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41. 发明授权

US4847000A Process for manufacturing synthesis gas or hydrogen by catalytic conversion of methanol in the liquid phase 失效
标题翻译：通过在液相中甲醇的催化转化来制造合成气或氢气的方法
公开(公告)号：US4847000A
公开(公告)日：1989-07-11
申请号：US156879
申请日：1988-02-18
申请人： Quang Dang Vu , Daniel Durand , Jean-Francois Le Page , Philippe Courty , Alain Forestiere
发明人： Quang Dang Vu , Daniel Durand , Jean-Francois Le Page , Philippe Courty , Alain Forestiere
IPC分类号： C01B3/22 , C01B3/32
CPC分类号： C01B3/22 , C01B3/323 , Y02P20/52
摘要： Process for manufacturing synthesis gas or hydrogen by catalytic conversion of methanol in the liquid phase, comprising simultaneously passing methanol (1), a liquid phase of hydrocarbons (6) and optionally water on the catalyst (9).
摘要翻译：通过液相中甲醇的催化转化制备合成气或氢的方法，包括同时使甲醇（1），烃（6）的液相和任选的水在催化剂（9）上通过。

42. 发明授权

US4544544A Plate reactors for chemical syntheses under high pressure in gaseous phase and with heterogeneous catalysis 失效
标题翻译：在高压下在气相和异相催化下进行化学合成的板式反应器
公开(公告)号：US4544544A
公开(公告)日：1985-10-01
申请号：US555260
申请日：1983-11-25
申请人： Quang Dang Vu , Claude Pradel , Jean-Paul Euzen , Jean-Francois Le Page
发明人： Quang Dang Vu , Claude Pradel , Jean-Paul Euzen , Jean-Francois Le Page
IPC分类号： B01J3/04 , B01J3/00 , B01J8/00 , B01J8/02 , B01J8/06 , C01C1/04 , C07C29/15 , C07C29/152 , C07C31/04 , C01B3/12
CPC分类号： C01C1/0417 , B01J8/0005 , B01J8/0242 , B01J8/0285 , C07C29/15 , B01J2208/0015 , B01J2208/022 , Y02P20/52
摘要： The invention relates to a process and to an apparatus for effecting chemical syntheses in gaseous phase, under pressure, in the presence of a solid catalyst, for instance, for ammonia synthesis from hydrogen and nitrogen or for the synthesis of methanol or higher homolog alcohols from hydrogen and at least one carbon oxide.The reactor (8) of substantially cylindrical shape, (see FIG. 4) contains a plurality of elongate compartments (9) of parallelipiped shape, adjacent to each other, the adjacent walls of the compartments or the common walls of the adjacent compartments being gas-tight walls (1), said tight walls forming hollow plates wherein are provided channels for the flow of a fluid heat carrier flowing through said walls under a pressure substantially equal to the pressure to which are subjected the reaction gases.
摘要翻译：本发明涉及一种在固体催化剂存在下，在压力下，在气相中进行化学合成的方法和装置，例如用于从氢和氮合成氨或用于合成甲醇或高级同系物的醇氢和至少一种碳氧化物。基本上圆柱形的反应器（8）（见图4）包含多个彼此相邻的平行形状的细长隔室（9），隔室的相邻壁或相邻隔室的公共壁是气体（1），所述紧密壁形成中空板，其中提供的通道用于在基本上等于受到反应气体的压力的压力下流过所述壁的流体热载体的流动。

43. 发明授权

US4498974A Process for converting a highly viscous hydrocarbon charge to a less viscous, more easily transportable and more easily refinable hydrocarbon fraction 失效
$Process for converting a highly viscous hydrocarbon charge to a less viscous, more easily transportable and more easily refinable hydrocarbon fraction$
标题翻译：将高粘度烃装料转化为较不粘稠，更容易运输和更容易可再生的烃馏分的方法
公开(公告)号：US4498974A
公开(公告)日：1985-02-12
申请号：US532928
申请日：1983-09-16
申请人： Alain Billon , Jean-Francois Le Page , Jean-Pierre Peries
发明人： Alain Billon , Jean-Francois Le Page , Jean-Pierre Peries
IPC分类号： C10G67/04 , C10G45/58
CPC分类号： C10G67/049
摘要： Process for reducing the viscosity of a highly viscous hydrocarbon charge containing 10-30% b.w. of constituents distilling above 375.degree. C., said treatment comprising hydrovisbreaking said charge to such an extent as to convert 10 to 30% of the 375.degree. C..sup.+ fraction to a 375.degree. C..sup.- fraction, fractionating the hydrovisbreaked product to separate a fraction comprising at least 90% of the constituents boiling below 375.degree. C. from a distillation residue, deasphalting said distillation residue and admixing at least a portion of the deasphalted distillation residue with at least a portion of said fraction comprising at least 90% of the constituents boiling below 375.degree. C.
摘要翻译：降低含有10-30％b.w的高粘性碳氢化合物的粘度的方法。的组分蒸馏高于375℃，所述处理包括将所述装料加氢裂化至将10％至30％的375℃+馏分转化为375℃馏分的程度，将水解产物分馏馏分包含来自蒸馏残余物的沸点低于375℃的组分的至少90％的组分，将所述蒸馏残渣脱沥青并将至少一部分脱沥青蒸馏残余物与所述级分的至少一部分混合，包含至少90％成分沸点低于375℃

44. 发明授权

US4424282A Process for the catalytic synthesis of hydrocarbons, particularly of methane, from hydrogen and carbon monoxide 失效
标题翻译：从氢气和一氧化碳催化合成烃，特别是甲烷的方法
公开(公告)号：US4424282A
公开(公告)日：1984-01-03
申请号：US348890
申请日：1982-02-16
申请人： Yves Chauvin , Dominique Commereuc , Andre Sugier , Jean-Francois Le Page
发明人： Yves Chauvin , Dominique Commereuc , Andre Sugier , Jean-Francois Le Page
IPC分类号： B01J8/02 , B01J23/00 , B01J23/46 , C07B61/00 , C07C1/00 , C07C1/04 , C07C9/04 , C07C67/00
CPC分类号： C07C1/048 , B01J23/462 , B01J8/0285 , C07C1/0425 , C07C1/0435 , C07C1/0445 , C07C1/046 , C07C1/0485 , B01J2208/0007 , B01J2208/00088 , B01J2208/00256 , B01J2208/00283 , C07C2521/04 , C07C2523/46
摘要： Methane is produced by passing hydrogen, carbon monoxide and an aqueous liquid phase downwardly through a fixed bed of a catalyst containing ruthenium on a carrier such as alumina, separating and externally coolng in a heat exchanger the resultant aqueous phase before recycling, thereby limiting the reaction temperature within a range from 200.degree. to 320.degree. C.
摘要翻译：通过将氢气，一氧化碳和水性液相通过载体如氧化铝上的含有钌的催化剂的固定床，在热交换器中分离和外部冷却，生成甲烷，所得水相在再循环之前由此限制反应温度在200〜320℃的范围内。

45. 发明授权

US4405442A Process for converting heavy oils or petroleum residues to gaseous and distillable hydrocarbons 失效
标题翻译：将重油或石油残渣转化为气态和可馏出的烃的方法
公开(公告)号：US4405442A
公开(公告)日：1983-09-20
申请号：US444268
申请日：1982-11-24
申请人： Andre Deschamps , Sigismond Franckowiak , Jean-Francois Le Page
发明人： Andre Deschamps , Sigismond Franckowiak , Jean-Francois Le Page
IPC分类号： C10G47/00 , C10G47/34 , C10G65/12 , C10G67/06 , C10G47/20
CPC分类号： C10G47/34 , C10G65/12 , C10G67/06 , Y10S208/95
摘要： This process for converting a charge of heavy oils or petroleum residues to gaseous and distillable hydrocarbons comprises the steps of (a) admixing said charge with a first hydrogenated recycle oil obtained in a subsequent step of the process, heating the mixture to 350.degree.-450.degree. C., admixing it with a reducing gas at a temperature of at least 800.degree. C. and maintaining a temperature of 530.degree.-850.degree. C. and a pressure of at least 20 bars for 0.1 to 60 seconds (b) admixing the resultant product with a second hydrogenated recycle oil whose temperature is lower than 300.degree. C., thereby decreasing the temperature of the resultant mixture to less than 450.degree. C., then contacting it with a steam-hydrogen stream, thereby vaporizing at least 80% of the liquid to a gaseous phase (c) treating the unvaporized remaining fraction with oxygen and steam to form a reducing gas at a temperature of at least 800.degree. C., used at least partly in step (a), (d) hydrogenating the gaseous phase from step (b) and recovering therefrom a light fraction distilling below 250.degree. C., recycling at least partly the remaining gaseous phase to step (b) after removal of CO.sub.2 and H.sub.2 S therefrom and (e) recycling the remaining hydrogenated heavy oil fraction, distilling above 250.degree. C., to steps (a) and (b).
摘要翻译：用于将重油或石油残余物转化成气态和可馏出烃的方法包括以下步骤：（a）将所述电荷与在该方法的后续步骤中获得的第一氢化循环油混合，将混合物加热至350-450℃ 将其与还原气体在至少800℃的温度下混合并保持530-850℃的温度和至少20巴的压力进行0.1至60秒（b）将得到的产物具有温度低于300℃的第二氢化循环油，从而将所得混合物的温度降低至低于450℃，然后使其与蒸汽 - 氢气流接触，从而汽化至少80％（c）用氧气和蒸汽处理未蒸发的剩余馏分以在至少800℃的温度下形成还原气体，至少部分地在步骤（a）中使用，（d）将来自ste的气相 p（b）并从其中回收低于250℃蒸馏的轻馏分，在从其中除去CO 2和H 2 S之后将至少部分剩余的气相再循环至步骤（b），和（e）回收剩余的氢化重油馏分，蒸馏高于250℃，步骤（a）和（b）。

46. 发明授权

US4340504A Catalyst for a process for dealkylating aromatic hydrocarbons in the presence of steam 失效
标题翻译：用于在蒸汽存在下使芳烃脱烷基化的方法的催化剂
公开(公告)号：US4340504A
公开(公告)日：1982-07-20
申请号：US206408
申请日：1980-11-12
申请人： Philippe Courty , Georgy L. Rabinovich , Victor N. Mojaiko , Jean-Francois Le Page
发明人： Philippe Courty , Georgy L. Rabinovich , Victor N. Mojaiko , Jean-Francois Le Page
IPC分类号： C07C4/20 , B01J23/656 , B01J23/68 , B01J23/89 , C07B61/00 , C07C1/00 , C07C15/00 , C07C67/00 , C10G45/62 , B01J23/36 , B01J23/48 , B01J23/58 , B01J23/72
CPC分类号： B01J23/8986 , B01J23/688 , C10G2400/30
摘要： Catalyst for dealkylating, in the presence of steam, a hydrocarbon charge, obtained for example from a catalytic reforming unit or from a unit for the production of aromatic hydrocarbons, and containing at least one alkylaromatic hydrocarbon such as toluene or a xylene, said catalyst containing an alumina carrier of a specific surface higher than 50 m.sup.2 /g and, by weight with respect to the catalyst, from 0.1 to 2% of rhodium, from 0.05 to 2% of at least one metal selected from copper, silver and gold, from 0.05 to 2% of rhenium and from 0.02 to 5% of at least one additional metal selected from lithium, sodium, potassium, rubidium, cesium, beryllium, magnesium, calcium, strontium, barium and uranium.
摘要翻译：在蒸汽存在下，使烷基化的催化剂，例如从催化重整单元获得的烃装料或用于生产芳族烃的单元，并含有至少一种烷基芳烃如甲苯或二甲苯，所述催化剂含有比表面积高于50m2 / g的氧化铝载体，相对于催化剂的重量，0.1-2％的铑，0.05-2％的至少一种选自铜，银和金的金属，来自 0.05至2％的铼和0.02至5％的至少一种选自锂，钠，钾，铷，铯，铍，镁，钙，锶，钡和铀的另外的金属。

47. 发明授权

US5498318A Reaction-distillation apparatus and its use 失效
标题翻译：反应蒸馏装置及其用途
公开(公告)号：US5498318A
公开(公告)日：1996-03-12
申请号：US100801
申请日：1993-08-02
申请人： Jacques Alagy , Alain Forestiere , Jean-Francois Le Page , Marie-Claire Marion , Jean-Charles Viltard
发明人： Jacques Alagy , Alain Forestiere , Jean-Francois Le Page , Marie-Claire Marion , Jean-Charles Viltard
IPC分类号： B01D3/16 , B01D3/00 , B01D3/22 , B01J8/02 , B01J8/04 , B01J19/30 , B01J19/32 , B01J32/00 , C07C41/06 , C07C43/04 , B01D3/14
CPC分类号： B01J8/02 , B01D3/009 , B01J19/30 , B01J8/048 , B01J2219/30223 , B01J2219/30226 , B01J2219/30408 , B01J2219/30475 , Y10S203/06
摘要： A reaction-distillation method is provided in which a chemical reaction and fractionation are conducted in an apparatus having at least one reaction-distillation zone (A,B) including at least one bed of solid elements disposed on a fluid-permeable support (5) having perforations small enough to retain the elements. The bed of solid elements includes loose solid catalytic particles (2) and at least one receptacle (3), containing at least one distillation packing body (4). The external jacket of the at least one receptacle (3) is permeable to fluids and impermeable to the solid catalytic particles (2) and the packing body (4). The apparatus can be used for carrying out chemical reactions and concomitant fractionation of the reaction mixture, for example, to synthesize ethers from olefins and alcohols.
摘要翻译：提供了一种反应 - 蒸馏方法，其中在具有至少一个反应蒸馏区（A，B）的装置中进行化学反应和分馏，所述反应蒸馏区包括设置在流体可渗透载体（5）上的至少一个固体元素床，具有足够小的孔以保持元件。固体元件床包括松散的固体催化剂颗粒（2）和至少一个包含至少一个蒸馏包装体（4）的容器（3）。所述至少一个容器（3）的外部护套可以渗透流体并且不可渗透固体催化颗粒（2）和包装体（4）。该装置可用于进行化学反应并伴随分离反应混合物，例如从烯烃和醇合成醚。

48. 发明授权

US4715946A Process for deasphalting a hydrocarbon charge containing asphaltenes 失效
标题翻译：使含有沥青质的烃装料脱沥青的方法
公开(公告)号：US4715946A
公开(公告)日：1987-12-29
申请号：US848083
申请日：1986-04-04
申请人： Jean-Francois Le Page , Alain Billon , Frederic Morel , Pierre Renard , Jean-Michel Biedermann , Michel Laborde , Jacques Bousquet
发明人： Jean-Francois Le Page , Alain Billon , Frederic Morel , Pierre Renard , Jean-Michel Biedermann , Michel Laborde , Jacques Bousquet
IPC分类号： C10G21/14 , C10G21/00 , C10C3/00
CPC分类号： C10G21/003
摘要： Process for deasphalting a hydrocarbon charge by means of a deasphalting solvent.The charge (1) is introduced, at 100.degree.-200.degree. C., in admixture with a deasphalting solvent (3and 4), into a settler (7). The deasphalted oil (24) is separated from the solvent (23). Asphalt (9) is washed in a column and then separated from the washing liquid (21).
摘要翻译：通过脱沥青溶剂使烃装料脱沥青的方法。将电荷（1）在100-200℃下与脱沥青溶剂（3和4）混合引入沉降器（7）中。脱沥青油（24）与溶剂（23）分离。将沥青（9）在柱中洗涤，然后与洗涤液（21）分离。

49. 发明授权

US4582630A Process for manufacturing synthesis gas, particularly useful for producing methanol 失效
标题翻译：制造合成气的方法，特别适用于生产甲醇
公开(公告)号：US4582630A
公开(公告)日：1986-04-15
申请号：US687231
申请日：1984-12-28
申请人： Dang V. Quang , Claude Raimbault , Regis Bonifay , Jean-Francois Le Page
发明人： Dang V. Quang , Claude Raimbault , Regis Bonifay , Jean-Francois Le Page
IPC分类号： C07C29/15 , C01B3/02 , C01B3/34 , C07C27/00 , C07C29/151 , C07C31/04 , C07C67/00 , C01B3/36
CPC分类号： C01B3/34
摘要： A synthesis gas for methanol production, containing hydrogen and carbon oxides, is obtained by performing, separately, a steam-reforming of hydrocarbons and a hydrocarbon combustion step: the effluents are admixed and the resultant mixture is subjected to steam-reforming.
摘要翻译：通过分别进行碳氢化合物和烃燃烧步骤的蒸汽重整来获得含有氢和碳氧化物的甲醇生产用合成气：混合流出物，对所得混合物进行蒸汽重整。

50. 发明授权

US4535067A Catalyst containing iron, chromium, potassium and lanthanum oxides, its manufacture and use in dehydrogenation reactions 失效
标题翻译：含有铁，铬，钾和氧化镧的催化剂，其制备和用于脱氢反应
公开(公告)号：US4535067A
公开(公告)日：1985-08-13
申请号：US561376
申请日：1983-12-14
申请人： Philippe Courty , Michel Roussel , Philippe Varin , Jean-Francois Le Page , Serge Leporq
发明人： Philippe Courty , Michel Roussel , Philippe Varin , Jean-Francois Le Page , Serge Leporq
IPC分类号： B01J23/86 , C07C5/333 , B01J21/16 , B01J23/10
CPC分类号： B01J23/862 , C07C5/3332
摘要： There are described catalysts containing, as oxides, iron, chromium and potassium, the latter being optionally partly in form of kaliophyllite Al.sub.2 O.sub.3, 2 SiO.sub.2, K.sub.2 O, as well as lanthanum, in a proportion, calculated in oxide weight, of 1-15% with respect to the final catalyst.The presence in the catalyst of lanthanum oxide, optionally previously combined with cobalt or vanadium, at least in part in the form of a mixed oxide of the perovskite type, confers to the catalyst an improved activity and/or selectivity in dehydrogenation reactions, particularly of ethylbenzene to styrene.
摘要翻译：描述了含有作为氧化物，铁，铬和钾的氧化物的催化剂，后者任选地部分地以氧化铝重量计为1-15％的亚氯酸铝Al 2 O 3，SiO 2，K 2 O以及镧的形式，相对于最终催化剂。至少部分以钙钛矿型混合氧化物的形式，任选地预先与钴或钒组合的氧化镧的催化剂中存在催化剂赋予催化剂在脱氢反应中更好的活性和/或选择性，特别是乙苯至苯乙烯。

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