products.
摘要翻译：由乙烯单元构成的乙烯共聚物和由密度为0.940〜0.955g / cm 3的至少一种其它1-烯烃组成的单元，其乙烯基端基含量为至少0.5个端基，基于1000个碳原子，其拉伸冲击强度 atn根据ISO 8256（1997）/ 1A在-30℃测量，大于或等于145kJ / m 2，并且其每1000个碳原子C x的共聚单体侧链含量高于通过式I定义的值， Cx = 128.7-134.62d'（I），其中d'是共聚物的密度d，单位为g / cm 3，及其制备方法及其作为吹塑制品的用途。

42. 发明申请

US20100317755A1 Process For Preparation Of Ethylene Polymers For Blown Films 失效
标题翻译：乙烯聚合物制备吹塑膜的工艺
公开(公告)号：US20100317755A1
公开(公告)日：2010-12-16
申请号：US12223234
申请日：2007-01-24
申请人： Wolfgang Rohde , Lutz-Gerd Heinicke , Rainer Karer , Manfred Hecker
发明人： Wolfgang Rohde , Lutz-Gerd Heinicke , Rainer Karer , Manfred Hecker
IPC分类号： C08J9/00 , C08F10/02
CPC分类号： C08F10/02 , C08F10/00 , C08F110/02 , C08J5/18 , C08J2323/08 , C08K5/005 , C08F4/025 , C08F4/24 , C08F2/34 , C08L23/04 , C08F2500/12 , C08F2500/04 , C08F2500/26 , C08F2500/17
摘要： Process for preparation of ethylene homopolymers or copolymers, comprising the steps of a) polymerization of ethylene or of ethylene with one or more other 1-olefins in the presence of a chromium catalyst at temperatures of from 20 to 200° C. and at pressures of from 0.1 to 20 MPa, where the chromium catalyst can be prepared via application of one or more chromium compounds to a silicate support and subsequent thermal activation under oxidative conditions at temperatures of from 620 to 900° C.; b) mixing of the polyethylene in the melt in the presence of from 1000 to 2000 ppm of an antioxidant comprising at least one sterically hindered phenol and comprising at least one phosphite in a mixing ratio of from 1:5 to 5:1, with specific energy input of at least 0.17 kWh/kg.
摘要翻译：乙烯均聚物或共聚物的制备方法，包括以下步骤：a）在铬催化剂存在下，在20〜200℃的温度下，在乙烯或乙烯与一种或多种其它1-烯烃的存在下，在 0.1至20MPa，其中可通过将一种或多种铬化合物施用于硅酸盐载体并随后在620-900℃的氧化条件下进行热活化来制备铬催化剂; b）在1000-2000ppm的包含至少一种空间位阻酚并且包含至少一种1:5至5:1的混合比的亚磷酸酯的抗氧化剂存在下，将聚乙烯混合在熔体中，能量输入至少为0.17 kWh / kg。

43. 发明申请

US20090311453A1 Molding compostion comprsing polyethlene for preparing films and process for preparing the molding composition in the presence of a mixed catalyst 审中-公开
标题翻译：用于制备膜的聚乙烯的成型组合物和在混合催化剂存在下制备模塑组合物的方法
公开(公告)号：US20090311453A1
公开(公告)日：2009-12-17
申请号：US11919166
申请日：2006-04-15
申请人： Shahram Mihan , Dieter Lilge , Heinz Vogt , Jennifer Kipke , Rainer Karer
发明人： Shahram Mihan , Dieter Lilge , Heinz Vogt , Jennifer Kipke , Rainer Karer
IPC分类号： B32B1/02 , C08F110/02 , C08L23/06 , C08F2/00 , C07F17/00 , B01J31/12 , B29C47/00
CPC分类号： C08J5/18 , C08F4/65912 , C08F4/65925 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , C08J2323/08 , C08L23/06 , C08L23/0815 , C08L2205/02 , C08L2314/04 , C08L2314/06 , Y02P20/52 , Y10T428/1352 , C08F4/69 , C08F4/025 , C08F4/65916 , C08L2666/06 , C08F2500/17 , C08F2500/12 , C08F2500/04 , C08F2500/26 , C08F2500/09 , C08F2500/18 , C08F210/14 , C08F4/6292 , C08F4/63904
摘要： Molding composition comprising polyethylene and having a density in the range from 0.915 to 0.955 g/cm, an MI in the range from 0 to 3.5 g/10 min, an MFR in the range from 5 to 50, a polydispersity Mw/Mn in the range from 5 to 20, and a z-average moiar mass Mz of less than 1 million g/mol, a process for preparing such a composition, a catalyst suitable for the preparation of the same, as well as films comprising this molding composition.
摘要翻译：包含聚乙烯并且密度在0.915至0.955g / cm 3，MI在0至3.5g / 10min范围内的MFR，5至50范围内的MFR，5分钟内的多分散性Mw / Mn 范围为5至20，z平均摩尔质量Mz小于100万g / mol，制备这种组合物的方法，适用于其制备的催化剂以及包含该模塑组合物的薄膜。

44. 发明申请

US20080299342A1 Catalyst Comprising Chromium and Zinc for Olefin Polymerization and Process for Preparing It 审中-公开
标题翻译：包含铬和锌用于烯烃聚合的催化剂及其制备方法
公开(公告)号：US20080299342A1
公开(公告)日：2008-12-04
申请号：US11628682
申请日：2005-06-09
申请人： Martin Schneider , Jan Gohre , Rainer Karer , Wolfgang Rohde , Anke Bold , Martin Lux , Ernst Fischer , Christoph Kiener
发明人： Martin Schneider , Jan Gohre , Rainer Karer , Wolfgang Rohde , Anke Bold , Martin Lux , Ernst Fischer , Christoph Kiener
IPC分类号： B32B1/08 , B01J23/06 , B01J23/26 , C08F4/44
CPC分类号： B01J23/26 , C08F10/00 , C08F110/02 , C08F210/16 , C08F2410/01 , C08F2410/02 , Y10T428/139 , C08F4/10 , C08F4/24 , C08F4/22 , C08F4/025 , C08F2500/12 , C08F2500/24 , C08F2500/13 , C08F2500/04 , C08F210/14 , C08F2500/18
摘要： Catalyst for the polymerization and/or copolymerization of olefins which has a chromium content of from 0.01 to 5% by weight, based on the element in the finished catalyst, is supported on a finely divided inorganic support and is obtainable by concluding calcination at temperatures of from 350 to 1050° C. and has a zinc content of from 0.01 to 10% by weight, based on the element in the finished catalyst.
摘要翻译：用于烯烃的聚合和/或共聚的催化剂负载在精细分散的无机载体上，铬含量为0.01-5重量％，基于成品催化剂中的元素，可通过在基于成品催化剂中的元素，其含量为350〜1050℃，锌含量为0.01〜10重量％。

45. 发明申请

US20080177012A1 Process and Apparatus For the Polymerization of Ethylene 有权
标题翻译：用于聚合乙烯的方法和装置
公开(公告)号：US20080177012A1
公开(公告)日：2008-07-24
申请号：US11883713
申请日：2006-01-30
申请人： Giuseppe Penzo , Cyrus Ahmadzade-Youssefi , Rainer Karer , Ulrich Nieken
发明人： Giuseppe Penzo , Cyrus Ahmadzade-Youssefi , Rainer Karer , Ulrich Nieken
IPC分类号： C08F2/34 , B01J8/00
CPC分类号： C08F10/02 , B01J8/0035 , B01J8/006 , B01J8/24 , B01J2208/00274 , B01J2208/00761 , B01J2219/00006 , C08F6/005 , C08F10/00 , C08F110/02 , C08F210/16 , Y02P20/582 , Y10S526/92 , C08L23/06 , C08L23/0815 , C08F4/69 , C08F2/34 , C08F2/01 , C08F210/08 , C08F210/14
摘要： Process for the polymerization of ethylene or of ethylene with further 1-olefins, in which the ethylene is polymerized in the presence of a catalyst in a gas-phase reactor and reaction gas comprising propane and unpolymerized ethylene is circulated to remove the heat of polymerization, wherein the polymer particles are discharged continuously or discontinuously from the reactor, the polymer particles are separated from the major part of the concomitantly discharged gas and the polymer particles are degassed, the gas is freed of entrained fine particles and is separated from a low-boiling fraction comprising ethylene or from a high boiling fraction containing further 1-olefins or alkanes having from 4 to 12 carbon atoms in a first separation stage, a propane fraction is separated off in a second separation stage and this propane fraction is used for degassing the polymer particles discharged from the reactor, with the proportion of ethylene in the propane fraction being less than 1 mol % and the proportion of 1-olefins and alkanes having from 4 to 12 carbon atoms in the propane fraction being less than 4 mol %, in each case based on the total propane fraction. Furthermore, an apparatus for carrying out the process. In this way, a high heat discharge from the reactor, satisfactory degassing of the discharged polymer particles and recovery of the reaction gas discharged together with the polymer particles and also the gas used for degassing the polymer particles are made possible.
摘要翻译：乙烯或乙烯与进一步的1-烯烃聚合的方法，其中乙烯在催化剂存在下在气相反应器和包含丙烷和未聚合乙烯的反应气体中聚合循环以除去聚合热，其中聚合物颗粒从反应器中连续或不连续地排出，聚合物颗粒与伴随排出气体的主要部分分离，聚合物颗粒脱气，气体不含夹带的细颗粒，并从低沸点在第一分离阶段，包含乙烯或含有另外的具有4至12个碳原子的1-烯烃或烷烃的高沸点馏分的馏分在第二分离阶段分离出丙烷馏分，该丙烷馏分用于使聚合物脱气从反应器排出的颗粒，丙烷馏分中乙烯的比例小于1mol ％，丙烷馏分中具有4至12个碳原子的1-烯烃和烷烃的比例小于4mol％，基于总丙烷馏分。此外，一种用于执行该过程的装置。以这种方式，可以从反应器的高热放电，排出的聚合物颗粒的令人满意的脱气和与聚合物颗粒一起排放的反应气体的回收以及用于使聚合物颗粒脱气的气体成为可能。

46. 发明申请

US20080014128A1 Apparatus and Process for the Gas-Phase Polymerization of Olefins 有权
标题翻译：用于烯烃气相聚合的装置和方法
公开(公告)号：US20080014128A1
公开(公告)日：2008-01-17
申请号：US11667417
申请日：2005-11-08
申请人： Eberhard Herrmann , Manfred Hecker , Rainer Karer , Klaus Berhalter , Paulus de Lange , Jorg Halpap , Cyrus Ahmadzade-Youssefi
发明人： Eberhard Herrmann , Manfred Hecker , Rainer Karer , Klaus Berhalter , Paulus de Lange , Jorg Halpap , Cyrus Ahmadzade-Youssefi
IPC分类号： C08F10/00 , B01J19/18
CPC分类号： B01J8/003 , B01J8/006 , B01J8/1872 , B01J2208/00256 , B01J2208/00274 , B01J2208/00761 , C08F10/00 , C08F110/02 , C08F2/34
摘要： Apparatus for the polymerization of olefins, in particular ethylene, comprising a gas-phase fluidized-bed reactor (1), a product offtake line (15) for taking polymer particles either continuously or discontinuously from the reactor (1), which line (15) is connected to a depressurization vessel (2) for separating polymer particles and gas, a recycle gas filter (3) for freeing the gas of entrained fine particles connected to the depressurization vessel (2), a compressor which compresses the gas which has been freed of fine particles and recirculates it into the reactor (1), with the recycle gas filter (3) having an inlet chamber (4) provided with a gas inlet (6), an outlet chamber (5) provided with a gas outlet (7), an essentially vertical sheet-like filter medium (9) for retaining the fine particles which separates the inlet chamber (4) from the outlet chamber (5) and a particle outlet (8). The inlet chamber (4) has a dividing wall (10) which is arranged essentially parallel to the filter medium (9) and separates the inlet chamber (4) into an inflow region (4a), which is connected to the gas inlet (6), and a filter region (4b) in which the filter medium is located and has an upper opening and a lower opening which are dimensioned so that from 60 to 90% of the volume flow flows through the upper opening so that flow along the filter medium (9) from the top downward results.
摘要翻译：用于烯烃聚合的设备，特别是乙烯，包括气相流化床反应器（1），用于从反应器（1）连续或不连续地获取聚合物颗粒的出口管线（15），该管线（15））连接到用于分离聚合物颗粒和气体的减压容器（2），用于释放连接到减压容器（2）的夹带的细颗粒的气体的循环气体过滤器（3），压缩已经被释放细颗粒并将其再循环到反应器（1）中，循环气体过滤器（3）具有设置有气体入口（6）的入口室（4），设置有气体出口的出口室（5） 7），用于保持将入口室（4）与出口室（5）分离的细颗粒和颗粒出口（8）的基本垂直的片状过滤介质（9）。入口室（4）具有基本上与过滤介质（9）平行布置的分隔壁（10），并将入口室（4）分离成入口区域（4a），该入口区域连接到气体入口 6）和过滤器区域（4b），其中过滤介质位于并具有上开口和下开口，其尺寸使得体积流量的60％至90％流过上开口，使得沿着过滤介质（9）从顶部向下的结果。

47. 发明授权

US06730753B2 Catalyst systems of the ziegler-natta type and a process for preparing them 失效
标题翻译：齐格勒 - 纳塔型催化剂系统及其制备方法
公开(公告)号：US06730753B2
公开(公告)日：2004-05-04
申请号：US09940368
申请日：2001-08-28
申请人： Klaus Föttinger , Stephan Hüffer , Rainer Karer
发明人： Klaus Föttinger , Stephan Hüffer , Rainer Karer
IPC分类号： C08F464
CPC分类号： C08F10/00 , C08F110/02 , C08F4/651 , C08F4/6567 , C08F4/6565 , C08F2500/17
摘要： Catalyst systems of the Ziegler-Natta type, which are suitable for the polymerization of olefins are prepared by: A) bringing an inorganic metal oxide on which a magnesium compound has been deposited into contact with a tetravalent titanium compound, B) if desired, bringing the intermediate obtained in this way into contact with an electron donor compound and C) bringing the intermediate obtained in step A) or B) into contact with a polysiloxane.
摘要翻译：适用于烯烃聚合的齐格勒 - 纳塔型催化剂体系是通过以下步骤制备的：A）使其上沉积有镁化合物的无机金属氧化物与四价钛化合物接触，B）如果需要，将以这种方式获得的中间体与电子给体化合物接触，和C）将步骤A）中得到的中间体或B）与聚硅氧烷接触。

48. 发明授权

US09266976B2 Method for activation of chromium containing catalyst precursor for polymerization and the resulting polymerization catalyst 有权
标题翻译：活化用于聚合的含铬催化剂前体的方法和所得的聚合催化剂
公开(公告)号：US09266976B2
公开(公告)日：2016-02-23
申请号：US13990490
申请日：2011-11-29
申请人： Manfred Hecker , Paulus De Lange , Rainer Karer
发明人： Manfred Hecker , Paulus De Lange , Rainer Karer
IPC分类号： C08F4/24 , B01J23/26 , B01J37/14 , B01J38/14 , B01J38/30 , B01J38/32 , C08F10/00
CPC分类号： C08F4/24 , B01J23/26 , B01J37/14 , B01J38/14 , B01J38/30 , B01J38/32 , C08F10/00 , Y02P20/584 , C08F4/69
摘要： The instant invention relates to an activation of a polymerization catalyst precursor by heat treatment comprising a support material and a catalyst precursor deposited thereon in a fluidized bed activator and to the use of the activated polymerization catalyst in the manufacture of polyolefins. The activation involves heat treatment in the presence of oxygen. After that activation the oxygen in the activator is replaced by inert gas via flushing until the fluidization gas emerging from the activator comprises oxygen in a maximum amount of up to 5 ppm. The catalyst prepared by that method is improved with respect to prevent reactor fouling during gas-phase polymerization or slurry polymerization either in stirred vessel or loop.
摘要翻译：本发明涉及通过热处理的聚合催化剂前体的活化，其包括在流化床活化剂中沉积在其上的载体材料和催化剂前体，以及活性聚合催化剂在制备聚烯烃中的用途。活化包括在氧气存在下的热处理。在该活化之后，通过冲洗将活化剂中的氧替代为惰性气体，直到从活化剂出来的流化气体包含最高达5ppm的氧气。通过该方法制备的催化剂相对于在搅拌容器或循环中的气相聚合或淤浆聚合期间防止反应器结垢而改进。

49. 发明授权

US09090762B2 Polyethylene composition suitable for the preparation of films and process for preparing the same 有权
标题翻译：适用于制备薄膜的聚乙烯组合物及其制备方法
公开(公告)号：US09090762B2
公开(公告)日：2015-07-28
申请号：US13301495
申请日：2011-11-21
申请人： Jennifer Kipke , Shahram Mihan , Rainer Karer , Jörg Auffermann , Manfred Hecker , Paulus De Lange , Harald Schmitz
发明人： Jennifer Kipke , Shahram Mihan , Rainer Karer , Jörg Auffermann , Manfred Hecker , Paulus De Lange , Harald Schmitz
IPC分类号： C08L23/04 , C08L23/08 , C08L23/06
CPC分类号： C08L23/04 , C08L23/06 , C08L23/0815 , C08L2205/02 , C08L2205/025 , C08L2205/035 , C08L2308/00 , C08L2314/06 , C08L2666/06 , C08L2666/02
摘要： A polyethylene composition, in particular suitable for the preparation of films, and a process for preparing the same are described. The polyethylene composition of the invention comprises from 50 to 89% by weight of a first polyethylene component comprising at least one multimodal polyethylene including a plurality of ethylene polymer fractions having distinct molecular weights and comonomer contents, at least one of said plurality of ethylene polymer fractions being prepared by the use of a single site catalyst, and from 50 to 11% by weight of a second polyethylene component comprising a low or medium density polyethylene.
摘要翻译：描述了特别适用于制备薄膜的聚乙烯组合物及其制备方法。本发明的聚乙烯组合物包含50至89重量％的第一聚乙烯组分，其包含至少一种多峰聚乙烯，其包含具有不同分子量和共聚单体含量的多种乙烯聚合物级分，所述多种乙烯聚合物级分中的至少一种通过使用单中心催化剂制备，以及50至11重量％的包含低密度或中密度聚乙烯的第二聚乙烯组分。

50. 发明授权

US08722833B2 Multimodal polyethylene composition, mixed catalyst and process for preparing the composition 有权
标题翻译：多峰聚乙烯组合物，混合催化剂及其制备方法
公开(公告)号：US08722833B2
公开(公告)日：2014-05-13
申请号：US12448449
申请日：2007-12-18
申请人： Jennifer Kipke , Shahram Mihan , Rainer Karer , Harald Schmitz
发明人： Jennifer Kipke , Shahram Mihan , Rainer Karer , Harald Schmitz
IPC分类号： C08L23/06 , C08F2/34 , C08F10/02 , C08F210/16 , C08L23/08 , B01J31/12
CPC分类号： B01J31/12 , C08F2/34 , C08F4/65912 , C08F10/00 , C08F10/02 , C08F210/16 , C08F2410/04 , C08J5/18 , C08J2323/04 , C08L23/04 , C08L23/06 , C08L23/0815 , C08L2205/03 , C08L2314/06 , Y02P20/52 , C08F4/65925 , C08F4/65916 , C08L23/00 , C08L2666/06 , C08F210/14 , C08F2500/07 , C08F2500/08 , C08F2500/04 , C08F2500/26 , C08F4/7042 , C08F4/61904
摘要： A multimodal polyethylene composition comprising at least three ethylene polymer fractions having distinct molecular weights or comonomer contents, the at least three ethylene polymer fractions comprising at least one first ethylene polymer fraction having a first molecular weight, at least one second ethylene polymer fraction having a second molecular weight higher than the first molecular weight, and at least one third ethylene polymer fraction having a third molecular weight higher than the first molecular weight, wherein the at least one first ethylene polymer fraction and the at least third ethylene polymer fraction are prepared by the use of a first and, respectively, third catalyst of the single site type.
摘要翻译：包含至少三种具有不同分子量或共聚单体含量的乙烯聚合物级分的多峰聚乙烯组合物，所述至少三种乙烯聚合物级分包含至少一种具有第一分子量的第一乙烯聚合物级分，至少一种具有第二分子量的第二乙烯聚合物级分分子量高于第一分子量，以及至少一种具有高于第一分子量的第三分子量的第三乙烯聚合物级分，其中至少一种第一乙烯聚合物级分和至少三级乙烯聚合物级分是通过使用单一位点型的第一和第三催化剂。

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