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31. 发明授权

US09266808B2 Method for the hydroformylation of olefins 有权
标题翻译：烯烃加氢甲酰化的方法
公开(公告)号：US09266808B2
公开(公告)日：2016-02-23
申请号：US12516855
申请日：2007-11-29
申请人： Marcus Sigl , Frank Poplow , Rainer Papp , Thomas Mackewitz , Dag Wiebelhaus , Rocco Paciello , Thomas Heldemann , Frank Heimann , Stefan Bitterlich , Martin Volland , Sven Crone , Christoph Obler
发明人： Marcus Sigl , Frank Poplow , Rainer Papp , Thomas Mackewitz , Dag Wiebelhaus , Rocco Paciello , Thomas Heldemann , Frank Heimann , Stefan Bitterlich , Martin Volland , Sven Crone , Christoph Obler
IPC分类号： C07C29/141 , C07C45/50 , C07C5/25 , C07C45/74
CPC分类号： C07C45/50 , C07C5/2506 , C07C29/141 , C07C45/74 , C07C47/02 , C07C11/08 , C07C31/125 , C07C47/21
摘要： The present invention relates to a process for preparing hydroformylation products of olefins having at least four carbon atoms, in which a high proportion of both the linear Ci-olefins having a terminal double bond comprised in the olefin-comprising feed used and of the linear Ci-olefins having an internal double bond is converted into hydroformylation products. Furthermore, the invention relates to a process for preparing 2-propylheptanol which comprises such a hydroformylation process.
摘要翻译：本发明涉及一种制备具有至少四个碳原子的烯烃的加氢甲酰化产物的方法，其中在所用含烯烃的原料中包含的具有末端双键的直链C 1 -C 20烯烃和线性C 1 具有内部双键的烯烃转化为加氢甲酰化产物。此外，本发明涉及一种制备2-丙基庚醇的方法，其包括这种加氢甲酰化方法。

32. 发明授权

US08969644B2 Method for providing an oxygen-containing gas stream for the endothermic reaction of an initial stream comprising one or more hydrocarbons 有权
标题翻译：提供用于包含一种或多种烃的初始流的吸热反应的含氧气流的方法
公开(公告)号：US08969644B2
公开(公告)日：2015-03-03
申请号：US12525830
申请日：2008-01-31
申请人： Gerhard Olbert , Franz Corr , Sven Crone
发明人： Gerhard Olbert , Franz Corr , Sven Crone
IPC分类号： C07C5/48 , F23C6/04 , B01J4/00 , C01B3/36 , F23L7/00
CPC分类号： F23C6/045 , B01J4/005 , C01B3/36 , C01B2203/0255 , C07C5/48 , F23C2900/06041 , F23L7/005 , Y02E20/344 , Y02P20/129 , C07C11/06 , C07C11/08
摘要： A method is proposed for providing an oxygen-containing gas stream for the endothermic reaction of an initial stream comprising one or more hydrocarbons, having a predetermined oxygen concentration and a predetermined temperature, wherein a fluid fuel stream is combusted with a primary air stream at λ values of the primary air stream to the fluid fuel stream of from 0.6 to 1.2 to obtain a combustion gas stream, and a secondary air stream is admixed to the combustion gas stream to obtain the oxygen-containing gas stream for the endothermic reaction, with the predetermined oxygen concentration and the predetermined temperature of the oxygen-containing gas stream being adjusted via the flow rate and the temperature of the secondary air stream.
摘要翻译：提出了一种方法，用于提供含有一种含氧气流，用于包含一种或多种具有预定氧浓度和预定温度的烃的初始流的吸热反应，其中流体燃料流与主空气流以λ 一次空气流到流体燃料流的值为0.6至1.2，以获得燃烧气体流，并且二次空气流与燃烧气体流混合以获得用于吸热反应的含氧气体流，其中预定的氧浓度和含氧气流的预定温度通过二次气流的流量和温度进行调节。

33. 发明授权

US07854906B2 Reactor for carrying out a reaction between two fluid starting materials over a catalyst bed with premixing of the fluid starting materials in a mixing-in device 有权
标题翻译：用于在催化剂床上进行两种流体起始材料之间的反应的反应器，其中流体原料在混合装置中预混合
公开(公告)号：US07854906B2
公开(公告)日：2010-12-21
申请号：US11959008
申请日：2007-12-18
申请人： Gerhard Olbert , Franz Corr , Sven Crone
发明人： Gerhard Olbert , Franz Corr , Sven Crone
IPC分类号： F28D7/00 , B01J8/00 , B01J8/04 , B01J8/08 , B01J35/02 , F28F1/00 , C10G55/02 , C10G51/02 , C10G35/10
CPC分类号： B01F5/0453 , B01F5/0456 , B01J8/008 , B01J8/0085 , B01J8/0214 , B01J8/0278 , B01J8/0453 , B01J8/0492 , B01J2208/00849 , B01J2208/00884 , B01J2219/1946 , Y10T137/87652
摘要： A reactor for carrying out a reaction between two fluid starting materials over a catalyst bed with premixing of the fluid starting materials before introduction into the catalyst bed within a delay time of less than 150 ms in a mixing-in device, wherein the mixing-in device is made up of the following elements which are arranged essentially transverse to the inflow direction of the first fluid starting material stream: two or three rows arranged behind one another of tubes which have turbulence generators on the outside and constrict the flow cross section for the first fluid starting material stream to from ½ to 1/10, with the second fluid starting material stream being passed through the interiors of the tubes and injected via openings in the tubes into the first fluid starting material stream; a perforated plate upstream of the tubes; and a perforated plate downstream of the tubes, is proposed.
摘要翻译：一种用于在催化剂床上进行两种流体起始材料之间的反应的反应器，其中在混合入装置内在延迟时间小于150ms之前，在引入催化剂床之前预先混合流体原料，其中混合装置由以下元件组成，其基本上横向于第一流体起始材料流的流入方向布置：两个或三个排布置在彼此后面的管，其在外部具有湍流发生器并且收缩流动截面第一流体起始物料流至1/2至1/10，其中第二流体起始物料流通过管的内部并通过管中的开口注入到第一流体原料流中; 在管的上游的多孔板; 并且提出了在管下游的多孔板。

34. 发明授权

US07838702B2 Direct amination of hydrocarbons 失效
标题翻译：碳氢化合物的直接胺化
公开(公告)号：US07838702B2
公开(公告)日：2010-11-23
申请号：US12280070
申请日：2007-02-13
申请人： Frederik Van Laar , Ekkehard Schwab , Joachim-Thierry Anders , Sven Crone , Karl Hoelemann , Wolfgang Mackenroth , Petr Kubanek
发明人： Frederik Van Laar , Ekkehard Schwab , Joachim-Thierry Anders , Sven Crone , Karl Hoelemann , Wolfgang Mackenroth , Petr Kubanek
IPC分类号： C07C209/02 , C07C209/60
CPC分类号： C07C209/02 , C07C211/46
摘要： A process for aminating hydrocarbons with ammonia, wherein the N2 content in the mixture at the reactor exit is less than 0.1% by volume based on the total volume of the mixture at the reactor exit.
摘要翻译：用氨胺化胺的方法，其中反应器出口处混合物中的N 2含量基于反应器出口处混合物的总体积小于0.1体积％。

35. 发明授权

US07741522B2 Direct amination of hydrocarbons 失效
标题翻译：碳氢化合物的直接胺化
公开(公告)号：US07741522B2
公开(公告)日：2010-06-22
申请号：US12280634
申请日：2007-02-15
申请人： Frederik Van Laar , Ekkehard Schwab , Joachim-Thierry Anders , Sven Crone , Karl Hoelemann , Wolfgang Mackenroth , Petr Kubanek
发明人： Frederik Van Laar , Ekkehard Schwab , Joachim-Thierry Anders , Sven Crone , Karl Hoelemann , Wolfgang Mackenroth , Petr Kubanek
IPC分类号： C07C209/02
CPC分类号： C07C209/02
摘要： A process for aminating hydrocarbons with ammonia in the presence of catalyst (i) which catalyzes the amination, which comprises supplying oxidizing agent to the reaction mixture and reacting the oxidizing agent with hydrogen which is formed in the amination in the presence of a catalyst (ii) which catalyzes this reaction with hydrogen.
摘要翻译：在催化胺化催化剂（ⅰ）的存在下，用氨胺化氨烃的方法，其中包括向反应混合物中供应氧化剂，并使氧化剂与在催化剂存在下在胺化中形成的氢反应（ii）），其与氢催化该反应。

36. 发明申请

US20090203941A1 DIRECT HYDROCARBON AMINATION 审中-公开
标题翻译：直接碳氢化合物
公开(公告)号：US20090203941A1
公开(公告)日：2009-08-13
申请号：US12064635
申请日：2006-08-21
申请人： Frederik Van Laar , Ekkehard Schwab , Hartwig Voss , Joachim-Thierry Anders , Sven Crone , Wolfgang Mackenroth
发明人： Frederik Van Laar , Ekkehard Schwab , Hartwig Voss , Joachim-Thierry Anders , Sven Crone , Wolfgang Mackenroth
IPC分类号： C07C209/02
CPC分类号： C07C209/02 , B01D53/228 , B01D67/0072 , B01D69/10 , B01D71/022 , B01D2323/12 , B01D2325/10 , C01B3/505 , C01B2203/041 , C01B2203/0465 , C01B2203/048 , C07C211/44 , C07C211/45 , C07C211/46
摘要： A process for aminating hydrocarbons comprises physically removing hydrogen from the reaction mixture.
摘要翻译：用于胺化胺的方法包括物理地从反应混合物中除去氢。

37. 发明授权

US07488857B2 Method for the production of butadiene and 1-butene 有权
标题翻译：制备丁二烯和1-丁烯的方法
公开(公告)号：US07488857B2
公开(公告)日：2009-02-10
申请号：US10584783
申请日：2004-12-30
申请人： Thorsten Johann , Götz-Peter Schindler , Andreas Brodhagen , Sven Crone , Regina Benfer , Marcus Sigl , Mark Duda
发明人： Thorsten Johann , Götz-Peter Schindler , Andreas Brodhagen , Sven Crone , Regina Benfer , Marcus Sigl , Mark Duda
IPC分类号： C07C5/333
CPC分类号： C07C5/327 , C07C5/333 , C07C5/48 , C07C11/167
摘要： The disclosure involves a process for the preparation of butadiene and 1-butene. The process includes at least a first catalytic dehydrogenation of n-butane to obtain a gas stream which is followed by at least a second oxidative dehydrogenation to form a second gas stream. The second gas stream is then subjected to distillation and isomeration steps to obtain butadiene and 1-butene.
摘要翻译：本公开涉及制备丁二烯和1-丁烯的方法。该方法至少包括正丁烷的第一催化脱氢以获得气流，随后进行至少第二氧化脱氢以形成第二气流。然后将第二气流进行蒸馏和异构化步骤以获得丁二烯和1-丁烯。

38. 发明申请

US20100233047A1 HORIZONTAL REACTOR FOR REACTING A FLUID EDUCT STREAM WITH A FLUID OXIDANT STREAM IN THE PRESENCE OF A SOLID CATALYST 审中-公开
标题翻译：用于在固体催化剂存在下用流体氧化物流反应流体流化床的水平反应器
公开(公告)号：US20100233047A1
公开(公告)日：2010-09-16
申请号：US12739829
申请日：2008-10-24
申请人： Gerhard Olbert , Franz Corr , Sven Crone
发明人： Gerhard Olbert , Franz Corr , Sven Crone
IPC分类号： B01J8/04
CPC分类号： B01J8/008 , B01F5/0451 , B01F5/0453 , B01F5/0456 , B01F5/0458 , B01F5/0618 , B01F13/1013 , B01F13/1016 , B01J8/048 , B01J8/0492 , B01J8/0496 , B01J2208/00194 , B01J2208/00769 , B01J2208/00814 , B01J2208/00884
摘要： A reactor (1) for reacting a fluid feed stream (2) with a fluid oxidant stream (3) in the presence of a solid catalyst (4) in two or more stages over two or more fixed catalyst beds (5) which are arranged horizontally, parallel to the longitudinal axis of a cylindrical reactor wall (6) in the interior space thereof, with caps (7) being installed in a detachable fashion at the ends of the reactor wall (6), with the fluid feed stream (2) flowing through the reactor (1) from the top downward, wherein the two or more fixed catalyst beds (5) are each formed by a plurality of modules, comprising in each case a cuboidal frame (8) which extends over the entire height of the fixed catalyst bed and in which one or more lower screens (9) and an upper screen (10) are installed and the solid catalyst (4) is present between the one or more lower screens (9) and the upper screen (10), all modules of a fixed catalyst bed (5) are enclosed in a cuboidal outer frame (11) which is arranged horizontally in the reactor (1) and extends essentially over the entire length and the entire width of the reactor (1) with the exception of the caps, and a mixing-in apparatus (12) for the fluid oxidant stream (3) is provided upstream of each fixed catalyst bed (5), is proposed.
摘要翻译：一种反应器（1），用于在固体催化剂（4）存在下，在两个或更多个固定催化剂床（5）上分两个或更多个阶段使流体进料流（2）与流体氧化剂流（3）反应，水平地平行于其内部空间中的圆柱形反应器壁（6）的纵向轴线，其中帽（7）以可拆卸的方式安装在反应器壁（6）的端部处，流体进料流（2））从顶部向下流动通过反应器（1），其中两个或更多个固定催化剂床（5）各自由多个模块形成，每个模块包括在每个壳体中的整个高度上延伸的立方形框架（8）固定催化剂床，其中安装有一个或多个下筛网（9）和上筛网（10），并且固体催化剂（4）存在于一个或多个下筛网（9）和上筛网（10）之间，，固定催化剂床（5）的所有模块都封闭在水平放置的立方形外框架（11）中反应器（1）并且基本上在反应器（1）的整个长度和整个宽度上延伸，除了盖子之外，并且用于流体氧化剂流（3）的混合装置（12）设置在提出了每个固定催化剂床（5）。

39. 发明授权

US07482500B2 Preparation of butadiene 有权
标题翻译：丁二烯的制备
公开(公告)号：US07482500B2
公开(公告)日：2009-01-27
申请号：US10584758
申请日：2004-12-30
申请人： Thorsten Johann , Götz-Peter Schindler , Andreas Brodhagen , Sven Crone , Regina Benfer , Thomas Hill , Mark Duda
发明人： Thorsten Johann , Götz-Peter Schindler , Andreas Brodhagen , Sven Crone , Regina Benfer , Thomas Hill , Mark Duda
IPC分类号： C07C5/327 , C07C5/32
CPC分类号： C07C5/333 , C07C5/48 , C07C11/167
摘要： The disclosure relates to a process for preparing butadiene. The process involves nonoxidatively catalytically dehydrogenating butane to obtain a product gas stream containing butane, 1-butene, 2-butene, butadiene, hydrogen and secondary constituents. The 1-butene and 2-butene of the product gas stream is then oxidatively dehydrogenated to give a second gas stream containing butane,2-butene, butadiene, hydrogen, steam and secondary constituents. Next, the butane,2-butene and butadiene are separated from the second gas stream and the butane and 2-butene are then separated from the butadiene product. The butane and 2-butene are then recycled into the nonoxidative catalytic dehydrogenating zone.
摘要翻译：本公开涉及一种制备丁二烯的方法。该方法涉及非氧化催化脱氢丁烷，以获得含有丁烷，1-丁烯，2-丁烯，丁二烯，氢和二次成分的产物气流。然后将产物气流的1-丁烯和2-丁烯氧化脱氢，得到含有丁烷，2-丁烯，丁二烯，氢气，蒸汽和二级成分的第二气流。接下来，将丁烷，2-丁烯和丁二烯与第二气流分离，然后从丁二烯产物中分离丁烷和2-丁烯。然后将丁烷和2-丁烯循环到非氧化催化脱氢区。

40. 发明申请

US20090023956A1 DIRECT AMINATION OF HYDROCARBONS 失效
标题翻译：油气的直接化学分析
公开(公告)号：US20090023956A1
公开(公告)日：2009-01-22
申请号：US12280634
申请日：2007-02-15
申请人： Frederik van Laar , Ekkehard Schwab , Joachim-Thierry Anders , Sven Crone , Karl Holemann , Wolfgang Mackenroth , Petr Kubanek
发明人： Frederik van Laar , Ekkehard Schwab , Joachim-Thierry Anders , Sven Crone , Karl Holemann , Wolfgang Mackenroth , Petr Kubanek
IPC分类号： C07C209/02
CPC分类号： C07C209/02
摘要： A process for aminating hydrocarbons with ammonia in the presence of catalyst (i) which catalyzes the amination, which comprises supplying oxidizing agent to the reaction mixture and reacting the oxidizing agent with hydrogen which is formed in the amination in the presence of a catalyst (ii) which catalyzes this reaction with hydrogen.
摘要翻译：在催化胺化催化剂（ⅰ）的存在下，用氨胺化氨烃的方法，其中包括向反应混合物中供应氧化剂，并使氧化剂与在催化剂存在下在胺化中形成的氢反应（ii）），其与氢催化该反应。

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